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1.
Understanding and control of the surface properties such as molecular orientations are of great importance in numerous applications of ionic liquids. However, there remain discrepancies among the previous experimental and theoretical studies on the surface orientation and structures of room temperature ionic liquids(RTIL) systems. In this article, the orientation of 1-butyl-3-methylimidazolium([bmin]) cation at the air/liquid interface of a characteristic RTIL, 1-butyl-3-methylimidazolium hexafluorophosphate([bmim][PF6]), was investigated by the sum frequency generation vibrational spectroscopy(SFG-VS). Detailed polarization and experimental configuration analyses of the SFG-VS spectra showed the possibility of a small spectral splitting in the CH3 symmetric stretching region, which can be further attributed to the probable existence of multiple orientations for the interfacial [bmim] cations. In addition, the(N)–CH3 vibrations were absent, ruling out the prediction by several recent molecular dynamics simulations which state that portions of the [bmim] cations orient with a standing-up(N)–CH3 group at the ionic liquid surface. Hence, new realistic theoretical models have to be developed to reflect the complex nature of the ionic liquid surface. 相似文献
2.
I. Paradela Pérez M. Groth M. Wischmeier D. Coster D. Brida P. David D. Silvagni M. Faitsch the ASDEX-Upgrade Team the EUROfusion MST Team 《等离子体物理论文集》2020,60(5-6):e201900166
SOLPS-ITER L-mode-like simulations with the full set of currents and drift velocities activated, and fluid neutrals have been carried out to interpret experimental results obtained in AUG. Drifts are critical to quantitatively reproduce the experimental results; however, simulations without drifts can also reproduce some trends qualitatively. The magnitude and dependence of the peak heat flux onto both targets on the upstream collisionality are, in general, in quantitative agreement within uncertainties with infrared thermography measurements in favourable field direction. The onset of power detachment is observed. In unfavourable toroidal field direction, a more symmetrical inner/outer target solution with regards to the power distribution is predicted, in agreement with experimental observations. However, also in unfavourable toroidal field direction, insufficient power is dissipated in the simulations and therefore qpeak, inn is overpredicted by up to a factor of 4 and qpeak, out by up to a factor of 1.5. The largest contribution to the sources due to radial transport in the energy balance equation is the radial divergence of the energy flux due to VE × B. 相似文献
3.
W. Hubschmid R. Bombach A. Inauen F. Güthe S. Schenker N. Tylli W. Kreutner 《Experiments in fluids》2008,45(1):167-182
Laser-induced fluorescence and chemiluminescence, both phase-locked to the dominant acoustic oscillation, are used to investigate
phenomena related to thermoacoustic instability in a swirl-stabilized industrial scale gas turbine burner. The observed sinusoidal
phase-averaged flame motion in axial (main flow) direction is analyzed using different schemes for defining the flame position.
Qualitative agreement between experimental data and theoretical analysis of the observed flame motion is obtained, interpreted
as originating primarily from variation of the burning velocity. The heat release variation during an acoustic cycle is determined
from the sinusoidally varying total OH* chemiluminescence intensity.
相似文献
W. HubschmidEmail: |
4.
In this letter, we solve three-dimensional time-dependent Newton equations for atoms interacting with a ten-cycle elliptically polarized laser pulse. The ionized electron momentum distributions show a tilt angle between the distribution density peak and the main polarization axis. The tilt angle’s behavior changes with an increasing laser intensity. We show that this behavior change is directly related to the release time of the electron from the atom. 相似文献
5.
Li Caldeira Balkeståhl Erik Thomé on behalf of the PANDA Collaboration 《Hyperfine Interactions》2014,229(1-3):79-83
Strangeness and charm production provide an excellent probe of QCD in the confinement domain. With the PANDA detector at FAIR, this can be studied in e.g., hyperon production in the p?p → ?Y reactions. In PANDA, all ground state strange hyperons and single charmed Λ’s will be accessible. Simulations show that the differential cross sections and spin observables can be well reconstructed for these reaction channels. 相似文献
6.
HAN Tao LU XiaoChun WANG Xue RAO YongNan ZOU DeCai YANG JianFei & WU YangYang National Time Service Center Xi'an China Key Laboratory of Precision Navigation Timing Technology Chinese Academy of Sciences Graduate University of the Chinese Academy of Sciences Beijing 《中国科学:物理学 力学 天文学(英文版)》2011,(6)
With the development of Global Navigation Satellite System (GNSS),the idea of GNSS interoperability is born and has become the focus of study in the field of satellite navigation.The popularity for GNSS to augment the interoperability with the existing ones necessitates the study of the assessment algorithm of this idea.In this paper,an assessment algorithm for interoperability comprehensive benefits based on the differential equation dynamical system is discussed.There are two important aspects in GNSS tha... 相似文献
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A. B. Kurepin A. V. Dermenev M. B. Golubeva the CASTOR Collaboration 《Bulletin of the Russian Academy of Sciences: Physics》2011,75(3):399-401
The creation of the CASTOR forward calorimeter in the compact muon spectrometer (CMS) experiment at the Large Hadron Collider
(LHC), CERN enabled us to perform experiments at energies corresponding to those of cosmic rays but at much greater intensities,
the most important factor in studying rare and anomalous phenomena. 相似文献