Magnetic properties of the mixed spin-5/2 and spin-3/2 Blume-Capel Ising system on the two-fold Cayley tree

We use exact recursion relations to study the magnetic properties of the half-integer mixed spin-5/2 and spin-3/2 Blume-Capel Ising ferromagnetic system on the two-fold Cayley tree that consists of two sublattices A and B. Two positive crystal-field interactions Δ₁ and Δ₂ are considered for the sublattice with spin-5/2 and spin-3/2 respectively. For different coordination numbers q of the Cayley tree sites, the phase diagrams of the model are presented with a special emphasis on the case q = 3, since other values of q reproduce similar results. First, the T = 0 phase diagram is illustrated in the (D _A = Δ₁/J,D _B = Δ₂/J) plane of reduced crystal-field interactions. This diagram shows triple points and coexistence lines between thermodynamically stable phases. Secondly, the thermal variation of the magnetization belonging to each sublattice for some coordination numbers q are investigated as well as the Helmoltz free energy of the system. First-order and second-order phase transitions are found. The second-order phase transitions become sharper and sharper when D _A or D _B increases. The first-order transitions only exist for some appropriate non-zero values of D _A and/or D _B . The corresponding transition lines never connect to the second-order transition lines. Thus, the non-existence of tricritical points remains one of the key features of the present model. The magnetic exponent β ₀ of the model is estimated and found to be ¼ at small values of D _A = D _B = D and β ₀ = ½ at large values of D. At intermediate values of D, there is a crossover region where the magnetic exponent displays interesting behaviours.     

Numerical study of the mixed spin-1 and spin-5/2 BEG model on the Bethe lattice

The mixed spin-1 and spin- \frac52\frac{5}{2} ferromagnetic Ising model with bilinear (J) and biquadratic (K) nearest-neighbor exchange interactions and a single-ion potential or crystal-field interaction (D) is studied on the Bethe lattice by means of exact recursion equations. First, the phase diagram of the system at zero temperature is obtained in the (D/Jq, K/Jq) plane, where q denotes the coordination number of the lattice. Second, the sublattice magnetizations as functions of the temperature, the crystal-field and the biquadratic interaction strengths are thoroughly investigated. For q = 3, the resulting phase diagrams show first and second order phase transitions as well as compensation points where the net magnetization of the whole lattice should vanish in the antiferromagnetic version of the model. One interesting feature of the model concerns the presence of tricritical points. Our calculations show that at non-zero temperature, none of the sublattice can order separately. However, under an external magnetic field, some interesting phase diagrams with partially ordered phases arise.     

The random distribution of the coordination numbers in the mixed spin-1/2 and spin-2 Blume-Capel model

The effects of random distribution of coordination numbers are investigated for the mixed spin-1/2 and spin-2 Blume-Capel model on the Bethe lattice in terms of exact recursion relations. The usual coordination numbers, i.e. $q=3,4$ and 6, corresponding to the honeycomb, square and simple cubic lattices, respectively, are considered. Two different q values are taken as couples and are varied randomly in terms of a standard-random approach on the shells of the Bethe lattice with some probabilities. It is found that the model gives either first- or second-order phase transitions for appropriate values of probability (p) and single ion anisotropy (d). One or two tricritical points are also observed depending on the given values of p and d, respectively.     

Phase diagrams in mixed spin-3/2 and spin-2 Ising system with two alternative layers within the effective-field theory

The phase diagrams in the mixed spin-3/2 and spin-2 Ising system with two alternative layers on a honeycomb lattice are investigated and discussed by the use of the effective-field theory with correlations. The interaction of the nearest-neighbour spins of each layer is taken to be positive (ferromagnetic interaction) and the interaction of the adjacent spins of the nearest-neighbour layers is considered to be either positive or negative (ferromagnetic or anti-ferromagnetic interaction). The temperature dependence of the layer magnetizations of the system is examined to characterize the nature (continuous or discontinuous) of the phase transitions and obtain the phase transition temperatures. The system exhibits both second-and first-order phase transitions besides triple point (T P ), critical end point (E), multicritical point (A), isolated critical point (C) and reentrant behaviour depending on the interaction parameters. We have also studied the temperature dependence of the total magnetization to find the compensation points, as well as to determine the type of behaviour, and N-type behaviour in N′eel classification nomenclature existing in the system. The phase diagrams are constructed in eight different planes and it is found that the system also presents the compensation phenomena depending on the sign of the bilinear exchange interactions.     

The statistical mechanics of spin-1 Ising model with AFM/AFM interactions on a bilayer Bethe lattice

The spin-1 Ising model is studied for the case of antiferromagnetic (AFM)/AFM interactions on the bilayer Bethe lattice by using the pairwise approach for several values of the coordination numbers q=3, 4 and 6 when the layers are linked with the external magnetic fields. The ground state (GS) phase diagrams, thermal variations of the order-parameters and the response functions are studied in detail to obtain the phase diagrams of the model. It was found that the system gives only one Néel temperature, T_N, for q=3. Two T_N's and first-order phase transition temperature, T_t, thus tricritical point, are found and the existence of two T_N's leads to the reentrant behavior when q=4 and 6 for some given system parameters.     

Dynamic compensation temperature in kinetic spin-5/2 Ising model on hexagonal lattice

We present a study of the dynamic behavior of a two-sublattice spin-5/2 Ising model with bilinear and crystal-field interactions in the presence of a time-dependent oscillating external magnetic field on alternate layers of a hexagonal lattice by using the Glauber-type stochastic dynamics. The lattice is formed by alternate layers of spins σ=5/2 and S=5/2. We employ the Glauber transition rates to construct the mean-field dynamic equations. First, we investigate the time variations of the average sublattice magnetizations to find the phases in the system and then the thermal behavior of the dynamic sublattice magnetizations to characterize the nature (first- or second-order) of the phase transitions and to obtain the dynamic phase transition (DPT) points. We also study the thermal behavior of the dynamic total magnetization to find the dynamic compensation temperature and to determine the type of the dynamic compensation behavior. We present the dynamic phase diagrams, including the dynamic compensation temperatures, in nine different planes. The phase diagrams contain seven different fundamental phases, thirteen different mixed phases, in which the binary and ternary combination of fundamental phases and the compensation temperature or the L-type behavior strongly depend on the interaction parameters.     

Trilayer Bethe lattices in the form of spin-(1/2,3/2,1/2)

The critical behaviors of the trilayer Bethe lattice in the form of spin-(1/2,3/2,1/2) with the exterior two layers consisting of spin-1/2 and the interior one having only spin-3/2 Ising spins are studied in terms of the recursion relations with either ferromagnetic or antiferromagnetic bilinear exchange interactions between the nearest-neighbor spins. The ground-state phase diagrams are calculated and it is found that the model presents six different ground state phase configurations. The thermal variations of the order-parameter and free energy are investigated, therefore, topologically different phase diagrams of the model are obtained. It is found that the model exhibits second- and first-order phase transitions, tricritical and bicritical points for the values of the coordination numbers q=3, 4 and 6 and, the reentrant behavior for q=4 and 6, respectively.     

Equilibrium properties of a spin-1 Ising system with bilinear,biquadratic and odd interactions

The equilibrium properties of the spin-1 Ising system Hamiltonian with arbitrary bilinear (J), biquadratic (K) and odd (L), which is also called dipolar-quadrupolar, interactions is studied for zero magnetic field in the lowest approximation of the cluster variation method. The odd interaction is combined with the bilinear (dipolar) and biquadratic (quadrupolar) exchange interactions by the geometric mean. In this system, phase transitions depend on the ratio of the coupling parameters, α = J/K; therefore, the dependence of the nature of the phase transition on α is investigated extensively and it is found that for α ⩽ 1 and α ⩾ 2000 a second-order phase transition occurs, and for 1 < α < 2000 a first-order phase transition occurs. The critical temperatures in the case of a second-order phase transition and the upper and lower limits of stability temperature in the case of a first-order phase transition are obtained for different values of α calculated using the Hessian determinant. The first-order phase transition temperatures are found by using the free energy values while increasing and decreasing the temperature. Besides the stable branches of the order parameters, we establish also the metastable and unstable parts of these curves and the thermal variations of these solutions as a function of the reduced temperature are investigated. The unstable solutions for the first-order phase transitions are obtained by displaying the free energy surfaces in the form of a contour map. Results are compared with the spin-1 Ising system Hamiltonian with the bilinear and biquadratic interactions and it is found that the odd interaction greatly influences the phase transitions.     

Dynamic phase transitions in the kinetic spin-1 Blume-Capel model on the Bethe lattice

The stationary states of the kinetic spin-1 Blume-Capel (BC) model on the Bethe lattice are analyzed in detail in terms of recursion relations. The model is described using a Glauber-type stochastic dynamics in the presence of a time-dependent oscillating external magnetic field (h) and crystal field (D) interactions. The dynamic order parameter, the hysteresis loop area and the dynamic correlation are calculated. It is found that the magnetization oscillates around nonzero values at low temperatures (T) for the ferromagnetic (F) phase while it only oscillates around zero values at high temperatures for the paramagnetic (P) phase. There are regions of the phase space where the two solutions coexist. The dynamic phase diagrams are obtained on the (kT/J,h/J) and (kT/J,D/J) planes for the coordination number q=4. In addition to second-order and first-order phase transitions, dynamical tricritical points and triple points are also observed.     

Spin-3/2 Ising model AFM/AFM two-layer lattice with crystal field

The spin-3/2 Ising model is investigated for the case of antiferromagnetic (AFM/AFM) interactions on the two-layer Bethe lattice by using the exact recursion relations in the pairwise approach for given coordination numbers q=3, 4 and 6 when the layers are under the influences of equal external magnetic and equal crystal fields. The ground state (GS) phase diagrams are obtained on the different planes in detail and then the temperature-dependent phase diagrams of the system are calculated accordingly. It is observed that the system presents both second- and first-order phase transitions for all q, therefore, tricritical points. It is also found that the system exhibits double-critical end points and isolated points. The model also presents two Néel temperatures, T_N, and the existence of which leads to the reentrant behaviour.     

The temperature-dependent phase diagrams of the spin-3/2 Ising model on a FM/AFM two-layer lattice with a crystal field

The temperature-dependent phase diagrams of the spin-3/2 Ising model on a two-layer Bethe lattice with ferromagnetic (FM)/antiferromagnetic (AFM) intra-layer and either FM or AFM type inter-layer interactions are investigated under a constant magnetic field (H) and in the presence of a crystal field (D) by using exact recursion equations in a pairwise approach for coordination numbers q=3,4 and 6, in detail. In the light of the ground-state (GS) phase diagrams, the temperature-dependent phase diagrams of the model are obtained by studying the thermal variations of the order parameters, response functions and free energy. Then, they are illustrated on the (kT/J₁,J₃/J₁) and (kT/J₁,J₂/J₁) planes for the given system parameters. It is observed that the system exhibits first- and second-order phase transitions for all q values, and hence, in some cases, tricritical points. The existence of critical-end points and that of isolated points are also observed. The re-entrant behavior owes its presence to the two Néel temperatures, T_N, that are present for all q.     

Dynamic compensation temperatures in a mixed spin-1 and spin-3/2 Ising system under a time-dependent oscillating magnetic field

We study the existence of dynamic compensation temperatures in the mixed spin-1 and spin-3/2 Ising ferrimagnetic system Hamiltonian with bilinear and crystal-field interactions in the presence of a time-dependent oscillating external magnetic field on a hexagonal lattice. We employ the Glauber transitions rates to construct the mean-field dynamic equations. We investigate the time dependence of an average sublattice magnetizations, the thermal behavior of the dynamic sublattice magnetizations and the total magnetization. From these studies, we find the phases in the system, and characterize the nature (continuous or discontinuous) of transitions as well as obtain the dynamic phase transition (DPT) points and the dynamic compensation temperatures. We also present dynamic phase diagrams, including the compensation temperatures, in the five different planes. A comparison is made with the results of the available mixed spin Ising systems.     

Dynamic Phase Transitions and Compensation Temperatures in a Mixed Spin-3/2 and Spin-5/2 Ising System

We examine the dynamic phase transitions and the dynamic compensation temperatures, within a mean-field approach, in the mixed spin-3/2 and spin-5/2 Ising system with a crystal-field interaction under a time-varying magnetic field on a hexagonal lattice by using Glauber-type stochastic dynamics. The model system consists of two interpenetrating sublattices with σ=3/2 and S=5/2. The Hamiltonian model includes intersublattice, intrasublattice, and crystal-field interactions. The intersublattice interaction is considered antiferromagnetic and to be a simple but interesting model of a ferrimagnetic system. We employ the Glauber transition rates to construct the mean-field dynamic equations, and we solve these equations in order to find the phases in the system. We also investigate the thermal behavior of the dynamic sublattice magnetizations and the dynamic total magnetization to obtain the dynamic phase transition points and compensation temperatures as well as to characterize the nature (continuous and discontinuous) of transitions. We also calculate the dynamic phase diagrams including the compensation temperatures in five different planes. According to the values of Hamiltonian parameters, five different fundamental phases, three different mixed phases, and six different types of compensation behaviors in the Néel classification nomenclature exist in the system.     

Critical and Compensation Temperatures of the Ising Bilayer System Consisting of Spin-1/2 and Spin-1 Atoms

The critical and compensation temperatures of the bilayer Bethe lattices with one of the layers having only spin-1/2 atoms and the other having only spin-1 atoms placed symmetrically are studied by using exact recursion relations in a pairwise approach. The Hamiltonian of the model consist of the bilinear intralayer coupling constants of the two layers J ₁ and J ₂ for the interactions of the atoms in layers with spin-1/2 and spin-1, respectively, and the bilinear interlayer coupling constant J ₃ between the adjacent atoms with spin-1/2 and spin-1 of the layers. After obtaining the ground state phase diagram with J ₁ > 0, the variations of the order-parameters and the free energy are investigated to obtain the phase diagram of the model by considering only the ferromagnetic ordering of the layers, i.e. J ₁ > 0 and J ₂ > 0, and ferromagnetic or antiferromagnetic ordering of the adjacent spins of the layers, J ₃ > 0 or J ₃ < 0, respectively. It was found that the system presents both second- and first-order phase transitions and, tricritical points. The compensation temperatures was also observed for the appropriate values of the system parameters. PACS: 05.50.+q 05.70.Fh 64.60.Cn 75.10.Hk     

Dynamic magnetic properties in the kinetic mixed spin-2 and spin-5/2 Ising model under a time-dependent magnetic field

We extend the recent paper [W. Jiang, V-C. Lo, B-D. Bai, J. Yang, Physica A 389 (2010) 2227-2233] to present a study, within a mean-field approach, the dynamic magnetic properties of the mixed spin-2 and spin-5/2 Ising ferrimagnetic system, which corresponds the molecular-based magnetic materials AFe^IIFe^III(C₂O₄)₃ [ A=N(n-C_nH_2n+1)₄, n=3-5], by using the Glauber-type stochastic dynamics. This mixed Ising ferrimagnetic system is used on a layered honeycomb lattice in which Fe^II (S=5/2) and Fe^III (σ=2) occupy sites. First, we investigate the time variations of average order parameters to find the phases in the system and then the thermal behavior of the dynamic order parameters to obtain the dynamic phase transition (DPT) points as well as to characterize the nature (first-or second-order) phase transitions. We also present the dynamic phase diagrams and study the dynamic magnetic hysteresis loop behaviors of the kinetic mixed spin-2 and spin-5/2 Ising ferrimagnetic system. The results are compared with some experimental and theoretical works and a good overall agreement is found.     

The crystal-field dependency of sound attenuation in the spin-3/2 ising model

The effects of crystal-field (D) on sound attenuation are considered for the spin-3/2 Ising model by using Onsager theory of irreversible thermodynamics. It is assumed that the sound wave couples to the order-parameter fluctuations, therefore, it decays mainly via order-parameter relaxation process. The order-parameters, magnetization and quadrupole moment, are defined in terms of exact recursion relations (ERR) on Bethe lattice (BL). After our analysis, two relaxation times are obtained and they are used to calculate the sound attenuation coefficient (α). Consequently, the critical behaviors of sound attenuation coefficient are investigated in terms of frequency (w) and Onsager coefficient (γ) for the coordination numbers q=3, 4 ad 6 near the second-order (T_c) and first-order (T_t) phase transition temperatures in the ferromagnetic phase regions for the negative and positive D values and the results are presented on the (k_BT/J, α) planes. It is found that the peaks about T_t’s are observed at the same temperature, but the peaks about T_c’s are observed shifted to lower and higher temperatures in increasing (w)’s and (γ)’s, respectively. In addition, the peaks are also obtained near the tricritical points for all q.     

Random crystal field effects for spin-3/2 Blume-Capel model

The effects of crystal field (Δ) which is randomly turned on with probability p or turned off with probability 1−p on the sites of the Bethe lattice are investigated to study the critical behavior of the spin-3/2 Blume-Capel model. The order-parameters are obtained in terms of the recursion relations and then the possible phase diagrams are calculated at finite temperatures for given system parameters p, Δ and coordination numbers z=3, 4, 5 and 6. It was found that the phase diagrams change drastically for given probability and randomness. The first-order phase transitions are only found for higher p values and the lines of which get shorter and eventually disappear as p decreases. The critical lines do not present any qualitative differences with z, but they are seen at higher temperatures for higher z.     

The kinetic spin-1 Blume-Capel model with Glauber dynamic

We study the dynamic phase transitions (DPT), within a mean-field approach, in the kinetic spin-1 Blume-Capel model by using the Glauber-type stochastic dynamics. The nature of the transition is characterized by investigating the behavior of the thermal variation of the dynamic order parameter and the Lyapunov exponent. The phase diagram is constructed in the temperatures (T) and single-ion anisotropy amplitude (D) plane. Our results predict first-order transitions at low temperature and large anisotropy strengths, which correspond in the phase diagram to the existence of a nonequilibrium tricritical point (TCP). We compare our results with the equilibrium phase diagram.     

Magnetic properties of a mixed spin-1 and spin-2 Heisenberg ferrimagnetic system: Green’s function study

The magnetic behaviors of a mixed spin-1 and spin-2 Heisenberg ferrimagnetic system on a square lattice are studied by using the double-time temperature-dependent Green’s function technique. In order to decouple the higher order Green’s functions, Anderson and Callen’s decoupling and random phase approximations have been used. The system is described in the presence of an external magnetic field. We illustrate the influences of the nearest- and next-nearest-neighbor interactions and the single-ion anisotropies with an external magnetic field on compensation and critical temperatures. We found that the system that includes only the nearest-neighbor interaction and the single-ion anisotropies does not have a compensation temperature. When the next-nearest-neighbor interactions exceed a certain minimum value, a compensation temperature begins to appear. For some negative values of single-ion anisotropies, there exist first-order phase transitions. The system has first-order phase transition properties when it is under the influence of an external magnetic field.