超强频率梳激光场驱动下多光子共振谐波辐射的相位突变研究

本文从理论上研究了在双色频率梳激光场驱动下多光子谐波辐射光谱中的相位突变现象。我们利用Floquet理论非微扰地模拟了频率梳激光场与原子分子等量子系统的相互作用过程。谐波辐射信号是多光子偶极跃迁相干叠加的结果,通过调节频率梳激光场间的相对相位,可以相干地控制谐波辐射信号的强度。通过对谐波信号进行傅里叶变换,可以提取不同跃迁路径的相对相位信息。我们通过改变频率梳组激光场的强度和频率组分实现多光子跃迁频率,让其跨越共振跃迁频率时,谐波相位会发生突变。从而可以观测超强激光场驱动下量子系统共振跃迁频率的斯塔克能移。     

利用高阶拉盖尔-高斯横模精确测量法布里-珀罗腔内原子的运动轨迹

研究了冷原子与法布里-珀罗腔内拉盖尔-高斯横模强耦合相互作用体系的透射光谱, 分析了透射光谱与原子在腔中运动轨迹的关系. 结果表明, 与厄米特-高斯横模相比, 拉盖尔-高斯横模的腔场与原子的最大耦合系数几乎不随阶数的增加而变化, 使得探测光谱的对比度受模式阶数的影响较小. 在拉盖尔-高斯横模场分布的圆环边缘附近, 原子运动轨迹的微小偏移会引起透射光谱的很大变化, 因此在这些位置可以实现原子运动轨迹的高精度探测.     

Modulation of multiphoton resonant high-order harmonic spectra driven by two frequency-comb fields

The frequency-comb structure in the extreme ultraviolet(XUV) and vacuum ultraviolet(VUV) regions can be realized by the high-order harmonic generation(HHG) process driven by frequency-comb fields, providing an alternative approach for the measurement of an unknown frequency in XUV or VUV. We consider the case of two driving frequency-comb fields with the same repetition frequency and the carrier frequencies of fundamental-and third-harmonics, respectively.The many-mode Floquet theorem(MMFT) is employed to provide a nonperturbative and exact treatment of the interaction between a quantum system and the frequency-comb laser fields. Multiphoton transition paths involving both fundamentaland third-harmonic photons are opened due to the coupling of the third-harmonic frequency-comb field. The multiphoton transition paths are superpositioned when the carrier-envelope-phase shifts(CEPs) fulfill the matching condition. And the interference of the multiphoton transition paths can be controlled by tuning the relative envelope delay between the fields.We find that the quasienergy structure, as well as the multiphoton resonant high-order harmonic generation(HHG) spectra,driven by the two frequency-comb fields can be coherently controlled via the interference of multiphoton transition paths.It is also found that the spectral intensities of the generated harmonics can be modulated, and the modulation behavior is harmonic-sensitive.     

对巧克力相变迟滞现象的理论解释——朗道-德冯谢亚理论以及铁电相变理论

巧克力作为生活中常见的事物，其储存方法一直是食品科学界研究的重要课题，而由相变产生的巧克力凝固和融化等现象对巧克力的储存产生了决定性的影响；但由于巧克力的成分复杂且晶体结构多变，目前只在生活中实现了控制巧克力保持良好性状的储存，而鲜少有研究分析其背后存在的相变机理。研究中首先基于朗道-德冯谢亚理论，使用序参量描述了影响相变的相关因素，初步解释了巧克力相变当中存在的迟滞现象；而后进行了相关实验，提出了一种对朗道理论的修正来解释实验现象；最后，通过研究巧克力的主要成分可可脂晶体的铁电相变，对德冯谢亚理论中未作出解释的势垒产生做出了阐述。