双奇核188Au的准粒子带结构研究

利用在束γ谱学实验技术, 通过¹⁷³Yb(¹⁹F,4nγ)反应 布居了¹⁸⁸Au的高自旋态, 并对其准粒子带结构进行了研究. 基于实验测量结果, 对原有的双奇核¹⁸⁸Au能级纲图做了较大的修改. 通过系统性比较, 对15⁺以上的能级结构进行了讨论.     

Full-Wave Analyses for a Multi-Layered Microstrip Patch Antenna

This paper describes numerical modelling of a dual band multi-layered microstrip patch antenna operating at 35GHz on an in-house semi-insulating GaAs substrate. The simulated and measured resonant frequencies at both lower and upper resonant frequencies will be compared to check the accuracy of the different numerical modelling techniques.     

High-sensitive elemental analysis using multi-parameter coincidence spectrometer: GEMINI-II

In this study, using neutron activation analysis with multi-parameter coincidence method which was developed at Japan Atomic Energy Agency (JAEA), a non-destructive, ultra-high sensitive multi-elemental determination has been realized. The multi-parameter coincidence method is carried out with an array of 19 germanium detectors, GEMINI-II. Using this system, very weak γ-rays emitted from trace amounts of elements can be detected. The iridium concentration has been determined by means of neutron activation analysis with multi-parameter coincidence method for Cuban sediment samples across the K/T boundary strata.     

Kopsifolines A–F: a New Structural Class of Monoterpenoid Indole Alkaloids from Kopsia

Six new indole alkaloids, named kopsifolines A–F ( 1 – 6 ), with an unprecedented hexacyclic carbon skeleton, constituting a new structural group of monoterpenoid indole alkaloids, were obtained from the leaf extract of a Malayan Kopsia species, and their structures were established by spectroscopic analysis.     

Locally adaptive bilateral clustering for universal image denoising

This paper presents a novel and efficient locally adaptive denoising method based on clustering of pixels into regions of similar geometric and radiometric structures. Clustering is performed by adaptively segmenting pixels in the local kernel based on their augmented variational series. Then, noise pixels are restored by selectively considering the radiometric and spatial properties of every pixel in the formed clusters. The proposed method is exceedingly robust in conveying reliable local structural information even in the presence of noise. As a result, the proposed method substantially outperforms other state-of-the-art methods in terms of image restoration and computational cost. We support our claims with ample simulated and real data experiments. The relatively fast runtime from extensive simulations also suggests that the proposed method is suitable for a variety of image-based products ?? either embedded in image capturing devices or applied as image enhancement software.     

Transition Metal (Mn,Fe, Co,Ni)‐Doped Graphene Hybrids for Electrocatalysis

The development of electrocatalysts is crucial for renewable energy applications. Metal‐doped graphene hybrid materials have been explored for this purpose, however, with much focus on noble metals, which are limited by their low availability and high costs. Transition metals may serve as promising alternatives. Here, transition metal‐doped graphene hybrids were synthesized by a simple and scalable method. Metal‐doped graphite oxide precursors were thermally exfoliated in either hydrogen or nitrogen atmosphere; by changing exfoliation atmospheres from inert to reductive, we produced materials with different degrees of oxidation. Effects of the presence of metal nanoparticles and exfoliation atmosphere on the morphology and electrocatalytic activity of the hybrid materials were investigated using electron microscopy, energy‐dispersive X‐ray spectroscopy, X‐ray photoelectron spectroscopy, and cyclic voltammetry. Doping of graphene with transition metal nanoparticles of the 4th period significantly influenced the electrocatalysis of compounds important in energy production and storage applications, with hybrid materials exfoliated in nitrogen atmosphere displaying superior performance over those exfoliated in hydrogen atmosphere. Moreover, nickel‐doped graphene hybrids displayed outstanding electrocatalytic activities towards reduction of O₂ when compared to bare graphenes. These findings may be exploited in the research field of renewable energy.     

Solid‐State Structural Transformations and Photoreactivity of 1D‐Ladder Coordination Polymers of PbII

An attempt has been made to design double‐stranded ladder‐like coordination polymers (CPs) of hemidirected Pb^II. Four CPs, [Pb(μ‐bpe)(O₂C‐C₆H₅)₂] ? 2H₂O ( 1 ), [Pb₂(μ‐bpe)₂(μ‐O₂C‐C₆H₅)₂(O₂C‐C₆H₅)₂] ( 2 ), [Pb₂(μ‐bpe)₂(μ‐O₂C‐p‐Tol)₂(O₂C‐p‐Tol)₂] ? 1.5 H₂O ( 3 ) and [Pb₂(μ‐bpe)₂(μ‐O₂C‐m‐Tol)₂(O₂C‐m‐Tol)₂] ( 4 ) (bpe=1,2‐bis(4′‐pyridyl)ethylene), have been synthesised and investigated for their solid‐state photoreactivity. CPs 2 – 4 , having a parallel orientation of bpe molecules in their ladder structures and being bridged by carboxylates, were found to be photoreactive, whereas CP 1 is a linear one‐dimensional (1D) CP with guest water molecules aggregating to form a hydrogen‐bonded 1D structure. The linear strands of 1 were found to pair up upon eliminating lattice water molecules by heating, which led to the solid‐state structural transformation of photostable linear 1D CP 1 into photoreactive ladder CP 2 . In the construction of the double‐stranded ladder‐like structures, the parallel alignment of C?C bonds in 2 – 4 is dictated by the chelating and μ₂‐η²:η¹ bridging modes of the benzoate and toluate ligands. The role of solvents in the formation of such double‐stranded ladder‐like structures has also been investigated. A single‐crystal‐to‐single‐crystal transformation occurred when 4 was irradiated under UV light to form [Pb₂(rctt‐tpcb)(μ‐O₂C‐m‐Tol)₂(O₂C‐m‐Tol)₂] ( 5 ).     

Convergence Analysis of an Infeasible Interior Point Algorithm Based on a Regularized Central Path for Linear Complementarity Problems

Most existing interior-point methods for a linear complementarity problem (LCP) require the existence of a strictly feasible point to guarantee that the iterates are bounded. Based on a regularized central path, we present an infeasible interior-point algorithm for LCPs without requiring the strict feasibility condition. The iterates generated by the algorithm are bounded when the problem is a P _* LCP and has a solution. Moreover, when the problem is a monotone LCP and has a solution, we prove that the convergence rate is globally linear and it achieves `-feasibility and `-complementarity in at most O(n ² ln(1/`)) iterations with a properly chosen starting point.     

Multiple Coulomb excitation of a 70Ge beam and the interpretation of the 02 + state as a deformed intruder

Electromagnetic properties of the low-lying states in a ⁷⁰Ge nucleus were studied through the multiple Coulomb excitation of a ⁷⁰Ge beam with a ^natPb target. Relative γ-ray intensities were measured as a function of emission angle relative to the scattered projectile. Sixteen E2 matrix elements, including diagonal ones, for 6 low-lying states have been determined using the least-squares search code GOSIA. The expectation values 〈Q ²〉 of 0₁ ⁺ and 0₂ ⁺ states in ⁷⁰Ge are compared with those in ^{72, 74, 76}Ge. Simple mixing calculations indicate that the 0₂ ⁺ states in ⁷⁰Ge and ⁷²Se can be treated as deformed intruder states. It is shown that the deformed intruder becomes the ground state in ⁷⁴Kr. These interpretations of the 0₂ ⁺ states in this region are compared with the potential-energy surface calculations by the Nilsson-Strutinsky model, which allow to interpret the experimental results in a qualitative way from the theoretical point of view. Received: 2 September 2002 / Accepted: 5 November 2002 / Published online: 25 February 2003 RID="a" ID="a"e-mail: sugawara@pf.it-chiba.ac.jp Communicated by D. Schwalm