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961.
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963.
964.
Plasma‐solution interface plays the important role in the systems of the electrical discharges with or in liquids (electrolyte solutions). Processes, which pass at this interface, influence on as plasma as liquid. In this paper, the theoretical and experimental results of studies of the double layer on the liquid surface are presented. Data of cathode region properties, kinetics of nonequilibrium vaporization, correlation between radiation intensity and fluxes from electrolyte cathode surface and energy consumptions per on one water molecule transfer are summarized. It is able to suggest the transfer mechanism at the plasma‐solution interface. (© 2013 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim) 相似文献
965.
Diffusion-weighted MRI images acquired at b-value greater than 1000 s mm− 2 measure the diffusion of a restricted pool of water molecules. High b-value images are accompanied by a reduction in signal-to-noise ratio (SNR) due to the application of large diffusion gradients. By fitting the diffusion tensor model to data acquired at incremental b-value intervals, we determined the effect of SNR on tensor parameters in normal human brains, in vivo. In addition, we also investigated the impact of field strength on the diffusion tensor model. Data were acquired at 1.5 and 3 T, at b-values 0, 1000, 2000 and 3000 s mm− 2 in twenty diffusion-sensitised directions. Fractional anisotropy (FA), mean diffusivity (MD) and principal eigenvector coherence (κ) were calculated from diffusion tensors fitted between datasets with b-values 0–1000, 0–2000, 0–3000, 1000–2000 and 2000–3000 s mm− 2. Field strength and b-value effects on diffusion parameters were analysed in white and grey matter regions of interest. Decreases in FA, κ and MD were found with increasing b-value in white matter. Univariate analysis showed a significant increase in FA with increasing field strength in highly organised white matter. These results suggest there are significant differences in diffusion parameters at 1.5 and 3 T and that the optimal results, in terms of the highest values of FA in white matter, are obtained at 3 T with a maximum b = 1000 s mm− 2. 相似文献
966.
采用共沉淀法制备了不同Eu3+掺杂浓度的Gd2(WO4)3纳米发光材料. 测量了纳米材料样品的X射线衍射谱(XRD) 和场发射扫描电镜, 对样品的结构和形貌进行了表征. 测量了各样品的发射光谱和激发光谱(声子边带光谱), 绘制了浓度猝灭曲线, 确定了最佳的掺杂浓度为20 mol%. 通过声子边带光谱计算了不同掺杂浓度样品的黄昆因子. 测量了不同浓度样品的荧光寿命, 利用Auzel模型对Eu3+ 5D0能级荧光寿命数据进行了拟合, 确定了5D0能级的固有寿命和猝灭过程中生成的声子数. 本文还根据荧光寿命数据计算了Eu3+之间的能量传递速率, 确定了能量传递速率与浓度的关系.
关键词:
钨酸盐
3+')" href="#">Eu3+
黄昆因子
能量传递速率 相似文献
967.
The promotion/prevention mechanism of dissolved gases on cavitation inception is essential for many high-tech industries and research. In the present study, large-scale molecular dynamics simulations are performed to investigate the effects of water cavitation caused by different gas types by using nitrogen and oxygen gases with TIP4P/2005 water. The cavitation inception behaviour is analyzed via Mean First Passage Time method. Water with dissolved gases has a higher nucleation rate and is easier to cavitate than pure water. At the same gas concentration, the cavitation of water with nitrogen is promoted to a greater extent than that with oxygen. The number and energy of hydrogen bond (HB) are further calculated by the Acceptor-Hydrogen-Donor method to explain this promotion mechanism. The number and energy of HB in water with gases decrease compared with those in pure water. The introduction of gases weakens the HB network and promotes cavitation inception because of weaker interactions between gas and water molecules. A model is developed to describe the relationship between nucleation rate and HB energy. Gas molecules assemble on the surface of bubbles during water cavitation, which may decrease the free energy of bubble surface, maintain the existing bubble, and contribute to the growth process. 相似文献
968.
Aniruddha Chakraborty 《Molecular physics》2013,111(17):1777-1786
We consider a suspended elastic rod under longitudinal compression. The compression can be used to adjust potential energy for transverse displacements from the harmonic to the double well regime. The two minima in potential energy curve describe two possible buckled states. Using transition state theory (TST) we have calculated the rate of conversion from one state to other. If the strain ? = 4? c the simple TST rate diverges. We suggest a method to correct this divergence for quantum calculations. We also find that zero point energy contributions can be quite large so that single mode calculations can lead to large errors in the rate. 相似文献
969.
J. Assaf 《辐射效应与固体损伤》2013,168(6):384-391
Dose rate effects on the noise characteristics of gamma-irradiated junction field effect transistors (JFETs) are presented. The dose rate varied between 0.5 and 19 kGy/h at a constant radiation dose of 600 kGy. Neither obvious nor non-general relationship was identified between noise and dose rate along the total dose rate range. Nevertheless, some explanations have been provided about the resulting effects when the total range was studied, as some partial ranges corresponded to low, medium and high dose rates. This explanation is based on the gamma interaction process in JFET structure and the electronic noise resulted. 相似文献
970.
Lingqing Wang 《辐射效应与固体损伤》2013,168(9):677-683
Radionuclides are released together with fly ash from the coal-fired power plant and thus add to the natural radiation. Fifty soil samples were collected around the Baoji coal-fired power plant from 25 locations and the natural radionuclide concentrations were determined by a gamma ray spectrometric system. The results show that the activity concentrations in soil samples range from 12.54 to 40.18 Bq kg?1, 38.02 to 72.55 Bq kg?1 and 498.02 to 1126.98 Bq kg?1 for 226Ra, 232Th and 40K with the mean values of 27.35, 52.66 and 764.72 Bq kg?1, respectively. In order to evaluate the radiological hazard of the natural radioactivity, the radium equivalent activity (Raeq), the absorbed dose rate (D) and the annual effective dose rate have been calculated and compared with the internationally approved values. The radium equivalent activity in all the soil samples is lower than the safe limit set in the Organization for Economic Cooperation and Development report (370 Bq kg?1). The average value of the calculated dose rates is higher than the global average value 55 nGy h?1, and the calculated annual effective dose rate is significantly lower than the average annual external effective dose rate (460 μSv y?1) of the normal background radiation. 相似文献