Fast neutron capture cross-section measurements of rare-earth nuclei

Measurements of neutron radiative-capture cross sections have been made using a Moxon-Rae detector and time-of-flight techniques. Cross-section ratios to In were determined for Sm, Eu, Gd, Tb, Dy, Ho, Er, Yb, Lu and Ta for 30, 65, 165 and 300 MeV neutron energies.     

Measurement of cross sections for inelastic cold-neutron scattering in metals and polymers by the method of (<Emphasis Type="Italic">n, γ</Emphasis>) analysis

The results obtained by measuring the cross sections for the inelastic scattering of very cold neutrons for a number of metals and polymers by the method of a neutron-irradiation analysis are presented. The method is based on simultaneously measuring events of inelastic scattering and neutron capture in the sample under investigation via recording gamma radiation with a semiconductor germanium detector. Neutron capture by a nucleus of the sample is accompanied by the prompt radiation of gamma rays having a known spectrum. Upon inelastic scattering, a neutron acquires thermal energy. Upon leaving the sample, this neutron is absorbed in a special converter that contains the isotope ¹⁰B. The capture of the neutron by a ¹⁰B nucleus is followed by the emission of a 477-keV gamma ray. The probabilities of capture and inelastic scattering are proportional to the respective neutron-interaction cross sections, and the ratio of the recorded detector counts corresponding to events of the two types does not depend on the spectrum of the incident flux of very cold neutrons or on the trajectory of neutron motion in the sample. The sought inelastic-scattering cross section at a fixed sample temperature is calculated by using this ratio and the known cross section for neutron capture by the sample isotope having a known gamma-radiation spectrum.     

Partial photoneutron cross sections for the isomeric state 180Tam

Photoneutron cross sections for (181)Ta(y, n) (180)Ta(m) were determined from simultaneous measurements of total cross sections (sigma(tot) and ground-state cross sections (sigma(gs)) for (180)Ta in photodisintegration of with laser Compton-backscattered rays. Techniques of direct neutron counting and photoactivation were used for the measurement of sigma(tot) and sigma(gs), respectively. The partial cross sections for the isomeric state serves as a novel probe of the nuclear level density of (180)Ta. Implications for the p- and s-process nucleosynthesis of (180)Ta(m) are given.     

Fast Neutron Capture Cross Section of Natural Molybdenum

The radiative capture cross sections of natural Mo relative to the ¹⁹⁷Au (n,γ) were measured in the 0.7—1.4MeV neutron energy range,using a large liquid scintillator detector and the time-of-flight method.In the 0.01—2.0MeV neutron energy range,the theoretical calculation of (n,γ) reaction cross section for Mo was performed.The result of calculation is compared with the experimental data.     

14MeV中子引起的Pb(n,x)203Hg, W(n,x)182Ta和W(n,x)183Ta的核反应截面测量

利用活化方法测量了14MeV中子引起的Pb(n,x)²⁰³Hg,W(n,x)¹⁸²Ta和W(n,x)¹⁸³Ta的反应截面.中子注量由监督反应⁹³Nb(n,2n)^92mNb给出,中子能量利用⁹⁰Zr(n,2n)^89m+gZr和⁹³Nb(n,2n)^92mNb反应的截面比来确定.     

间接测量中重放射性核中子俘获截面——替代比率法

s过程中的放射性核素中子俘获截面对天体核合成和核素丰度有重大影响, 在直接测量异常困难的情况下, 替代比率法是获得放射性核素中子俘获截面数据的一种间接新方法。 简单介绍了替代比率法理论, 并简要论述了用替代比率法推导中重核区放射性核素中子俘获截面的可行性。 The radioactive nuclei neutron capture cross section is very important to nuclearsynthesis and nuclide abundance in s process, but it is difficult to be measured directly because of the target production. A new method, surrogate ratio method which is developed from surrogate method, could be used to determine the cross section of radioactive nuclei neutron capture. In this paper, the surrogate ratio method was introduced and the feasibility was discussed to deduce the desired neutron capture cross sections with surrogate ratio method.     

MEASUREMENTS OF NEUTRON CAPTURE CROSS SECTIONS OF WOLFRAM AND GADOLINIUM BETWEEN 560 AND 1610keV

Neutron capture cross sections of W and Gd were measured relative to that of Au at six neutron energy values by using a large liquid scintillator tank and time-of-flight technique.The accelerator used was a 2.5MV pulsed van de Graff.The present results agree well with other recent measurement.     

锂玻璃探测器中子探测效率的刻度

为了精确测量keV能区的中子俘获截面,中国原子能科学研究院正在建造一台4π 全吸收型γ 探测装置---GTAF,锂玻璃探测器将会作为中子束流监视器测量中子能谱。利用5SDH-2 加速器刻度了锂玻璃探测器在两个入射中子单能点(250 和565 keV) 的探测效率,并使用EANT4 和MCNP 程序模拟计算了锂玻璃探测器的相对探测效率。通过归一化实验数据和模拟结果,得到了锂玻璃探测器在10keV~1 MeV 能区的中子探测效率曲线。对于把锂玻璃探测器测量得到的飞行时间谱转化为中子束流能谱,是一项非常重要的工作,同时为探测器效率刻度提供了新方法。In order to accurately measure the neutron capture cross section in the energy range of keVMeV, 4 πgamma-ray total absorption facility (GTAF) is being constructed at China Institute of Atomic Energy (CIAE). The lithium glass detector will be used as a neutron beam monitor for GTAF. The detection efficiency of the lithium glass detector at two incident neutron energy points (250, 565 keV) was calibrated in 5SDH-2 accelerator, and the relative detection efficiency was simulated by GEANT4 and MCNP code. By the normalization of the experimental data and simulation result, the neutron detection efficiency curve of the lithium glass detector between 10 keV and 1 MeV was obtained. This work will be important to convert the Time-of-flight spectrum that be measured by Li-glass detector to the energy spectrum of neutron beam, and provide the new method for calibration of detection efficiency.     

Measurement of Cross Sections for Pb(n,x)203Hg,W(n,x)182Ta and W(n,x)183Ta Reactions Induced by 14 MeV Neutrons

The cross sections for Pb(n,x)²⁰³Hg,W(n,x)^l82Ta and W(n,x)¹⁸³Ta reactions have been measured by the activation method. The neutron fluences were determined by the cross sections of ⁹³Nb (n,2n)^92mNb reaction. The neutron energies in the measurements were determined by the cross section ratios of Zr(n,2n)^89m+gZr and Nb(n,2n)^92mNb reactions.     

Small-angle elastic scattering of 14.8 mev neutrons

The 14.8 MeV neutron elastic scattering differential cross sections of U, Pb, Hg, Ta, Sn and Al have been measured for angles extending from 10° down to 1.8° and for U and Pb down to 0.35°. Nuclear cross sections extrapolated to 0° have been compared with the Wick limit. The U nuclear cross sections did not rise as sharply toward 0°, and were not in as serious disagreement with the spherical optical model, as in earlier measurements. The smallest-angle data verified the Schwinger prediction.     

Deformed even-even nuclei in a quark-meson coupling model with tensor coupling

Neutron total cross sections of ¹⁹⁷Au and ^natTa have been measured at the nELBE photoneutron source in the energy range 0.1–10MeV with a statistical uncertainty of up to 2% and a total systematic uncertainty of 1%. This facility is optimized for the fast neutron energy range and combines an excellent time structure of the neutron pulses (electron bunch width 5ps) with a short flight path of 7m. Because of the low instantaneous neutron flux transmission measurements of neutron total cross sections are possible, that exhibit very different beam and background conditions than found at other neutron sources.     

The energy dependence of Delbrück scattering investigated at Z = 73, 82 and 92

Using neutron capture γ-rays from a ¹⁴⁰CeO₂ source installed in the Grenoble high-flux reactor, differential cross sections for the elastic scattering of photons by Ta, Pb and U through θ = 120° have been measured for E = 4.291 and 4.767 MeV. These data have been supplemented by measuring elastic differential cross sections for U, θ = 120° and energies ranging from 0.279 to 1.332 MeV, using radioactive sources. The experimental differential cross sections below 1 MeV confirm the predicted Rayleigh amplitudes based on the second-order S-matrix within 3%. An excellent agreement between experiment and lowest-order Delbrück theory is observed between 1.0 and 1.4 MeV, showing that Coulomb corrections are small close to the threshold for pair production. At 4.291 and 4.767 MeV experiment and lowest-order Delbrück theory agree within ~12%     

New experimental measurement of natSe(n, γ) cross section between 1 eV to 1 keV at the CSNS Back-n facility

The ⁷⁴Se is one of 35 p-nuclei, and ⁸²Se is a r-process only nucleus, and their (n, γ) cross sections are vital input parameters for nuclear astrophysics reaction network calculations. The neutron capture cross section in the resonance range of isotopes and even natural selenium samples has not been measured. Prompt γ-rays originating from neutron-induced capture events were detected by four C₆D₆ liquid scintillator detectors at the Back-n facility of China Spallation Neutron Source (CSNS). The pulse height weighting technique (PHWT) was used to analyze the data in the 1 eV to 100 keV region. The deduced neutron capture cross section was compared with ENDF/B-VIII.0, JEFF-3.2, and JENDL-4.0, and some differences were found. Resonance parameters were extracted by the R-matrix code SAMMY in the 1 eV-1 keV region. All the cross sections of ^natSe and resonance parameters are given in the datasets. The datasets are openly available at http://www.doi.org/10.11922/sciencedb.j00113.00019.     

Radiative capture of fast neutrons by 89Y and 140Ce

The γ-ray spectra from the reactions ⁸⁹Y(n, γ)⁹⁰Y and ¹⁴⁰Ce(n, γ)¹⁴¹Ce have been measured in the neutron energy range of 6.2–15.6 MeV. The pulse-height spectra were recorded with NaI(Tl) spectrometers and time-of-flight techniques were used to improve signal-to-background ratio. Capture cross sections were determined for γ-ray transitions to the two $\text{2}\text{d}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}$ levels at 0 and 203 keV of ⁹⁰Y and to the $\text{2}\text{f}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}$ ground state of ¹⁴¹Ce as well as integrated cross sections to bound states in these nuclei. The observed γ-ray spectra and partial radiative capture cross sections were compared with predictions of the direct-semidirect capture theory. The resonance behaviour with neutron energy of both the ground-state and integrated partial capture cross sections shows the validity of the semidirect model for ⁸⁹Y and ¹⁴⁰Ce in the region of neutron energy encompassing the giant-dipole resonance. The observed symmetry of the cross sections about the peak of the resonance argues strongly for the complex form of the particle-vibration coupling interaction. A detailed comparison of the predictions of the DSD model using the complex coupling interaction shows that the capture cross sections are relatively insensitive to the real part of the interaction.     

恒星能量下核子俘获反应率的晕核效应

恒星能量下俘获截面很难直接测量。¹⁰Be（n，γ）¹¹Be俘获反应涉及到非均匀宇宙大爆炸核合成，无直接测量实验截面数据。利用转移反应¹⁰Be（d，p）¹¹Be的渐近归一化系数（ANC）方法，计算了¹⁰Be（n，γ）¹¹Be俘获反应截面和反应率。¹¹Be是中子晕核。研究表明，在恒星能量下俘获到晕态的截面和反应率显著增大。     

Proton-inclusive cross sections from 600 MeV proton-nucleus reactions

Proton-inclusive cross sections were measured for 600 MeV proton bombardment of ²⁷Al and ¹⁸¹Ta targets using the SREL synchrocyclotron. Proton energies were measured with a plastic scintillator time-of-flight system, and a 10.2 cm thick NaI detector was used for particle identification. The results of classical many-body and knock-on calculations are compared with the data.     

Measurement of (n,p) cross sections on isotopes of Cd,Sn and Te for 14 MeV neutrons

For several isotopes of Cd, Sn and Te, cross sections for the (n, p) process have been measured by activation relative to ²⁷Al(n, α)²⁴Na. As target materials, natural Cd, Sn and TeO₂ of high purity have been used. Measurements were carried out by γ-detection using a Ge(Li) detector. For measuring short-lived activities, a pneumatic tube system was used. The neutron energy was 14.6±0.2 MeV for all activations. The results obtained for the total (n, p) cross sections show decreasing values with increasing number of neutrons for a given proton number. This trend obviously follows the behaviour of the difference of the proton and neutron separation energies, determining the competition between proton and neutron emission.     

Triton-emission cross sections with 30 MeV d(Be) break-up neutrons

Triton-emission cross sections were measured for Al, Ti, V, Cr, Mn, Fe, Co, Ni, Cu, Nb, Mo, Ag, Ta, Tl, Pb and Bi with a 30 MeV d(Be) break-up neutron spectrum characterized by a multiple-foil activation technique. The accumulated tritium was separated by vacuum extraction and measured by low-level gas-phase β^? counting. The systematic trend in the cross sections is somewhat similar to that in the 53 MeV d(Be) break-up neutron spectrum; apart from some initial decrease as a function of Z, the cross section is almost constant over the entire range of Z = 22 to 83. The magnitudes of the cross sections lie between those with 14 MeV neutrons and 53 MeV d(Be) break-up neutrons. Hauser-Feshbach calculations show that the statistical model describes the triton-emission cross sections for nuclei in the (2s, ld) shell within a factor of 2; for the heavier nuclei, however, the calculated cross sections are much smaller than the experimental values.     

Resonance-spin memory in low-energy-gamma-ray spectra from Sb, Tb, Ho, and Ta odd-odd compound nuclei

The low-energy-gamma-ray spectra from neutron resonance capture with natural samples of Sb, Tb, Ho, and Ta were measured using the HPGe detector at the IBR-30 pulsed reactor at the JINR, Dubna. The resonance-spin-memory effect in the spectra from the odd-odd compound nuclei of ¹²²Sb, ¹⁶⁹Tb, and ¹⁶⁶Ho was found to be quite distinct. For the ¹⁸²Ta compound nucleus, it proved to be rather weak.