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We adopt the nonequilibrium Green's function method to theoretically study the Kondo effect in a deformed molecule, which is treated as an electron-phonon interaction (EPI) system. The self-energy for phonon part is calculated in the standard many-body diagrammatic expansion up to the second order in EPI strength. We find that the multiple phonon-assisted Kondo satellites arise besides the usual Kondo resonance. In the antiparallel magnetic configuration the splitting of main Kondo peak and phonon-assisted satellites only happen for asymmetrical dot-lead couplings, but it is free from the symmetry for the parallel magnetic configuration. The EPI strength and vibrational frequency can enhance the spin splitting of both main Kondo and satellites. It is shown that the suppressed zero-bias Kondo resonance can be restored by applying an external magnetic field, whose magnitude is dependent on the phononic effect remarkably. Although the asymmetry in tunnel coupling has no contribution to the restoration of spin splitting of Kondo peak, it can shrink the external field needed to switch tunneling magnetoresistance ratio between large negative dip and large positive peak. 相似文献
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The nonequilibrium Kondo effect is studied in a molecule
quantum dot coupled asymmetrically to two ferromagnetic electrodes
by employing the nonequilibrium Green function technique. The
current-induced deformation of the molecule is taken into account,
modeled as interactions with a phonon system, and
phonon-assisted Kondo satellites arise on both sides of the usual main
Kondo peak. In the antiparallel electrode configuration, the
Kondo satellites can be split only for the asymmetric dot-lead
couplings, distinguished from the parallel configuration where
splitting also exists, even though it is for symmetric case. We also
analyze how to compensate the splitting and restore the suppressed
zero-bias Kondo resonance. It is shown that one can change the TMR
ratio significantly from a negative dip to a positive peak only by
slightly modulating a local external magnetic field, whose value is
greatly dependent on the electron--phonon coupling strength. 相似文献
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从双子晶格Hubbard模型出发,应用变分泛函积分方法,研究了巡游电子反铁磁性.该方法的关键在于:对Hubbard哈密顿量的相互作用部分作Stratonovich-Hubbard变换时,采用连续分解方案,导致自旋涨落与电荷涨落的分离,从而能更好地描述两类涨落所具有的相反倾向的性质.在连续分解中所引入的参数由变分原理确定,从而消除了泛函积分理论中的“不确定性”困难.本文还对半满带情形作了数值研究,计算了基态性质,奈耳温度,磁化强变以及顺磁磁化率等.与Hasegawa理论比较,在磁化率的温度依赖行为方面有一定
关键词: 相似文献
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针对X光谱分析研究中经常遇到的谱峰重叠问题,提出了一种基于标准差关联的高斯混合模型(GMM-SDR)和粒子群算法的重叠谱峰解析方法。首先,介绍了重叠峰的GMM-SDR模型,并以GMM-SDR参数构成粒子位置,给出了粒子目标函数及适应度值的快速算法;然后,利用粒子群算法的群体搜索能力,以搜索最优GMM-SDR模型,进而实现重叠峰的分解。初始值采用随机设定,将测量的所有随机数据作为一个整体,以其对模型的概率匹配程度作为适应度值,故该方法避免了初值设定不当带来的局部收敛问题,克服了传统曲线拟合方法对原始有用数据的破坏,所搜索到的模型是一个全局最优解。通过对四个及以下重叠谱峰的分解表明,该方法分解精度较高,其中,两峰重叠谱分解后的峰位、峰面积及标准差最大相对误差分别为0.4%,0.05%和2.07%,三峰重叠谱分解后的峰位、峰面积及标准差最大相对误差分别为1.2%,0.04%和0.74%,可适用于各种严重重叠谱峰的分解。 相似文献
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