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81.
82.
We consider the relaxation dynamics of two quantum levels coupled to a stochastic bath. We emphasize that even if the matrix elements of the fluctuating Hamiltonian are Gaussian, a second-order cumulant truncation is not exact. For various stochastic models, including the case of a spin-1/2 particle in a fluctuating magnetic field, we calculate 1/T
1, the population relaxation rate, and 1/T
2, the phase relaxation rate, up to fourth order in perturbation theory. We show that unlike the commonly accepted second-order result that 1/T
21/2T
1, when fourth-order terms are included, in some instances 1/T
2<1/2T
1. 相似文献
83.
The relation between the aperiodic solution of the Lorenz model and that of a stochastic anharmonic oscillator is explored. The stochastic oscillator is constructed by replacing (t) in the Lorenz model by a stochastic variable(t) of specified statistics. The resulting system is of course not isomorphic to the Lorenz model, but does share with it a number of statistical properties. Thus, within the confines of these measures the two systems are physically very similar. 相似文献
84.
Darian E Hnizdo V Fedorowicz A Singh H Demchuk E 《Journal of computational chemistry》2005,26(7):651-660
A method of statistical estimation is applied to the problem of evaluating the absolute entropy of internal rotation in a molecule with two torsional degrees of freedom. The configurational part of the entropy is obtained as that of the joint probability density of an arbitrary form represented by a two-dimensional Fourier series, the coefficients of which are statistically estimated using a sample of the torsional angles of the molecule obtained by a stochastic simulation. The internal rotors in the molecule are assumed to be attached to a common frame, and their reduced moments of inertia are initially calculated as functions of the two torsional angles, but averaged over all the remaining internal degrees of freedom using the stochastic-simulation sample of the atomic configurations of the molecule. The torsional-angle dependence of the reduced moments of inertia can be also averaged out, and the absolute internal-rotation entropy of the molecule is obtained in a good approximation as the sum of the configurational entropy and a kinetic contribution fully determined by the averaged reduced moments of inertia. The method is illustrated using Monte Carlo simulations of isomers of stilbene and halogenated derivatives of propane. The two torsional angles in cis-stilbene are found to be much more strongly correlated than those in trans-stilbene, while the degree of the angular correlation in propane increases strongly on substitution of hydrogen atoms with chlorine. 相似文献
85.
A novel hybrid optimization method called quantum stochastic tunneling has been recently introduced. Here, we report its implementation within a new docking program called EasyDock and a validation with the CCDC/Astex data set of ligand-protein complexes using the PLP score to represent the ligand-protein potential energy surface and ScreenScore to score the ligand-protein binding energies. When taking the top energy-ranked ligand binding mode pose, we were able to predict the correct crystallographic ligand binding mode in up to 75% of the cases. By using this novel optimization method run times for typical docking simulations are significantly shortened. 相似文献
86.
In this paper, we establish the discrete approximation of continuous-state nonlinear branching processes in Lévy random environments by using tightness and convergence sequence in infinite dimensional product space via stochastic differential equations. Taking α-stable branching as an example, the conditions which are given to discretize continuous-state nonlinear branching processes in Lévy random environments are verified. © 2022 Chinese Academy of Sciences. All rights reserved. 相似文献
87.
本文研究了数值求解非自治随机微分方程的正则Euler-Maruyama分裂(CEMS)方法,该方程的漂移项系数带有刚性且允许超线性增长,扩散项系数满足全局Lipschitz条件.首先,证明了CEMS方法的强收敛性及收敛速度.其次,证明了在适当条件下CEMS方法是均方稳定的.进一步,利用离散半鞅收敛定理,研究了CEMS方法的几乎必然指数稳定性.结果表明,CEMS方法在漂移系数的刚性部分满足单边Lipschitz条件下可保持几乎必然指数稳定性.最后通过数值实验,检验了CEMS方法的有效性并证实了我们的理论结果. 相似文献
88.
该文讨论了一类带扰动的随机脉冲泛函微分方程解的渐近性.通过比较扰动方程的解和原方程的解,得到了两者逼近的充分条件.首先,两者在有限的时间区间上相互逼近;其次,当扰动趋于零时,区间长度趋于无穷大,在这个区间上两个解仍然是相互逼近的.最后,举例说明了结果的有效性. 相似文献
89.
90.
形状记忆合金(SMA)是二十一世纪具有形状记忆效应的新型智能材料.针对具有非对称约束的SMA梁,本文构造了碰撞振动系统.在无碰撞和有碰撞两种情况下,利用随机平均法给出了近似解析结果.数值模拟作为验证解析结果的工具.结果表明,系统能量的概率响应曲线具有非光滑特性.当约束位置发生变化时,系统会出现随机P分岔和D分岔. 相似文献