Spin-1 chain doped with mobile S = 1/2 fermions

We investigate the doping of a two-orbital chain with mobile S = 1/2 fermions as a valid model for Y2-xCaxBaNiO5. The S = 1 spins are stabilized by strong, ferromagnetic Hund's rule couplings. We calculate correlation functions and thermodynamic quantities by density matrix renormalization group methods and find a new hierarchy of energy scales in the spin sector upon doping. Gapless spin excitations are generated at a lower energy scale by interactions among itinerant polarons created by each hole and coexist with the larger scale of the gapful spin-liquid background of the S = 1 chain accompanied by a finite string order parameter.     

Interaction of the ground state of quarter-filled one-dimensional strongly correlated electronic system with localized spins

We study numerically the ground-state properties of the one-dimensional quarter-filled strongly correlated electronic system interacting antiferromagnetically with localized S = 1/2 spins. It is shown that the charge-ordered state is significantly stabilized by the introduction of relatively small coupling with the localized spins. When the coupling becomes large the spin and charge degrees of freedom behave quite independently and the ferromagnetism is realized. Moreover, the coexistence of ferromagnetism with charge order is seen in the strongly interacting region. The present theoretical results are to be compared with the experiments on phthalocyanine compounds.     

Formation of an Antiferromagnetic Metal Phase in the Electron-Doped Sr0.98La0.02MnO3 Oxide According to 17O NMR Data

JETP Letters - The spin density distribution of itinerant electrons, neg, and their effect on pairwise correlations of localized spins S(t2g) of Mn4+ ions in cubic Sr1 − xLaxMnO3...     

Alternating-spin S = 3/2 and <Emphasis Type="Italic">σ</Emphasis> = 1/2 Heisenberg chain with isotropic three-body exchange interactions

The promotion of collinear classical spin configurations as well as the enhanced tendencytowards nearest-neighbor clustering of the quantum spins are typical features of thefrustrating isotropic three-body exchange interactions in Heisenberg spin systems. Basedon numerical density-matrix renormalization group calculations, we demonstrate that theseextra interactions in the Heisenberg chain constructed from alternating S = 3/2 and σ = 1/2 site spins can generate numerous specific quantum spinstates, including some partially-polarized ferrimagnetic states as well as adoubly-degenerate non-magnetic gapped phase. In the non-magnetic region of the phasediagram, the model describes a crossover between the spin-1 and spin-2 Haldane-typestates.     

The Charged and the Spin-Excitation Gaps in the Double-Exchange Model: a Rigorous Result

We extend a previous result of ours [G.S. Tian, Phys. Rev. B58 (1998) 76121 on the charged gap and the spin-excitation gap of the half-filled Kondo lattice model to the doubleexchange model. In our original approach, this model cannot be dealt with since its localized spins have a large spin number S=3/2. By following a construction argument due to Zener and rewriting the double-exchange Hamiltonian, we are able to overcome this difficulty and re-establish the same relation for this model.     

Entanglement of spin pairs in alternating open spin-1/2 chains with the XY Hamiltonian

We investigate entanglement of spin pairs in alternating open spin chains (s = 1/2) with spin-spin interactions (SSI) in the thermodynamic equilibrium state in an external magnetic field. The reduced density matrix of an arbitrarily chosen spin pair was calculated. The entanglement of a spin pair was evaluated with the Wootters criterion. The temperature at which the entangled state arises in the chosen pair was determined. Entanglement (concurrence) is shown to oscillate as a function of the position of a spin pair in the chain. The results demonstrate the dependence of the entanglement in arbitrarily chosen pairs of neighboring spins on the temperature, the position of the spin pair in the chain, chain length, and the ratio between the SSI constants. Qualitative explanation of these dependences is offered. The role of the terminal spins in the generation of entanglement is explained.     

Thermodynamics of a quasi-one-dimensional spin system for molecule-based ferrimagnets

A physical picture of electron spin alignments in organic molecule-based ferrimagnets is given from numerical calculations of magnetic specific heat (C) and magnetic susceptibility (χ) as functions of temperature and static magnetic field (B) in terms of an Ising Hamiltonian for an alternating spin chain. The double-peak structure of specific heat appears for different parameter ratios and different magnetic field B, indicating that one peak originates from the ferromagnetic nature and the other from the antiferromagnetic nature. Meanwhile, we study successively the influence of intermolecular and intramolecular interaction on the magnetic susceptibility, showing that the ferromagnetic spin alignment in the alternating molecular chains of biradicals and monoradicals is equivalent to the ferromagnetic alignment of the effective S=1/2 spins. Our results are consistent with those of the Quantum Monte Carlo simulations and the exact diagonalization method and in qualitative agreement with the experimental ones.     

Fully Optical Detection of Hyperfine Electron–Nuclear Interactions in Spin Centers in 6H-SiC Crystals with a Modified 13C Isotope Content

JETP Letters - Optically induced alignment and polarization of electron and nuclear spins in color centers with electron spin $$S = 3{\text{/}}2$$ , which lead to giant changes in photoluminescence...     

Heisenberg-Dirac-van Vleck vector model for a 1D antiferromagnetic chain of localized spins <Emphasis Type="Italic">S</Emphasis> = 1

Magnetic properties of anisotropic crystals with localized spins S = 1 are investigated; for these crystals, the Hamiltonian is derived in the Heisenberg-Dirac-van Vleck form, which includes biquadratic contributions apart from bilinear terms. The ground-state energy of the antiferromagnetic chain of spins S = 1 is calculated in the model of nearest neighbors, and the interaction constant is renormalized using the renorm group method in the case of coarsening of the system. The temperature criterion for the formation of long-range order in the system is obtained. The excitations of this chain in the linear approximation have a dispersion relation differing from that for antiferromagnets with spin S = 1/2 and are separated by an energy gap from the ground state. Allowance for nonlinear contribution leads to the formation of a solitary wave in the form of a dark-bright soliton.     

Delay of Spatial Quantum Correlations in Magnetic Nanostructures

Simultaneous quantum correlations between two spins in magnetic nanostructures are considered in the model of a linear chain of a finite number of atoms with exchange interaction between electron spins of neighboring atoms in the framework of the Heisenberg ferromagnetism theory. We assume that in the initial state, the spins of all chain atoms except the first two are oriented along the same direction. The spins of the first two atoms are flipped. Due to the exchange interaction, this initial state generates a spin flip wave along the chain. The expressions obtained for nonstationary quantum amplitudes of the flip probability waves for an even number of spins can be used for calculating quantum correlations between two spins separated by a large distance in a chain. Numerical calculations of the spin correlator reveal that the correlation between two spins in the chain occurs with a delay on the order of the time of propagation of the exchange interaction along the spin chain. After the delay, the spin correlation amplitude abruptly increases followed by subsequent oscillatory temporal behavior.     

Energy structure of a finite Haldane chain in Y2BaNi0.96Mg0.04O5 studied by high field electron spin resonance

This Letter presents the fine structure of energy levels for the edge states of a Haldane chain. In order to investigate the edge states, we have performed high field and multifrequency electron spin resonance (ESR) measurements of finite length S=1 antiferromagnetic chains in Y2BaNi0.96Mg0.04O5. Owing to the high spectral resolution by high fields and high frequencies, observed ESR signals can be separated into the contributions of the finite chains with various chain lengths. Our results clearly show that the edge spins actually interact with each other through the quantum spin chain and the interaction depends on the chain length N. This N dependence has been obtained experimentally for the first time, and shows that the correlation length xi in the real system is somewhat larger than that calculated by a simple Heisenberg model.     

Field-dependent nuclear relaxation of spins 1/2 induced by dipole-dipole couplings to quadrupole spins: LaF3 crystals as an example

A general theory of spin-lattice nuclear relaxation of spins I=1/2 caused by dipole-dipole couplings to quadrupole spins S1, characterized by a non-zero averaged (static) quadrupole coupling, is presented. In multispin systems containing quadrupolar and dipolar nuclei, transitions of spins 1/2 leading to their relaxation are associated through dipole-dipole couplings with certain transitions of quadrupole spins. The averaged quadrupole coupling attributes to the energy level structure of the quadrupole spin and influences in this manner relaxation processes of the spin 1/2. Typically, quadrupole spins exhibit also a complex multiexponential relaxation sensed by the dipolar spin as an additional modulation of the mutual dipole-dipole coupling. The proposed model includes both effects and is valid for an arbitrary magnetic field and an arbitrary quadrupole spin quantum number. The theory is applied to interpret fluorine relaxation profiles in LaF3 ionic crystals. The obtained results are compared with predictions of the 'classical' Solomon relaxation theory.     

Dynamics of multiple quantum coherences in dipole-coupling spins in solid

A perturbation method deals with dipolar coupling spins in solids is presented. As example of application the method, the multiple-quantum coherence dynamics in clusters of a linear chain of four nuclear spins and a ring of six spins coupled by dipole-dipole interaction are considered. The calculated 0Q and 2Q intensities in a linear chain of four nuclear spins and 6Q intensity in a ring of six spins vs. the duration of the preparation period agree well with the exact solutions (for linear chain of four nuclear spins) and simulation data (for linear chain of four nuclear spins and a ring of six spin).     

Single particle nature of the yrast line at high angular momentum in 152Dy

Linear polarization and Doppler shift recoil-distance decay curves for γ-ray transitions deexciting very high spin yrast states up to spin 36? in ¹⁵²Dy were measured with a delayed-promt γ-γ coincidence technique via the reactions ¹²²Sn (³⁴S, 4n) and ¹²⁴Sn(³²S, 4n), at 150 MeV incident beam energy. The deduced experimental transition probabilities are consistent with those obtained for non-rotational nuclei indicating that the yrast angular momentum originates mainly from the alignment of individual particle spins.     

Measurements of g-Factor of Rotational Band States in 82Sr

The g-factors of the positive parity rotational states up to spin I = 8^＋ for the ground state band in even-even nuclei S2Sr have been measured by a transient-magnetic-field ion implantation perturbed angular distribution method. The experimentally measured 9-factors increase with the increasing spin along the band and show that the g9/2 proton aligns only and the alignment starts from I =6^＋. The measured g-factors also indicate that the nuclei ^82Sr gain their spins by the quasi-proton alignment at higher spin.     

Two-qubit cells made of boron nitride nanotubes for a quantum computer

The electronic structure of boron nitride nanotubes (8, 0) with intercalated alkali metal atoms and alkaline-earth metal ions is studied. It is shown by calculation that the spin density is localized on individual atoms or ions. The antiferromagnetic state of a linear chain of atoms and ions turns out to be energetically more favorable. Exchange interaction between spins is fairly weak. Such systems are suggested to be used as two-qubit cells for a quantum computer.     

Exact solution of a coupled spin–electron linear chain composed of localized Ising spins and mobile electrons

Exact solution of a coupled spin–electron linear chain composed of localized Ising spins and mobile electrons is found. The investigated spin–electron model is exactly solvable by the use of a transfer-matrix method after tracing out the degrees of freedom of mobile electrons delocalized over a couple of interstitial (decorating) sites. The exact ground-state phase diagram reveals an existence of five phases with different number of mobile electrons per unit cell, two of which are ferromagnetic, two are paramagnetic and one is antiferromagnetic. We have studied in particular the dependencies of compressibility and specific heat on temperature and electron density.     

Phase diagram of the random Heisenberg antiferromagnetic spin-1 chain

We present a new perturbative real space renormalization group (RG) to study random quantum spin chains and other one-dimensional disordered quantum systems. The method overcomes problems of the original approach which fails for quantum random chains with spins larger than S=1/2. Since it works even for weak disorder, we are able to obtain the zero temperature phase diagram of the random antiferromagnetic Heisenberg spin-1 chain as a function of disorder. We find a random singlet phase for strong disorder. As the disorder decreases, the system shows a crossover from a Griffiths to a disordered Haldane phase.     

Ferromagnetism in diluted magnetic semiconductor quantum dot arrays embedded in semiconductors

We present an Anderson-type model Hamiltonian with exchange coupling between the localized spins and the confined holes in the quantum dots to study the ferromagnetism in diluted magnetic semiconductor (DMS) quantum dot arrays embedded in semiconductors. The hybridization between the quantum-confined holes in the quantum dots and the itinerant holes in the semiconductor valence band makes possible hole transfer between the DMS quantum dots, which can induce the long range ferromagnetic order of the localized spins. In addition, it makes the carrier spins both in the quantum dots and in the semiconductors polarized. The spontaneous magnetization of the localized spins and the spin polarization of the holes are calculated using both the Weiss mean field approximation and the self-consistent spin wave approximation, which are developed for the present model.Received: 17 Mars 2003, Published online: 30 January 2004PACS: 75.75. + a Magnetic properties of nanostructures - 75.30.Ds Spin waves - 75.50.Dd Nonmetallic ferromagnetic materials - 75.50.Pp Magnetic semiconductors     

Spin superstructure and noncoplanar ordering in metallic pyrochlore magnets with degenerate orbitals

We study double-exchange models with itinerant t(2g) electrons in spinel and pyrochlore crystals. In both cases the localized spins form a network of corner-sharing tetrahedra. We show that the strong directional dependence of t(2g) orbitals leads to unusual Fermi surfaces that induce spin superstructures and noncoplanar orderings for a weak coupling between itinerant electrons and localized spins. Implications of our results to ZnV(2)O(4) and Cd(2)Os(2)O(7) are also discussed.