Femtosecond measurements of the time of flight of photons in a three-dimensional photonic crystal

We report on experimental measurements of the propagation behavior of short optical pulses in a three-dimensional photonic crystal in the visible spectrum. The propagation delay of 70 fs light pulses transmitted through a sample of a fcc synthetic opal at frequencies lying in a photonic stop band was measured directly using a time-of-flight technique. Taking into account spectral reshaping of the transmitted pulses as well as the residual frequency chirp of the incoming pulses, it is found that the pulses significantly slow down at the photonic band edges.     

Dispersion-insensitive low-coherent pulses emerging from nonlinear polarization switching

We have experimentally investigated low-repetition nanosecond pulses delivered from an erbium-doped fiber (EDF) laser operating in ultra-large anomalous dispersion regime. The output pulses with rectangular profile and Gaussian spectrum almost keep invariable when they propagate through either normal- or anomalous-dispersion fibers. After nanosecond pulses are amplified via a two-stage EDF amplifier, they are broken up and exhibited as flatly broadened supercontinuum from 1520 to 1700 nm if amplified pulses are launched into a 10-km single-mode fiber, whereas the pulses retain the same duration with a broadband supercontinuum from 1200 to 1750 nm if they are input into a 100-m highly-nonlinear low-dispersion photonic-crystal fiber (PCF). The experimental observations demonstrate that the nanosecond pulses result from nonlinear polarization switching and can be regarded as dispersion-insensitive low-coherent pulses rather than compressible pulses.     

Ultrafast pulse retiming by cross-phase modulation in an anomalous-dispersion polarization-maintaining fiber

Retiming of signal pulses by orthogonally polarized control pulses copropagating in an anomalous-dispersion low-birefringence polarization-maintaining fiber is demonstrated. Through walk-off-free cross-phase modulation in a 500 m long fiber, optical pulses at a 10 GHz rate are retimed by as much as +/- 2 ps.     

19 fs shaped ultraviolet pulses

We report the generation of shaped tunable ultrashort ultraviolet pulses with full control over the spectral phase and amplitude. The output of a noncollinearly phase-matched optical parametric amplifier is shaped in phase and amplitude by a liquid-crystal spatial light modulator. The resulting structured visible pulses are transferred into the ultraviolet by sum-frequency mixing with strongly chirped 775 nm pulses. Single, double, and triple pulses at 344 nm with subpulses as short as 19 fs are explicitly demonstrated. The method can easily be adapted to arbitrarily shaped pulses throughout the 295-370 nm range.     

Mutual coherence of supercontinuum pulses collinearly generated in bulk media

We report the collinear generation of white light pulses in bulk media by phase-locked and time-delayed intense laser pulses. The mutual phase coherence of the pump pulses is fully transferred to the two supercontinua, which thus show a highly-modulated two-pulse spectrum extending from all of the visible down to the near-infrared. We have investigated the effects of changing the relative delay between the pulses as well as the role of imbalances in the pump energy, and we have found that, at least in a limited energy interval, the mutual phase coherence of the two white-light pulses is surprisingly robust.     

Linear phase slope in pulse design: application to coherence transfer

Using optimal control methods, robust broadband excitation pulses can be designed with a defined linear phase dispersion. Applications include increased bandwidth for a given pulse length compared to equivalent pulses requiring no phase correction, selective pulses, and pulses that mitigate the effects of relaxation. This also makes it possible to create pulses that are equivalent to ideal hard pulses followed by an effective evolution period. For example, in applications, where the excitation pulse is followed by a constant delay, e.g. for the evolution of heteronuclear couplings, part of the pulse duration can be absorbed in existing delays, significantly reducing the time overhead of long, highly robust pulses. We refer to the class of such excitation pulses with a defined linear phase dispersion as ICEBERG pulses (Inherent Coherence Evolution optimized Broadband Excitation Resulting in constant phase Gradients). A systematic study of the dependence of the excitation efficiency on the phase dispersion of the excitation pulses is presented, which reveals surprising opportunities for improved pulse sequence performance.     

Pattern pulses: design of arbitrary excitation profiles as a function of pulse amplitude and offset

A novel class of pulses is presented which can be regarded as a generalization of both frequency-selective pulses and B1-selective pulses. The excitation profile of these pulses forms a pre-defined pattern in two dimensions, which are spanned by pulse offset and radio-frequency (RF) amplitude. The presented pulses were designed numerically based on principles of optimal control theory. For simple test patterns, we demonstrate the flexibility of this approach by simulations and experiments. This previously unknown flexibility may trigger novel applications in NMR spectroscopy and imaging. As a first practical application, we demonstrate a direct approach for calibrating RF pulses.     

Propagation of femtosecond pulses in large-mode-area, higher-order-mode fiber

We demonstrate propagation of 14 nJ femtosecond pulses through a large-mode-area, higher-order-mode (HOM) fiber with an effective area of 2100 microm2. The pulses propagate stably in the LP07 mode of the fiber through lengths as long as 12 m. The strongly chirped pulses exiting the amplifier fiber are dechirped by the high-order-mode fiber, resulting in pulses with a peak power of 61 kW after propagation in 5 m of the positive-dispersion fiber. A small amount of self-phase modulation is observed in the compressed pulses and is described well by a nonlinear Schr?dinger equation model that takes into account the measured effective area and dispersion of the HOM fiber.     

Supercontinuum generation in a standard fiber pumped by noise-like pulses from a figure-eight fiber laser

We report the experimental study of broadband spectrum generation in a piece of standard fiber (SMF-28) using as the pump a train of noise-like pulses, or sub-nanosecond packets of sub-ps pulses with randomly varying amplitudes. The pulses are generated by an erbium-doped figure-eight fiber laser, and present a wide (∼50 nm) optical spectrum, which represents a significant advantage to seed the generation of new frequencies. Another advantage of the pulses is their relatively large energy, as they are made up of a large number of ultrashort pulses. After amplification with an Erbium Doped Fiber Amplifier (EDFA), the pulses were injected in a 0.75 km length of SMF-28 fiber. We obtained experimentally at the end of the fiber an output signal spectrum extending from 1530 nm to at least 1750 nm (the upper limit of the spectrum analyzer) for pump pulses with an average power of 20.4 mW, corresponding to a few kilowatts peak power. The spectral broadening is due to Raman self-frequency shift (SFS). It is noteworthy that the spectrum of the newly created frequencies was extremely uniform over the range of measurement. Considering that the Raman shift is directly related to the pump pulse duration, spectral flatness is a direct consequence of the random distribution of amplitudes and durations of the pulses in the packet. Finally, the results show the capabilities of noise-like pulses from a fiber laser for applications in supercontinuum generation based on nonlinear phenomena such as Raman SFS.     

Mid-infrared pulse generation using a sub-picosecond OPO

We describe a synchronously pumped LBO parametric oscillator pumped by a cw mode-locked Ti:Sapphire laser. We demonstrate the synchronization between the pump pulses and the signal pulses by measuring a 100 fs cross correlation. We then generate pulses tunable from 2.6 to 5.3 µm by mixing the signal and idler pulses in an AgGaS₂ crystal and obtain as much as 400 µW of average power.     

石墨烯被动锁模全正色散掺镱光纤激光器中的暗脉冲及其谐波

报道了一种基于石墨烯被动锁模的全正色散掺镱环形光纤激光器. 在激光器腔中应用激光诱导沉积法制备的石墨烯可饱和吸收体, 通过调节抽运光功率和偏振控制器的角度分别得到了明脉冲及其二阶谐波, 暗明脉冲对和暗脉冲及其二、三阶谐波这三类不同的脉冲. 其中, 暗明脉冲对和暗脉冲在基于石墨烯被动锁模的掺镱光纤激光器实验中都是第一次被观察到. 本文根据实验结果结合模拟分析了暗脉冲的产生机理, 并研究对比了明脉冲谐波和暗脉冲谐波产生的原因.     

Transform-limited spectral compression by self-phase modulation of amplitude-shaped pulses with negative chirp

Spectral compression by self-phase modulation of amplitude- and phase-shaped pulses is demonstrated as superior compared to pulses that have only been phase shaped. We synthesize linearly negatively chirped parabolic pulses, which we send through a nonlinear photonic crystal fiber, in which self-phase modulation compresses the spectrum of the pulses to within 20% of the Fourier transform limit.     

Shaping of few-cycle laser pulses via a subwavelength structure

We theoretically investigate the propagation of few-cycle laser pulses in resonant two-level dense media with a sub- wavelength structure, which is described by the full Maxwell-Bloch equations without the frame of slowly varying envelope and rotating wave approximations. The input pulses can be shaped into shorter ones with a single or less than one optical cycle. The effect of the parameters of the subwavelength structure and laser pulses is studied. Our study shows that the media with a subwavelength structure can significantly shape the few-cycle pulses into a subcycle pulse, even for the case of chirp pulses as input fields. This suggests that such subwavelength structures have potential application in the shaping of few-cycle laser pulses.     

High-average-power femtosecond pulse generation in the blue using BiB3O6

Efficient generation of tunable femtosecond pulses in the blue is reported in the nonlinear crystal BiB3O6. By use of fundamental pulses from a mode-locked Ti:sapphire laser at 76 MHz, single-pass second-harmonic average powers of as much as 830 mW have been generated at 50% conversion efficiency, and a tunable range of 375-435 nm in the blue is demonstrated. Temporal measurements using cross correlation of the fundamental and second-harmonic pulses in a 100-microm-thick beta-BaB2O4 crystal result in blue pulse durations of 220 fs for 130-fs fundamental pulses. Direct experimental comparison with beta-BaB2O4 confirms the superior performance BiB3O6 for second-harmonic generation of femtosecond pulses.     

Pulse properties of a synchronously mode-locked,cavity dumped,picosecond dye laser system

A synchronously mode-locked, cavity-dumped picosecond dye laser is described. The structure and intensity of the picosecond pulses measured under different conditions are reported. It was found that the structure of the pulses from the synchronously pumped dye laser depends critically on the length of the Ar⁺ laser pulses. At the shortest Ar⁺ laser pulses of about 70 ps the dye pulses are as short as 1.1 ps. With Ar⁺ laser pulses of 200 ps the dye laser pulses contains a broad satellite pulse which contains a large fraction of the total intensity. When a cavity dumper is added to the system one gets dye laser pulses 15–20 ps long with a substructure, which indicates incomplete mode-locking. Well mode-locked 1.5–2.0 ps pulses were obtained in the red part of the dye laser action spectrum, i.e. 620–650 nm for R6G, 595–608 nm for R 110 and 657–662 nm for RB, respectively. Addition of mode-locking dyes also improved the pulse quality at some wavelengths.     

Generation of intense,carrier-envelope phase-locked few-cycle laser pulses through filamentation

Intense, well-controlled light pulses with only a few optical cycles start to play a crucial role in many fields of physics, such as attosecond science. We present an extremely simple and robust technique to generate such carrier-envelope offset (CEO) phase locked few-cycle pulses, relying on self-guiding of intense 43-fs, 0.84 mJ optical pulses during propagation in a transparent noble gas. We have demonstrated 5.7-fs, 0.38 mJ pulses with an excellent spatial beam profile and discuss the potential for much shorter pulses. Numerical simulations confirm that filamentation is the mechanism responsible for pulse shortening. The method is widely applicable and much less sensitive to experimental conditions such as beam alignment, input pulse duration or gas pressure as compared to gas-filled hollow fibers. PACS 45.65.Ky; 42.65.Re     

Femtosecond terahertz radiation from femtoslicing at BESSY

Femtosecond far-infrared radiation pulses in the THz spectral range were observed as a consequence of the energy modulation of 1.7 GeV electrons by femtosecond laser pulses in the BESSY storage ring in order to generate femtosecond x-ray pulses ("femtoslicing"). In addition to being crucial for diagnostics of the laser-electron interaction, the THz radiation itself is useful for experiments where intense ultrashort THz pulses of well-defined temporal and spectral characteristics are required.     

圆偏振光和线偏振光在正常色散材料中的时空自压缩

实验研究了圆偏振和线偏振高强度飞秒激光脉冲在正常色散材料中传输时的时空自压缩现象。实验中利用BK7玻璃作为正色散材料,比较研究了不同偏振入射情况下脉冲波形及频谱的变化规律。圆偏振光入射时,可以获得更短脉冲宽度的压缩脉冲和更窄的光谱宽度。在圆偏振光入射条件下,50 fs入射脉冲成功地自压缩到了19 fs,获得了大于2.5倍的压缩倍率。所以利用圆偏振光可以获得更短压缩脉冲,更大能量,更好光束质量的激光。     

Impact of third-order dispersion on the generation of wave-breaking free pulses in ultrafast fiber lasers

Wave-breaking free pulses generated in passively mode-locked fiber lasers can tolerate a certain cubic phase delay induced by third-order dispersion without losing pulse quality. We demonstrate that the spectral as well as the temporal profile of the pulses become asymmetric. The generated pulses had a pulse energy up to 3.5nJ and could be externally compressed down to 145fs. The fact that the pulses could always be dechirped within 10% of the Fourier limit points out the linearity of the chirp. The pulse asymmetry was also observed in the output coupling characteristic of the mode-locking mechanism.     

Generation of 2-nJ pulses from a femtosecond ytterbium fiber laser

We report a mode-locked ytterbium fiber laser that generates femtosecond pulses with energies as large as 2.2 nJ. This represents a 20-fold improvement in pulse energy compared with that of previously reported femtosecond Yb fiber lasers. The laser produces pulses as short as 52 fs, which are to our knowledge the shortest pulses to date from a Yb fiber laser. The laser is diode pumped by a wavelength-division multiplexing coupler, which leads to excellent stability.