Rectangular arrays of pyramidal recesses coated by silver film are investigated by means of polarization‐resolved nonlinear microscopy at 900 nm fundamental wavelength, demonstrating strong dependence of the dipole‐allowed SHG upon the lattice parameters. The plasmonic band gap causes nearly complete SHG suppression in arrays of 650 nm periodicity, whereas a sharp resonance at 550 nm periodicity is observed due to excitation of band edge Bloch states at fundamental frequency, accompanied by symmetry‐constrained interactions with similar modes at the second‐harmonic frequency. Additionally, coupling with modes at the bottom side of the silver film may lead to extraordinary optical transmission, opening a channel for SHG from the highly nonlinear GaAs substrate. Changing the lattice geometry enables SHG intensity modulation over three orders of magnitude, while the effective nonlinear anisotropy can be continuously switched between the two lattice directions, reaching values as high as ±0.96.
We demonstrate a high optoelectronic performance and application potential of our random network, with subwavelength diameter, ultralong, and high‐quality silver nanowires, stabilized on a substrate with a UV binder. Our networks show very good optoelectronic properties, with the single best figure of merit of ∼1686, and excellent stability under harsh mechanical strain, as well as thermal, and chemical challenge. Our network transparency strongly exceeds the simple shading limit. We show that this transmission enhancement is due to plasmonic refraction, which in an effective medium picture involves localized plasmons, and identify the inhomogeneous broadening as the key factor in promoting this mechanism. Such networks could become a basis for a next generation of ultrahigh‐performance transparent conductors.
The so‐called ‘flat optics’ that shape the amplitude and phase of light with high spatial resolution are presently receiving considerable attention. Numerous journal publications seemingly offer hope for great promises for ultra‐flat metalenses with high efficiency, high numerical aperture, broadband operation… We temperate the expectation by referring to the current status of metalenses against their historical background, assessing the technical and scientific challenges recently solved and critically identifying those that still stand in the way.
Due to the broad scattering spectral profiles, localized surface plasmon resonances (LSPRs) of Pd nanoparticles have low resolution and limited sensitivity for hydrogen detection. In this work, we use a simple light‐irradiation method to demonstrate that free‐space light can be efficiently coupled into and from the microfiber whispering‐gallery modes (WGMs) by the Pd nanoantennas. The nanoantenna–microfiber cavity system provides strong intermodal coupling between LSPRs and WGMs, and induces significant modulation of the scattering spectra. A measured full width at half‐maximum of 3.2 nm at 622.7 nm is obtained, which is the narrowest in Pd nanoparticle‐based LSPR structures reported up to now. The ultranarrow resonances offer enhanced sensitivity to hydrogen gas detection with a figure of merit reaching ∼2.22. Other advantages of the Pd nanoantenna–microfiber cavity system including independence of precise alignment of excitation light, large tunability of the resonant wavelengths, easy and low‐cost fabrication of the system, have also been demonstrated.
Traditional detour‐phase hologram is a powerful optical device for manipulating phase and amplitude of light, but it is usually not sensitive to the polarization of light. By introducing the light‐metasurface interaction mechanism to the traditional detour phase hologram, we design a novel plasmonic nano‐slits assisted polarization selective detour phase meta‐hologram, which has attractive advantages of polarization multiplexing ability, broadband response, and ultra‐compact size. The meta‐hologram relies on the dislocations of plasmonic slits to achieve arbitrary phase distributions, showing strong polarization selectivity to incident light due to the plasmonic response of deep‐subwavelength slits. To verify its polarization sensitive and broadband responses, we experimentally demonstrate two holographic patterns of an optical vortex and an Airy beam at p‐ and s‐polarized light with wavelengths of 532nm, 633nm and 780nm, respectively. Furthermore, we realize an application example of the meta‐hologram as a polarization multiplexed photonic device for multi‐channel optical angular momentum (OAM) generation and detection. Such meta‐holograms could find widespread applications in photonics, such as chip‐level beam shaping and high‐capacity OAM communication.
Surface plasmon polaritons (SPPs) have sparked enormous interest on nanophotonics beyond the diffraction limit for their remarkable capabilities of subwavelength confinements and strong enhancements. Due to the inherent polarization sensitivity of the SPPs [transverse‐magnetic (TM) polarization], it is a great challenge to couple the s‐polarized free‐space light to the SPPs. Here, an ultrasmall defect aperture (<λ2/2) is designed to directionally couple both the p‐ and s‐polarized incident beams to the single SPP mode in a broad bandwidth, which is guided by a subwavelength plasmonic waveguide. Simulations show that hot spots emerge at the sharp corners of the defect aperture when the incident beams illuminate it from the back side. The strong radiative fields from the hot spots are directionally coupled to the SPP mode because of the symmetry breaking of the defect aperture. By adjusting the structural parameters, both the unidirectional and bidirectional SPP coupling from the two orthogonal linear‐polarization incident beams are experimentally demonstrated. The polarization‐free coupling of the SPPs is of importance in circuits for fully optical processing of information with a deep‐subwavelength footprint.
The ability of generating arbitrary surface plasmon (SP) profiles in a controllable manner is of particular interest in designing plasmonic imaging, lithography and forcing devices. During the past decades, holography has gained enormous interest and achievements in free‐space three‐dimensional displays. Here, by applying a two‐dimensional version of holography, we experimentally demonstrate a generic method to control the SP profiles. Through controlling the orientation angles of two separated slits under circular polarization incidence, the amplitude and phase of the excited SPs can be freely manipulated, which allows direct generation of the desired SP profiles. A series of controllable SP holography schemes are theoretically and experimentally demonstrated, where the holographic SP profiles with high imaging quality can be dynamically modulated by varying the circular polarization handedness or orientation angle of linear polarization. The universality and simplicity of the proposed design strategies would offer promising opportunities for practical plasmonic applications.
Light manipulation is paramountly important to the fabrication of high‐performance optoelectronic devices such as solar cells and photodetectors. In this study, a high‐performance near‐infrared light nanophotodetector (NIRPD) was fabricated based on a germanium nanoneedles array (GeNNs array) with strong light confining capability, and single‐layer graphene (SLG) modified with heavily doped indium tin oxide nanoparticles (ITONPs), which were capable of inducing localized surface plasmon resonance (LSPR) under NIR irradiation. An optoelectronic study shows that after modification with ITONPs the device performance including photocurrent, responsivity and detectivity was considerably improved. In addition, the ITONPs@SLG/GeNNs array NIRPD was able to monitor fast‐switching optical signals, the frequency was as high as 1 MHz, with very fast response rates. Theoretical simulations based on finite‐element method (FEM) revealed that the observed high performance was not only due to the strong light‐confining capability of the GeNNs array, but also due to the plasmonic ITONPs‐induced hot electron injection. The above results suggest that the present NIRPD will have great potential in future optoelectronic devices application.
We report on the realisation of ultra‐small‐mode‐volume tunable dye lasers based on hemispherical open microcavities. The cavity mode volume is of the order of cubic micrometers, such that self‐diffusion of the dye molecules allows continuous wave operation over several minutes without the need for driven circulation. Such micro lasers could be integrated into lab‐on‐a‐chip devices. A rate‐equation model that incorporates the diffusion mechanism is used to predict the effect of the microcavity parameters on the lasing threshold.
Transport of subwavelength electromagnetic (EM) energy has been achieved through near‐field coupling of highly confined surface EM modes supported by plasmonic nanoparticles, in a configuration usually on a two‐dimensional (2D) substrate. Vertical transport of similar modes along the third dimension, on the other hand, can bring more flexibility in designs of functional photonic devices, but this phenomenon has not been observed in reality. In this paper, designer (or spoof) surface plasmon resonators (‘plasmonic meta‐atoms’) are stacked in the direction vertical to their individual planes in demonstrating vertical transport of subwavelength localized surface EM modes. The dispersion relation of this vertical transport is determined from coupled‐mode theory and is verified with a near‐field transmission spectrum and field mapping with a microwave near‐field scanning stage. This work extends the near‐field coupled resonator optical waveguide (CROW) theory into the vertical direction, and may find applications in novel three‐dimensional slow‐light structures, filters, and photonic circuits.
All‐optical signal processing on nonlinear photonic chips is a burgeoning field. These processes include light generation, optical regeneration and pulse metrology. Nonlinear photonic chips offer the benefits of small footprints, significantly larger nonlinear parameters and flexibility in generating dispersion. The nonlinear compression of optical pulses relies on a delicate balance of a material's nonlinearity and optical dispersion. Recent developments in dispersion engineering on a chip are proving to be key enablers of high‐efficiency integrated optical pulse compression. We review the recent advances made in optical pulse compression based on nonlinear photonic chips, as well as the future outlook and challenges that remain to be solved.
Dewetting of thin metal films is one of the most widespread method for functional plasmonic nanostructures fabrication. However, simple thermal‐induced dewetting does not allow to control degree of nanostructures order without additional lithographic process steps. Here we propose a novel method for lithography‐free and large‐scale fabrication of plasmonic nanostructures via controllable femtosecond laser‐induced dewetting. The method is based on femtosecond laser surface pattering of a thin film followed by a nanoscale hydrodynamical instability, which is found to be very controllable under specific irradiation conditions. We achieve control over degree of nanostructures order by changing laser irradiation parametrs and film thickness. This allowed us to exploit the method for the broad range of applications: resonant light absorbtion and scattering, sensing, and potential improving of thin‐film solar cells.
A spaser is a nanoplasmonic counterpart of a laser, with photons replaced by surface plasmon polaritons and a resonant cavity replaced by a metallic nanostructure supporting localized plasmonic modes. By combining analytical results and first‐principle numerical simulations, we provide a comprehensive study of the ultrafast dynamics of a spaser. Due to its highly‐nonlinear nature, the spaser is characterized by a large number of interacting degrees of freedom, which sustain a rich manifold of different phases we discover, describe and analyze here. In the regime of strong interaction, the system manifests an irreversible ergodic evolution towards the configuration where energy is equally shared among all the available degrees of freedom. Under this condition, the spaser generates ultrafast vortex‐like lasing modes that are spinning on the femtosecond scale and whose direction of rotation is dictated by quantum noise. In this regime, the spaser acquires the character of a nanoparticle with an effective spin. This opens up a range of interesting possibilities for achieving unidirectional emission from a symmetric nanostructure, stimulating a broad range of applications for nanoplasmonic lasers as unidirectional couplers and random information sources.
We uncover that the breaking point of the ‐symmetry in optical waveguide arrays has a dramatic impact on light localization induced by the off‐diagonal disorder. Specifically, when the gain/loss control parameter approaches a critical value at which ‐symmetry breaking occurs, a fast growth of the coupling between neighboring waveguides causes diffraction to dominate to an extent that light localization is strongly suppressed and the statistically averaged width of the output pattern substantially increases. Beyond the symmetry‐breaking point localization is gradually restored, although in this regime the power of localized modes grows upon propagation. The strength of localization monotonically increases with disorder at both broken and unbroken ‐symmetry. Our findings are supported by statistical analysis of parameters of stationary eigenmodes of disordered‐symmetric waveguide arrays and by analysis of dynamical evolution of single‐site excitations in such structures.
Entangled photon pairs must often be spatially separated for their subsequent manipulation in integrated quantum circuits. Separation that is both deterministic and universal can in principle be achieved through anti‐coalescent two‐photon quantum interference. However, such interference‐facilitated pair separation (IFPS) has not been extensively studied in the integrated setting, which has important implications on performance. This work provides a detailed review of IFPS and examines how integrated device dependencies such as dispersion impact separation fidelity and interference visibility. The analysis applies equally to both on‐chip and in‐fiber implementations. When coupler dispersion is present, the separation performance can depend on photon bandwidth, spectral entanglement and the dispersion. By design, reduction in the separation fidelity due to loss of non‐classical interference can be perfectly compensated for by classical wavelength demultiplexing effects. This work informs the design of devices for universal photon pair separation of states with tunable arbitrary properties.
About twenty years ago, in the autumn of 1996, the first white light‐emitting diodes (LEDs) were offered for sale. These then‐new devices ushered in a new era in lighting by displacing lower‐efficiency conventional light sources including Edison's venerable incandescent lamp as well as the Hg‐discharge‐based fluorescent lamp. We review the history of the conception, improvement, and commercialization of the white LED. Early models of white LEDs already exceeded the efficiency of low‐wattage incandescent lamps, and extraordinary progress has been made during the last 20 years. The review also includes a discussion of advances in blue LED chips, device architecture, light extraction, and phosphors. Finally, we offer a brief outlook on opportunities provided by smart LED technology.
This article presents a novel III‐V on silicon laser. This work exploits the phenomenon that a passive silicon cavity, side‐coupled to a III‐V waveguide, will provide high and narrow‐band reflectivity into the III‐V waveguide: the resonant mirror. This results in an electrically pumped laser with a threshold current of 4 mA and a side‐mode suppression ratio up to 48 dB.
Open‐access microcavities are emerging as a new approach to confine and engineer light at mode volumes down to the λ3 regime. They offer direct access to a highly confined electromagnetic field while maintaining tunability of the system and flexibility for coupling to a range of matter systems. This article presents a study of coupled cavities, for which the substrates are produced using Focused Ion Beam milling. Based on experimental and theoretical investigation the engineering of the coupling between two microcavities with radius of curvature of 6 m is demonstrated. Details are provided by studying the evolution of spectral, spatial and polarisation properties through the transition from isolated to coupled cavities. Normal mode splittings up to 20 meV are observed for total mode volumes around . This work is of importance for future development of lab‐on‐a‐chip sensors and photonic open‐access devices ranging from polariton systems to quantum simulators.
We report on the theoretical investigation of plasmonic resonances in metallic Möbius nanorings. Half‐integer numbers of resonant modes are observed due to the presence of an extra phase π provided by the topology of the Möbius nanostrip. Anomalous plasmon modes located at the non‐orientable surface of the Möbius nanoring break the symmetry that exist in conventional ring cavities, thus enable far‐field excitation and emission as bright modes. The far‐field resonant wavelength as well as the feature of half‐integer mode numbers is constant to the change of charge distribution on the Möbius nanoring due to the topology of Möbius ring. Owing to the ultra‐small mode volume induced by the remaining dark feature, an extremely high sensitivity as well as a remarkable figure of merit is obtained in our numerical calculations for sensing performance. The topological metallic nanostructure provides a novel platform for the investigation of localized surface plasmon modes exhibiting unique phenomena for potential plasmonic applications.
Owing to the unique ability of nanostructured metals to confine and enhance light waves along metal‐dielectric interfaces, plasmonics has enabled unprecedented flexibility in manipulating light at the deep‐subwavelength scale. With regard to the spectral behavior of plasmonic resonances, the spectral location of a resonance can be tailored with relative ease while the control over the spectral linewidth represents a more daunting task. In this paper, we present sharp resonance features by introducing dark plasmonic modes in diatomic gratings. The induced asymmetry in the metallic structure facilitates the generation of a dark mode with significantly suppressed radiative loss leading to an ultra‐sharp spectral feature ∼5 nm wide. We further use this metallic structure as an optoelectronic platform for the transduction of light waves to electrical signals via a plasmoelectric effect. The light concentrating ability of dark plasmonic modes, in conjunction with the ultra‐sharp resonance feature at a relatively low loss offers a novel route to enhanced light‐matter interactions with high spectral sensitivity for diverse applications.
