On the stability of the nuclei of element 108 withA=263–265

In bombarding²⁰⁹Bi and^{207, 208}Pb targets by⁵⁵Mn and⁵⁸Fe ions the yields of “cold fusion” reactions have been determined using a sensitive technique for detectingT _1/2≧1 ms spontaneous fission and theα-decay of heavy actinide elements. It has been shown that theA = 263–265 isotopes of element 108, including the even-even isotope²⁶⁴108, undergo mainlyα-decay. The obtained results, together with the known data on the properties of the isotopes of elements 104 and 106, provide evidence for the enhanced stability of theZ=108 nuclei against spontaneous fission.     

Development of tBu-phenyl Acetamide Appended Thiacalix[4]arene as “Turn-ON” Fluorescent Probe for Selective Recognition of Hg(II) Ions

Journal of Fluorescence - Herein, a novel N-(4-(tert-butyl)-phenyl)-2-chloroacetamide functionalized thiacalix[4]arene architecture, viz TCAN2PA has been synthesized and the sensing behaviour...     

On the properties of the element 106 isotopes produced in the reactions Pb+54Cr

In⁵⁴Cr ion bombardments of targets prepared from enriched lead isotopes the spontaneous fission probability for the isotopes of element 106 formed in the reactions Pb(⁵⁴Cr, 1,2n)106 was investigated. The spontaneous fission half-life of the doubly-even isotope²⁶⁰106 has been shown to beT _SF?5 ms. The half-lives of neighbouring oddmass isotopes have also been estimated:T _SF(²⁵⁹106)?0.1 s andT _SF(²⁶¹106)?0.4 s. The results of the experiments are discussed in comparison with the latest theoretical calculations.     

Synthesis of 292116 in the 248Cm + 48Ca reaction

We report on the observation of the first decay event of the new nuclide ²⁹²116 produced in an experiment devoted to the synthesis of Z=116 nuclei in the ²⁴⁸Cm + ⁴⁸Ca reaction. The implantation of a heavy recoil in the focal-plane detector was followed in 46.9 ms by an α particle with E _α=10.56MeV. The energies and decay times of the descendant nuclei are in agreement with those observed in the decay chains of the even-even isotope ²⁸⁸114, previously produced in the ²⁴⁴Pu + ⁴⁸Ca reaction. Thus, the first α decay should be attributed to the parent nuclide ²⁹²116 produced via the evaporation of four neutrons in the complete fusion of ²⁴⁸Cm and ⁴⁸Ca. The experiment is in progress at Flerov Laboratory for Nuclear Reactions (FLNR, JINR, Dubna).     

Growth morphology of zinc tris(thiourea) sulphate crystals

The growth morphology of crystals of zinc tris(thiourea) sulphate (ZTS) is investigated experimentally, and computed using the Hartman-Perdok approach. Attachment energies of the observed habit faces are calculated for determining their relative morphological importance. A computer code is developed for carrying out these calculations. A special procedure is adopted for computing the cohesive energy of a slice of the structure parallel to any rational crystallographic plane. For estimating the cohesive energies, formal charges on the experimentally determined atomic positions in the molecules of ZTS are calculated by ab initio molecular-orbital computations, with wave functions obtained by the Hartree-Fock procedure. Fairly good agreement with the observed crystal morphology is obtained for a model of growth mechanism in which ZTS is assumed to exist in solution sa szinc tris(thiourea) ions and sulphate ions.     

Synthesis of superheavy nuclei in 48Ca+244Pu interactions

This article reports the results of experiments aimed at producing hypothetical long-lived superheavy elements located near the spherical-shell closures with Z≥114 and N≥72. For the synthesis of superheavy nuclei, we used a combination of neutron-rich reaction partners, with a ²⁴⁴Pu target and a ⁴⁸Ca projectile. The sensitivity of the present experiment exceeded by more than two orders of magnitude previous attempts at synthesizing superheavy nuclides in reactions of ⁴⁸Ca projectiles with actinide targets. We observed new decay sequences of genetically linked alpha decays terminated by spontaneous fission. The high measured alpha-particle energies, together with the long decay times and spontaneous fission terminating the chains, offer evidence for the decay of nuclei with high atomic numbers. The decay properties of the synthesized nuclei are consistent with the consecutive alpha decays originating from the parent nuclides ^288,289114, produced in the 3n-and 4n-evaporation channels with cross sections of about a picobarn. The present observations can be considered experimental evidence for the existence of the “island of stability” of superheavy elements and are discussed in terms of modern theoretical approaches.     

Relative wavefunctions, vertex functions and coupling constants for the virtual decay of 4He

The d + d, t + p and h + n relative wavefunctions and their asymptotic normalizations are considered in the framework of the generator coordinate method (GCM) and compared with ATMS (amalgamation of two-body correlation into multiple scattering processes) method which used the realistic Reid soft core interaction. The asymptotic normalization of relative wavefunctions provide various coupling constants, the cluster probability amplitude (the so-called Z ^1/2-factor) and matter RMS radii. These wavefunctions are also used to obtain ⁴He − d − d, ⁴He − t − p and ⁴He − h − n vertex functions in the virtual decay of ⁴He. The extrapolation of vertex functions for negative values of q ² upto the corresponding poles provide the vertex constants which are comparable with other estimates. It is noticed that in GCM the coupling constants C ² for ⁴He − d − d vertex is less than 2 as has been obtained in the forward dispersion relation technique.