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Klas Källström 《Tetrahedron letters》2006,47(42):7477-7480
An efficient chiral N-heterocyclic carbene ligand for the Ir-catalyzed asymmetric hydrogenation of largely unfunctionalized tri-substituted olefins has been developed. The Ir-NHC-thiazole catalyst is able to reduce a large variety of substrates with excellent conversions and good enantioselectivities with ee’s ranging from 34% to 90%, depending on the geometry around the double bond of the substrates. 相似文献
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Conditions for determination of quaternary ammonium compounds and amines by two-phase titration have been calculated on the basis of extraction constants for the ion-pairs between the titrant (lauryl sulphate), the indicator (Methyl Yellow) and the sample. Methods for determination of extraction constants are presented. The precision and selectivity of the method are demonstrated by titrations of ammonium ions with different structures and degrees of substitution. The results are in agreement with the theoretical calculations. 相似文献
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This paper describes a full-scale mathematical model used for the analysis of temperature conditions of an RBMK nuclear reactor in the event of its complete deenergization. The results of the verification and some computational results are presented. 相似文献
7.
In this paper we discuss how partial knowledge of the density of states for a model can be used to give good approximations
of the energy distributions in a given temperature range. From these distributions one can then obtain the statistical moments
corresponding to e.g. the internal energy and the specific heat. These questions have gained interest apropos of several recent
methods for estimating the density of states of spin models. As a worked example we finally apply these methods to the 3-state
Potts model for cubic lattices of linear order up to 128. We give estimates of e.g. latent heat and critical temperature,
as well as the micro-canonical properties of interest.
相似文献
8.
Klas Markström 《Journal of Graph Theory》2014,76(2):101-105
For ordinary graphs it is known that any graph G with more edges than the Turán number of must contain several copies of , and a copy of , the complete graph on vertices with one missing edge. Erd?s asked if the same result is true for , the complete 3‐uniform hypergraph on s vertices. In this note, we show that for small values of n, the number of vertices in G, the answer is negative for . For the second property, that of containing a , we show that for the answer is negative for all large n as well, by proving that the Turán density of is greater than that of . 相似文献
9.
Given a group G, the model denotes the probability space of all Cayley graphs of G where each element of the generating set is chosen independently at random with probability p. In this article we show that for any and any family of groups Gk of order nk for which , a graph with high probability has diameter at most 2 if and with high probability has diameter greater than 2 if . We also provide examples of families of graphs which show that both of these results are best possible. Of particular interest is that for some families of groups, the corresponding random Cayley graphs achieve Diameter 2 significantly faster than the Erd?s‐Renyi random graphs. © 2014 Wiley Periodicals, Inc. Random Struct. Alg., 45, 218–235, 2014 相似文献
10.
The E. Amar and G. Henkin theorem on the bounded extendability of bounded holomorphic functions from certain closed complex
submanifolds of strictly pseudoconvex domains to the whole domain is generalized to the case of finite type convex domains
and their intersections with affine linear hyperplanes. Suitable integral operators of Berndtsson–Andersson type are constructed
and estimated for this purpose.
Received: 7 July 2000 相似文献