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We investigate the structural properties of liquid Sn. With the help of the internal friction (tanФ) method, it is found that a peak appears in the tan Ф - T curve, suggesting that an anomalous discontinuous temperatureinduced structure change may take place in liquid Sn. From the experimental data of pair distribution functions, we calculate the viscosity η and the excess entropy S and it is found that there are a peak of viscosity in the η-T curve and a bend of excess entropy in the S - T curve, which give a positive support to the appearance of the internal-friction peak in the tan Ф- T curve. 相似文献
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The recently proposed scaling law relating the diffusion coefficient and the excess entropy of liquid [Samanta A et al. 2004 Phys. Reu. Lett. 92 145901; Dzugutov M 1996 Nature 381 137], and a quasi-universal relationship between the transport coefficients and excess entropy of dense fluids [Rosenfeld Y 1977 Phys. Rev. A 15 2545],are tested for diverse liquid metals using molecular dynamics simulations. Interatomic potentials derived from the glue potential and second-moment approximation of tight-binding scheme are used to study liquid metals.Our simulation results give sound support to the above-mentioned universal scaling laws. Following Dzugutov,we have also reached a new universal scaling relationship between the viscosity coefficient and excess entropy.The simulation results suggest that the reduced transport coefficients can be expressed approximately in terms of the corresponding packing density. 相似文献
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用熔融共混法制备了不同组分的聚苯乙烯(PS)与聚氧化乙烯(PEO)共混物(PS/PEO).在玻璃转变温度Tg及其以上温区,利用相对能量耗散技术研究了该共混物的动力学行为.结果发现,在能量耗散-温度曲线上出现了两个弛豫型的耗散峰(α峰和α′峰).分析表明,α峰是与PS玻璃转变有关的特征耗散峰; α′峰则对应于一种“液-液转变”.两者的弛豫时间τ都不满足Arrhenius关系.此外,还研究了组分对这两个弛豫型耗散峰的影响,并给予了定性的解释.
关键词:
相对能量耗散
玻璃转变
力学弛豫 相似文献
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由中国物理学会内耗与超声衰减专业委员会、广州中山大学物理系和中国科学院固体物理研究所、中国科学技术大学内耗与固体缺陷开放研究实验室联合主办的第六届全国固体内耗与超声衰减学术会议暨中国物理学会第五届内耗与超声衰减专业委员会全体会员大会于 2 0 0 0年 10月 2 0— 2 3日在广州中山大学召开 .来自全国 13个单位的 4 7名代表参加了会议 ,会议代表向大会提交了 38篇学术论文(其中 4篇为特邀报告 ) ,共有 34篇学术论文在大会上宣读 .4篇特邀报告“凝聚态物质切变波共振吸收谱仪的原理”(张进修 ,中山大学 )、“结构弛豫与玻璃化转… 相似文献
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采用粉末冶金发泡法制备的泡沫铝试样,研究了室温下低频范围(0.04—4Hz)泡沫铝的内耗与孔结构(孔隙率和孔径)、频率、振幅之间的关系.结果表明泡沫铝的内耗具有以下特征:孔径一定时,内耗随孔隙率的增加而增大;孔隙率一定时,内耗随孔径的减小而增大;在测量频率范围内,内耗与频率近似无关;小应变振幅时内耗随振幅的增大而增大,具有正常振幅效应.提出了泡沫铝的内耗产生机制,根据等效夹杂方法和钉扎位错内耗特点进行了理论分析,较理想地解释了实验结果
关键词: 相似文献