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1.
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李玉  程倩  戚大伟  王继亮  张晶  王爽  关晶 《中国物理 B》2011,20(11):117502-117502
Ac susceptibility at low temperatures of Pr0.75Na0.25Mn1-xFexO3 (0 ≤ x ≤ 0.30) is investigated. The peak value of the real component of ac susceptibility χ' at the freezing temperature Tf is suppressed with the increasing frequency. The peak value of χ' shows a linear relation between Tf and the logarithm of the frequency ω. The normalized slope P = ΔTf/TfΔlgω, which is much lower than canonical insulating spin glass systems in which 0.06 ≤ P ≤ 0.08. The peak value of the imaginary component of the ac susceptibility χ' at Tf for the x = 0, 0.02, 0.30 samples increases with increasing frequency, suggesting a cluster glass ground state with a coexistence of charge-ordered phase and correlated ferromagnetic clusters in spin glass matrix. The peak value of χ' at Tf for the x = 0.10 sample decreases with increasing frequency, suggesting a phase separation ground state. The peak value of χ' at Tf for the x = 0.05 sample decreases with increasing frequency for ω ≤ 52 Hz and increases subsequently till 701 Hz, and then decreases with further increasing frequency for ω ≥ 1501 Hz. This complex behaviour is ascribed to the competition between the effects of large and little ferromagnetic clusters in the sample. The ground state of x = 0.05 sample is a transition state from cluster glass to phase separation.  相似文献   

2.
The amplitude-dependent ac susceptibility of high-temperature superconductors is shown to obey some empirical scaling relations. We try to analyze this behavior by extending a dc nonlinear response function of mixed state to the ac cases. The derived equations for critical current and ac susceptibility X(T) agree with the scaling relations of experimental data.  相似文献   

3.
Magnetite particles of different diameters were synthesized by chemical co-precipitation technique and the same are dispersed in dodecane to prepare a magnetic fluid. The results of X-ray diffraction, magnetization measurements, ac susceptibility and viscosity measurements are analyzed and discussed in the text.  相似文献   

4.
The amplitude-dependent ac susceptibility of high-temperature superconductors is shown to obey some empirical scaling relations. We try to analyze this behavior by extending a dc nonlinear response function of mixed state to the ac cases. The derived equations for critical current and ac susceptibility ξ(T) agree with the scaling relations of experimental data.  相似文献   

5.
测量了居里点TC=36 0K的钙钛矿La0 6 7Pb0 33MnO3在 2K 相似文献   

6.
The dynamic scaling behaviour of late-stage phase separation and coarsening mechanisms of L12 and D022 in Ni75AlxV25-x (3 ≤ x ≤ 10, at.%) alloys are studied using the microscopic phase-field dynamic model. The microelaso ticity field is incorporated into the diffusion dynamic model. The results show the morphology and coarsening dynamics being greatly changed by the elastic interactions among different precipitates, the particles aligning along the dominant directions, the average domain size (ADS) of L12 and D022 deviating from the exponent of temporal power-law, and the growth slowing down due to the increasing of elastic interactions. The dynamic scaling regime of late-stage coarsening of the precipitates is attained. Thus the scaling behaviour of structure function is also applicable for elastic interaction systems. It is also found that the variations of ADS and scaling function depend on the volume fraction of precipitates.  相似文献   

7.
The effect of Eu3+ ion doping in the La sites of single-crystal La4/3Srs/3Mn2O7 was investigated. Electron spin resonance (ESR) was applied to La4/3Sr5/3Mn2O7 and (Lao.8Euo.2)4/3Sr5/3Mn2O7 single crystals. A phase separation and phase transitions were observed from the ESR spectra data. Between 350 K and 300 K, both paramagnetic resonance (PMR) and anisotropic ferromagnetic resonance (FMR) lines were observed in the ab plane and the c axis direction, suggesting a coexistence of the paramagnetic (PM) phase and the ferromagnetic (FM) phase. The magnetization measurement reveals a spin-glass-like behavior in single-crystal (Lao.8Euo.2)4/3 Sr5/3Mn2O7 below the temperature of spin freezing Tf (- 29.5 K).  相似文献   

8.
Yttria-stabilized zirconia (YSZ) samples with different Fe concentrations were prepared to study the effects of Fe doping on crystalline and optical properties of YSZ. The former properties were determined by X-ray diffraction, while the latter properties were determined by diffuse reflectance (DR) and photoluminescence (PL) spectroscopies. Lattice contraction of YSZ caused by the Fe doping was observed. We revealed that the DR spectra of the 3 and 6 mol% Fe-doped YSZ samples originate from the Fe ions dissolved and undissolved in the YSZ, respectively. Moreover, two PL bands centered around 440 and 530 nm were observed for the YSZ sample, whereas one PL band centered around 440 nm was observed for the Fe-doped YSZ samples. The Fe doping reduced the PL intensity of YSZ and quenched the PL band around 530 nm. This could be explained by considering that the concentration of Fe ions near the surface of YSZ is much larger than that in the bulk of YSZ or by considering that the Fe doping enhances surface band bending of YSZ.  相似文献   

9.
The 57Fe Mössbauer technique has been used to investigate the effect of zinc oxide substitution in (25???x)MnO–xZnO–15Fe2O3–60B2O3 glass system (x?=?0, 5, 10, 15 and 20 mol% of ZnO ). Mössbauer absorption spectra for all the samples recorded at room temperature suggest the existence of the two paramagnetic quadrupole doublets. The observed variations in hyperfine parameters have been explained on the basis of cations distribution and exchange interaction at the lattice sites and it is concluded that B–B interaction increases while the metal–metal interaction decreases due to replacement of manganese oxide by zinc oxide. These results suggest that the present glass system exhibits a paramagnetic behaviour that changes towards the weak paramagnetic when manganese oxide was replaced with zinc oxide.  相似文献   

10.
11.
The improvement of the acetone-soaking treatment to the performance of polymer solar cells based on the P3HT/PCBM bulk heterojunction is reported. Undergoing acetone-soaking, the PCBM does not distribute uniformly in the vertical direction, a PCBM enrichment layer forms on the top of the active layer, which is beneficial to the collec- tion of the carriers and blocking the inverting diffusion carriers. X-ray photoelectron spectroscopy (XPS) analysis reveals that the PCBM weight ratio on the top of the active layer increases by 20% after the acetone-soaking treatment. Due to the nonuniform distribution of PCBM, the short-circuit current density, the open-circuit voltage, and the fill factor are enhanced significantly. Finally, the power conversion efficiency of the acetone-soaking device increases by 31% compared with the control device.  相似文献   

12.
The spherical model of a ferromagnet is investigated for various (external) boundary conditions. It is shown that, besides the well-known critical point, a second one can be produced by the boundary conditions. Although the main asymptotic of the free energy is analytic at the new critical point, theO(N1–2/d) asymptotic possesses a singularity here. A natural order parameter of the model has singularities at both critical points. The magnetization profile is studied for the whole range of the model's parameters and at different scales. It is shown that (in an appropriate regime) below the second critical temperature the magnetization profile freezes, that is, becomes temperature independent. Distributions of the single spin variables and some macroscopic observables (including normalized total spin) are studied for the whole temperature range including the critical points.  相似文献   

13.
The mixed valent manganites (La0.85Ag0.15)MnO3 with perovskite structure has been prepared by doping up to 50% of Co at the Mn site. Paramagnetic (PM) to ferromagnetic (FM) transitions have been observed in all the prepared materials. However, the long-range magnetic ordering observed in (La0.85Ag0.15)MnO3 is systemically reduced to cluster glass-type (short-range) of FM ordering due to the introduction of Co. The FM transition temperature was found to decrease with increase in Co doping up to 20% and for further increase in Co doping, the Tc was found to increase. They are explained on the basis of competition between FM double exchange interactions in Mn–O–Mn and Co–O–Co networks. In addition to PM–FM transition, evidences of FM to antiferromagnetic (AFM), and AFM to reentrant spin-glass transitions have been observed. The shift in spin-glass freezing temperature, Tf has been observed from the frequency variation of ac susceptibility measurements. The observed magnetic transitions are explained on the basis of magnetic interactions in different Mn–O–Mn, Mn–O–Co and Co–O–Co networks and such transitions are also observed from the measurement of third harmonic susceptibility. Metal–insulator transition and colossal magneto-resistivity have been observed up to 10% of Co doping.  相似文献   

14.
运用元胞自动机模型研究单车道路面上设立限速区对交通流的影响.计算机模拟结果显示,在交通流与密度的基本图中存在饱和交通流量,其大小取决于限速区的最大速度.限速区的设立导致不同相的分离.在确定性的模型中,当车辆密度较低时,存在两种不同的自由流相;而当车辆密度较高时,出现最大交通流相和自由流相.在随机模型中,车辆密度较高时,出现最大交通流相-堵塞相-自由流.对交通流以及临界密度等量给出一些解析结果.  相似文献   

15.
Dynamical spin susceptibility χs(q,ω) of the dp model in the over doping region is investigated by using the auxiliary boson technique. It includes higher order terms of the 1/N-expansion within the random phase approximation (RPA) of the local vertex, where frequency dependence of the quasi-particle interaction is taken into account. The incommensurate spin fluctuation is obtained due to the nesting effect in the low energy region (ωω*), whereas the commensurate one in the high energy region (ωω*), the characteristic energy ω* is estimated to be about 30 meV. Both of the spin–lattice relaxation rate 1/T1 and the spin–spin relaxation rate 1/Tg monotonically increase as T decreases, while the spin Knight shift K is almost independent of T.  相似文献   

16.
Zuo Xiaoxi 《Optik》2005,116(7):361-364
Fe:LiNbO3 and In:Fe:LiNbO3 crystals were grown by Czochralski method. The absorption spectra were measured to investigate their defect structure. The photo damage resistance and photorefractive properties were measured. The photo damage resistance of the In:Fe:LiNbO3 crystal in which the In concentration is above the threshold value is one order of magnitude higher than that of the Fe:LiNbO3 crystal. The mechanisms of the violet shift of the absorption edge and the enhancement of the photorefractive effect of In:Fe:LiNbO3 crystals were investigated.  相似文献   

17.
The effects of Fe-doping and Fe-N-codoping on the magnetic properties of SnO2, prepared by chemical co-precipitation technique, are investigated in details. We found that the paramagnetism is the dominant magnetic interaction in Fe doped SnO2. A weak antiferromagnetic coupling between Fe2+ ions is also confirmed through Zero field-cooled (ZFC) and field-cooled (FC) magnetization studies. On the other hand, hystersis behavior is observed for Fe-N-codoped SnO2 samples with coercivity Hc∼420 and 352 Oe for x=0.05 and 0.10, respectively. As no other secondary or impurity phase is detected by XRD study and the presence of N is confirmed by EDX analysis, this observed ferromagnetism is originated due to the substitution of N in Sn1−xFexO2. N doping at the oxygen site can be regarded as defect and introduces a hole in this system. As a result, a hole-induced ferromagnetism might be the origin of the observed ferromagnetism in Fe-N-codoped SnO2 samples.  相似文献   

18.
利用折射率椭球基本理论对线性电光效应进行了分析,对单轴晶体铌酸锂电光相位调制器的温度特性进行了研究。通过计算机进行数值模拟计算,分析了加电场时光通过LiNbO3电光调制器后出射光的相位变化与温度间的关系,得出在横向和纵向调制中温度对相位改变的影响。研究发现,无论在横向还是在纵向调制下,入射光偏振方向不同但其各自受温度影响的相位变化趋势大体一致,即随着晶体中温度的增加而增大。计算结果表明,LiNbO3电光调制的最佳使用方案为:电场沿x主轴方向施加,入射光偏振方向为感应主轴x’方向,且LiNbO3电光调制器粟用横向相位调制方式。  相似文献   

19.
基于微观相场动力学模型,运用原子图像、平均长程序参数和平均成分偏离序参数,研究了Al浓度对Ni75Cr25-xAlx合金中L12相和D022相形核孕育期的影响以及孕育期与沉淀相析出顺序之间的关系.结果表明,L12相和D022相的形核孕育期不仅与Al浓度有关,而且与两相析出的先后顺序密切相关.当Al浓度小于7.5%时,先析出相为D022相,随着Al浓度的增大,D022相形核孕育期延长,后析出的L12相的形核孕育期也延长,L12相的原子簇聚速度加快;当Al浓度大于7.5%时,先析出相为L12相,随着Al浓度的增大,L12相的形核孕育期缩短,后析出的D022相形核孕育期也缩短.当Al浓度为7.5%时,L12相和D022相几乎同时析出,两者的孕育期没有明显的差别.  相似文献   

20.
We use exact recursion relations to study the magnetic properties of the half-integer mixed spin-5/2 and spin-3/2 Blume-Capel Ising ferromagnetic system on the two-fold Cayley tree that consists of two sublattices A and B. Two positive crystal-field interactions Δ1 and Δ2 are considered for the sublattice with spin-5/2 and spin-3/2 respectively. For different coordination numbers q of the Cayley tree sites, the phase diagrams of the model are presented with a special emphasis on the case q = 3, since other values of q reproduce similar results. First, the T = 0 phase diagram is illustrated in the (D A = Δ1/J,D B = Δ2/J) plane of reduced crystal-field interactions. This diagram shows triple points and coexistence lines between thermodynamically stable phases. Secondly, the thermal variation of the magnetization belonging to each sublattice for some coordination numbers q are investigated as well as the Helmoltz free energy of the system. First-order and second-order phase transitions are found. The second-order phase transitions become sharper and sharper when D A or D B increases. The first-order transitions only exist for some appropriate non-zero values of D A and/or D B . The corresponding transition lines never connect to the second-order transition lines. Thus, the non-existence of tricritical points remains one of the key features of the present model. The magnetic exponent β 0 of the model is estimated and found to be ¼ at small values of D A = D B = D and β 0 = ½ at large values of D. At intermediate values of D, there is a crossover region where the magnetic exponent displays interesting behaviours.  相似文献   

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