Alpha-gamma decay studies of $$^{247}$$ Md

The European Physical Journal A - The goal of the present paper is twofold. First, a novel expansion many-body method applicable to superfluid open-shell nuclei, the so-called Bogoliubov in-medium...     

New results on elements 111 and 112

Experiments on the synthesis and identification of the nuclei ²⁷²111 and ²⁷⁷112 were performed in order to confirm previous results. Three additional decay chains were measured in the reaction ⁶⁴Ni + ²⁰⁹Bi →²⁷³111^*. The study revealed considerably improved data on the decay chain originating from ²⁷²111. One additional chain was measured in the reaction ⁷⁰Zn + ²⁰⁸Pb →²⁷⁸112^*. The decay properties of the chain starting at ²⁷⁷112 are in excellent agreement with the second chain of the first experiment down to ²⁶⁵Sg, where the new chain ends by a previously unknown spontaneous-fission branch. A re-analysis of all the data on elements 110, 111, and 112 measured at GSI since 1994 (a total of 34 decay chains was investigated) revealed that for 2 chains (the second chain of ²⁶⁹110 measured in 1994 and the first chain of ²⁷⁷112 measured in 1996) the results of the new analysis differed from the previous one. In all other cases the earlier data are exactly reproduced. Received: 21 December 2001 / Accepted: 15 January 2002     

Decay studies of K isomers in 254No

A detailed $ \gamma$ spectroscopic decay study of two K isomers in ²⁵⁴No was performed. In addition to the previously reported $ \gamma$ lines two new transitions of E = 778 , 856keV could be attributed to the decay pattern of ^254m1No ( T _1/2 = 275±7 ms). The population of an excited band built up on this isomer ( $\ensuremath K^{\pi} =8^{-}$ by the decay of ^254m2No ( T _1/2 = 198±13 μs) could be proven by measuring delayed $ \gamma$ - $ \gamma$ coincidences between transitions stemming from the decay of both isomeric states. The energies of the band members could be established up to $\ensuremath I^{\pi} = 15^{-}$ . A spontaneous fission branch of (2.0±1.2)×10^-4 was measured for ^254m1No , an upper limit of $ \le$ 1.2×10^-4 was estimated for ^254m2No . These values demonstrate the high stability of multi-quasiparticle configurations against spontaneous fission. Evidence for an $ \alpha$ decay branch of ^254m1No in the order of 1×10^-4 was found.     

Isomeric states in 214Th and 213Th

Isomeric states in ²¹⁴Th and ²¹³Th were identified by means of γ -rays measured in delayed coincidence with the implanted evaporation residues. These were produced in irradiations of ¹⁶⁴Dy with ⁵⁴Cr projectiles and separated in-flight by the velocity filter SHIP. An isomeric state of I ^π = 8⁺ with a half-life of (1.24±0.12) μs was identified in ²¹⁴Th . The configuration π[1h _9/2 ⊗ 2f _7/2] was assigned to this state. An isomeric state with a half-life of (1.4±0.4) μs was observed in ²¹³Th . Tentatively it was assigned to an I ^π = 13/2⁺ state.     

Measurement of evaporation residue cross-sections of the reaction 30Si + 238U at subbarrier energies

The reaction ³⁰Si + ²³⁸U → ²⁶⁸Sg^* was studied at beam energies close to the Coulomb barrier. At a center-of-mass energy of E _c.m. = 144.0MeV for reactions at half thickness of the target we measured three decay chains of ²⁶³Sg produced by evaporation of five neutrons. The cross-section was ( 67⁺⁶⁷ _-37) pb. At E _c.m. = 133.0MeV we measured three spontaneously fissioning nuclei which we assigned to the isotope ²⁶⁴Sg. The production cross-section was ( 10⁺¹⁰ _-6) pb and a half-life of ( 120⁺¹²⁶ _-44) ms was determined. This half-life is a factor of twenty shorter than theoretical predictions. At E _c.m. = 128.0MeV an upper cross-section limit of 15pb was measured. The cross-section data reveal a strong influence of the orientation of the deformed target nucleus on the production yield. Compared to excitation functions measured for the lighter system ¹⁶O + ²³⁸U → ²⁵⁴Fm^*, a reduction of the fusion probability was observed at low beam energies indicating increasing competition from quasifission processes.     

Early onset of ground state deformation in neutron deficient polonium isotopes

In-source resonant ionization laser spectroscopy of the even-A polonium isotopes (192-210,216,218)Po has been performed using the 6p(3)7s (5)S(2) to 6p(3)7p (5)P(2) (λ=843.38 nm) transition in the polonium atom (Po-I) at the CERN ISOLDE facility. The comparison of the measured isotope shifts in (200-210)Po with a previous data set allows us to test for the first time recent large-scale atomic calculations that are essential to extract the changes in the mean-square charge radius of the atomic nucleus. When going to lighter masses, a surprisingly large and early departure from sphericity is observed, which is only partly reproduced by beyond mean field calculations.     

Alpha-decay properties of <Superscript>261</Superscript>Bh

The isotope ²⁶¹Bh was produced in the reaction ²⁰⁹Bi(⁵⁴Cr, 2n)²⁶¹Bh and its \( \alpha\) decay has been remeasured. It was found that it populates by an unhindered transition of \( \approx\) 10 MeV an excited level at E ^* > 350 keV in the daughter nucleus ²⁵⁷Db . The latter decays by internal transitions either into the isomeric state or the ground state. A somewhat improved half-life value of T _1/2 = 11.8^+3.9 _-2.4 ms was obtained for ²⁶¹Bh . The data support the previous assignment of the \( \alpha\) activities ²⁵⁷Db (1) and ²⁵⁷Db (2) to the isomer and to the ground state, respectively. No evidence for an isomeric state in ²⁶¹Bh decaying by \( \alpha\) emission was found. Based on the experimental results and theoretical calculations a partial decay scheme of ²⁶¹Bh including spin and parity assignments of the ground-state and excited levels in the daughter nucleus ²⁵⁷Db populated by the \( \alpha\) decay and succeeding internal transitions have been suggested. ²⁶¹Bh represents so far the heaviest nucleus for which such an attempt has been made. No spontaneous fission (SF) events that could be attributed to ²⁶¹Bh were observed, resulting in an SF branching b _SF < 0.05 . The measured production cross-section is (64±15) pb at E ^* = 22 MeV.     

Radioactive decay of 217Pa

The radioactive decay of ²¹⁷Pa was investigated by means of α-γ-spectroscopy. Fine structure in the ground-state α-decay was established. Ambiguities in the fine structure of the α-decay of the previously known isomeric state could be clarified by α-γ-coincidence measurements. A previously unknown α-transition of E _α = (8306 ± 5) keV was detected and identified by means of delayed α-α- and α-γ-γ-coincidence measurements. A second isomeric state decaying by α-emission was not observed. The quality of the previously reported data of the α-decay fine structure of ²¹⁷Th was improved. Received: 29 April 2002 / Accepted: 17 June 2002 / Published online: 19 November 2002 RID="a" ID="a"e-mail: f.p.hessberger@gsi.de Communicated by J. ?yst?