LiNbO_3:Fe晶体的光折变对喇曼光谱的影响(Ⅱ)

继文献[1]之后,我们又研究了掺Fe浓度为0.07％的LiNbO_3:Fe晶体的光折变对喇曼光谱的影响。发现在x(zx)z和y(zy)z配置下出现异常。这可以由异常声子的极化电场与光折变在晶体中形成的强空间电荷场的相互作用来解释。     

在局域非线性响应的光折变晶体中的对称光扇

在具有非局域非线性响应的所有光折变晶体中几乎都能观察到光折变光扇效应．最近我们在具有局域非线性响应的光折变晶体（LiNbO₃∶Fe）观察到对称光扇．基于前向简并三波作用，从理论上研究了这种对称光扇的形成 关键词：     

运动折射率相位栅和背向光折变散射

本文按照Kukhtarev的光折变理论讨论了在LiNbO₃:Fe晶体内自发形成的运动折射率相位栅和由它所引起的强烈的背向光折变散射。 关键词：     

光生伏打-光折变介质中光学涡旋孤子

简化了描述光生伏打光折变效应的模型方程.给出了光生伏打空间电荷场的形式解.讨论了单光束在光生伏打、自散焦光折变介质(LiNbO3∶Fe晶体)中的三维传播行为.指出在适当近似条件下,光生伏打光折变非线性可以维持圆对称的涡旋孤子. 关键词：     

LiNbO3:Fe晶体的光折变对喇曼光谱的影响

我们观察到了LiNbO₃:Fe晶体中某些几何配置下十分异常的喇曼光谱现象。这一现象是与该晶体光折变后出现的异常光散射现象相联系的。 关键词：     

光生伏打LiNbO3:Fe晶体从自散焦到等效“自聚焦”的动态转换

实验研究了在一定条件下LiNbO₃:Fe晶体中从自散焦到等效“自聚焦”转换的动态行为,提出了出现自聚焦的物理机理为双相位共轭的法布里珀罗干涉腔中的多光束干涉与光折变效应的共同结果.该效应有希望在光折变自散焦介质中形成亮空间孤子 关键词： 自散焦 自聚焦 光折变     

c向切割LiNbO3∶Fe晶体中光折变光散射

提出了一个新的理论机理:c向切割LiNbO₃∶Fe晶体中光折变背向光散射是由光生伏特电流的不均匀性引起的,并经过理论计算,比较成功的解释了实验观察到的各种现象 关键词： 光折变 散射 光生伏特     

快速响应的光致折射率改变效应的实验研究

在LiNbO₃∶Fe晶体薄片中观察到快速响应（<0.1s）、各向同性、并具有信息存储功能的一种光致折射率改变效应.基于它的特征及其与光折变效应的区别，初步讨论了产生该效应的物理机理. 关键词： 光致折射率改变效应 光折变效应 热释电效应     

光折变光子晶格中空间二次谐波的产生

用干涉法在自散焦光折变晶体 LiNbO₃：Fe中写入光子晶格的动态过程中，发现了双光束干涉条纹一分为二，四光束干涉点阵一分为四的分裂现象. 研究证明：这是干涉条纹空间频率的倍频现象，是入射的干涉光场与写入的光子晶格之间相互作用的结果. 本实验说明利用光折变效应可以容易地实现干涉光场空间频率的倍频和空间高次谐波的产生，并可利用产生的空间谐波感应出二倍频和高倍频的光折变光子晶格. 关键词： 光折变晶体 光子晶格 空间谐波     

铟掺杂对Fe∶LiNbO3晶体近红外光折变性能的影响

采用在Fe∶LiNbO3中掺入了铟离子生长的双掺杂In∶Fe∶LiNbO3晶体,以波长为1064nm的近红外会聚光束作为记录光源,通过数字观测装置,对比研究了铟离子掺入前后Fe∶LiNbO3晶体和In∶Fe∶LiNbO3晶体的光折变性能。实验研究结果表明,铟离子掺入后晶体的光折变响应速度和抗光折变能力明显提高,饱和折射率变化量降低。初步分析认为,In∶Fe∶LiNbO3晶体光折变性能的增强是由于掺入的铟离子取代了部分光折变敏感中心,降低了光敏中心的数量,导致晶体光电导增大,响应时间随之缩短。     

LiNbO3:Fe晶体中光感应自衍射观察

用He-Ne激光束沿LiNbO₃:Fe晶体的x轴或y轴方向聚焦照射较薄样品时,在晶体后面的屏上观察到十分规则的衍射图样。这与前人在该晶体中观察到的由晶体中光折变形成的位相噪音栅引起的光感应光散射现象迥然不同。我们观察到的这种自衍射图样,可用聚焦激光束入射时在晶体中形成的复杂类透镜效应和自衍射理论来解释。它可以清楚地表明聚焦激光束入射时晶体中光折变过程的特点、还可由衍射条纹的数目直接推算晶体中光折变△n的最大值。文中还实验研究与讨论了光感应自衍射的形成条件及其与光感应光散射的竞争关系。 关键词：     

新型聚偶氮苯取向增强光折变效应及全息存储

合成了新型偶氮分子偶氮二苯胺ADPA(Azo-diphenylamine),将其掺入聚乙烯咔唑Poly(N-Vinylcarba-zole)(PVK)和聚丙烯丁酯(Poly-butylacrylate)(PBA)的聚合物(PVK-PBA)以及三硝基芴酮2,4,7-trinitro-9-flu-orenone(TNF)聚合制成薄膜器件。结果表明掺杂偶氮苯聚合物薄膜在非共振吸收下具有强的光致取向增强光折变效应。光致折射率变化值Δn达到1.3×10-3以上。样品在两相干光束作用下,可建立光折射率光栅,其衍射效率可超过30%,实现了光全息存储。讨论了影响折射率光栅的因素,并对全息存储相关结果形成的机制进行了分析。     

Femtosecond laser embedded grating micromachining of flexible PDMS plates

We report on the femtosecond laser micromachining of photo-induced embedded diffraction grating in flexible Poly (Dimethly Siloxane) (PDMS) plates using a high-intensity femtosecond (130 fs) Ti: sapphire laser (λ_p = 800 nm). The refractive index modifications with diameters ranging from 2 μm to 5 μm were photo-induced after the irradiation with peak intensities of more than 1 × 10¹¹ W/cm². The graded refractive index profile was fabricated to be a symmetric around from the center of the point at which femtosecond laser was focused. The maximum refractive index change (Δn) was estimated to be 2 × 10⁻³. By the X-Y-Z scanning of sample, the embedded diffraction grating in PDMS plate was fabricated successfully using a femtosecond laser.     

Laser induced memory bits in photorefractive LiNbO3 and LiTaO3

We study experimentally the formation of refractive index voxels (volume elements) in photorefractive LiNbO₃ and LiTaO₃ crystals illuminated with high irradiance femtosecond laser pulses. We used 150 fs pulses at 800 nm wavelength (energy 6–50 nJ) tightly focused inside the crystals in a single shot regime. This resulted in a formation of a micrometer size region of elevated refractive index, which may be used as memory bits in information storage/retrieval application. The maximum refractive index change of 5×10⁻⁴ was recorded in undoped LiNbO₃ at an average light intensity of ∼TW/cm² that is close to the breakdown threshold. A simple setup for photorefractive recording and in situ monitoring of the refractive index changes has been proposed. M. Sūdžius leaves from: the Institute of Materials Science and Applied Research of Vilnius University, Lithuania.     

Composition-tuned refractive index and oscillator parameters in TlGaxIn1−xS2 layered mixed crystals (0≤x≤1)

The optical properties of TlGa_xIn_1?xS₂ mixed crystals have been studied through transmission and reflection measurements in the wavelength range 400–1100 nm. These measurements allowed determination of the spectral dependence of the refractive index for all compositions of the mixed crystals studied. The dispersion of the refractive index is discussed in terms of the Wemple–DiDomenico single-effective-oscillator model. The compositional dependences of the refractive index dispersion parameters (oscillator energy, dispersion energy and zero-frequency refractive index) were revealed.     

一维新型阶梯函数光子晶体透射特性

研究了阶梯型折射率n₂₂、n₁₁(阶梯分布高度)的大小、对应的分布厚度、不同入射角以及缺陷模对阶梯函数型光子晶体透射特性的影响.由费马原理给出光在函数光子晶体中的运动方程,再由电磁传播理论给出函数光子晶体的传输矩阵,进一步推导出函数光子晶体的透射率以及电场分布的表达式.研究表明,1)随n₂₂,n₁₁大小或者厚度改变,其禁带变宽;2)随光的入射角增加,其禁带变窄;3)当加入缺陷层时,随着缺陷层介质折射率增加,缺陷模强度减小且位置发生红移;4)在函数光子晶体中,缺陷层前电场分布保持不变,而在缺陷层处以及之后的电场强度都明显增强,这不同于常规光子晶体的电场分布仅在缺陷层处局域增强.     

Photosensitive post tuning of chalcogenide Te20As30Se50 narrow bandpass filters

We present an experimental study on the photosensitive properties of narrow bandpass filters based on a chalcogenide Te₂₀As₃₀Se₅₀ (TAS) spacer. The transmittance curve of single TAS layer was shifted towards long wavelength direction after 2 h exposure by Xenon arc lamp. The refractive index and extinction coefficient were both increased together with a red shift of optical gap. A maximum 1.7% photo-induced effect was observed. Narrow band filters constituted by TAS and cryolite were manufactured by electron beam deposition. The transmittance spectrum of the filter during the exposure by a wide band source was in situ measured and the resonant wavelength was observed to turn longer gradually till saturation. A spatially localized central wavelength change up to 5.7 nm was finally obtained. The stability of the photo-induced effect was studied and some comments were given at the end of this paper.     

低功率近红外光的偏振方向对光致折射率变化影响的实验研究

研究了利用低功率近红外光辐照In:Fe:LiNbO3晶体时写入光束的偏振方向对光致折射率变化(Δn)的影响.分别采用正常偏振(o光)和非常偏振(e光)的近红外细激光束,在In:Fe:LiNbO3晶体中进行了光折变实验.研究表明,两种偏振方向引起晶体的Δn实测曲线相似,但变化规律恰好相反,o光引起的折射率变化量约是e光的3倍左右.近红外光写入下两种偏振光束引起晶体的Δn分布规律都不同于可见光,尤其是e光辐照区域中心晶体的折射率升高.因此,通过选择不同偏振方向的近红外光可以在光折变晶体中制作不同折射率分布的非线性光学器件.     

Anisotropy of the refractive index and electro-optical effect in Tl<Subscript>1–x</Subscript>Ag<Subscript>x</Subscript>GaSe<Subscript>2</Subscript> crystals (0 ≤ <Emphasis Type="Italic">x</Emphasis> ≤ 0.025)

Anisotropy of the refractive index and electro-optical effect in Tl_1–xAg_xGaSe₂ crystals (0 ≤ x ≤ 0.025) is studied. It is shown that the refractive indices increase as they approach the intrinsic absorption band. It is established that when light and an external electric field are directed along a selected c crystallographic axis, the electro-optical effect is quadratic; if the field is oriented perpendicular to the c axis and light propagates along the latter, the electro-optical effect is linear.