Observation of filamentation-induced continuous self-frequency down shift in air

We observed a new filamentation nonlinear process: continuous self-frequency down shift inside the filament zone during the propagation of a femtosecond laser pulse in air. The frequency shift depends strongly on the length of the self-guided column (filament). PACS 42.65.Dr; 42.65.Jx; 52.35.Mw     

Self-transformation of a powerful femtosecond laser pulse into a white-light laser pulse in bulk optical media (or supercontinuum generation)

We present experimental and theoretical results on white-light generation in the filamentation of a high-power femtosecond laser pulse in water and atmospheric air. We have shown that the high spatio-temporal localization of the light field in the filament, which enables the supercontinuum generation, is sustained due to the dynamic transformation of the light field on the whole transverse scale of the beam, including its edges. We found that the sources of the supercontinuum blue wing are in the rings, surrounding the filament, as well as at the back of the pulse, where shock-wave formation enhanced by self-steepening takes place. We report on the first observation and demonstration of the interference of the supercontinuum spectral components arising in the course of multiple filamentation in a terawatt laser pulse. We demonstrate that the conversion efficiency of an initially narrow laser pulse spectrum into the supercontinuum depends on the length of the filament with high intensity gradients and can be increased by introducing an initial chirp. PACS 42.65.Jx; 42.65.Re; 42.25.Bs; 42.50.Hz     

Computer simulation of laser pulse filament generation in rain

Initiation of femtosecond laser pulse filamentation in rain conditions is investigated numerically. It is shown that coherent scattering on rain water particles generates filament initiation sites. Results of computer simulation are consistent with full-scale experimental data. PACS 42.65.Jx; 42.68.Jg; 42.60.Jf     

Self-stabilization of third-harmonic pulse during two-color filamentation in gases

Self-stabilization of the laser pulse parameters is demonstrated during the two-color filamentation of ultrashort and intense laser pulses in gases. Experimental data and results of numerical simulations show, in good qualitative agreement, that the root-mean-square values of the intensity fluctuations decrease below the initial value for the near-infrared pump pulse and the perturbative limit for the third-harmonic pulse in the filament. It is found that the stabilization of the third-harmonic intensity and energy are due to intensity clamping of the pump pulse and a constant ‘volume’ of the laser pulse during the nonlinear propagation inside the filament. PACS 42.65.Ky; 42.65.Jx; 52.35.Mw     

Continuum generation of the third-harmonic pulse generated by an intense femtosecond IR laser pulse in air

The continuum generation by intense femtosecond IR laser pulses focused in air including the effect of third-harmonic generation is investigated. We have used a theoretical model that includes the full spatio-temporal dynamics of both the fundamental and the third-harmonic pulses. Results of our numerical calculations show that a two-color filamentation effect occurs, in which the third-harmonic conversion efficiency remains almost constant over the whole filament length. It is found that this effect is rather independent of the wavelength of the input beam and the focal geometry. During the filamentation process the third-harmonic pulse itself generates a broad continuum, which can even overlap with the continuum of the fundamental pulse for the longer pump wavelengths. In consequence, the continuum generation generated by intense IR laser pulses is further extended into the UV. PACS 42.65.Jx; 42.65.Ky; 52.35.Mw     

Spatial optimization of filaments

We demonstrate the spatial homogenization of intense laser pulses by adaptive minimization of spatial chirp of the spectrally broadened output pulses of a filament. A liquid-crystal-based two-dimensional spatial light modulator is used to control the spatial phase of the driver pulse. An evolutionary algorithm finds the optimal spatial laser phase distribution that introduces minimal distortions during filamentation and enhances the beam quality of the output pulse. A homogeneous intensity distribution favours efficient temporal compression close to the bandwidth limit without the need for spatial filtering after the filament. PACS 42.65.-k; 42.65.Re; 41.85.Ct     

Two-dimensional organization of a large number of stationary optical filaments by adaptive wave front control

We present an adaptive technique for the formation of multiple co-propagating and stationary filaments in a gaseous medium. Wavefront shaping of the initial beam is performed using a deformable mirror to achieve a complete two-dimensional control of the multi-spot intensity pattern in the laser focus. The spatial organization of these intensity spots yields reliable formation of up to five stable and stationary filaments providing a test bed for fundamental studies on multiple filamentation. PACS 42.65.Jx; 52.38.Hb; 42.65.Sf     

Comparison of the filamentation and the hollow-core fiber characteristics for pulse compression into the few-cycle regime

The gas-filled hollow-core fiber compression and the optical filamentation technique are compared experimentally in a parameter regime suitable for intense few-cycle pulse generation. In particular, pointing stability, spectral properties, and spatial chirp are investigated. It is found that in the case of filamentation, the critical parameter for pointing stability is gas pressure inside the generation cell whereas for the hollow-core fiber it is alignment that plays this role. The hollow-core fiber technique yields spectra that are better suited for chirped-mirror pulse compression whereas filamentation offers higher throughput and prospects for easy-to-implement self-compression. We present spectral phase interferometry for direct electric-field reconstruction (SPIDER) measurements that directly show the transition in the spectral phase of the output continua into the self-compression regime as the gas pressure is increased. PACS 42.65.Re; 42.65.Jx; 42.65.Tg     

Pressure independence of intensity clamping during filamentation: theory and experiment

Because of the dynamic equilibrium between Kerr self-focussing and plasma induced defocusing and the inexistence of collisional ionization the critical intensity during femtosecond laser filamentation in air is independent of pressure. An analytical analysis is given which is justified by a direct experimental verification. PACS 42.65.Jx; 52.38.Hb; 52.70.Kz     

Long-range self-channeling of infrared laser pulses in air: a new propagation regime without ionization

We report long-range self-channeling in air of multiterawatt femtosecond laser pulses with large negative initial chirps. The peak intensity in the light channels is at least one order of magnitude lower than required for multiphoton ionization of air molecules. A detailed comparison is made between experiments and realistic 3+1-dimensional numerical simulations. It reveals that the mechanism limiting the growth of intensity by filamentation is connected with broken revolution symmetry in the transverse diffraction plane. PACS 42.65.Sf; 42.25.Bs; 42.65.Jx; 52.38.Hb     

Frequency-stabilized Nd:YVO4 thin-disk laser

We have developed a Nd:YVO₄ thin-disk laser at 914 nm with single-frequency operation and active frequency stabilization to a low-finesse reference cavity. The spectral density of laser frequency noise is analysed by means of noise measurements at the error point of the frequency control loop. To address the 3¹S₀→3³P₁ magnesium intercombination line at 457 nm, we use an external frequency doubling stage based on periodically poled KTiOPO₄ for the generation of more than 150-mW output power at 457 nm. Optical beat signal measurements at 457 nm with a frequency-stable dye laser show a short-time line width of the thin-disk laser of less than 100 kHz. PACS 42.55.Xi; 42.60.Lh; 42.62.Fi; 42.65.Ky     

Observation of discrete supercontinuum spectra from a multi-pulse pumped distributed feedback dye laser

A new approach to the generation of uniformly sliced supercontinuum is reported. It is based on a multi-pulse pumped distributed feedback dye laser rather than on the conventional propagation of femtosecond pulses through air or photonic molecules. Recent developments in supercontinuum generation and laser filamentation are critically reviewed to relate our findings to published work. Novelty of the proposed technique, in terms of ease of generation and economy, makes the method an attractive alternative. This work was carried out by pumping dye solution with six beams of a Q. switched and mode-locked Nd:YAG laser. A total energy of 421 J was used to generate a 5.5 nm wide discrete supercontinuum consisting of nine distinct coherent lines. The principle of multiple line generation may be extended to any desired spectral range depending upon the available gain medium and number of pumping pulses. Threshold power intensity for sliced supercontinuum generation using a frequency doubled Nd:YAG laser for solution of R6G in ethanol is found to be less than 24×10⁸ W/cm². Successful design and operation of a coherent off-white discrete supercontinuum source is also presented. PACS 42.60.By; 42.65.Re; 42.25.Bs     

Femtosecond filament amplification in liquids

We study the femtosecond filamentation in a liquid amplifying medium, sulphorhodamine 640 in a methanol solvent. In the presence of population inversion, the energy of the filament increases while its diameter expands because of peak intensity clamping. PACS 42.25.Bs; 42.65.Jx; 42.65.Re; 42.65.Sf     

Sub-picosecond ultraviolet laser filamentation-induced bulk modifications in fused silica

We present experiments with sub-picosecond ultraviolet laser pulses (248 nm, 450 fs) tightly focused in the bulk of fused-silica samples. The high laser intensities attained generate plasma through multi-photon absorption and electron avalanche processes in the bulk of the material. Depending on the initial experimental conditions three distinct types of structural changes in the material are observed, from small changes of the refractive index to birefringence, and even cracks and voids. We also observe the creation of micro-channels, up to 115 m in length, inside the material due to self-guiding and filamentation of the laser pulses in the transparent material. The selective change of the refractive index is a promising method for the fabrication of photonic structures such as waveguides and three-dimensional integrated optical devices. PACS  52.38.Hb; 42.65.-k; 42.70.-a     

Measurement and calculation of nonlinear absorption associated with femtosecond filaments in water

We investigate the filamentation dynamics of 200 fs, 527 nm laser pulses in water. By comparing the experimental results with the numerical simulations that use an extended propagation model, the influence of several physical effects, particularly nonlinear losses and free electron plasma generation, is studied. It is shown that a set of relevant numerical values, related to multiphoton absorption, can be extracted with reasonable accuracy. PACS 42.65.Jx; 42.25.Bs     

Green light generation in a periodically poled Zn-doped LiNbO3 planar waveguide fabricated by He+ implantation

An optical planar waveguide is investigated in ZnO-doped periodically poled lithium niobate formed by He⁺ implantation. Optical losses were found to be 2 dB/cm. Second-harmonic generation is used to produce a green laser beam by quasi-phase matching in the obtained waveguide. The conversion efficiency was found to be 10^-2%/W. Photorefractive resistance properties are reported and discussed relating to un-doped periodically poled lithium niobate. PACS 42.65.-k; 42.65.Wi; 42.82.-m     

Dependency of injection seeding and spectral purity of a single resonant KTP optical parametric oscillator on the phase matching condition

For spectroscopic and remote sensing applications injection seeded optical parametric oscillators (OPOs) are well established. In this paper we study the dependencies of signal resonant injection seeding of an OPO on its resonator length, phase matching angle and pump power in detail. The quality of the seeding process is assessed by stabilising the seed laser on a molecular absorption line of water vapour and using a water vapour absorption cell as a narrow bandwidth filter for the injection seeded radiation. A reduction of the acceptance of injection seeding is observed with increasing pump power. For small phase mismatch injection seeding with a spectral purity of 99.7% was observed at 13-fold OPO threshold. A signal pulse energy of 38 mJ with 50% pump depletion was achieved with a beam parameter M² of about 6. PACS 42.65.Yj; 42.79.Nv; 42.79.Qx     

Conical four-wave mixing in sodium vapour excited by femtosecond laser pulses

Broadband (sometimes exceeding 1500 cm^-1) red-shifted (with respect to the sodium 3S–3P transition frequency) conical emission has been observed with the pump wavelength tuned in the range between 540 and 589 nm. Such broadband emission was attributed to the generation and amplification of light at the Rabi sideband frequencies in the field of intense femtosecond laser pulses. It has been shown that the cone angle of the emitted radiation is determined by the process of four-wave mixing under the conditions of longitudinal (Cherenkov-type) phase matching. PACS 42.65.Ky; 42.65.Re; 42.50.Hz     

Short pulse Z -scan investigations of optical nonlinearities of a novel organometallic complex: [(C2H5)4N]2[Cu(dmit)2] at 532 and 1064?nm

A novel dmit organometallic complex: [(C₂H₅)₄N]₂[Cu(dmit)₂] (dmit^2-=1,3-dithiole-2-thione-4,5-dithiolate), abbreviated as EtCu, was synthesized. Afterwards its optical nonlinearities in acetone solution at 532 nm and 1064 nm were studied by the Z-scan technique with laser pulses of picosecond duration. The two-photon absorption at 1064 nm and the saturable absorption at 532 nm were observed. The Z-scan curves also revealed that EtCu sample solutions exhibited self-defocusing effects at both wavelengths. The origins were analyzed for the differences between the results. All the outcomes suggest that this material is potential for nonlinear optical device applications. PACS 42.65.An; 42.65.Hw; 42.65.Jx; 81.20.Ka; 78.30.Jw