频率啁啾脉冲下里德堡锂原子量子态布局跃迁

采用含时多态展开方法（TDMA）,结合B样条技术,计算了频率啁啾脉冲激光场中里德堡锂原子五个量子态之间的跃迁情况,并分析了激光场的四个主要参数对跃迁的影响。结果表明当取合适的激光参数时,可以实现布居数在量子态间的有效跃迁,从而一定程度上可以实现量子态的人工控制.     

频率啁啾脉冲下里德堡锂原子量子态布居跃迁

采用含时多态展开方法(TDMA),结合B样条技术,计算了频率啁啾脉冲激光场中里德堡锂原子五个量子态之间的跃迁情况,并分析了激光场的四个主要参数对跃迁的影响.结果表明当取合适的激光参数时,可以实现布居数在量子态间的有效跃迁,从而一定程度上可以实现量子态的人工控制.     

啁啾微波场中里德伯钠原子高激发态的布居跃迁

采用含时多态展开方法, 结合B样条函数和单电子原子模型势研究微波场中钠原子里德伯高激发态的性质, 得到钠原子的能级结构及在微波场中的布居数迁移, 实现对量子态的操纵与控制. 结果表明: 含时多态展开方法结合B样条函数和单电子原子模型势是有效研究微波场中碱金属原子性质的一种方法; 选择合适的啁啾率、振幅等参数, 可以实现布居数在量子态之间的完全迁移和量子态囚禁.     

里德伯钠原子经绝热快速通道的布居数跃迁相干控制

运用含时多态展开方法和B-样条函数研究了啁啾频率微波场中里德伯钠原子的量子态之间的布居数迁移.计算了里德伯钠原子n=70-77的开普勒频率.计算了在不同的微波场中六个态的布居数从n=70到n=77随时间的迁移,布居数跃迁到最终态n=77达到了98%,这可以通过连续的单光子跃迁来实现.结果表明,通过优化微波脉冲参数可以实现从低态到较高态的布居跃迁的相干控制.     

绝热条件下通常的脉冲序列和反直觉的脉冲序列对布居数转移和相干的影响

本文研究了绝热条件下，三能级Λ系统实现布居数转移和相干的两种方法，并比较了激光脉冲序列对布居数转移效率和相干的影响。运用自洽方程和密度矩阵方程，得出了相干控制量子态和布居数的数值模拟图。我们可以看到运用反直觉的脉冲序列比通常的脉冲序列在实现布居数转移和相干上更容易更优越。     

微波场中里德堡锂原子的高激发跃迁

运用含时多态展开方法研究微波场中里德堡锂原子高激发态的性质,得到锂原子在微波场中的跃迁几率,实现对量子态的操纵与控制。结果表明：选择合适的振幅、频率等参数,可以实现布居数在量子态之间的完全跃迁。     

微波场中里德堡锂原子的高激发跃迁

运用含时多态展开方法研究微波场中里德堡锂原子高激发态的性质,得到锂原子在微波场中的跃迁几率,实现对量子态的操纵与控制.结果表明:选择合适的振幅、频率等参数,可以实现布居数在量子态之间的完全跃迁.     

太赫兹场中里德堡铷原子的相干操控

采用含时多态展开方法研究了太赫兹场中里德堡铷原子布居数迁移的动力学过程,计算了一个太赫兹脉冲序列与三能级里德堡铷原子系统相互作用后的布居数分布,以及多脉冲序列对多量子态里德堡铷原子系统的相干操控,给出了同一主量子数n中不同角量子数l态布居数的含时演化过程.结果表明:通过优化太赫兹脉冲序列参数,铷原子布居数可由初态被抽运到较高的目标态,在太赫兹频率范围实现里德堡原子的操纵与控制.     

太赫兹场中里德堡铷原子的相干操控

采用含时多态展开方法研究了太赫兹场中里德堡铷原子布居数迁移的动力学过程,计算了一个太赫兹脉冲序列与三能级里德堡铷原子系统相互作用后的布居数分布,以及多脉冲序列对多量子态里德堡铷原子系统的相干操控,给出了同一主量子数n中不同角量子数l态布居数的含时演化过程.结果表明:通过优化太赫兹脉冲序列参数,铷原子布居数可由初态被抽运到较高的目标态,在太赫兹频率范围实现里德堡原子的操纵与控制.     

多维傅里叶变换光谱

二维或多维傅里叶变换谱的概念最早是在核磁共振(NMR) 谱学中提出的,随着激光技术 的发展,飞秒脉冲激光的实现使多维傅里叶变换谱的概念被引入到了光学领域,以脉冲激光代 替NMR 中的射频(RF) 场,激光波长从红外延伸到可见光波段。多维傅里叶变换光谱可以同时 提供的信息包括量子态上布居数以及量子态间的耦合,所以多维谱可以提供一维谱所无法获取的 反映量子系统演化动力学的信息,如量子系统中的能量转移以及分子间的相互作用等。人们使用 多维傅里叶变换光谱的方法对碱金属原子、量子阱、分子等量子系统中的动力学过程进行了一系 列的研究。     

Coherent population transfer in Rydberg potassium atom by a single frequency-chirped laser pulse

By using the time-dependent multilevel approach, we have calculated the coherent population transfer among the quantum states of potassium atom by a single frequency-chirped laser pulse. The results show that the population can be efficiently transferred to a target state and be trapped there by using an `intuitive' or a `counter-intuitive' frequency sweep laser pulse in the case of `narrowband' frequency-chirped laser pulse. It is also found that a pair of sequential `broadband' frequency-chirped laser pulses can efficiently transfer population from one ground state of the \La atom to the other one.     

Population transfer via adiabatic passage in the Rydberg potassium atom

Using the time-dependent multilevel approach, we have calculated the coherent population transfer between the quantum states of potassium atom by a single frequency-chirped laser pulse. The result shows that a pair of sequential `broadband' frequency-chirped laser pulses can efficiently transfer population from the initial state of the ladder system to the target state. It is also found that the population can be efficiently transferred to a target state and trapped there by using an `intuitive' or a `counterintuitive' frequency sweep laser pulse in the case of `narrowband' frequency-chirped laser pulse. Our research shows that the complete population transfer is related to the pulse duration, chirp rate, and amplitude of the laser pulse.     

Population transfer by femtosecond laser pulses in a ladder-type atomic system

The population transfer in a ladder-type atomic system driven by linearly polarized sech-shape femtosecond laser pulses is investigated by numerically solving Schr6dinger equation without including the rotating wave approximation （RWA）. It is shown that population transfer is mainly determined by the Rabi frequency （strength） of the driving laser field and the chirp rate, and that the ratio of the dipole moments and the pulse width also have a prominent effect on the population transfer. By choosing appropriate values of the above parameters, complete population transfer can be realized.     

Coherent population transfer in four-level ladder systems by single frequency-chirped laser pulse

Adiabatic passage induced by a frequency-chirped laser pulse in four-level ladder systems is investigated. Two different strategies for efficient population transfer (intuitive and counterintuitive laser pulse) are analyzed. For the larger detuning, the four-level ladder system can be reduced to a two-level system with which we are familiar. For the smaller detuning, the main conditions for realization of population transfer are the following: the width of the transform-limited laser pulse envelope frequency spectrum (without chirp) must be smaller and the peak Rabi frequency of the pulse must be larger than the detuning ε₂₁ and ε₂₁∼ε₃₂ in the case of the three-photon resonance. With this laser pulse, it is possible to achieve complete population via the intermediate levels by three successive adiabatic passages. Complete inversion is also obtained by a counterintuitive direction of the frequency sweep.     

双色脉冲激光与原子相互作用过程的研究

本文研究了双色脉冲激光与多电子原子相互作用过程,计算了高激发态的粒子数和总离子数随时间的变化,并对计算的结果进行了分析.     

The influence of femtosecond laser parameters on the wavepacket and population of the diabatic excited states of NaLi

Using the three-state model and time-dependent wavepacket method, the influence of the parameters of the intense femtosecond laser field on the wavepacket dynamic process of the double-minimum potential state 5¹Σ⁺ and the population of the ground and diabatic electronic states of NaLi are investigated. The calculations show that different femtosecond laser parameters result in different influences on the evolution of the wavepacket and the population of NaLi. With increasing laser intensity and wavelength the diabatic coupling strength between A and B states first strengthens and then weakens. The population interchanges between A and B states when the laser pulse disappears. The above results provide the suggestions and useful information for one to achieve quantum manipulation of the molecule in an experiment.     

On the detection of closed orbits in time-dependent systems by using double-pulse lasers

In the photodetachment of atoms or negative ions by a double-pulse laser, the first pulse of the double-pulse laser generates waves and the delayed second pulse may detect them. The phenomenon of the excitation and detection of waves by a double-pulse laser can be used to identify the closed orbits in the system. We demonstrate this phenomenon with a negative hydrogen ion (H⁻) by analyzing the total population excited by a double-pulse laser in a time-dependent field for different physical parameters. By analyzing the total excited population using a double-pulse laser, we can uncover all the closed orbits existing in the system. We demonstrate that this can be realized by scanning the first pulse position and the time delay between the two pulses.     

啁啾激光场中钾原子的激发

采用含时多态展开方法研究了高斯啁啾激光激发钾原子布局数跃迁的动力学过程,得到了不同激光脉冲强度、频率啁啾场中里德堡钾原子布局数跃迁,实现了布局数向目标态的跃迁.     

受激发射损耗荧光显微镜的模型设计及参量优化

受激发射损耗荧光显微镜利用荧光饱和和激发态荧光受激损耗的非线性关系,通过限制损耗区域,可突破远场光学显微术的衍射极限分辨力并实现三维成像。基于对粒子速率方程组的修正,建立了描述荧光团各能级粒子数概率时间特性的模型,并定义了时间平均损耗效率判据。采用高斯函数模拟两束入射激光脉冲通过对模型的数值计算,模拟了激发脉冲的SIED激光脉冲的光强、脉冲宽度以及两束光的延迟时间等参量与损耗效率之间的关系,并获得了各参量的最佳值,优化了损耗效率,为提高系统分辨力提供了有效的途径。