Ar气对~(39)K_2分子C~1Ⅱ_u→X~1∑_g~+LIF光谱的碰撞猝灭效应

实验测量了缓冲气体Ar气对~(39)K_2分子C~1Π_u(v′=O,J′=53)→X~1∑_g~+(v″=5,6,J″=52,54)LIF光谱的碰撞猝灭效应.用稳态碰撞模型推导出LIF光谱强度I对气体压强P=P_(Ar)+P_K的函数关系.用上述模型拟合出的I-P曲线和实验数据的符合,对拟合所得参数C_1的进一步分析指出:热管炉后向探测LIF光谱方法比非增益荧光探测法的灵敏度可提高2倍以上.     

Ar~+激光激发的LiArA~2Ⅱ→X~2∑漫射谱发射

用Ar~+的457.9,476.5,496.5,514.5nm激光激发充有Ar气的Li热管,获得Vander Waal's分子LiAr在650—760nm波长范围A~2П→X~2∑的漫射发射光谱。讨论了产生这种发射的动力学机制。     

Theoretical study of quasi-phase-matching fourth harmonic generation in periodically poled lithium tantalate

The direct fourth harmonic generation (FHG) is theoretically demonstrated based on quasi-phase-matching (QPM) configuration in periodically poled lithium tantalate (PPLT). The wavelength dependence of the period of FHG QPM gratings is calculated. Bandwidths of fundamental wavelength, temperature, and incident angle are also studied. A very wide bandwidth, as large as 119.5 nm, of fundamental wavelength near 3699 nm is found with the QPM period of 9.442 μm and the crystal length of 1 cm.     

I型准相位匹配周期性极化铌酸锂倍频蓝光输出

在周期为 14 .5 μm的周期性极化铌酸锂中 ,利用d3 1,得到了一阶I型EωYEωY-E2ωZ (oo-e)准相位匹配蓝光二次谐波。在 15 0℃下 ,由 114 μJ抽运光 ,得到了 5 2 μJ ,0 .4 73μm倍频蓝光 ,对应于平均最大转换效率 4 5 .6 %。制备了一阶和三阶周期分别为 4 .5 μm和 13.5 μm的周期性极化铌酸锂。在EωZEωZ-E2ωZ (ee -e)准相位匹配 0 .4 73μm蓝光倍频中 ,15 0℃下 ,分别得到了 4 1.3%和 19%的倍频转换效率。oo -e准相位匹配比传统的ee -e准相位匹配有较大的光栅周期 ,尤其在短波长区域倍频输出应用中 ,降低了周期性结构制作的困难 ,其较大的容许带宽在实验中提高了频率转换效率。实验结果表明了在周期性极化铌酸锂中准相位匹配倍频的偏振相关性。     

Generation of the numerator=2 rational harmonic mode-locked pulses in fiber ring lasers

In conventional rational harmonic mode-locking, optical pulse trains with the repetition rate of (pn+1)f_c are generated when the modulation frequency of the in-cavity modulator is set at f_m = (n+1/p)f_c, where n and p are both integers, f_c is the fundamental cavity frequency. In this paper, we report that rational harmonic mode locking phenomenon takes place in the fiber lasers when the modulation frequency is set at f_m =(n+2/p)f_c. The pulse generations are experimentally demonstrated when the numerator of the rational corresponds to 2 in 5th and 7th order rational harmonic mode-locking.     

Generation of broadband and multiple-peak THz radiation in aperiodically poled lithium niobate

Terahertz (THz) regime has become the most attracting frequency range in the electromagnetic radiation in re- cent years[1-3]. Single-cycle THz waves intrinsically pos- sess a broad bandwidth[1]. Unfortunately, the generated THz waveform is very weak and inhomogeneous for the THz frequency. It has been proved experimentally[2-4] that the velocity mismatch between the THz pulse and the optical femto-second pulse in the periodically poled lithium niobate (PPLN) allows the generation of ult…     

K_2分子2~3∏_g—1~3∑_u~+漫射谱强度的碰撞诱导增强效应

用4415.6ACW激光线获得了5730A附近的K_2分子2~3∏_g—1~3∑_u~+漫射荧光谱。实验研究了缓冲气体Ar气压强P对漫射谱峰值强度I_(diff)的碰撞诱导增强效应。用稳态碰撞模型描述了C~1∏_u—2~3∏_g间的能量转移过程,推导出了I_(diff)-P函数关系,对实验数据进行了令人满意的拟合。这种拟合表明:适当变更实验装置,利用本文模型可以得到C~1∏_u—2~3∏_g间的能级交叉速率和碰撞诱导转移速率。     

~(39)K_2分子C~1Ⅱ_u-X~1∑_9~+(J′=105)Q支激光诱导荧光光谱及电偶极跃迁矩变化率研究

用4415.6(?)CW激光线获得了~(39)K_2分子C~1II_u(v′=0,J′=105)-X~1∑_g~+(v″=1～10,J″=105)Q支激光诱导荧光(LIF)光谱.用最小二乘法拟合出了~(39)K_2分子X~1∑_g~+态振动常数和C~1II_u态电子谱项值T_e.光谱分析表明C~1II_u态T_e=22968cm~(-1)是合适的.用~(39)K_2分子Morse势计算了(V′=0,J′=105)-(v″=1～10,J″=105)跃迁的Franck-Condon因子和跃迁强度,强度计算值和激光诱导荧光光谱测量值之间有令人满意的符合,进一步的r重心近似分析给出了~(39)K_2分子C~1II_u→X~1∑_g~+电偶极跃迁矩R_(?)随核间距r的归一化变化率为-0.157～-0.168 debye/(?)(4.22(?)相似文献   

基于集成光学的ICF脉冲整形系统

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