两种烷基碘化物分子理论研究及其发射谱测量

利用密度泛函理论(DFT)的B3LYP方法, 对烷基碘化物分子C2H2F3I和n-C3H4F3I的C—I解离势能曲线进行了理论计算, 并采用B3LYP方法和MPn(n=2, 3, 4)方法精确计算了C—I键解离能. 解离能计算进行了零点振动能(ZPVE)校正, 并运用完全均衡校正法对基函数重叠误差(BSSE)进行校正. 利用微波放电激励方法, 对C2H2F3I和n-C3H4F3I的发射谱进行观测. 实验结果表明, 通过微波放电激励这两种分子, 均可产生1315 nm发射谱, 说明利用微波放电可使C2H2F3I和n-C3H4F3I分子的C—I键解离, 从而产生碘原子.     

介质参数对受激布里渊散射特性的影响

 采用一维瞬态模型对受激布里渊散射（SBS）过程进行了数值模拟，研究了介质参数对SBS特性的影响规律；选取FC-72、FC-75、CCl₄、CS₂、丙酮、苯以及CCl₂/乙醇的混合溶液等作为散射介质，在Nd∶YAG调Q激光系统下进行了实验研究，比较了各种介质所产生的SBS脉宽、能量反射率和波形之间的差异，由此讨论了介质参数对SBS特性的影响。结果表明，介质增益系数越大，吸收系数越小，SBS能量反射率就越大；吸收系数越大，产生的SBS脉宽就越窄；声子寿命越短，SBS波形前沿就越陡，并且越容易出现调制现象。     

混合介质的SBS参数随混合比变化的研究

从混合介质的折射率、黏度、密度和声速等物理量随混合比的变化关系入手,推导出了混合介质的布里渊线宽、声子寿命和增益系数等受激布里渊散射(SBS)参数随混合比的变化关系.数值模拟了HT-70/FC-72混合介质的布里渊线宽、声子寿命和增益系数随FC-72体积分数的变化关系,并测定了该混合介质的吸收系数和光学击穿阈值随FC-72体积分数的变化关系.结果表明,HT-70/FC-72混合介质的SBS参数随FC-72体积分数单调变化,不出现极值现象.混合介质的选用不仅增加了SBS介质的种类,而且能够满足SBS系统对不 关键词： 受激布里渊散射 混合介质 SBS参数     

Investigation of stimulated Brillouin scattering for broadband KrF laser

Stimulated Brillouin scattering (SBS) numerical mode for broadband multimode KrF laser pump with optical breakdown has been built up in this paper. The basic premises of the model are that KrF spectrum is composed of an umber of lines and SBS arises from these lines with coupling to some extent. The broadband SBS threshold strongly depends on pump bandwidth. SBS and optical breakdown occur nearly simultaneously when broadband SBS and breakdown have the same threshold. The decrease of saturation reflectivity for broadband pump radiation is explained with this model. Experimental results agree well with the model.     

Theoretical calculation of the triple differential cross sections of the 2p orbital of argon in a coplanar highly asymmetric（e,2e） reaction

The triple differential cross sections of the 2p electron of argon in a coplanar highly asymmetric geometry have been calculated with the modified distorted wave Born approximation (DWBA) and the target Hartree－Fock approximation methods. The damping polarization of the semi-classical short-range potentials and the M_ee factor are included in the distorting potentials of the modified DWBA. Theoretical results are compared with a recent experiment. The dynamic mechanism of inner shell ionization in a coplanar highly asymmetric geometry (e, 2e) reaction are also discussed.     

A new method for measuring the threshold of stimulated Brillouin scattering

A new method for measuring the threshold of stimulated Brillouin scattering (SBS) based on the generation location of a Stokes beam is proposed for the first time to our knowledge. The length of the medium cell is selected to be longer than the free gain length of pump pulses in the Brillouin medium. The reflected light from a certain mirror in front of the medium cell is chosen as the reference beam, and the SBS threshold is measured by the "jump" of the delay between the Stokes beam and the reference beam. An 8-ns Q-switched single-longitudinal-mode pulse is used as the pump and the typical SBS medium FC-72 is selected as the nonlinear medium in our experiment. The SBS threshold intensity is measured to be 173-178 mW/cm 2 , which is consistent with existing results measured with the transmitted energy limiting method.     

受激布里渊散射相位共轭激光组束规律的研究

提出了一种新的SBS激光组束的方法。此方法中,一束按时间分布的激光脉冲序列作为泵浦光从SBS放大池的一端入射,另一束Stokes频移种子光从SBS池的另一端入射,Stokes种子光在SBS池的相互作用区提取泵浦光能量。研究了组束效率和输出脉宽随脉冲串个数、间隔和泵浦功率密度等的变化规律。研究结果表明种子注入型泵浦脉冲串的受激布里渊散射相位共轭组束是一种高效的组束方法。     

对受激布里渊散射激光进行组束的数值模拟及方案设计

提出了时间上串行的多路激光脉冲通过受激布里渊散射(SBS)池进行组束的方法,并对其进行了数值模拟研究。利用6束每束能量为45J的KrF激光进行组束, 可获得能量为141.89J,脉宽为670ps的Stokes输出光。根据模拟结果设计出了时间上串行的SBS激光组束的两个方案, 对其进行了讨论。数值模拟还发现在介质的增益系数更大、声子寿命更短的情况下,输出激光脉冲的脉宽可以压缩得更窄。     

杂质颗粒对受激布里渊散射介质光学击穿阈值影响的研究

建立了受激布里渊散射介质中热作用破坏的物理模型, 数值模拟了杂质颗粒的温度随其半径的变化曲线.结果显示,杂质颗粒存在一个最大热作用半径, 介质所含颗粒的尺寸在此半径附近时,介质最容易发生光学击穿现象, 其光学击穿阈值最低.在Continuum Nd: YAG种子注入式激光系统中,选取FC-3283, GF-180和HFE-7100介质, 通过不同孔径的过滤膜进行过滤,并研究了过滤前后的光学击穿阈值和能量反射率. 结果表明,随着过滤孔径的变小,介质光学击穿阈值逐渐提高, 且过滤之后介质的能量反射率有了明显的提高.介绍了一种利用He-Ne激光透射光光斑变化来判断是否发生光学击穿现象的方法,该方法具有方便、 准确的特点,可有效地减小由于肉眼观测引起的误差.     

BBO，LBO，KDP晶体光参量啁啾脉冲放大特性的比较研究

对BBO,LBO,KDP晶体I类非共线匹配下的光参量啁啾脉冲放大的相位匹配、参量范围、增益特性等进行了理论分析,重点对BBO和LBO的光参量啁啾脉冲放大特性进行了比较。结果表明对于以光参量啁啾脉冲放大系统代替800nm中心波长的Ti:sappire再生放大系统,用BBO晶体可获得更宽的增益带宽,而对1 053nm中心波长的种子光用LBO晶体更好。