离子极化势对钙原子共面对称(e,2e)反应影响的数值研究

本文使用扭曲波波恩近似方法(DWBA)研究了共面对称条件下钙原子的电子碰撞电离反应((e,2e)反应),在DWBA理论的基础上,考虑了原子极化势和离子极化势对三重微分散射截面的影响.采用发展的DWBA方法,我们研究了出射电子能量从6.75 e V到29.25 e V范围内电子与钙原子的碰撞电离过程,计算了电离三重微分截面.通过与已有理论和实验数据进行比较发现,离子极化势对钙原子的共面对称(e,2e)反应散射微分截面有较大的影响,很好的描述了碰撞电离微分截面的结构效应,特别是在散射角度较小时(≦60o),本文计算结果与实验测量非常一致.     

电子碰撞原子(e,2e)反应的复极化势

研究包括连续通道等非处理通道的复极化势对(e,2e)碰撞过程三重微分截面的影响,即将耦合通道光学势方法得到的复极化势附加到畸变波玻恩近似方法的畸变势中,在靶态的HF近似下,计算了Ar原子和Ne原子在非共面对称几何条件下(e,2e)反应的三重微分截面.对于较高的入射能量,在实验的误差范围内,计算结果与电子动量谱的实验数据符合较好,复极化势的影响很小;对于较低的入射能量,复极化势的作用明显增大. 关键词： 复极化势 (e;2e)反应 三重微分截面 电子动量谱     

离子极化势对钙原子共面对称(e,2e)反应影响的数值研究

本文使用扭曲波波恩近似方法(DWBA)研究了共面对称条件下钙原子的电子碰撞电离反应( (e,2e)反应 ),在DWBA理论的基础上,考虑了原子极化势和离子极化势对三重微分散射截面的影响。采用发展的DWBA方法,我们研究了出射电子能量从6.75eV到29.25eV范围内电子与钙原子的碰撞电离过程,计算了电离三重微分截面。通过与已有理论和实验数据进行比较发现,离子极化势对钙原子的共面对称(e,2e)反应散射微分截面有较大的影响,很好的描述了碰撞电离微分截面的结构效应,特别是在散射角度较小时(≦60o),本文计算结果与实验测量非常一致。     

共面双对称几何条件下Ne原子(e,2e)反应的三重微分截面

利用标准一阶扭曲波玻恩近似方法（DWBA）计算了共面双对称几何条件下不同能量电子碰撞电离Ne原子的三重微分截面(TDCS),与Nixon和Murray 最新的实验测量数据进行比较.当入射电子能量较低时,理论计算结果和实验数据符合较差;随着入射电子能量的增加,而符合程度逐渐改善.     

低能电子碰撞He+(e,2e)反应绝对三重微分截面的理论研究

利用Berakdar和Briggs对BBK波函数Sommerfeld参数的修正结果，即考虑第三个粒子存在对两个粒子间相互作用的影响，考虑了入射道的库仑相互作用及出射粒子的交换对称性，计算了在共面等能分配几何情况下低能电子碰撞He⁺(e,2e)反应绝对三重微分截面.结果表明，入射道库仑场对较低的入射能量及小的碰撞参数的三重微分截面影响较大. 关键词：     

共面双对称几何条件下Ne原子(e,2e)反应的三重微分截面

利用标准一阶扭曲波玻恩近似方法(DWBA)计算了共面双对称几何条件下不同能量电子碰撞电离Ne原子的三重微分截面(TDCS),与Nixon和Murray[1]最新的实验测量数据进行比较.当入射电子能量较低时,理论计算结果和实验数据符合较差;而随着入射电子能量的增加,符合程度逐渐改善.     

共面不对称条件下Ag+(4p,4d)(e,2e)反应三重微分截面的理论研究

采用扭曲波玻恩近似(DWBA)理论计算了共面不对称几何条件下Ag⁺(4p⁶) 及Ag⁺(4d¹⁰)在不同入射电子能量和散射电子角度下(e,2e)反应的三重微分截面. 散射电子角度为4°, 10°和20°. 计算结果表明, Ag⁺(4p⁶)(e,2e)反应的三重微分截面其binary峰峰位或劈裂峰的谷位与动量转移方向有较大差别, 这可能是由于一种两次两体碰撞造成的. 另外, 还发现Ag⁺(4p⁶)(e,2e)反应三重微分截面的binary峰出现了反常劈裂现象, 这表明离子靶内壳层电离(e,2e)反应过程较外壳层更为复杂.对Ag⁺(4p⁶)及Ag⁺(4d¹⁰), 除binary峰和recoil峰以外, 在其他敲出电子角度出现了新的峰, 本文用几种两次两体碰撞过程对这些新的峰进行了解释.     

C3+与Ne碰撞过程纯电离绝对截面的测量和研究

介绍了离子-原子碰撞过程中双微分绝对截面的计算方法.利用符合技术测量了中能区C3++Ne碰撞系统的纯电离微分绝对截面.将实验结果与多体经典蒙特卡罗方法计算结果进行对比后发现,纯电离截面随入射能量变化的趋势基本一致,对理论与实验产生差异的原因作了分析.对多重电离的电离机制分析表明:高价态的反冲离子主要来自于俄歇贡献;随着入射能量的升高,电子-电子间的库仑作用也逐渐显现.此实验方法可以用于相同实验装置上的各种反应出射道的绝对截面测量,入射离子种类及入射离子能量范围将得到拓展.     

C3+与Ne碰撞过程纯电离绝对截面的测量和研究

介绍了离子-原子碰撞过程中双微分绝对截面的计算方法.利用符合技术测量了中能区C³⁺+Ne碰撞系统的纯电离微分绝对截面. 将实验结果与多体经典蒙特卡罗方法计算结果进行对比后发现，纯电离截面随入射能量变化的趋势基本一致，对理论与实验产生差异的原因作了分析. 对多重电离的电离机制分析表明：高价态的反冲离子主要来自于俄歇贡献；随着入射能量的升高，电子-电子间的库仑作用也逐渐显现. 此实验方法可以用于相同实验装置上的各种反应出射道的绝对截面测量，入射离子种类及入射离子能量范围将得到拓展. 关键词： 离子-原子碰撞 绝对截面 纯电离     

共面不对称条件下低能电子碰撞电离Ar(3p)的三重微分截面

采用修正的扭曲波玻恩近似方法, 在共面不对称几何条件下, 计算了能量为70.8 eV电子与Ar(3p)碰撞电离的(e, 2e)三重微分截面, 并与最新实验数据进行了比较. 结果表明电子交换效应和后碰撞相互作用在低能电子碰撞的(e, 2e)过程中起着重要作用. 关键词： (e,2e)三重微分截面 扭曲波玻恩近似 后碰撞相互作用 电子交换效应     

The (e, 2e) triple differential cross sections of Cu+ (3p) in coplanar asymmetric geometry

The three-body distorted-wave Born approximation has been used to calculate the (e,2e) triple differential cross sections (TDCSs) of Cu+ (3p) in different kinematical variables in coplanar asymmetric geometry.The angles 4,10 and 20 were selected as the scattering electron angles.Under high incident energy (≥ 500 eV) and high asymmetric detection energy,the binary peaks showed abnormal splits.Such abnormal splits have not been observed in atomic target and outer valence orbitals of ionic target,which indicates that an (e,2e) process for inner valence orbitals of ionic target would be more complicated than outer valence orbitals.Furthermore,some pronounced peaks appeared at certain ejected angles.We considered that these pronounced peaks are probably related to one kind of double-binary collision.     

Study of (e, 2e) process on potassium at 6 eV—60 eV above threshold in second-order Born approximation

The standard distorted wave Born approximation (DWBA) method has been extended to second-order Born amplitude in order to describe the multiple interactions between the projectile and the atomic target. Second-order DWBA calculations have been preformed to investigate the triple differential cross sections (TDCS) of coplanar doubly symmetric (e, 2e) collisions for alkali target potassium at excess energies of 6 eV-60 eV. Comparing with the first-order DWBA calculations before, the present theoretical model improves the degree of agreement with experiments, especially for backward scattering angle region of TDCS. This indicates that the present second-order Born term is capable to give a reasonable correction to DWBA model in studying coplanar symmetric (e, 2e) problems in low and intermediate energy range.     

Study of （e, 2e） process on potassium at 6 eV-60 eV above threshold in a second-order Born approximation

The standard distorted wave Born approximation(DWBA) method has been extended to second-order Born amplitude in order to describe the multiple interactions between the projectile and the atomic target.Second-order DWBA calculations have been preformed to investigate the triple differential cross sections(TDCS) of coplanar doubly symmetric(e,2e) collisions for the alkali target potassium at excess energies of 6 eV-60 eV.Compared with the previous first-order DWBA calculations,the present theoretical model improves the degree of agreement with experiments,especially for the backward scattering angle region of TDCS.This indicates that the present second-order Born term is capable of giving a reasonable correction to the DWBA model in studying coplanar symmetric(e,2e) problems in low and intermediate energy ranges.     

Triple differential cross-sections of Ne (2s<Superscript>2</Superscript>) in coplanar to perpendicular plane geometry

The distorted wave Born approximation (DWBA) with the spin averaged static exchange potential has been used to calculate the triple differential cross-sections (TDCSs) for Ne (2s ²) ionization by electron impact in coplanar to perpendicular plane symmetric geometry at 110.5 eV incident electron energy. The present theoretical results at gun angles (coplanar symmetric geometry) and (perpendicular plane geometry) are in satisfactory agreement with the available experimental data. A deep interference minimum appears in the TDCS in the coplanar symmetric geometry and a strong peak at scattering angle caused by the single collision mechanism has been observed in the perpendicular plane geometry. The TDCSs at the gun angles , and are predicted.Received: 16 July 2002, Published online: 22 July 2003PACS: 34.80.Gs Molecular excitation and ionization by electron impact - 34.80.Dp Atomic excitation and ionization by electron impact     

非共面双对称几何条件下电子离化He的（e,2e）反应

运用修正后的BBK理论计算了入射能为27.6 eV,29.6 eV和34.6 eV,非共面双对称几何条件下,电子入射离化氦原子的三重微分截面,计算结果与实验结果进行比较发现两者符合的较好,验证了低入射能时修正后的BBK模型同样适用于非共面双对称条件下的(e,2e)过程,从碰撞的微观机理上分析了影响出射电子角分布的原因.     

（e, 2e） triple-differential cross sections for Ag＋（4p, 4s） in coplanar symmetric geometry

The (e, 2e) triple-differential cross sections of Ag + (4p, 4s) are calculated based on the three-body distorted-wave Born approximation considering post-collision interaction in coplanar symmetric geometry. The energy of the outgoing electron is set to be 50, 70, 100, 200, 300, 500, 700, and 1000 eV, and the intensity and splitting of forward and backward peaks are discussed in detail. Some new structures are observed around 15° and 85° for 4p and 4s orbitals. Structures in triple-differential cross sections at 15° are reported for the first time. A double-binary collision is proposed to explain the formation of such structures. The structures at 85° are also considered as the result of one kind of double-binary collision.     

共面双对称条件下电子碰撞Ar原子单电离的一阶扭曲波Born近似

在共面双对称几何条件下,利用一阶扭曲波Born近似计算了中低能电子碰撞Ar原子(3p壳层电子)单电离的三重微分截面,并与最近的实验数据做了比较.结果表明,对于Ar原子,当入射电子能量比电离阈高40 eV以上,随着入射能量的增加,binary和recoil碰撞机理逐渐占据支配地位;在近阈能量范围,上述碰撞机理不再处于支配地位,扭曲效应明显.要完备地描述中低能入射条件下Ar原子的电子碰撞电离过程,理论模型必须同时考虑多种散射机理.     

(e,2e)反应中电子的角度分布

利用修正的BBK理论模型,在共面,等能分享,固定相对角度几何条件下,计算了能量分别为58.4,68,81.6,108.8和174.4eV的入射电子碰撞He⁺(1s)(e,2e)反应三重微分截面(TDCS),并讨论了交换,关联与干涉效应及入射道库仑场对TDCS的影响。结果表明,这些效应对决定TDCS的角度分布及大小是非常重要的。