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1.
This study was aimed at providing the baseline data of terrestrial gamma dose rates and natural radioactivity to assess the corresponding health risk in the ambient environment of the Pahang State. Terrestrial gamma radiation (TGR) from 640 locations was measured with the mean value found to be 176?±?5 nGy h?1. Ninety-eight soil samples were analysed using a high-purity germanium detector (HPGe), and the mean concentrations of the radionuclides 226Ra, 232Th and 40K are 110?±?3, 151?±?5 and 542?±?51 Bq kg?1, respectively.226Ra and 232Th concentrations were found to be three times the world average, while that of 40K is quite higher than the world average value. The acid-intrusive geological formation has the highest mean concentrations for 226Ra (215?±?6 Bq kg?1), 232Th (384?±?12 Bq kg?1) and 40K (1564?±?153 Bq kg?1). The radium equivalent activities (Req) and the external hazard index (Hex) for the various soil types were also calculated. Some of the soil types were found to have values exceeding the internationally recommended levels of 370 Bq kg?1 and the unity value, respectively.  相似文献   

2.
ABSTRACT

The specific activities of 226Ra, 232Th and 40K of 26 samples of granite produced in Xinjiang of China were measured by a high-purity germanium detector, and their radiological hazards of radium equivalent, external hazard index, internal hazard index, absorbed dose rate, annual effective dose rate, gamma index and alpha index were evaluated. The results indicate that the overall average specific activities of 226Ra, 232Th and 40K obtained in the investigated samples are below the world’s average granite values. The average radium equivalent is within the recommended limit of 370?Bq?kg?1. The results obtained further show that the mean values of external hazard index, internal hazard index, absorbed dose rate, annual effective dose rate, gamma index and alpha index are 0.65, 0.77, 111.7?nGy?h?1, 0.55 mSv?y?1, 0.89 and 0.23, respectively. These mean values established that radiological hazards are also found to be below the international recommended values. The results are compared with granite samples from other countries or China-Taiwan province. It can be noticed that the specific activity values of granite samples produced in China are lower or similar to that of other countries or China-Taiwan province, however there are higher specific activity values for 226Ra and 232Th in individual samples, which need to provide proper radiation monitoring before use considering the long term health effect.  相似文献   

3.
Twenty soil and 25 sediment samples were collected from the banks and bottom of the River Nile in the surroundings of biggest cities located close to it. Natural radioactivity concentrations of 226Ra, 232Th and 40K have been evaluated for all samples by means of γ spectrometric analysis. The radioactivity levels of soil and sediment samples fall within the internationally recommended values. Nevertheless, high natural background radiation zones are detected in the Kafr El-Zayat region due to the presence of a fertilizer factory, and in the Rosetta region due to the presence of black sand deposits. The absorbed dose rate, the γ index and excess life time cancer risk are calculated. High values for some of the radiation health parameters are detected in the Kafr El-Zayat and Rosetta regions representing a serious problem to public health because the soil and sediment are used as constructing material for buildings. Furthermore, the isotope analysis of uranium for representative collected sediment samples via α spectrometry showed average specific activities of 18.7?±?3.6, 0.087?±?0.0038 and 18.6?±?3.8 Bq kg–1 for 234U, 235U and 238U, respectively. In general, these values confirm the balance in the isotopic abundance of U isotopes.  相似文献   

4.
In the present study, the distribution of natural radionuclides in soil samples collected from different geological units of Kumaun Himalayas are assessed using gamma ray spectrometer with Nal(Tl) detector. The naturally occurring radioactivity concentration of 226Ra, 232Th and 40K were found to vary from 36.4 Bq/kg to 166.6 Bq/kg, 15.3 Bq/kg to 94.7 Bq/kg and 645.9 Bq/kg to 1378.9 Bq/kg, respectively. The total absorbed gamma dose rate was found to vary from 80 nGy/h to 179.6 nGy/h. The resulting dose due to the presence of these radionuclides was estimated from radiation protection point of view. The significance of this investigation is also discussed in details.  相似文献   

5.
Natural radioactivity is one of the essential components of the environment. Unlike the Sudety mountains area in Poland, the Tatra Mountains were not the subject of wide survey as regards the levels of natural radioactivity. Especially, the concentrations of radon (natural radioactive gas) have not been investigated there in terms of their possible negative health impact. Within the frame of bilateral cooperation between the Institute of Nuclear Physics in Kraków, Poland, and the Jo?ef Stefan Institute in Ljubljana, Slovenia, the measurements of natural radioactive elements in old uranium mines in the Tatra National Park were performed in June 2010. The investigated sites were located in Dolina Bia?ego (The Valley of the White). One of the mines is situated near the tourist path. The paper presents the results of complex measurements of natural radioactivity in both uranium drifts. The concentration of radon gas inside the mining drifts exceeded 28,000 Bq m?3. Also, very high gamma dose rates were observed (up to 5600 nSv h?1). The maximum concentrations of natural radioactive elements (potassium 40K, radium 226Ra, thorium 232Th) in rock samples amounted to 535, 2137, and 18 Bq kg?1, respectively. The effective dose rates due to radon and thoron inhalation have been assessed as 0.013 mSv h?1 (for the lowest concentration) and 0.121 mSv h?1 (for the highest concentration).  相似文献   

6.
The radiation survey of the ambient environment was conducted using two gamma detectors, and the measurement results were used in the computation of the mean external radiation dose rate, mean-weighted dose rate and annual effective dose, which are 144 nGy h?1, 0.891 mSv y?1 and 178 μSv, respectively. A high-purity germanium detector was used to determine the activity concentrations of 232Th, 226Ra and 40K in soil samples. The results of the gamma spectrometry of the soil samples show radioactivity concentration ranges from 19±1 to 405±13 Bq kg?1 with a mean value of 137±5 Bq kg?1 for 232Th, from 21±2 to 268±9 Bq kg?1with a mean value of 78±3 Bq kg?1 for 226Ra and from 23±9 to 1268±58 Bq kg?1 with a mean value of 207±13 Bq kg?1 for 40K. Radium equivalent activity (Raeq) and external hazard index (Hex) were 290 Bq kg?1 and 0.784, respectively, which were safe for the population. The mean lifetime dose and lifetime cancer risk for each person living in the area with average lifetime (70 y) were 12.46 mSv and 7.25×10?4 Sv year, respectively. The results were compared with values given in United Nations Scientific Committee on the Effects of Atomic Radiation 2000.  相似文献   

7.
Radionuclides are released together with fly ash from the coal-fired power plant and thus add to the natural radiation. Fifty soil samples were collected around the Baoji coal-fired power plant from 25 locations and the natural radionuclide concentrations were determined by a gamma ray spectrometric system. The results show that the activity concentrations in soil samples range from 12.54 to 40.18 Bq kg?1, 38.02 to 72.55 Bq kg?1 and 498.02 to 1126.98 Bq kg?1 for 226Ra, 232Th and 40K with the mean values of 27.35, 52.66 and 764.72 Bq kg?1, respectively. In order to evaluate the radiological hazard of the natural radioactivity, the radium equivalent activity (Raeq), the absorbed dose rate (D) and the annual effective dose rate have been calculated and compared with the internationally approved values. The radium equivalent activity in all the soil samples is lower than the safe limit set in the Organization for Economic Cooperation and Development report (370 Bq kg?1). The average value of the calculated dose rates is higher than the global average value 55 nGy h?1, and the calculated annual effective dose rate is significantly lower than the average annual external effective dose rate (460 μSv y?1) of the normal background radiation.  相似文献   

8.
《Radiation measurements》2009,44(1):102-110
Determination of the natural radioactivity has been carried out, by means of gamma-ray spectrometry system, in surface soil samples collected from various geological formations in urban areas of the northern highlands of Jordan. These highlands, extending from Yarmouk River in the north to Wadi Wala in the south, form the agriculturally important regions of Jordan. Soils of the study region, at which about 70% of the total population of the country are living, mainly originated from limestones that are locally used in construction materials, making the evaluation of environmental radioactivity and estimating the current radiation hazards to the population an interesting issue. The total average concentrations of radionuclides 226Ra, 238U, 232Th, and 40K were 42.5, 49.9, 26.7, and 291.1 Bq kg−1, respectively. Correlations made among these radionuclides prove the existence of secular equilibrium in the investigated soils. The total average absorbed dose rate in the study areas is found to be 51.5 nGy h−1, whereas the annual effective dose equivalent has an average value of 63.2 μSv y−1. The external and internal hazard indices, the radium equivalent activity, and the annual gonadal dose equivalent associated with the investigated soils do not exceed the permissible limits except for soils originated from phosphate rocks. Moreover, the radio-elemental concentrations of uranium, thorium and potassium, evaluated for the various geological features in the study areas were calculated to indicate whether relative depletion/enrichment of radioisotopes had occurred. The results of the present study were discussed and compared with internationally recommended values.  相似文献   

9.
The activity concentrations of 226Ra, 232Th and 40K have been measured by gamma spectroscopy in samples of soil collected from the different zones of around Huelva (Spain). The average activity concentrations of 226Ra (Bq kg?1) in the active phosphogypsum (PG) stacks, unrestored and restored zones were 647, 573 and 83 respectively. The corresponding values for 232Th and 40K (Bq kg?1) were 8, 10 and 25 and 33, 47 and 225 respectively. As a measure of radiation hazard to the occupational workers and public, the Ra equivalent activities, representative level index and dose rates due to natural radionuclides at 1 m above the ground surface were estimated. The average of absorbed dose rates due to 226Ra, 232Th and 40K (nGy/h) from active PG stacks, unrestored and restored zones are 284, 255 and 55.The calculated external γ-radiation average dose (mSv/y) received by the workers of the phosphogypsum piles are estimated to be 0.293, 0.262 and 0.057 which is far below the international agreed dose limit of 20 mSv/y (ICRP-60, 1990) for workers. Also, the radiation dose to a member of the public resulting from the use of PG is negligible compared to the average annual effective dose from natural sources (2.4 mSv/y).  相似文献   

10.
The activity concentrations of 226Ra, 232Th and 40K in commercial marble materials have been determined using a NaI(Tl) γ-ray spectrometer with a matrix-inversion-based spectral stripping technique. Knowledge of radioactivity present in marble materials enables one to assess any possible radiological risks to human health. The concentrations of 226Ra, 232Th and 40K in Chinese commercial marble range from 8.4 to 157.4, 5.6 to 165.5 and 44.1 to 1352.7 Bq kg?1, respectively. The natural radionuclide concentration varied with color and production site of commercial marble. The activity concentrations of 226Ra, 232Th and 40K in white, gray, black, green and yellow marble samples are comparatively smaller than those in brown and red marble samples. The radium equivalent activity (Raeq), the external hazard index (H ex), the internal hazard index (H in) and the annual gonadal dose equivalent were also calculated and compared with the internationally recommended values. One type of brown commercial marble (TSB) of China does not satisfy the universal standards.  相似文献   

11.
ABSTRACT

The concentration of natural radioactivity in rice is an important parameter for the determination of population exposure by the ingestion of natural radionuclides during habitual consumption of food. All types of food including rice contain a detectable amount of natural radioactivity which successively relocate into the human body via the ingestion pathway. Rice is the main cultivated crop in Bangladesh and most of the Bangladeshi people consume rice as their staple food. Hence, studies on the evaluation of natural radioactivity in rice have been performed by gamma-ray spectrometry using High Purity Germanium (HPGe) detector in order to estimate various radiation hazards due to rice consumption. The average activity levels of natural radionuclides 226Ra, 228Ra and 40K in the rice samples were 1.09?±?0.31, 0.17?±?0.21 and 4.70?±?1.59?Bq?kg?1, respectively. The estimated effective doses for the respective radionuclides caused by the rice consumption were 43.69, 16.39 and 4.15?µSv?y?1, respectively which was below the UNSCEAR compiled value. The calculated excess lifetime cancer risk (ELCR) values via rice consumption were found below the acceptable limit of 0.29?×?10?3 for radiological risk.  相似文献   

12.
Studies of the natural γ-emitting radionuclides in different types of cements manufactured by different companies in Egypt (e.g. Iron (HI), Karnak (HK), and Super fine (HSu) products from Helwan Ltd.) have been done to determine their natural levels of radioactivity using a high-purity germanium detector (HPGe). Knowledge of radioactivity present in cement materials enables one to assess any possible radiological risks to human health. The results show that the highest mean values of 226Ra and 232Th activity are 234.01±20.12 and 46.56±4.65 Bq kg?1, respectively, measured in cement sample ‘Iron’ from Helwan company (HI). The corresponding value of 40K is 333.53±26.68 Bq kg?1 measured in cement sample ‘Karnak’ from Helwan company (HK). For 137Cs, this value is 3.27±0.31 Bq kg?1 measured in cement sample (HI). The average concentrations of measured radionuclides in the different cement samples are 72.21±6.39, 24.98±2.24, 134.49±10.45, and 0.58±0.08 Bq kg?1 for 226Ra, 232Th, 40K, and 137Cs, respectively. The measured activity concentrations for these radionuclides were compared with the reported data of other countries. Radium equivalent (Raeq) activities and different hazard indices were calculated to assess the radiation hazard. Iron HI cement sample shows a higher Raeq activity of 311.91±31.10 Bq kg?1. Calculations of absorbed doses in nGy h?1 show that the Iron (HI), Karnak (HK), and Super fine (HSu) products from Helwan company have higher activities than the permissible level (80 nGy h?1). On the basis of the external hazard index (H ex), Raeq activities, and annual effective dose rates for organs (H organ), the natural radioactivity of cement samples is not greater than the recommended values in the established standards and hence safe for use in building constructions and therefore for inhabitants.  相似文献   

13.
The primordial radionuclides activity concentrations (226Ra, 40K and 232Th) are measured in some granite samples in this study. The collected granite materials are analyzed with NaI(Tl) gamma-ray spectrometry. The specific activity of 226Ra, 232Th and 40K values are in range 2.60?±?0.10 to 178.9?±?0.6?Bq?kg?1, 1.46?±?0.10 to 162.50?±?0.75?Bq?kg?1 and 19.8?±?0.3 to 579.7?±?2.8?Bq?kg?1 respectively. The radium’s equivalent activity, annual effective dose, absorbed dose rate, hazard index, radioactivity level index, activity utilization’s index and exposure rate are calculated for determination of radiological risk. The concentration of 226Ra (in the 71.4% of samples), 232Th (in the 71.4% of samples) and 40K (in the 14.3% of samples) in the granite samples are higher than average radioactivity concentrations of this radio-isotopes defined by ICRP (35.0, 30.0 and 400.0?Bq?kg?1, respectively).  相似文献   

14.
In Rechna Doab, samples of the most common vegetation, perennial grass Desmostachya bipinnata (dab), were collected along with soil samples from 29 sites. Natural radioactivity of 226Ra, 232Th/228Ac and 40K was measured by using high purity germanium-based gamma ray spectrometer. Activity concentration levels of 226Ra, 232Th/228Ac and 40K in soil were found to be 46.8±6.2 (36.0–57.6), 61.4±5.9 (48.2–73.2) and 644.8±73.9 (537.7–868.4) Bq kg?1 (dry mass), respectively, and those in vegetation were 2.74±1.70 (1.00–6.39), 2.24±0.59 (1.56–2.61) and 172.72±113.37 (53.14–469.24) Bq kg?1 (dry mass), respectively. The measured values of the activity concentration in vegetation are comparable with some other international data. Calculated soil to vegetation transfer factors of 226Ra, 228Ac and 40K were 0.06±0.03 (0.02–0.14), 0.04±0.01 (0.03–0.04) and 0.26±0.16 (0.09–0.69). The mean outdoor absorbed dose rate in air for the area under study was determined as 8.22 nGy h?1 and the mean indoor absorbed dose rate in air was 11.52 nGy h?1. The total annual effective dose to the general public from the vegetation was found to be (0.02–0.16) mSv, which is below the recommended limit value of 1 mSv y?1 for the general public. The dab vegetation under study was found to be radiologically safe for the population and environment.  相似文献   

15.
Natural and anthropogenic radioactivity of sand and water samples collected from the four big rivers of Punjab province, Pakistan, was measured using a high-purity germanium detector coupled with a high resolution multichannel analyser. The average concentration of the naturally occurring radionuclides 226Ra, 232Th and 40K in all the sand samples from the rivers Jhelum, Chenab, Ravi and Indus was found to be 22±0.6, 36±1 and 287±10 Bq?kg ?1, respectively, while the concentration of the anthropogenic radionuclide 137Cs was found to be below the minimum detectable activity, i.e. ~ 1.2 Bq?kg ?1. All the sand samples have Raeq concentrations lower than the limit of 370 Bq?kg ?1. Indoor (H in) and outdoor (H out) radiation hazard indices were calculated for the samples to assess the radiation hazards arising due to the use of this sand in construction, and were found to be less than unity in the study area. Calculated values of the absorbed dose rate were less than the typical world average value of 59 nGy?h ?1, and the annual effective dose rate was also less than the typical world value of 70 μSv, except in the Indus river, in which it is slightly higher then the world average. Results show that the measured values are comparable with other global radioactivity measurements. None of the studied riverbeds was considered a radiological hazard, and their sand can be safely used in construction.  相似文献   

16.
Ever since studies on uranium miners established the presence of a positive risk coefficient for the occurrence of lung cancer in miners exposed to elevated levels of 222Rn and its progeny, there was a great upsurge of interest in the measurement of 222Rn in the environment. Subsequently, considerable data is being generated on the levels of 222Rn in the environment across the worlds and is being periodically reported by UNSCEAR reports. In contrast to this, data pertaining to 220Rn in indoors and workplace environment is scaree due to the genral perception that its levels are negligible due to its shorter half life, and subsequently its contribution to the total inhalation dose is ignored, in the presence of other significant sources of natural radiation. This may not be true. Globally many locations have higher levels of natural background radiation due to elevated levels of primordial radio nuclides in the soil and their decay products like radon (222Rn), and thoron (220Rn) in the environment. Of late, technologically enhanced naturally occurring radioactive material has also contributed to the burden of background radiation. It is estimated that inhalation of 222Rn, 220Rn and their short lived progenies contribute more than 54% of the total natural background radiation dose received by the general population. 220Rn problem exists in industries which use thorium nitrate. Including India, lamps using thoriated gas mantles are still being used for indoor and outdoor lighting and by hawkers in rural as well as urban areas. Considering the fact that large amount of thorium nitrate is being handled by these industries, contribution to the inhalation dose of workers from 220Rn gas emanated and build up of the progeny in ambient air may also be quite significant. In this paper current status of 220Rn levels in the indoor environment and workplaces as well as in other industries where large amount of 232Th is being handled is being summarized. Methods of measurement and reported levels are also summarized.  相似文献   

17.
《Radiation measurements》2009,44(3):223-231
A multidisciplinary study of the Roc de Marsal Cave gave us the opportunity to re-examine the known problem posed by U-series disequilibria in sediments in the field of palaeodosimetric dating. Apart from burnt flints and heated limestones, the material being dated, THAT IS our principal concern here, is made of burnt sediment samples collected from a reddish layer that forms the very base of the Roc de Marsal Mousterian sequence (Couche B). U-series disequilibria of long life nuclides in sediments were observed: as a general trend, the activity of 238U is greater than that of 226Ra. Important discrepancies in age determination can occur according to the origin of the disequilibrium and its kinetics. To characterise these ancient modifications of radioactivity and constrain the range of possible variations of annual doses, a statistical study of 238U, 226Ra and 232Th activities, measured by gamma spectrometry, was carried out. It shows that the sediment was mainly enriched in mobile uranium. This conclusion is in accordance with the results of complementary measurements of 230Th and 234U performed by alpha spectrometry. On the kinetics side, two models of time-variation of U and daughter concentrations are compared, taking experimental data into account. A detailed presentation of the methodology and the method of calculation of dose rates, and particularly time-averaged dose rates in such a situation, is given.  相似文献   

18.
This study entails the measurement of the specific activity of natural radionuclides (226Ra, 40K and 232Th) in 18 tooth samples obtained from the clinic of the Universiti Sains Malaysia (USM), Penang, by using an HPGe detector. The specific activity of 226Ra, 40K and 232Th was measured to estimate the hazard index of the radionuclides, radium equivalent activities (Raeq), external, internal hazard indices (Hex, Hin), and absorbed dose (Dout, Din). The maximum values of concentration of 226Ra, 232Th and 40K in the tooth samples were found to be 60.82, 60.29 and 594.22?Bq kg?1, respectively. Maximum values of Raeq, Hex, Hin, Dout and Din were found to be 192.78?Bq kg?1, 0.520, 0.685, 89.29 and 169.81?nGy h–1, and as 0.702 and 0.304, respectively. The results were lower than the average world value (UNSCEAR). In addition, a strong correlation was found between the concentrations of 226Ra and Raeq, between energy and net area, as well as between radionuclides (226Ra, 40K and 232Th) in tooth samples and age of volunteers. This study showed that the concentrations and hazard indices of tooth samples are below the recommended safe levels; therefore, the study area is considered safe in terms of radiological health hazards.  相似文献   

19.
《Radiation measurements》2008,43(8):1402-1407
Radiological impacts of phosphate rocks mining and manufacture could be significant due to the elevated radioactivity contents of the naturally occurring radioactive materials (NORM), such as 238U series, 232Th series and 40K, in some phosphate deposits. Over the last decades, the land reclamation and agriculture activities in Saudi Arabia and other countries have been widely expanded. Therefore, the usage of chemical fertilizers is increased. Selected phosphate fertilizers samples were collected and the specific activities of NORM were measured using a gamma ray spectrometer based on a hyper pure germanium detector and alpha spectrometer based on surface barrier detector.The obtained results show remarkable wide variations in the radioactivity contents of the different phosphate fertilizer samples. The mean (ranges) of specific activities for 226Ra, 210Po, 232Th and 40K, and radium equivalent activity are 75 (3–283), 25 (0.5–110), 23 (2–74), 2818 (9–6501) Bq/kg and 283 (7–589) Bq/kg, respectively. Based on dose calculations, the increment of the public radiation exposure due to the regular agricultural usage of phosphate fertilizers is negligible. Its average value 1 m above the ground is about 0.12 nGy/h where the world average value due to the NORM in soil is 51 nGy/h. Direct radiation exposures of the farmers due to phosphate fertilizers application was not considered in our study.  相似文献   

20.
Textile dyes are among the most problematic pollutants because of their toxicity on several organisms and ecosystems. Many of the chemicals used in the textile industry may represent some health concerns. The determination of the radioactivity in textile dyes is therefore very important for both human health and environment. The study was designated to determine, for the first time, the values of 238U, 232Th and 40K in nine different dyes employed in the textile industry using gamma spectrometry with a Hyper Pure Germanium (HPGe) detector. The mean activity concentrations of 238U, 232Th and 40K were 29.37?±?4.48, 1.15?±?0.13 and 565?±?4 Bq/kg, respectively. The calculated radium equivalents for all samples were lower than the maximum admissible value (370 Bq/kg). The absorbed dose rates due to the natural radioactivity of the investigated samples ranged from 2.94?±?0.05 to 166?±?3 nGy/h. So, the absorbed dose rates for all samples of textile dyes were lower than the international recommended value (55 nGy/h) except the yellow dye (166?±?3 nGy/h), which recorded a significant radiological hazard. The external hazard index was also calculated. Conclusively, the results have indicated that the textile dyes may possess a measurable amount of radioactivity that should be taken into account. Therefore, safety rules and precautions should be applied for dyes used in the textile industry and for people working in this field.  相似文献   

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