高离化态Hg和U离子的双电子复合过程的理论研究

在相对论多组态Dirac-Fock理论基础上，利用近期发展的计算双电子复合截面的程序，系统研究了高离化态类氦到类硼Hg和U离子的KLL双电子复合过程. 讨论了Breit效应和量子电动力学(QED)效应对Hg离子共振双激发态能级的贡献，得到了双激发态的共振能、总线宽和相应的双电子复合共振强度，所得结果与其他理论和实验结果都符合得很好. 在此基础上进一步研究了高离化态U离子的KLL双电子复合过程，并与已有的实验和理论结果作了比较.     

类锂离子KLL双电子复合过程研究

采用相对论扭曲波方法,理论研究了高离化态类锂离子I~(50+)、Ho~(64+)、Bi~(80+)的KLL双电子复合过程,得到了双电子激发态的共振能量和双电子复合截面,利用自电离和辐射跃迁速率,得到了对应谱线的总宽度,并与已有的理论和实验结果进行了对比,理论较好地解释了最近的实验结果.     

类锂离子KLL双电子复合过程研究

采用相对论扭曲波方法,理论研究了高离化态类锂离子I50+、Ho64+、Bi80+的KLL双电子复合过程,得到了双电子激发态的共振能量和双电子复合截面,利用自电离和辐射跃迁速率,得到了对应谱线的总宽度,并与已有的理论和实验结果进行了对比,理论较好地解释了最近的实验结果。     

类氦铀离子的双电子激发态辐射衰变特性

讨论了类氢铀离子与H2分子碰撞中,经KLL共振转移和激发过程形成类氦铀离子双电子激发态的机制,分析了实验测量到的X射线能谱和各种竞争过程对X射线能谱的贡献.对由于纯电子-电子相互作用形成的双激发态的Kα辐射衰变的超级卫星线的角分布测量结果表明,角分布呈各向异性,电子态布居存在很强的定向排列.     

Fe~(24+)离子双电子复合以及和H_2 碰撞的共振转移与激发X射线发射过程的研究

以准相对论Hartree-Fock理论为基础,对Fe~(24+)离子KLn(n=L,M,N,O,P)共振激发态可能辐射衰变通道的双电子复合过程的共振强度进行了系统的理论计算研究,计算了KLL共振激发态谱项能级电偶极允许跃迁的共振强度和截面,在此基础上,根据已有H_2分子的实验Compton轮廓,进一步计算了能量在300—800 MeV范围内,抛射体Fe~(24+)离子俘获H_2分子靶电子的KLn(n=L,M,N,O,P)共振电荷转移与激发X射线发射截面,计算结果与最新实验值或者其他理论计算结果做了对比分析,研究表明,对于Fe~(24+)离子KLn(n=L,M,N,O,P)的双激发态,Kα辐射衰变通道对双电子复合过程的共振强度贡献最大,是起主导性作用的重要通道,Kα辐射衰变X射线的波长范围λ为1.850—1.880A,而非Kα辐射衰变的波长范围λ为1.460—1.601 A,两者共振X射线的波长位置并不重叠。     

W^71＋离子态—态双电子复合速度系数的计算

基于Ｃｏｗａｎ相对论多组态ＨＦＲ程序，计算了高离化类锂钨离子在０．１－９ｋｅＶ能量范围内，对应于Δｎ＝０．１的态－态双电子复合速率系数。讨论了速率系数随电子温度，复合类型及中间双激发态中俘获电子的主量子数的变化。     

W~（71＋）离子态─态双电子复合速率系数的计算

基于Ｃｏｗａｎ相对论多组态ＨＦＲ程序，计算了高离化类锂钨（Ｗ７１＋）离子在０．１～９ｋｅＶ能量范围内，对应于△ｎ＝０，１的态─态双电子复合速率系数。讨论了速率系数随电子温度，复合类型及中间双激发态中俘获电子的主量子数的变化。     

高离化类Ne铕离子的双电子伴线结构的理论研究

在对高离化态类Ne铕离子及其临近的类Na、类Mg离子的n=3→2跃迁的波长和强度详细计算的基础上，考虑了等离子体中单个谱线的展宽和谱线之间的重叠，得到了类Ne铕离子n=3→2的共振线及其类Na和类Mg离子双电子伴线的结构，并系统地分析了这些伴线对共振线波长和强度的影响.     

类钠Ni~(17+)离子双电子复合过程理论研究

使用基于相对论多组态方法的FAC程序,研究了类钠Ni17+(3s)离子通过双激发态Ni16+(3pnl,3dnl)(Δn=0激发)的双电子复合过程,得到了态选择的双电子复合截面和速率系数,并与文献中的实验和理论数据进行了对比.结果发现,计算通过3p3/210l和3p1/211l共振态的双电子复合积分截面在实验误差范围内与实验测量很好地符合,并好于全相对论的多体微扰理论计算结果.结合量子亏损理论,发现包含高里德伯态的共振双激发态的辐射跃迁和自电离速率具有较好的标度关系,利用该关系给出了近激发阈值的所有共振态的双电子复合积分截面和速率系数.比较3pnl和3dnl两个系列,发现在低温(大约小于100eV)等离子体情况下前者速率系数比后者大,更高的温度后者大.     

基态类Ne锗离子双电子复合的半相对论计算

采用半相对论多组态Ｈａｒｔｒｅｅ一Ｆｏｃｋ模型，计算了类Ｎｅ锗离子经过３ｌ３ｌ＇和４ｌ４ｌ＇双激发态到类Ｎａ离子单激发态的态对态双电子复合速率系数，同时给出了描写上述复合过程的参数Ｂ和。通过对求和而获得的部分双电子复合速率系数与其它理论计算结果进行了比较。     

The KLL dielectronic recombination processes for highly charged krypton, iodine and barium ions

The KLL dielectronic recombination (DR) processes of ions from highly charged helium-like to oxygen-like krypton, iodine and barium ions are studied systematically in the relativistic distorted-wave approximation with configuration interaction. The KLL DR resonant energies, the corresponding resonant strengths and the theoretical spectra for each highly charged ion species are obtained. The results accord well with other available values. The behaviour of KLL resonant strengths for He-like ions with atomic number Z is analysed.     

Theoretical study of the KLL dielectronic recombination for highly charged iodine ions

With a developed program for calculation of dielectronic recombination (DR) process, which is based on multi-configuration Dirac-Fock (MCDF) method, the KLL DR processes of the highly charged helium-like to carbon-like iodine ions have been studied systematically. The contributions to doubly excited states from quantum electrodynamic (QED) and Breit effects have been discussed. The KLL DR resonant energies and corresponding resonant strengths have been calculated. The behavior of KLL resonant strengths with increasing Z are analyzed for He-like ions in particular. The theoretical DR spectra for each highly charged ion species are obtained in the KLL region. Comparison has been made between the present calculations and the latest experiments in Tokyo-EBIT.     

KLL dielectronic recombination process of He-like to O-like xenon ions

In this work, the KLL dielectronic recombination (DR) processes of highly charged He-like to O-like xenon ions are studied systematically by using a DR program, which is based on the multi-configuration Dirac-Fock (MCDF) method. The KLL DR resonant energies and the corresponding resonant strengths are calculated, asizing especially the effect of the Breit interaction on the DR strengths. The theoretical KLL DR spectra are obtained and compared with the latest experimental results obtained in the Shanghai Electron Beam Ion Trap.     

Theoretical study on photorecombination of C V ion

The partial and total photorecombination cross sections of the ground-state C V ion in the KLL and KLM resonant energy regions were calculated in detail by using the Dirac atomic R-matrix code based on a fully relativistic R-matrix method. Meanwhile, the principal resonant lines in each photorecombination channel have been classified according to the calculated transition energies and probabilities from the KLL and KLM resonant states to the 1s2nl(n = 2, 3 and l = s, p, d)final states. The validity of these calculations is assessed by comparison with previously published experimental and theoretical data. The good agreement between the present calculated results and those obtained using different approaches confirms the accuracy of the present results. In addition, it is found that the damping effect can be neglected for the KLL resonant, but not for the KLM resonant.     

KLn Dielectronic Recombination Process of B- Through He-like Cu Ions

The KLn dielectronic recombination processes of trapped highly charged B-like through He-like Cu ions are studied theoretically, and the theoretical results are used to analyse our previous experimental data at Heidelberg electron beam ion trap （EBIT）. The theoretical resonant positions agree with the experimental resonant positions to a precision of 0.4%, in comparison with the resonant positions of those highest peaks between theory and experiment. The experimental spectra are then fitted using a formula with the theoretical resonant energies and strengths, the result shows good overall agreement between theory and experiment over a wide electron energy range. The distribution of highly charged states is obtained from the fitting parameters.     

Measurement of the KLL Dielectronic Recombination Resonances in He-like to C-like Kr Ions

The KLL dielectronic recombination processes of highly charged He-like to C-like Kr ions have been studied experimentally. The measurement was performed on the newly developed Shanghai electron beam ion trap （Shanghai-EBIT） facility. Characteristic x-rays from both dielectronic recombination and radiative recombination are detected as the electron beam energy is scanned through the resonances. The KLL resonant strengths obtained are 5.41×10^-19, 4.33×10^-19, 3.59×10^-19, 2.05×10^-19 and 0.98×10^-19 cm^2 eV for He-like to C-like Kr ions, respectively.     

Structure and dynamics of highly charged heavy ions studied with the electron beam ion trap in Tokyo

In this paper, we present the structure and the dynamics of highly charged heavy ions studied through dielectronic recombination (DR) observations performed with the Tokyo electron beam ion trap. By measuring the energy dependence of the ion abundance ratio in the trap at equilibrium, we have observed DR processes for open shell systems very clearly. Remarkable relativistic effects due to the generalized Breit interaction have been clearly shown in DR for highly charged heavy ions. We also present the first result for the coincidence measurement of two photons emitted from a single DR event.     

State-selective quantum interference observed in the recombination of highly charged Hg 75+...78+ mercury ions in an electron beam ion trap

We present experimental data on the state-selective quantum interference between different pathways of photorecombination, namely, radiative and dielectronic recombination, in the KLL resonances of highly charged mercury ions. The interference, observed for well resolved electronic states in the Heidelberg electron beam ion trap, manifests itself in the asymmetry of line shapes, characterized by "Fano factors," which have been determined with unprecedented precision, as well as their excitation energies, for several strong dielectronic resonances.     

Dielectronic recombination at low energy range with Boron-like Ar13+at the CSRm

In order to extend the dielectronic recombination (DR) experiments from the main cooler storage ring CSRm with intermediate charge state ions to the experimental cooler storage ring CSRe with highly charged ions and even radioactive ions, a test electron-ion recombination experiment of B-like Ar¹³⁺ ions was performed with a section of the new electron beam energy detuning system, which will be installed at the CSRe. We present the measured and also the calculated DR spectra for the ∆n = 0 resonances from 0 to 3 eV. The experimental results agree very well with the previous DR experimental data from CRYRING, and the energy resolution reached 30 meV full width at half maximum. This test experiment demonstrates that the reliability and stability of the newly developed electron beam energy detuning system are satisfactory for the upcoming DR experiments at the CSRe. However, we found large discrepancies between the experimental result and the calculation in both resonance positions and the intensities of the recombination spectrum below 0.7 eV, which indicate that precise calculation of the DR spectrum of multielectron ions is still a challenge.