On the influence of anisotropy on the magnetic small-angle neutron scattering of superparamagnetic particles |
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Authors: | A Michels J Weissmüller |
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Institution: | Institut für Nanotechnologie, Forschungszentrum Karlsruhe, Karlsruhe, Germany Technische Physik, Universit?t des Saarlandes, Postfach 151150, Bau 43.2, 66041 Saarbrücken, Germany, DE
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Abstract: | This paper presents a calculation of the magnetic small-angle neutron scattering cross-section resulting from a dilute ensemble
of superparamagnetic particles exhibiting uniaxial magnetic anisotropy. We focus on the two experimentally relevant scattering
geometries in which the incident neutron beam is perpendicular or parallel to an applied magnetic field, and we discuss several
orientations of the anisotropy axes with respect to the field. Magnetic anisotropy has no influence on the magnetic small-angle
neutron scattering when the particles are mobile, as is the case e.g. in ferrofluids, but, when the particles are embedded
in a rigid non-magnetic matrix and the orientations of the anisotropy axes are fixed, significant deviations compared to the
case of negligible anisotropy are expected. For the particluar situation in which the anisotropy axes are parallel to the
applied field, closed-form expressions suggest that an effective anisotropy energy or anisotropy-energy distribution can be
determined from experimental scattering data.
Received 8 November 2001 |
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Keywords: | PACS 61 12 Ex Neutron scattering techniques (including small-angle scattering) – 75 30 Gw Magnetic anisotropy – 75 50 Tt Fine-particle systems nanocrystalline materials |
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