Spatial-temporal dispersion of the kinetic coefficients near the Anderson transition

A generalization of the Vollhardt-Wölfle localization theory is proposed to make it possible to study the spatial-temporal dispersion of the kinetic coefficients of a d-dimensional disordered system in the low-frequency, long-wavelength range (ω?_F and q?k _F ). It is shown that the critical behavior of the generalized diffusion coefficient D(q,ω) near the Anderson transition agrees with the general Berezinskii-Gor’kov localization criterion. More precisely, on the metallic side of the transition the static diffusion coefficient D(q,0) vanishes at a mobility threshold λ _c common for all q: D(q, 0)∝t=(λ _c ?λ)/λ _c →0, where λ=1/(2π?_F τ) is a dimensionless coupling constant. On the insulator side, q≠0 D(q,ω)∝?iω as ω→0 for all finite q. Within these limits, the scale of the spatial dispersion of D(q,ω) decreases in proportion to t in the metallic phase and in proportion to ωξ ², where ξ is the localization length, in the insulator phase until it reaches its lower limit ～λ _F. The suppression of the spatial dispersion of D(q,ω) near the Anderson transition up to the atomic scale confirms the asymptotic validity of the Vollhardt-Wölfle approximation: D(q,ω)?D(ω) as |t|→0 and ω→0. By contrast, the scale of the spatial dispersion of the electrical conductivity in the insulator phase is of order of the localization length and diverges in proportion to |t|^?v as |t|→0.     

Kinetic theory of classical liquids. I. Basic theory

A somewhat new approach to a kinetic theory of classical liquids is presented, and it is used to calculate the dynamical structure factor S(qω). It gives correctly the zeroth, second, and fourth frequency moments of S(qω), and it goes correctly over to the free particle value for large q. For small q and ω it goes over to proper hydrodynamics, including the coupling to heat diffusion. Results of numerical calculations on liquid argon are presented and they show very good agreement with available neutron scattering and molecular dynamics data.     

Non-equilibrium structure factor for the disordering of adsorbed monolayers

We consider the non-equilibrium, time-dependent elastic-scattering structure factor S(q,t), for the disordering of an ordered overlayer, initially in equilibrium at temperature T_I and characterized by the structure factor S(q,0)=x(q,T_I, upon a sudden increase in temperature T_I→T_F at constant coverage, such that the adsorbates equilibrate at T_F in a disordered phase. The initial decay of a peak in x(q,T_I) proceeds exponentially in time, $\text{exp}\text{(−}\text{t}\text{τ}{}_{\mathrm{q}}\text{)}$, where τ_q is a wavevector-dependent lifetime, before it crosses over to a power-law, t⁻¹ decay. When x(q,T_I) is peaked at the boundaries of the Brillouin zone (BZ), the peak approximately maintains its shape in q-space as it decays exponentially. Except near the center of the BZ, after the peak has decayed sufficiently, the dependence of S(q,t) on q is as though the spins quasi-equilibrate to the equilibrium structure factor associated with T_F, x(q,T_F), in that the ratio $\text{S(q,t)}\text{x(q,T}{}_{\mathrm{<mtext>F</mtext>}}\text{)}$ is independent of q, is dependent on time, approaching unity as t⁻¹ for large t. For systems exhibiting an initial peak for q ≈ 0, the peak decays exponentially but does not preserve its shape, since τ_q strongly depends on q, diverging as q⁻² for q→0. For these systems too, away from the center of the BZ, $\text{S}\text{(q,t)}\text{x(q,T}{}_{\mathrm{<mtext>F</mtext>}}\text{)}$ rapidly evolves to a slowly decaying function of $\text{t}\text{t}{}_{\mathrm{w}}$, independent of q. In this case, however, the characteristic time scale, t_w, is anomalously long, proportional to ξ², where ξ is the correlation length associated with the initial state. This behavior of t_w can be related to the random walk of domain boundaries.     

Scattering of conduction electrons in Fe(t x , Å)/Cr(10 Å) superlattices with ultrathin iron layers

IR magnetoreflection spectra, diagonal σ _xx and off-diagonal σ _xy components of the effective optical conductivity tensor, and magnetic properties of Fe(t _x , Å)/Cr(10 Å) superlattices have been studied. The abrupt decrease in the amplitude of dissipative function ?ωImσ _xy (ω) (ω is the cyclic frequency of light wave) in the superlattices with ultrathin Fe layers (t _Fe = 3.2, 2.6, 2.1 Å) has been analyzed. It has been found that the magnetorefractive effect in nanostructures with ultrathin iron layers is due to scattering of conduction electrons by magnetic interfacial layers formed in the Cr matrix with complete consumption of deposited iron atoms. The parameters of the interfacial scattering of electrons in the spin-up (└) and spin-down (┌) conduction channels have been discussed.     

The electronic structure and optical and magnetooptical properties of the CaCo<Subscript>2</Subscript> compound synthesized at a high pressure: Experiment and theory

The optical properties (the real ε₁ and imaginary ε₂ permittivity parts, optical conductivity σ, and reflectivity R) of the new ferromagnetic compound CaCo₂ in the Laves cubic phase (C15) synthesized at a pressure of 8.0 GPa were studied over the spectral range ?ω = 0.2–9 eV. The field and spectral (?ω = 0.5–4.2 eV) dependences of the equatorial Kerr effect were determined. The electronic structure and optical characteristics of CaCo₂ were calculated using the electron density functional theory by the linearized augmented-plane-wave method. The main band structure parameters of the compound were determined. The experimental and theoretical σ(ω) and R(ω) dependences were in satisfactory agreement with each other. The formation of the main absorption bands was found to be caused by the (p,d → d,p)-type electronic transitions related to the cobalt and calcium atoms. The exchange splitting of the 3d band of CaCo₂ was estimated, 2Δ_exc ～ (1–1.3) eV.     

Classical Motion in Force Fields with Short Range Correlations

We study the long time motion of fast particles moving through time-dependent random force fields with correlations that decay rapidly in space, but not necessarily in time. The time dependence of the averaged kinetic energy 〈p ²(t)〉/2 and mean-squared displacement 〈q ²(t)〉 is shown to exhibit a large degree of universality; it depends only on whether the force is, or is not, a gradient vector field. When it is, 〈p ²(t)〉～t ^2/5 independently of the details of the potential and of the space dimension. The stochastically accelerated particle motion is then superballistic in one dimension, with 〈q ²(t)〉～t ^12/5, and ballistic in higher dimensions, with 〈q ²(t)〉～t ². These predictions are supported by numerical results in one and two dimensions. For force fields not obtained from a potential field, the power laws are different: 〈p ²(t)〉～t ^2/3 and 〈q ²(t)〉～t ^8/3 in all dimensions d≥1.     

Excitation spectrum and T=0 dynamics of the one-dimensional planar spin-12 ferromagnet

The T=0 dynamics of the one-dimensional $\text{S}\text{=}\text{1}\text{2}$ ferromagnet with planar exchange anisotropy is studied by finite-chain calculations and a Green function approach. We demonstrate that the excitation spectrum relevant for appropriate low-T inelastic neutron scattering experiments is much more complex than predicted by linear spin-wave theory. It includes two continua and a set of discrete branches. Some of the low-lying excitations predicted by rigorous calculations, on the other hand, are shown to contribute no spectral weight to the T=0 dynamic structure factor S_zz(q,ω). We provide quantitative results for the spectral-weight distribution in S_zz(q,ω) at T=0 from bound states and continuum states, including a detailed analysis of the singularity in S_zz(q,ω) at the lower band edge. Further evidence is found for the prediction that some T=0 critical properties of the planar $\text{S}\text{=}\text{1}\text{2}$ ferro- and antiferromagnet are governed by exponents which depend continuously on the planar anisotropy.     

Quantum integrable systems related to lie algebras

Some quantum integrable finite-dimensional systems related to Lie algebras are considered. This review continues the previous review of the same authors [83] devoted to the classical aspects of these systems. The dynamics of some of these systems is closely related to free motion in symmetric spaces. Using this connection with the theory of symmetric spaces some results such as the forms of spectra, wave functions, S-matrices, quantum integrals of motion are derived. In specific cases the considered systems describe the one-dimensional n-body systems interacting pairwise via potentials g²v(q) of the following 5 types: v_I(q) = q^?2, v_II(q) = sinh^?2q, v_III(q) = sin^?2q, $\text{v}{}_{\mathrm{<mtext>IV</mtext>}}\text{(q) =}\text{P}\text{(q)}$, v_V(q) = q^?2 + ω²q². Here $\text{P}\text{(q)}$ is the Weierstrass function, so that the first three cases are merely subcases of the fourth. The system characterized by the Toda nearest-neighbour potential exp(q_jq_{j+ 1}) is moreover considered.This review presents from a general and universal point of view results obtained mainly over the past fifteen years. Besides, it contains some new results both of physical and mathematical interest.     

Bi-solitons for a class of non-linear equations with quadratic non-linearity. II

We generalize to any order q, the methods developed in a companion paper for q = 2,3 for finding bi-solitons, solutions of the class of non-integrable non-linear equations L_qK = K²; L_q = ? + Σ_i+j≤qa_ij?_xⁱ?_lⁱ, ? ≠ 0 in 1 + 1 dimensions. We call bi-solitons K(ω₁,ω₂) of the exponential type variables ω_i = exp(γ_ix + ρ_it), i = 1,2 and deal only with the so-called “non trivial” solutions which may be written as a finite sum K = Σ^lmax₀ω¹₂F_i(Z)_, F₁ rational function of Z = ω₁Z = ω₁ + ω₁. To any such polynomial K, we associate a linear transformation such that L_qK has only the power ω¹₂ of K² and we find that there are particular polynomialswhere the above restriction provide a factorization of the linear operator L_q in the product of smaller order differential operators. After this linear phase, we show in a second step that these forms yield solutions for the full non linear equation which can be derived in an intrinsic manner. Examples in the monomial and binomial cases are given.     

Inelastic neutron scattering study of spin waves in MnO

The dispersion relation E(q) for spin waves in MnO has been measured at 4.2°K by neutron inelastic scattering. The isotropic exchange integrals as well as the anisotropy constants have been determined by fitting the Hamiltonian to the data. It is found that the exchange striction plays main role in the anomaly in the magnetic interactions in MnO and the biquadratic exchange interaction j₁(S₁·S₂)² is almost absent (j₁/J₁ ? 0.002).     

Consistent MFA correlation functions of Ising models for all temperatures

A correct calculation of the Ising model correlation function C(q) = 〈(S(q) ? 〈S(q)〉) (S(-q) ? 〈S(-q)〉)〉 in the MFA results in

$\text{C(q)=}\text{〈S}{}^2\text{〉?〈〉}{}^2\text{1?(〈S}{}^2\text{〉?〈S〉}{}^2\text{βJ(q}\text{1}\text{N}\text{∑}\text{q}\text{1}\text{1?〈S〉}{}^2\text{βJ(q)}{}^{\mathrm{?1}}\text{C(q) fulfills the exact sum rule N}{}^{-1}\text{Σ}{}_{\mathrm{q}}\text{C(q) = 〈S}{}^2\text{〉 ? 〈S〉}{}^2$

. Previous literature supposed a violation of this sum rule to be a characteristic disadvantage of this approximation.     

Spin dynamics of layered triangular antiferromagnets with uniaxial anisotropy

The spin dynamics of the semiclassical Heisenberg model with uniaxial anisotropy, on the layered triangular lattice with antiferromagnetic coupling for both intralayer nearest neighbor interaction and interlayer interaction is studied both in the ordered phase and in the paramagnetic phase, using the Monte Carlo-molecular dynamics technique. The important quantities calculated are the full dynamic structure function S(q,ω)$S(\mathbf{q},\omega )$, the chiral dynamic structure function _Schi(ω)$S_{\mathrm{chi}}(\omega )$, the static order parameter and some thermodynamic quantities. Our results show the existence of propagating modes corresponding to both S(q,ω)$S(\mathbf{q},\omega )$ and _Schi(ω)$S_{\mathrm{chi}}(\omega )$ in the ordered phase, supporting the recent conjectures. Our results for the static properties show the magnetic ordering in each layer to be of coplanar 3-sublattice type deviating from 120^°${120}^{°}$ structure. In the presence of magnetic trimerization, however, we find the 3-sublattice structure to be weakened along with the tendency towards non-coplanarity of the spins, supporting the experimental conjecture. Our results for the spin dynamics are in qualitative agreement with those from the inelastic neutron scattering experiments performed recently.     

Spin susceptibility of cuprates in the model of a 2D frustrated antiferromagnet: Role of renormalization of spin fluctuations in describing neutron experiments

Experimental data on the spin susceptibility of HTSC cuprates are reproduced on the basis of a spherically symmetric approach in the frustrated Heisenberg model. The inclusion of real and imaginary renormalizations in spin Green’s functions makes it possible to explain the evolution of spin excitation spectrum ω(q) and susceptibility spectrum χ(q, ω) in the range from insulator to optimal doping. In the low-frustration limit corresponding to the weakly doped mode, the saddle singularity of ω(q) and scaling of χ_2D(ω) =∫d q Im χ(q, ω) are reproduced and an analytic expression is derived for the scaling function. In the strong frustration (optimal doping) mode, the stripe scenario is demonstrated; this leads to a peak of χ_2D (ω) in the region of ω～60 meV.     

Optical conductivity in the t − J model

Frequency dependent conductivity σ(ω) is calculated for the t ? J model by applying the memory function technique in terms of the Hubbard operators. The relaxation rate due to electron scattering on spin and charge dynamical fluctuations is calculated and a generalized Drude law for σ(ω) is obtained. For a model with an incoherent spectrum for one-hole excitations we obtain a universal form for frequency dependence of relaxation rate and conductivity in terms of the scaling function γ(ω/kT). The relaxation rate for the t ? J model is quite different from that one for the conventional Hubbard model in the strong coupling limit where it vanishes due to an exact cancellation of the intraband scattering and virtual interband transitions.     

Streuung an Kristallen mit Ionenspin-Gitter-Kopplung

The dependence of the Heisenberg exchange interaction on the ion positions couples the lattice with the ion spins. The resulting phonon damping depends on the magnetic order of the crystal. We calculate the Phonon Greens Function (PGF) by solving the equation of motion of the coupled spin-phonon system. The scattering functionsS(q,ω) andS(q) of the crystal can be determined with the PGF. In the region of great spin fluctuations an additional diffuse scattering intensity appears. This determines spin-lattice coupling parameters at least in the case of scattering of X-rays which do not interact directly with magnetism. The ordering temperature is assumed to be small compared to the Debye temperature. The magnetic influence on the diffuse scattering intensity is then of the order of a few per cent.     

On asymptotic behaviour of four spin correlation functions in a linear chain of spins

Second and fourth moments of the four spin frequency correlation functions S^Z_i(t) S^Z_i+1 (t) S^Z_j+1 〉_k,ω and 〈S^x_i(t) S^z_i+1 (t) S^x_jS^z_j+1 〉_kω have been calculated in the high temperature limit for an arbitrary spin with an isotropic Heisenberg Hamiltonian.     

Nonlinear susceptibility x;(3) in a direct gap semiconductor derived from coupled inter-and intraband equations of motion

A set of generalized Maxwell Bloch Equations describing a two band semiconductor as a system of interacting two level atoms is used to calculate the nonlinear dielectric susceptibility x;⁽³⁾ (ω, ? ω, ω). For near resonance conditions (ω ≈ ω_g) we find a simplified expression for χ⁽³⁾ that is compared with other theories. A fit using parameters relevant for InSb leads to good agreement with experimental results.