噁嗪750激光染料分子在醇类溶剂中超快动力学研究

利用飞秒时间分辨荧光亏蚀光谱技术,研究了噁嗪750激光染料分子在典型的醇类溶剂中超快动力学过程.实验发现两个超快动力学过程:飞秒量级的快速弛豫过程和皮秒量级的慢速弛豫过程.快速弛豫过程来源于分子内振动能量再分配(IVR)和溶剂分子超快惯性弛豫动力学过程,而慢速弛豫过程对应于溶剂化的扩散分子弛豫动力学过程.实验结果表明慢速弛豫过程的时间常数随醇溶剂分子间氢键键能的增强而增大.     

In situ SEOP polarised He neutron spin filter for incident beam polarisation and polarisation analysis on neutron scattering instruments

We discuss the development and characterisation of a new in situ spin exchange optical pumping (SEOP) based ³He neutron spin filter polarisation device. We present results from a recent test of the prototype system developed with the Institut Laue-Langevin. The polariser was installed on the polarised reflectometer CRISP at ISIS in the analyser position. The ³He was pumped continuously in situ on the beamline. The system also integrated a ³He adiabatic fast passage spin flipper that allowed reversal of the ³He and therefore neutron polarisation state, allowing for measurement of all four polarisation cross-sections. The system was run for a number of days reaching a ³He polarisation of 63%.     

Increasing the pump-up rate to polarize He gas using spin-exchange optical pumping method

In recent years, polarized ³He gas has increasingly been used as neutron polarizers and polarization analyzers. Two of the leading methods to polarize the ³He gas are the spin-exchange optical pumping (SEOP) method and the meta-stable exchange optical pumping (MEOP) method. At present, the SEOP setup is comparatively compact due to the fact that it does not require the sophisticated compressor system used in the MEOP method. The temperature and the laser power available determine the speed, at which the SEOP method polarizes the ³He gas. For the quantity of gas typically used in neutron scattering work, this speed is independent of the quantity of the gas required, whereas the polarizing time using the MEOP method is proportional to the quantity of gas required. Currently, using the SEOP method to polarize several bar-liters of ³He to 70% polarization would require 20−40 h. This is an order of magnitude longer than the MEOP method for the same quantity of gas and polarization. It would therefore be advantageous to speed up the SEOP process. In this article, we analyze the requirements for temperature, laser power, and the type of alkali used in order to shorten the time required to polarize ³He gas using the SEOP method.     

光磁共振实验中扫场和水平场关系的探究

光泵磁共振实验中,在磁共振信号观察时,常常会有光抽运信号同时出现的现象,这严重影响了实验的有效观察和准确测量。本文阐述了取合适的扫场和水平场的大小的关系,从而避免实验过程中磁共振信号和光抽运信号的同时出现,以确保实验的精准。     

Spectral and temporal features of multiple spontaneous NMR-maser emissions

When a system composed of dissolved laser-polarized xenon with negative spin temperature is put inside a high field NMR magnet, a series of spontaneous maser emissions can be observed. We report here their spectral and temporal features using a processing model derived from the solution of the Bloch equations in the presence of radiation damping. We show, in particular, that by combining Fourier transformation and squared modulus, a parameter allowing the characterization of the burst of transverse magnetization can be determined. This parameter is shown to be correlated with the radiated energy. Moreover, this processing clearly reveals features which can probably be assigned to effects resulting from distant dipolar fields. Finally, the analysis of the experimental data reveals an unexpected behavior of the ¹²⁹Xe transverse self-relaxation.     

LD抽运Cr,Tm,Ho∶YAG微片激光器单纵模运转特性的研究

研究了LD抽运的单纵模Cr,Tm,Ho∶YAG微片激光器,激光器厚度为1?mm,在用波长785?nm的LD进行端面抽运时,激光器阈值为1060?mW,单纵模激光最大输出功率为31?mW. 对激光器输出功率随温度变化特性进行了研究,验证了CTH∶YAG晶体的温度敏感性. 还研究了激光器的温度调谐特性,实验测得激光器的温度调谐系数为14?GHz/℃. 关键词： 激光光学 CTH∶YAG微片激光器 LD抽运 单纵模运转     

High repetition rate laser pulses amplified by Nd/Cr:YAG ceramic amplifier under CW arc-lamp-light pumping

Laser pulses with high repetitive rate generated from a Q-switch microchip Nd:YAG oscillator were amplified by Active mirror composed of Nd/Cr:YAG ceramic pumped by CW arc-lamp. The laser pulses were amplified, and saturation of averaged output laser power was observed. Repetitive ratio of injected laser pulses was changed from 20 to 100 kHz. Averaged output laser power and gain were measured, and gain coefficient and power-extraction efficiency were evaluated. Output laser power was calculated and compared to experimentally measured one, and the calculated results are consistent with the experimental ones. For amplification of laser pulses with high repetitive ratio, this laser material can realize very high laser gain with low pumping power density and high optical-optical conversion efficiency under CW-lamp-light pumping.     

光泵磁共振实验探究

本文分析了光磁共振实验中,观察到光抽运信号和磁共振信号的条件,并重点对方波和三角波扫场对光抽运信号和磁共振信号的作用和影响进行了讨论,阐明了应如何选择方波和三角波扫场信号的大小和方向,才能得到理想的光抽运信号和磁共振信号。     

Rb87基态超精细塞曼能级跃迁的偏振激发特性

本论述了Rb^87基态超精细塞曼能级光泵磁共振的偏振激发特性,给出了塞曼能级跃迁谱线随抽运光偏振特性的变化。     

A standing wave model for acoustic pumping effect in microchannels

An acoustic impedance pump is comprised of a compressible section coupled at both ends to sections of different acoustic impedances. Liquid can be pumped from one end to another if the compressible section is actuated at certain locations. This paper presents an analytical model on the acoustic pumping effect in microchannels. A one-dimensional wave equation is developed for acoustic pressures in the compressible section, taking into account the actuations as acoustic source terms. The solution for the acoustic pressure is a set of standing waves established inside the compressible section, corresponding to the actuations. The pumping effect is attributed to the second-order terms of the acoustic pressures. Two control parameters are identified. One is the resonance frequency associated with the sound wave speed and length of the compressible section, and the other is the damping factor. The analytical results are compared with the experimental data, and a qualitative agreement is observed in terms of frequency characteristics of the pumping pressure.