Tunneling in suspended carbon nanotubes assisted by longitudinal phonons

Current-voltage characteristics of suspended single-wall carbon nanotube quantum dots show a series of steps equally spaced in voltage. The energy scale of this harmonic, low-energy excitation spectrum is consistent with that of the longitudinal low-k phonon mode (stretching mode) in the nanotube. Agreement is found with a Franck-Condon-based model in which the phonon-assisted tunneling process is modeled as a coupling of electronic levels to underdamped quantum harmonic oscillators. A comparison with this model indicates a rather strong electron-phonon coupling factor of order unity.     

Experimental evidence of a dynamic Jahn-Teller effect in C60(+)

Detailed analysis of the highest occupied molecular orbital band shape in the photoelectron spectrum of gaseous C60 reveals a dynamic Jahn-Teller effect in the ground state of C60(+). The direct observation of three tunneling states asserts a D(3d) geometry for the isolated cation, originating from a strong vibronic coupling. These results show that the ionic motion plays an important role in the electron-phonon interaction.     

Dispersion of incoherent spectral features in systems with strong electron-phonon coupling

We study (inverse) photoemission from systems with strong coupling of doped carriers to phonons. Using an adiabatic approximation, we develop a method for calculating spectra. This method is particularly simple for systems where the electron-phonon coupling can be neglected in the initial state, e.g., the undoped t-J model. The theory then naturally explains why the electron-phonon coupling just leads to a broadening of spectra calculated without electron-phonon coupling, without changing the dispersion. This is in agreement with recent angle-resolved photoemission spectroscopy (ARPES) on undoped cuprates, and it supports the interpretation in terms of strong electron-phonon interaction. The theory also shows that for systems with strong electron-phonon coupling in the initial state, the result cannot in general be related to the spectrum obtained without electron-phonon coupling.     

Spin-dependent transport through quantum dot with inelastic interactions

Using the Keldysh nonequilibrium Green function method, we theoretically investigate the electron transport properties of a quantum dot coupled to two ferromagnetic electrodes, with inelastic electron-phonon interaction and spin flip scattering present in the quantum dot. It is found that the electron-phonon interaction reduces the current, induces new satellite polaronic peaks in the differential conductance spectrum, and at the same time leads to oscillatory tunneling magnetoresistance effect. Spin flip scattering suppresses the zero-bias conductance peak and splits it into two, with different behaviors for parallel and anti-parallel magnetic configuration of the two electrodes. Consequently, a negative tunneling magnetoresistance effect may occur in the resonant tunneling region, with increasing spin flip scattering rate.     

Spatially dependent inelastic tunneling in a single metallofullerene

We have measured the elastic and inelastic tunneling properties of isolated Gd@C(82) molecules on Ag(001) using cryogenic scanning tunneling spectroscopy. We find that the dominant inelastic channel is spatially well localized to a particular region of the molecule. Ab initio pseudopotential density-functional theory calculations indicate that this channel arises from a vibrational cage mode. We further show that the observed inelastic tunneling localization is explained by strong localization in the molecular electron-phonon coupling to this mode.     

Theory of resonant tunneling through quantum dots in the presence of electron-phonon interaction

Structures where the electrons of a two-dimensional electron gas are confined to disconnected regions can be fabricated by the use of appropriate gate geometries. The transport between these electrostatically defined quantum dots takes place by tunneling. Using the tunneling Hamiltonian approach we present a theoretical model of the system including electron-phonon interaction. The relevant coupling constants are determined from realistic wave functions for the expected confinement potentials. The phonon part of the Hamiltonian is diagonalized using a canonical transformation. Starting from the determination of the transmission matrix for the interacting system we calculate the current-voltage characteristics for different temperatures and phonon coupling strengths.     

共振拉曼效应和电子-声子耦合对线性多烯分子共振拉曼光谱的影响

线性多烯分子具有高强度且信息丰富的共振拉曼光谱,在生物学、光电材料和医学等方面都有一定应用.而含有共轭双键的短链β胡萝卜素分子是多烯分子中极具有代表性的分子.在激发光作用下π电子与CC键振动相互作用影响着吸收光谱和拉曼光谱,而共振拉曼效应和电子-声子耦合影响着共振拉曼光谱的强度、频率和线型.测量了β胡罗卜素分子在二氯乙...     

Non-stationary effects in the coupled quantum dots influenced by the electron-phonon interaction

We analyzed time evolution of the localized charge in the system of two interacting single level quantum dots coupled with the continuous spectrum states in the presence of electron-phonon interaction. We demonstrated that electron-phonon interaction leads to an increase in localized charge relaxation rate. We also found that several time scales with different relaxation rates appear in the system in the case of non-resonant tunneling between the dots. We revealed the formation of oscillations in the filling numbers time evolution caused by the emission and adsorption processes of phonons.     

The ratio of energy gap to transition temperature in amorphous superconductors

Using results of tunneling measurements, values of 2Δ(o)/kT_c for a number of amorphous transition-metal based superconductors are found to be 3.5±0.1 in agreement with the BCS theory in the weak-coupled limit unlike previously reported results suggesting strong electron-phonon coupling in amorphous non-transition metals such as Ga and Pb-Bi alloys. A comparison of our results with existing data for amorphous soft-metal alloys and A-15 compounds suggests that non-crystallinity alone does not give rise to a significantly enhanced electron-phonon interaction.     

N-S多层薄膜结构的超导临界温度讨论

本文推广了McMillan隧道模型,并应用于厚度小于超导相干长度的超导和正常膜组成的N-S多层薄膜结构。计算了它的序参量和超导临界温度。由于界面区域电声子作用的修正以及不同原子的掺杂所引起的T_c增强的可能性也作了讨论。 关键词：     

Surface-acoustic-wave-induced transport in a double quantum dot

We report on nonadiabatic transport through a double quantum dot under irradiation of surface acoustic waves generated on chip. At low excitation powers, absorption and emission of single and multiple phonons are observed. At higher power, sequential phonon assisted tunneling processes excite the double dot in a highly nonequilibrium state. The present system is attractive for studying electron-phonon interaction with piezoelectric coupling.     

Beyond Eliashberg superconductivity in MgB2: anharmonicity, two-phonon scattering, and multiple gaps

Density-functional calculations of the phonon spectrum and electron-phonon coupling in MgB (2) are presented. The E(2g) phonons, which involve in-plane B displacements, couple strongly to the p(x,y) electronic bands. The isotropic electron-phonon coupling constant is calculated to be about 0.8. Allowing for different order parameters in different bands, the superconducting lambda in the clean limit is calculated to be significantly larger. The E(2g) phonons are strongly anharmonic, and the nonlinear contribution to the coupling between the E(2g) modes and the p(x,y) bands is significant.     

Electron-longitudinal-phonon coupling in a transition metal: Ta

Recent tunneling studies of tantalum using a proximity technique reveal stronger coupling to the longitudinal modes relative to the transverse modes than observed previously for any transition metal. This result has implications for modeling the electron-phonon coupling mechanism and for future tunneling investigations. We obtain parameter values for Ta of $\text{λ = 0.73, μ}{}_{\mathrm{ph}}{}^1\text{= 0.10}$,in agreement with optimized conventional results.     

Phonon-assisted tunneling and shot noise in double barrier structures in a longitudinal magnetic field

The phonon-assisted resonant tunneling is studied for the double barrier structures in a longitudinal magnetic field. Using the scattering matrix approach with an appropriate one-particle Green's function we are able to calculate the current and the zero frequency shot noise power spectrum in a large range of the magnetic field and to any order of the electron-phonon interaction. Obtained results describe well the relevant experimental data and provide new suggestions for further examinations.     

Polaron effects in the nearly atomic limit of the Hubbard model

The Hubbard Model of electron correlation effects in solids is unified with Holstein's molecular crystal model for small polarons as a first step in studying electron-phonon coupling in π-bonded organic solids. Some implications of the electron-lattice coupling on both the single particle excitation spectrum and the effective Heisenberg exchange energy are discussed.     

Calculation of the vibronic spectrum of excitonic luminescence in AgBr:I

The radiative decay of an exciton bound to a substitutional iodine ion in AgBr is investigated theoretically. The vibronic spectrum showing multiphonon replicas is calculated under the assumptions of linear electron-phonon coupling. The experimental intensity of the one-phonon spectrum as a function of frequency could satisfactorily be reproduced only by considering coupling coefficients up to fifth neighbors. This result indicates that the bound exciton influences the dynamics of the lattice over an extended neighborhood of the iodine.     

The polaron state of a crystal

The quantum mechanics of an electron-nuclear system with strong electron-phonon coupling is considered. First, a two-site model is treated in the adiabatic approximation. As the coupling constant increases, electron transfer undergoes qualitative changes; more specifically, a potential barrier forms in the adiabatic potential, the electron transfer becomes associated with the tunneling of nuclei through the barrier, and the level splitting in the system falls off exponentially. The properties of a similar crystal model are discussed. It is shown that electron transfer in a crystal in the case of strong coupling is likewise associated with the tunneling of nuclei through barriers in the deformation space. Strong coupling modifies the electron-electron interaction terms. The Hamiltonian (exchange) terms, which are not associated with electron transfer, are only weakly modified. At the same time, the terms involving transfer (the band terms) undergo exponential reduction and vanish in the limit as M → ∞ (M is the ion mass) and the carriers become small polarons. This reduction provides a basis for the natural mechanism of enhancement of the isotope effect.     

Optical absorption of piezoelectric polarons

The optical absorption of piezoelectric polarons is calculated for all values of the electron-phonon coupling. The spectrum shows a series of peaks due to internal transitions of the polaron superposed on a background resulting from emission and absorption of acoustical phonons.     

Ab initio analysis of electron-phonon coupling in molecular devices

We report a first principles analysis of electron-phonon coupling in molecular devices under external bias voltage and during current flow. Our theory and computational framework are based on carrying out density functional theory within the Keldysh nonequilibrium Green's function formalism. Using a molecular tunnel junction of a 1,4-benzenedithiolate molecule contacted by two aluminum leads as an example, we analyze which molecular vibrational modes are most relevant to charge transport under nonequilibrium conditions. We find that the low-lying modes are most important. As a function of bias voltage, the electron-phonon coupling strength can change drastically while the vibrational spectrum changes at a few percent level.     

Electron and phonon cooling in a superconductor-normal-metal-superconductor tunnel junction

We present evidence for the cooling of normal-metal phonons, in addition to the well-known electron cooling, by electron tunneling in a superconductor-normal-metal-superconductor tunnel junction. The normal-metal electron temperature is extracted by comparing the device current-voltage characteristics to the theoretical prediction. We use a quantitative model for the heat transfer that includes the electron-phonon coupling in the normal metal and the Kapitza resistance between the substrate and the metal. It gives a very good fit to the data and enables us to extract an effective phonon temperature in the normal metal.