| Femtosecond Dynamics of Energy Transfer in Native B800-B850 and B800-Released LH2 Complexes of Rhodobacter Sphaeroides |
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| 作者姓名： | 刘伟民 朱荣毅 夏辰安 刘源 徐春和 钱士雄 |
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| 作者单位： | [1]DepartmentofPhysics,FudanUniversity,Shanghai200433 [2]NationalKeyLaboratoryofSurfaceScience,FudanUniversity,Shanghai200433 [3]ShanghaiInstituteofPlantPhysiologyandEcology,ShanghaiInstituteforBiologicalSciences,ChineseAcademyofSciences,Shanghai200032 |
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| 摘 要： | Two kinds of antenna complexes LH2 of Rhodobacter sphaeroides, wild type RS601 and the removal of B800pigments (B800-released), were used in our experiment. These two LH2 complexes show quite different behaviour in absorption and femtosecond dynamics. By using the femtosecond pump-probe technique, the energy transfer processes occurring in two complexes were studied. Because of removing the B800 pigment from the LH2 in B800-released LH2 complex, the energy transfer between the B800 to B850 pigment was completely eliminated, while the pure internal energy transfer within the exciton states of B850 pigment could be carefully investigated. The results show that, at B800 absorption band, B800-released LH2 obviously shows a dominated transient absorption different from the photobleaching observed in RS601; while at the B850 band, these two complexes show similar photobleaching behaviour.
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| 关 键 词： | 飞秒力学 能量传递 飞秒泵探针技术 光合作用 吸收光谱 光子动力学 延迟时间 |
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