Nature of quasiparticles in itinerant correlated electron systems with geometrical frustration

Using the exact diagonalization technique, we study the effect of geometrical frustration on single-particle, spin and charge excitations in the Hubbard model in a metallic state close to half-filling. As the frustration increases, the magnetic order in the system is suppressed and the peak in the single-particle spectrum becomes sharper, indicating enhanced quasiparticle formation. Careful examination of spin and charge excitations shows that increasing frustration also leads to the merge of spin and charge excitation energies to that of the single-particle excitation. This is consistent with a Fermi liquid having well-defined quasiparticles with both spin and charge characteristics. The calculated results show that geometrical frustration plays an important role in defining the nature of quasiparticles in itinerant correlated electron systems.     

Macroscopic signature of protected spins in a dense frustrated magnet

The inability of systems of interacting objects to satisfy all constraints simultaneously leads to frustration. A particularly important consequence of frustration is the ability to access certain protected parts of a system without disturbing the others. For magnets such "protectorates" have been inferred from theory and from neutron scattering, but their practical consequences have been unclear. We show that a magnetic analogue of optical hole-burning can address these protected spin clusters in a well-known, geometrically frustrated Heisenberg system, gadolinium gallium garnet. Our measurements additionally provide a resolution of a famous discrepancy between the bulk magnetometry and neutron diffraction results for this magnetic compound.     

Quantum phase transitions of spin chiral nanotubes

Recently many interesting magnetic nanostructures have been fabricated and much attention is arising on the rich magnetic properties that originate in the quantum effects eminent in the nanoscale world. One of the peculiar aspects of the quantum effects is the spin excitation gap. In the spin-1/2 low-dimensional systems, the spin gap often appears when the lattice dimerization or the frustration in the spin–spin interaction are introduced. In the present study, we investigate the ground-state property of the spin-1/2 antiferromagnetic spin chiral nanotubes with the spatial modulation in the spin–spin interaction. The ground-state phase diagrams of them are determined by observing the behavior of the expectation value of the Lieb–Schultz–Mattis slow-twist operator calculated by the quantum Monte Carlo method with the continuous-time loop algorithm. We discuss the relation between the characteristic of the topology of the phase diagram and the chiral vector of the nanotubes.     

Electron spin resonance of magnetic materials in high fields and high frequencies

Observation and analysis of electron spin resonance of many kinds of magnetic materials have been performed with high frequencies provided by Gunn oscillators, backward traveling wave tubes and far-infrared lasers and also with a vector network analyzer in both pulsed high magnetic fields up to 40 T and steady field up to 20 T. The magnetic behavior of quantum spin systems and metallic materials has been investigated.     

Role of surface anisotropy for magnetic impurities in electron dephasing and energy relaxation and their size effect

Recently the electron dephasing and energy relaxation due to different magnetic impurities have been extensively investigated experimentally in thin wires, and in this Letter these quantities are theoretically studied. It was shown earlier that a magnetic impurity in a metallic host with strong spin-orbit interaction experiences a surface anisotropy of the form H=K(d)(nS)(2) which causes size effects for impurities with integer spin. Here we show that the dephasing and the energy relaxation are influenced by the surface anisotropy in very different ways for integer spin having a singlet ground state. That must result also in strong size effects and may resolve the puzzle between the concentrations estimated from the two kinds of experiments.     

Magnetic Phase Transition Driven by Frustrated Interactions in a Longitudinal‐Field Ising Chain

The ground‐state magnetic phase transitions in a classical spin chain with long‐range interactions in a system of trapped ions are investigated. The tunable competing interactions, mediated by both longitudinal and transverse photon modes, lead to competition among different spins, due to which magnetic frustration occurs. Various ground‐state spin configurations are separated by multiple phase transitions when the strength and sign of these interactions are tuned continuously. The spin chains are highly degenerated because of the frustration, so there is some melting of several magnetic phases.     

具有次近邻相互作用的五量子比特XXZ海森伯自旋链的热纠缠

研究具有次近邻相互作用五量子比特XXZ海森伯自旋链在磁场作用下的热纠缠性质,利用数值计算求出最近邻两量子比特和次近邻两量子比特的共生纠缠度(concurrence),分别记为C_(12)和C_(13).研究结果表明,阻挫参数对配对热纠缠具有重要影响,而且阻挫参数的变化对C_(12)和C_(13)的影响也各不相同;温度、磁场、Dzyaloshinkii-Moriya相互作用以及各向异性参数对配对热纠缠有着不同程度的影响;通过选择适当的模型参数,可以有效地调节和提高五量子比特XXZ海森伯自旋链的配对热纠缠.     

Non-Kondo mechanism for resistivity minimum in spin ice conduction systems

We present a mechanism of resistivity minimum in conduction electron systems coupled with localized moments, which is distinguished from the Kondo effect. Instead of the spin-flip process in the Kondo effect, electrons are elastically scattered by local spin correlations which evolve in a particular way under geometrical frustration as decreasing temperature. This is demonstrated by the cellular dynamical mean-field theory for a spin-ice-type Kondo lattice model on a pyrochlore lattice. Peculiar temperature dependences of the resistivity, specific heat, and magnetic susceptibility in the non-Kondo mechanism are compared with the experimental data in metallic Ir pyrochlore oxides.     

Theory of two-magnon Raman scattering in iron pnictides and chalcogenides

Although the parent iron-based pnictides and chalcogenides are itinerant antiferromagnets, the use of local moment picture to understand their magnetic properties is still widespread. We study magnetic Raman scattering from a local moment perspective for various quantum spin models proposed for this new class of superconductors. These models vary greatly in the level of magnetic frustration and show a vastly different two-magnon Raman response. Light scattering by two-magnon excitations thus provides a robust and independent measure of the underlying spin interactions. In accord with other recent experiments, our results indicate that the amount of magnetic frustration in these systems may be small.     

Relaxation effects in Fe17 and Fe19 oxo-bridged iron clusters

The magnetic properties of a new type of iron clusters are studied by means of Mössbauer spectroscopy in an applied magnetic field. The results obtained agree with the ones obtained from magnetic susceptibility measurements. They are well explained in terms of relaxation determined by fluctuations in the hyperfine field due to spin-spin interaction. The triangular arrangement of the iron ions plays an essential role in this mechanism giving rise to spin frustration effects.     

Chiral-like critical behavior in the antiferromagnet cobalt glycerolate

Critical exponents closely matching those of the N=2 chiral universality class have been obtained for the layered magnetic system cobalt glycerolate using muon spin relaxation. This class was originally introduced to represent geometrically frustrated triangular stacked-layer XY magnets with chiral noncollinear spin structures. Since the present magnetic system is a canted XY system without geometrical frustration or chiral degeneracy, the results indicate that the order parameter for canting in this system plays a similar role to the chiral order parameter in the geometrically frustrated systems, strongly suggesting that both types of noncollinear system share the same universality class.     

Unconventional magnetism in a nitrogen-containing analog of cupric oxide

We have investigated the magnetic properties of CuNCN, the first nitrogen-based analog of cupric oxide CuO. Our muon-spin relaxation, nuclear magnetic resonance, and electron-spin resonance studies reveal that classical magnetic ordering is absent down to the lowest temperatures. However, a large enhancement of spin correlations and an unexpected inhomogeneous magnetism have been observed below 80 K. We attribute this to a peculiar fragility of the electronic state against weak perturbations due to geometrical frustration, which selects between competing spin-liquid and more conventional frozen states.     

人工自旋冰中阻挫现象的研究进展

磁学中的阻挫现象近些年来是实验及理论研究的热点.本文就磁学中阻挫研究的新进展进行了介绍.描述了用显微刻蚀制备的人工自旋冰的研究,讨论了其潜在的应用前景以及计算机模拟的结果.     

Precursor phenomena in frustrated systems

To understand the origin of the dynamical transition, between high-temperature exponential relaxation and low-temperature nonexponential relaxation, that occurs well above the static transition in glassy systems, a frustrated spin model, with and without disorder, is considered. The model has two phase transitions, the lower being a standard spin glass transition (in the presence of disorder) or fully frustrated Ising (in the absence of disorder), and the higher being a Potts transition. Monte Carlo results clarify that in the model with (or without) disorder the precursor phenomena are related to the Griffiths (or Potts) transition. The Griffiths transition is a vanishing transition which occurs above the Potts transition and is present only when disorder is present, while the Potts transition which signals the effect due to frustration is always present. These results suggest that precursor phenomena in frustrated systems are due either to disorder and/or to frustration, giving a consistent interpretation also for the limiting cases of Ising spin glass and of Ising fully frustrated model, where also the Potts transition is vanishing. This interpretation could play a relevant role in glassy systems beyond the spin systems case.     

Single-particle excitation spectrum of the Hubbard model with magnetic frustration at finite temperature

The single-particle excitation spectrum of the Hubbard model with magnetic frustration at finite temperature is examined using numerical exact diagonalization techniques. The magnetic frustration is introduced by a proper choice of the Hamiltonian parameters, which lead to rich low-energy spin excitation behavior, resembling those observed in heavy fermion systems. At finite temperature, the low-lying excited states become thermally populated with significant weight. As a result, the calculated spectrum shows interesting temperature dependent evolution. The calculated results are presented and discussed in a many-body picture to gain insight into the photoelectron spectroscopy of strongly correlated electron systems.     

Impurity spin dynamics and quantum coherence in mesoscopic rings

We investigate the effects of impurity spin dynamics on quantum coherence in mesoscopic metallic rings. Spin relaxation induces temporal current fluctuations which are closely related to persistent currents in such systems. The persistent current is suppressed in the presence of magnetic impurities. We discuss spin-polarisation effects, spin-glass ordering, and the Kondo effect which are shown to restore the current even in the presence of magnetic scattering.     

Nonextensive quantum method for itinerant-electron ferromagnetism: Factorization approach

Magnetic and thermodynamical properties of itinerant-electron (metallic) ferromagnets described by the Hubbard model have been discussed with the use of the generalized Fermi-Dirac (GFD) distribution for nonextensive quantum systems. We have derived the GFD distribution within the superstatistics, which is equivalent to that obtained by the maximum-entropy method to the Tsallis entropy with the factorization approximation. By using the Hartree-Fock approximation to the electron-electron interaction in the Hubbard model, we have calculated magnetic moment, energy, specific heat and Curie-Weiss-type spin susceptibility, as functions of the temperature and entropic index q expressing the degree of the nonextensivity: q=1.0 corresponds to the Boltzmann-Gibbs statistics. It has been shown that by increasing the nonextensivity of |q−1|, the temperature dependence of magnetic moment becomes more significant and the low-temperature electronic specific heat is very much increased. This is attributed to enlarged Stoner excitations in the GFD distribution, which is elucidated by an analysis with the use of the generalized Sommerfeld expansion. We discuss the difference and similarity between the effects of the nonextensivity on metallic and insulating ferromagnets.     

Spin freezing in the van der Waals material Mn2Ga2S5

Geometrical frustration in low-dimensional magnetic systems has been an intriguing research aspect, where the suppression of conventional magnetic order may lead to exotic ground states such as spin glass or spin liquid. In this work we report the synthesis and magnetism study of the monocrystalline Mn$_2$Ga$_2$S$_5$, featuring both the van der Waals structure and a bilayered triangular Mn lattice. Magnetic susceptibility reveals a significant antiferromagnetic interaction with a Curie-Weiss temperature $\theta_{\rm w}\sim-260$ K and a high spin $S=5/2$ Mn$^{2+}$ state. However, no long range magnetic order has been found down to 2 K, and a spin freezing transition is found to occur at around 12 K well below its $\theta_{\rm w}$. This yields a frustration index of $f = -\theta_{\rm w}/T_{\rm f} \approx 22$, an indication that the system is highly frustrated. The absence of a double-peak structure in magnetic specific heat compared with the $TM_2$S$_4$ compounds implies that the spin freezing behavior in Mn$_2$Ga$_2$S$_5$ is a result of the competition between exchange interactions and the 2D crystalline structure. Our results suggest that the layered Mn$_2$Ga$_2$S$_5$ would be an excellent candidate for investigating the physics of 2D magnetism and spin disordered state.     

Low temperature cluster glass behavior in Nd5Ge3

Various experimental evidence obtained from dc and ac magnetization measurements indicates that Nd(5)Ge(3) undergoes a spin glass transition from a high temperature antiferromagnetic state. Below the Néel temperature of 49 K, it shows distinct properties that characterize a cluster glass state, thereby indicating that it is an example of a reentrant spin glass system. Dynamical behavior of the magnetic susceptibility and the magnetic relaxation clearly give evidence of frustration in the material. Geometric frustration arising from the triangular arrangement of Nd atoms seems to be the main reason behind the spin glass state. A field-induced structural distortion accompanying the Néel transition may also be responsible for the frustration and the spin glass state.     

阻挫三角反铁磁AgCrO2螺旋自旋序的第一性原理研究

基于密度泛函理论的广义梯度近似(GGA)和投影缀加波(PAW)方法,分别从共线和非共线磁性结构出发,研究了自旋阻挫三角反铁磁AgCrO₂的基态、磁性以及电子结构,从理论计算的角度给出了基态磁性结构.计算结果表明:AgCrO₂具有120°螺旋自旋序反铁磁基态,其自旋螺旋面平行于(110)面或(11^-0)面;由于Cr离子间的自旋几何阻挫,导致沿晶体的a,b和a+b方向上均形成了螺旋自旋转动角为120°的 关键词： 第一性原理 交换相互作用 阻挫 反铁磁