Low-threshold, 12-MHz, multipass-cavity femtosecond Cr4+: Forsterite laser

We report on the development of an extended-cavity, low-threshold femtosecond Cr⁴⁺:forsterite laser operating near 1270 nm. The resonator was end-pumped by a continuous-wave Yb-fiber laser at 1060 nm. The 195-MHz short cavity could be operated with absorbed threshold pump powers as low as about 300 mW. To scale up the pulse energy, the cavity length was increased by using a q-preserving multipass cavity (MPC) consisting of a flat and a curved (R = 4 m), notched high-reflector. Kerr-lens mode locking was used to generate femtosecond pulses and double-chirped mirrors were included in the cavity for dispersion compensation. With an absorbed pump power of 1250 mW, the mode-locked laser produced 4 nJ of pulse energy at an average output power of only 47 mW. The corresponding repetition rate of the extended cavity was 11.7 MHz. The pulse-width was 90 fs and the spectral bandwidth was 23 nm, corresponding to a time-bandwidth product of 0.37.     

Low-cost low-threshold diode end-pumped Tm:YAG laser at 2.016?μm

We report a low-threshold continuous-wave Tm:YAG laser that can be excited near 785?nm with low-cost, single-mode AlGaAs laser diodes. Low-threshold operation was achieved using a tightly focused, astigmatically compensated x-cavity containing a 2-mm-thick Tm:YAG crystal with 5?% Tm³⁺ concentration. Two linearly polarized single-mode diodes operating at 785.8?nm were polarization coupled to end pump the resonator. With a 6?% output coupler, as high as 32?mW of output power could be obtained at 2016?nm with 184?mW of incident pump power. The output could be further tuned in the 1935?C2035?nm range. Slope efficiency measurements indicated that cross-relaxation was very effective at this doping level. With a 2?% output coupler, lasing could be obtained with as low as 32.3?mW of pump power. In the limit of vanishing output coupling, the incident threshold pump power could be reduced to as low as 25?mW. To our knowledge, this is among the lowest lasing thresholds reported to date for continuous-wave, room-temperature thulium lasers.     

Intracavity-pumped Cr2+:ZnSe laser with ultrabroad tuning range between 1880 and 3100 nm

We obtained, what is to our knowledge, record tuning from an intracavity-pumped gain-switched Cr2+:ZnSe laser. In the experiments, a polycrystalline Cr2+:ZnSe sample with an absorption of about 43% at 1570 nm was used to minimize reabsorption losses at the lasing wavelengths below 2000 nm. By placing the gain medium inside the cavity of a pulsed KTP optical parametric oscillator (OPO) operating at 1570 nm, smooth, continuous tuning was achieved in the 1880-3100 nm range with four different sets of cavity optics. As high as 145 mW of average laser output power was obtained at 2365 nm with 1.2 W of intracavity OPO power.     

Synthesis and characterization of poly(acrylic acid) stabilized cadmium sulfide quantum dots

Cadmium sulfide (CdS) nanoparticles (NPs) capped with poly(acrylic acid) (PAA) were prepared in aqueous solutions from Cd(NO3)2 and Na2S. Influence of the COOH/Cd ratio (0.8-12.5), reaction pH (5.5 and 7.5), and PAA molecular weight (2100 and 5100 g/mol) on the particle size, colloidal stability, and photoluminescence were investigated. A Cd/S ratio of <1 causes ineffective passivization of the surface with the carboxylate and therefore results in a red shift of the absorption band and a significant drop in photoluminescence. Therefore, the Cd/S ratio was fixed at 1.1 for all experiments studying the mentioned variables. PAA coating provided excellent colloidal stability at a COOH/Cd ratio above 1. Absorption edges of PAA-coated CdS NPs are in the range of 460-508 nm. The size of the NPs increases slightly with increasing PAA molecular weight and COOH/Cd ratio at pH 7.5. It is demonstrated that there is a critical COOH/Cd ratio (1.5-2) that maximizes the photoluminescence intensity and quantum yield (QY, 17%). Above this critical ratio, which corresponds to smaller crystal sizes (3.7-4.1 nm) for each reaction set, the quantum yield decreases and the crystal size increases. Moreover, CdS NPs prepared at pH 7.5 have significantly higher QY and absorb at lower wavelengths in comparison with those prepared at pH 5.5. Luminescence quenching has not been observed over 8 months.     

Energy scaling of a carbon nanotube saturable absorber mode-locked femtosecond bulk laser

We report successful energy scaling of a room-temperature femtosecond Cr⁴⁺: forsterite laser by using a single-walled carbon nanotube saturable absorber (SWCNT-SA). By incorporating a q-preserving multipass cavity, a repetition rate of 4.51?MHz was realized, and the oscillator produced 121?fs, 10?nJ pulses at 1247?nm, with an average output power of 46?mW. To the best of our knowledge, the peak power of 84?kW is the highest generated to date from a SWCNT-SA mode-locked oscillator. Furthermore, energy scaling of a femtosecond multipass-cavity laser, mode-locked using a SWCNT-SA, is demonstrated for the first time.     

Injection-seeded, gain-switched tunable Cr:ZnSe laser

We report a narrow-linewidth, tunable, gain-switched Cr:ZnSe laser operating between 2255 and 2455 nm. The spectral width of the laser was reduced from 125 nm to 0.3 nm by using injection seeding. Seeding was achieved with a second tunable CW Cr:ZnSe laser. The output wavelength was varied by tuning the wavelength of the seed laser. The seeded oscillator produced as high as 157 μJ pulses with 598 μJ incident pump pulse energy at a repetition rate of 1 kHz. The slope efficiency was determined to be 26%.     

Nanoscale plasmonic devices for dynamically controllable beam focusing and scanning

We have performed simulations to investigate the variable focusing and scanning capability of metallic nano-slit configurations. In a symmetric nanorod configuration inside an aperture with adjustable offset of the center rod, the focal position is found to be variable in the 0.5–3.5 μm range. In a ladder configuration of the rods, the transmitted beam is found to be deflected up to 23°. Horizontal displacement of rods allows for finer control of angular scanning up to 4°. Such slit geometries offer the potential to be controlled by using nano-positioning systems for applications in dynamic beam shaping and scanning on the nanoscale.     

Lasing at 1065 nm in bulk Nd-doped telluride-tungstate glass

We have achieved, for the first time to our knowledge, lasing in a new type of telluride-tungstate glass host doped with neodymium: Nd³⁺:(0.8)TeO₂-(0.2)WO₃. Lasing was obtained at 1065 nm with two samples containing 0.5 mol% and 1.0 mol% Nd₂O₃. During gain-switched operation, slope efficiencies of 12% and 10% were obtained with the 0.5 mol% and 1.0 mol% doped samples, respectively, at a pulse repetition rate of 1 kHz. Judd-Ofelt analysis was further employed to determine the emission cross section σ_e at 1065 nm from the absorption spectra and lifetime data. The emission cross section from the Judd-Ofelt analysis came to 3.23 ± 0.09 × 10⁻²⁰ cm², in reasonable agreement with the value of 2.0 ± 0.13 × 10⁻²⁰ cm² obtained from the analysis of laser threshold data.     

Bulk Nd3+-doped tellurite glass laser at 1.37 μm

We have demonstrated, for the first time to our knowledge, lasing at 1.37 μm in a tellurite-based glass host doped with 0.5 mol.% neodymium: Nd³⁺:(0.8)TeO₂–(0.2)WO₃. The gain-switched laser could be operated with 59 μJ threshold pulse energy as well as 5.5% slope efficiency. As high as 6 μJ-pulses with a duration of 1.74 μs were obtained. The pulse repetition rate was 1 kHz. The emission cross section from the threshold analysis turned out to be 1.57×10^?20 cm² at 1370 nm by taking into account excited-state absorption from ⁴F_3/2 to ⁴G_7/2 energy level. Furthermore, the ratio of excited-state absorption to the emission cross section was found out to be 0.78 by using the slope efficiency value.     

Direct generation of 81 nJ pulses and external compression to a subpicosecond regime with a 4.9 MHz chirped-pulse multipass-cavity Cr⁴⁺:forsterite oscillator

We report direct generation of 81 nJ chirped pulses from a room-temperature, Kerr lens mode-locked Cr??:forsterite oscillator operating at 1258 nm. To increase the pulse energy, the pulse repetition rate of the short x-type resonator was lowered from 143 to 4.9 MHz by the addition of a q-preserving multipass cavity, which provided an additional effective optical path length of 59.4 m. The duration of the chirped pulses was around 5.5 ps with a spectral width of 21 nm. The pulses were externally compressed to 607 fs by using a diffraction grating pair. To our knowledge, this is the highest reported pulse energy directly generated from a room-temperature mode-locked Cr??:forsterite laser.