基于开口环阵列结构的表面晶格共振产生及二次谐波增强

理论研究了二维周期排列的金开口环谐振器的磁共振模式与周期阵列的衍射模式发生强耦合所需满足的条件及其对二次谐波产生效率的影响.通过控制阵列结构在x和y方向的周期大小,使得衍射模式只在其中一个方向产生,当衍射模式的电场方向与入射光电场偏振方向一致时,衍射模式才会与开口环谐振器的磁共振模式发生强耦合作用,产生表面晶格共振进而实现近场场增强.在此基础上,进一步计算了金开口环谐振器阵列的二次谐波产生效率,随着阵列周期逐渐增大,即开口环谐振器的数密度减小,二次谐波强度呈现先增加后降低的趋势,当开口环谐振器数密度降为原来的1/4左右时,二次谐波强度可以增强2倍以上.本文的研究为金属超表面二次谐波产生效率的提高提供了一种新的可能途径.     

双折射吸收非线性介质薄膜中倍频的产生

从二次谐波电场满足的波动方程出发，考虑到介质对二次谐波的吸收以及把完全边界条件应用于基频波和二次谐波在介质的入射面和出射面之间的反射效应，推导出了单光轴非线性薄膜介质中的二次谐波输出功率的计算式.结果表明：当采用复折射率的概念时，可以把非线性无吸收介质的二次谐波输出功率计算式应用到非线性吸收介质二次谐波输出功率计算式中去.     

超高真空中C60光聚合效应光学二次谐波的研究

利用１．０６４μｍ基频超短脉冲激光，使用光学二次谐波方法研究了超高真空中蒸镀在多晶银表面上的Ｃ６０薄膜紫外光照射下的光聚合现象，发现聚合以后的Ｃ６０二阶非线性响应增强，同时观察到光聚合的饱和效应，Ｃ６０光聚合二阶非线性的提高可以用电四极了磁偶极子对二次谐波贡献的增强来解释。     

光合色素分子吸附膜的非线性增强效应

吸附在光学表面上的细菌叶绿素和藻兰素生物分子膜.在基波(λ=1.06μm)激光作用下,观察到谐波效应.文中对藻兰素只产生三次谐波而不产生二次谐波做了分析.     

高效全固化紫外四倍频激光器的研究

用半导体激光器抽运的调Q YLF倍频激光器抽运掺钛蓝宝石激光器，用LBO晶体在腔内产生二次谐波，再聚焦到BBO晶体上产生四次谐波深紫外激光。为了提高谐波转换效率，在腔内分别插入了单片、组合双折射滤光片和聚焦透镜，在平均功率为3.6W，波长为527nm的抽运光下得到410mW，417nm的蓝光。用长焦距的透镜聚焦二次谐波，得到34mW，208nm的紫外脉冲激光。从实验上详细研究了基频光的线宽对二次谐波效率的影响，二次谐波的线宽对四次谐波效率的影响、基频光的波长对四次谐波产生效率的影响。全面地分析了单片和组合大拆射滤光片及抽运功率对钛蓝宝石激光器基频光的脉宽、线宽等参量的影响。     

表面等离子激元波的光学二次谐波效应及应用 Ⅰ.长程等离子激元波的二次谐波效应

运用光束传播方法推导了长程表面等离子激元波产生的二次谐波场强公式,并首次在银膜与各向同性的均匀介质的多层膜结构中观察到长程表面等离子激元波产生的二次谐波增强效应。理论分析与实验结果基本一致。     

空气对C60薄膜拉曼谱的影响

采用拉曼光谱方法和光学二次谐波方法，观察蒸镀在石英玻璃上的Ｃ６０薄膜在空气中的变化，根据实验中观察的Ｃ６０薄膜１４６９ｃｍ＾－１拉曼谱的演变情况，结合二次谐波的测量结果，初步推断Ｃ６０分子发生了聚合反应和氧化反应。     

双折射吸收非线性介质薄膜中倍频的产生

从二次谐波电场满足的波动方程出发,考虑到介质对二次谐波的吸收以及把完全边界条件应用于基频波和二次谐波在介质的入射面和出射面之间的反射效应,推导出了单光轴非线性薄膜介质中的二次谐波输出功率的计算式.结果表明：当采用复折射率的概念时,可以把非线性无吸收介质的二次谐波输出功率计算式应用到非线性吸收介质二次谐波输出功率计算式中去. 关键词： 非线性 倍频 二次谐波功率     

二维矩形波导管中的非线性声传播

本文采用部分波和二阶微扰理论对二维矩形波导管内声波的非线性传播问题进行了研究。由二次谐波的边界条件和初始条件，可得到物理图象清晰、便于计算的二次谐波声场解析式。结果表明，不同基波传播模式间的相互作用不存在二阶非线性，管内任意振幅分布的稳态激发源产生的二次谐波为各个模式二次谐波之和，且二次谐波声场分布具有对称性。     

超热电子产生的靶后相干渡越辐射光谱实验研究

利用OMA光学多道分析仪测量了激光与薄膜靶相互作用中产生的辐射光谱，在靶后观察到红移的二次谐波发射. 这种二次谐波是v×B加热产生的、具有微脉冲结构的超热电子束在等离子体-真空边界产生的相干渡越辐射(CTR). 随着激光能量的增大，红移峰向长波方向移动，光谱同时发生展宽. 分析认为，等离子体临界面的迅速膨胀是导致二次谐波红移的主要原因. 随着预脉冲能量的增大，临界面膨胀速度增大，导致了发射峰更大的红移. 实验还测量了靶面法线方向的辐射光谱，观察到基频辐射的红移和展宽. CTR为诊断临界面的运动方向和速度提供了一种新的方法. 关键词： 相干渡越辐射 超热电子 超短超强激光 等离子体相互作用     

Imaging theory of nonlinear second harmonic and third harmonic generations in confocal microscopy

ItisreportedrecentlythatnonlinearopticalphenomenonofSHGandTHGhasbeenobservedinmanybiologicaltissues[16].SHGandTHGhavebeenusedtoperformthethree-dimensionalimaginginlivingtissuesandhaveattractedmuchattentionrecently.TherearemanyadvantagesofusingSHGandTHGtoperformthethree-dimensionalimaginginlivingtissues,suchasnoninvasiveandnophotobleaching,inadditiontotheimagingpropertiesofmulti-photonfluorescenceimaging[7—9].Firstly,unlikeinthesingle-andmulti-photonfluorescenceprocesses,onlyvirtualstat…     

Voigt位型下电介质/反铁磁/电介质结构二次谐波生成非倒易性研究

利用非线性传递矩阵方法研究了Voigt位型下电介质/反铁磁/电介质 结构二次谐波生成的非倒易性. 研究发现外加静磁场反向和电介质层排序翻转均对二次谐波输出产生影响, 出现了二次谐波生成的非倒易性. 二次谐波生成非倒易性频率区域在反铁磁共振区, 此区间正处于THz频段. 随着入射角度的增加, 非倒易性的效果越来越明显. 研究二次谐波生成的非倒易性, 可为反铁磁器件的设计加工提供理论支持.     

Second harmonic generation of propagating collective excitations in Bose－Einstein condensates

We consider a possible second harmonic generation (SHG) of propagating collective excitations in a two-component Bose－Einstein condensate (BEC) with repulsive atom－atom interactions. We show that the phase-matching condition for the SHG can be fulfilled if the wave vectors and frequencies of the excitations are chosen adequately from different dispersion branches. We solve the nonlinear amplitude equations for the SHG derived using a method of multiple-scales and provide SHG solutions similar to those obtained for a SHG in nonlinear optical media. A possible experimental realization of the SHG for the propagating collective modes in a cigar-shaped two-component BEC is also discussed.     

Magnetization-induced anisotropy of second harmonic generation in thin cobalt films

Magnetization-induced effects in the symmetry properties of optical second harmonic generation (SHG) are studied in thin cobalt films. We demonstrate that the application of an external magnetic field leads to the appearance of a strong SHG azimuthal anisotropy from the isotropic Au/Co structure. Symmetry analysis of the SHG dependencies, supported by the SHG interferometry measurements, indicates that the effective magnetic and crystallographic second-order susceptibilities are both of the same order of magnitude.     

Evaluating cutaneous photoaging by use of multiphoton fluorescence and second-harmonic generation microscopy

The photoaging process of facial skin is investigated by use of multiphoton fluorescence and second-harmonic generation (SHG) microscopy. We obtain the autofluorescence (AF) and SHG images of the superficial dermis from the facial skin of three patients aged 20, 40, and 70 years. The results show that areas of AF increase with age, whereas areas of SHG decrease with age. The results are consistent with the histological findings in which collagen is progressively replaced by elastic fibers. The AF and SHG changes in photoaging are quantified by a SHG to autofluorescence aging index of dermis (SAAID). Our results suggest that SAAID can be a good indicator of the severity of photoaging.     

Analysis of second-harmonic generation microscopy under refractive index mismatch

On the basis of the vector diffraction theory and Green＇s function method, this paper investigates the effects of refractive index mismatch on second-harmonic generation （SHG） microscopy. The polarization distribution and SHG intensity are calculated as functions of the sample radius and probe depth. The numerical results show that refractive index mismatch can result in peak intensity degradation, increase secondary lobes and extension of second- harmonic polarization distribution. Because of the attenuation of polarization intensity, the detected SHG intensity significantly decreases with increasing probe depth, which can limit the imaging depth of SHG microscopy inside thick samples. Forward SHG intensity decays slowly than backward SHG, due to the combination of extension second-harmonic polarization distribution and strong dependency of forward SHG on sample radius.[第一段]     

Investigation on high efficiency temporal phase modulated broadband second harmonic laser

In this paper, it is the first time to experimentally demonstrate the second harmonic generation (SHG) of temporal phase modulated broadband laser. The SHG conversion efficiency and the characteristic of SHG spectrum are investigated in detail and the relation between SHG conversion efficiency and incident fundamental light intensity is obtained. The highest efficiency of nearly 70% is achieved at the fundamental pulse intensity of 1.6 GW/cm². The experimental results show that the SHG spectrum widths under high and low intensity are both half of the incident fundamental lights, and don’t result in the spectrum narrowing. The obtained results are very useful for operation at the second harmonic wavelength in inertial confinement fusion (ICF) laser facility.     

Phase Matching of SHG in Arbitrary Directions of Biaxial Crystals

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Phase Matching of SHG in Arbitrary Directions of Biaxial Crystals

In this paper, propagation and polarization characteristics of optical waves in arbitrary directions in a biaxial crystal are analyzed, and universal relationships of refractive index dependence on their propagation directions and the principal refractive indices for two perpendicular polarization waves propagating in arbitrarily directions are derived from indicatrix equation. By using these relationships, methods of collinear phase matching (PM) of SHG are developed, and general expressions of the collinear PM angle dependent of the principal indices are given for SHG in arbitrarily directions. The expressions may be used to make optimization design of PM by computer for the SHG and to select optimum PM direction and to raise the SHG conversion efficiencies.     

晶体和基团倍频系数间的普遍变换公式

本文使用倍频系数的不可约张量表示法,得到了离子基团的微观倍频系数与晶体宏观倍频系数间的一般变换公式,从而为晶体中不同取向的基因对宏观倍频系数的贡献提供了普遍的计算公式。应用这一计算方法可方便地计算各种碘酸盐的倍频系数,结果相当满意。本文对于探索新型倍频材料,提供了明确的空间结构条件。 关键词：