Singlet–triplet oscillations and far-infrared spectrum of four-minima quantum-dot molecule

We study ground states and far-infrared spectra (FIR) of two electrons in four-minima quantum-dot molecule in magnetic field by exact diagonalization. Ground states consist of altering singlet and triplet states, whose frequency, as a function of magnetic field, increases with increasing dot–dot separation. When the Zeeman energy is included, only the two first singlet states remain as ground states. In the FIR spectra, we observe discontinuities due to crossing ground states. Non-circular symmetry induces anticrossings, and also an additional mode above ω₊ in the spin-triplet spectrum. In particular, we conclude that electron–electron interactions cause only minor changes to the FIR spectra and deviations from the Kohn modes result from the low-symmetry confinement potential.     

Quantum confinement effects on the optical phonons of CdTe quantum dots

We present Raman-scattering results for CdTe nanocrystals in doped glasses which clearly show the confinement effects on the phonon spectra as a function of the quantum-dot size. We observed optical phonon modes, surface phonons and some of their overtone combinations. We show that the surface-phonon scattering intensity increases as the quantum-dot size decreases. Our results also show a decrease in the electron–phonon coupling as the nanocrystal size is decreased. These confinement effects are observed by changing the laser excitation energy, and thus by tuning to resonance with the optical transitions for quantum dots of different sizes within their broad size distribution in semiconductor-doped glasses.     

Far-infrared spectroscopy of quantum wires and dots, breaking Kohn’s theorem

We review far-infrared experiments on quantum wires and dots. In particular, we show that with tailored deviations from a parabolic external lateral confinement potential one can break Kohn’s theorem. This allows a detailed investigation of the internal relative motion in quantum dots and wires and the study of electron–electron interaction effects, for example, the formation of compressible and incompressible states in quantum dots and antidots.     

量子限制效应对δ掺杂GaAs/AlAs多量子阱中铍受主态寿命的影响

采用远红外时间分辨光谱,研究了量子限制效应对δ掺杂在GaAs/AlAs多量子阱中铍（Be）受主态寿命的影响.在低温下的远红外吸收谱中,清楚地观察到了三条主要吸收线,它们分别来源于铍受主从基态到它的三个奇宇称激发态的跃迁.实验结果表明：随着量子限制效应的增强,受主激发态寿命而减少,实验测得体材料中Be受主2p激发态的寿命是350 ps,而阱宽10 nm的多量子阱中的寿命是55 ps.量子限制效应对布里渊区折叠声学声子模的影响增强了受主带内空穴与声学声子相互作用,从而加快了受主带内空穴的弛豫过程. 关键词： 量子限制效应 受主态寿命 时间分辨光谱 δ掺杂')" href="#">δ掺杂     

Optical spectroscopy of CdTe/ZnTe quantum-dot superlattices

Studies of CdTe/ZnTe quantum-dot superlattices (self-assembled quantum-dot multilayers) have been carried out by optical spectroscopy methods in a wide range of temperatures. It has been shown that the ZnTe spacer layer thickness affects the properties of these quantum-dot superlattices due to changes in the elastic strain distribution pattern. An additional luminescence band appearing in the spectrum of the structure with the thinnest ZnTe spacer layer exhibits an anomalous shift of the peak position and an unusual behavior of integral intensity with the temperature increase. We assume that the spectrum of CdTe/ZnTe quantum-dot superlattices with the thinnest ZnTe spacer is caused by two kinds of excitonic states—spatially indirect and spatially direct.     

Discrepancy between photoluminescence and photoresponse intensities in n-InAs/GaAs and InAs/n-GaAs quantum-dot heterostructures

We report a discrepancy between near-infrared photoluminescence (PL) and far-infrared photoresponse (PR) efficiencies in self-assembled InAs/GaAs quantum-dot (QD) heterostructures with silicon doping in either InAs QDs or GaAs barriers. The structure with n-GaAs barriers reveals a much higher PR intensity in spite of a weaker PL intensity in comparison with n-InAs QD structure. This discrepancy is explained by differences in the electron occupation of QD sublevel associated with the Fermi-level position and in the mean free path of photogenerated carriers in GaAs barriers due to impurity scattering.     

Measurement and analysis of optical gain spectra in 1.6 to 1.8 μm InAs/InP (100) quantum-dot amplifiers

Small signal modal gain measurements have been performed on two-section ridge waveguide InAs/InP (100) quantum-dot amplifiers that we have fabricated with a peak gain wavelength around 1.70 μm. The amplifier structure is suitable for monolithic active-passive integration, and the wavelength region and wide gain bandwidth are of interest for integrated devices in biophotonic applications. A 65 nm blue shift of the peak wavelength in the gain spectrum has been observed with an increase in injection current density from 1,000 to 3,000 A/cm². The quantum-dot amplifier gain spectra have been analyzed using a quantum-dot rate-equation model that considers only the carrier dynamics. The comparison between measured and simulated spectra shows that two effects in the quantum-dot material introduce this large blue shift in the gain spectrum. The first effect is the carrier concentration dependent state filling with carriers of the bound excited and ground states in the dots. The second effect is the decrease in carrier escape time from the dots to the wetting layer with decreasing dot size.     

Two-electron quantum dot in tilted magnetic fields: Sensitivity to the confinement model

Semiconductor quantum dots are conventionally treated within the effective-mass approximation and a harmonic model potential in the two-dimensional plane for the electron confinement. The validity of this approach depends on the type of the quantum-dot device as well as on the number of electrons confined in the system. Accurate modeling is particularly demanding in the few-particle regime, where screening effects are diminished and thus the system boundaries may have a considerable effect on the confining potential. Here we solve the numerically exact two-electron states in both harmonic and hard-wall model quantum dots subjected to tilted magnetic fields. Our numerical results enable direct comparison against experimental singlet-triplet energy splittings. Our analysis shows that hard and soft wall models produce qualitatively different results for quantum dots exposed to tilted magnetic fields. Hence, we are able to address the sensitivity of the two-body phenomena to the modeling, which is of high importance in realistic spin-qubit design.     

Photoluminescence structure of highly excited quantum dots of type II

The photoluminescence (PL) due to decay of exciton-like e–e–h complex X– (expected to appear for higher levels of activation) in electrically defined quantum dots of type II is analyzed within the Hartree approach for Gaussian confining potential, where the existence of metastable (against far-infrared interband dipole transitions) states is predicted, due to interplay of bare confinement with Coulomb interaction between the carriers. As we will show, when three-particle complexes (e–e–h) are taken into account, three PL peaks can occur at zero magnetic field, which further split into four peaks when external magnetic field is applied, which stands in a good correspondence with the experimental observations. The QD size and external magnetic field dependencies of the PL spectrum are analyzed, also finding good experimental confirmation.     

Water pair and three-body potential of spectroscopic quality from Ab initio calculations

We present the first pair plus three-body potential of water from ab initio calculations that quantitatively reproduces the experimental far-infrared spectra of the water dimer and trimer. The dimer spectrum was obtained from the pair potential through rigorous six-dimensional quantum calculations of the vibration-rotation-tunneling levels. The three-body interactions, together with the pair potential, produce an accurate representation of the hydrogen bond torsional levels of the water trimer.     

Optical studies of localized excitons in symmetric coupled quantum wells

We present evidence for coupling between spatially separated excitonic states in a GaAs symmetric coupled quantum well. A split excitonic peak is observed in the photoluminescence spectrum of our sample and is identified as due to islands of monolayer fluctuation in the well width. We use the technique of far-infrared modulated photoluminescence to show that a resonant coupling exists between the excitonic states when the incident far-infrared photon energy is approximately equal to the splitting as measured in the photoluminescence spectrum. The most likely mechanism for this coupling is the dipole–dipole interaction.     

Far-infrared response of quantum-dot molecules

We report an analysis of the dipole response of a symmetric quantum-dot molecule as a function of the dot-dot separation and intensity of a perpendicular magnetic field. The potential barrier is assumed proportional to the interdot distance using a two-center oscillator potential. The results are obtained within the symmetry-unrestricted TDLSDA. It is shown that the FIR details, specially the fragmentation of the low-energy brach, are quite sensitive to the interdot separation and that in both the small and large separation limits the results converge towards the analytic Kohn's magnetoplasmon energies. The validity of the LSDA is checked by comparison with the Hartree-Fock dipole spectrum in one case. Received 29 November 2000     

A Deductive Method for the Incomplete Far-Infrared Reflection Spectrum Analysis

We report a deductive method used in the incomplete far-infrared reflection spectrum analysis. The inherent restriction between the oscillator model and Kramers-Kronig relation is used to deduct the dielectric constant. In this way, one can analysis the incomplete far-infrared reflection spectrum of a crystal by combining both oscillator model and Kramers-Kronig relation.     

Dynamical localization of two electrons in triple-quantum-dot shuttles

The dynamical localization phenomena in two-electron quantum-dot shuttles driven by an ac field have been investigated and analyzed by the Floquet theory. The dynamical localization occurs near the anti-crossings in Floquet eigenenergy spectrum. The oscillation of the quantum-dot shuttles may increase the possibility of the dynamical localization. Especially, even if the two electrons are initialized in two neighbor dots, they can be localized there for appropriate intensity of the driven field. The studies may help the understanding of dynamical localization in electron shuttles and expand the application potential of nanoelectromechanical devices.     

Study of the electric capacitance spectra on symmetric quantum-dot pattern

We have calculated the ground-state energy of the symmetric quantum-dot pattern by the ab initio calculation method, i.e. unrestricted Hartree-Fock-Roothaan (UHFR) method based on the Gaussian basis, and studied their electric capacitance spectra, assuming each quantum dot of quantum-dot pattern to be confined in a three-dimensional spherical potential well of finite depth. For the systems in question, our results show that our method and theoretical model not only give the electric capacitance peaks similar to s-shell and p-shell atom-like quantum dot, but also show some new fine-structure of electric capacitance in the symmetric quantum-dot pattern system. This method might be a feasible tool to study few-electron problems on the symmetric quantum-dot pattern system.     

Free electron laser spectral dynamics with a modulation of electron beam energy

Recent experimental and theoretical works on free electron laser spectral dynamics have pointed out the difficulty to obtain a narrow and stable spectrum operation. This goal can only be achieved by avoiding the sideband generation leading to a broadband and unstable spectrum. Tapered wiggler and two-frequency wiggler are well suited for combining sharp spectrum and high efficiency but are not really compatible with a wide tunability of laser light. Filtering sidebands is a good way for lower power experiments but it seems to be difficult to conceive wideband filters, specially in the far-infrared region. Modulation of electron energy is a new potential soft way for controlling the spectral dynamics of longpulse free electron laser. Spectral dynamics under the modulation is investigated in the linear and non-linear regimes in the far-infrared region. Simulations show that a pulsed and sharp spectrum behavior can be obtained by optimizing the modulation parameters. The interest of such a method for the far-infrared experiments is discussed.     

The light-baryon spectrum in a relativistic quark model with instanton-induced quark forces

This is the second of a series of three papers treating light-baryon resonances up to 3 GeV within a relativistically covariant quark model based on the three-fermion Bethe-Salpeter equation with instantaneous two- and three-body forces. In this paper we apply the covariant Salpeter framework (which we developed in the first paper, U. L?ring, K. Kretzschmar, B.Ch. Metsch, H.R. Petry, Eur. Phys. J. A 10, 309 (2001)) to specific quark model calculations. Quark confinement is realized by a linearly rising three-body string potential with appropriate spinorial structures in Dirac space. To describe the hyperfine structure of the baryon spectrum we adopt 't Hooft's residual interaction based on QCD-instanton effects and demonstrate that the alternative one-gluon exchange is disfavored on phenomenological grounds. Our fully relativistic framework allows to investigate the effects of the full Dirac structures of residual and confinement forces on the structure of the mass spectrum. In the present paper we present a detailed analysis of the complete non-strange-baryon spectrum and show that several prominent features of the nucleon spectrum such as, e.g., the Roper resonance and approximate “parity doublets” can be uniformly explained due to a specific interplay of relativistic effects, the confinement potential and 't Hooft's force. The results for the spectrum of strange baryons will be discussed in a subsequent paper, see U. L?ring, B.Ch. Metsch, H.R. Petry, this issue, p. 447. Received: 27 March 2001 / Accepted: 17 April 2001     

An inter-comparison of far-infrared line-by-line radiative transfer models

A considerable fraction (>40%) of the outgoing longwave radiation escapes from the Earth's atmosphere-surface system within a region of the spectrum known as the far-infrared (wave-numbers less than 650 cm⁻¹). Dominated by the line and continuum spectral features of the pure rotation band of water vapor, the far-infrared has a strong influence upon the radiative balance of the troposphere, and hence upon the climate of the Earth. Despite the importance of the far-infrared contribution, however, very few spectrally resolved observations have been made of the atmosphere for wave-numbers less than 650 cm⁻¹. The National Aeronautics and Space Administration (NASA), under its Instrument Incubator Program (IIP), is currently developing technology that will enable routine, space-based spectral measurements of the far-infrared. As part of NASA's IIP, the Far-Infrared Spectroscopy of the Troposphere (FIRST) project is developing an instrument that will have the capability of measuring the spectrum over the range from 100 to 1000 cm⁻¹ at a resolution of 0.6 cm⁻¹. To properly analyze the data from the FIRST instrument, accurate radiative transfer models will be required. Unlike the mid-infrared, however, no inter-comparison of codes has been performed for the far-infrared. Thus, in parallel with the development of the FIRST instrument, an investigation has been undertaken to inter-compare radiative transfer models for potential use in the analysis of far-infrared measurements. The initial phase of this investigation has focused upon the inter-comparison of six distinct line-by-line models. The results from this study have demonstrated remarkably good agreement among the models, with differences being of order 0.5%, thereby providing a high measure of confidence in our ability to accurately compute spectral radiances in the far-infrared.     

The study of the valence bond property in a two—different—quantum—dot molecule

The electronic energy spectrum and wavefunction of a quantum-dot molecule are studied by means of the finite-element solution of the single electron Schr?dinger equation. We find that the nature of the coupling can be covalent, ionic, or "intermediate" new mixed states, depending on various parameters such as the separation distance between two dots, the height of potential barrier, matching of the energies and parities of the orbital localized on each dot. The bond property can be used to explain the experimental result obtained by Oosterkamp et al. (1998 Nature 395 873).     

Optimal control of charge with local gates in quantum-dot lattices

Semiconductor quantum dots are among the leading candidates for next-generation nanoscale devices due to their tunable size, shape, and low energy consumption. Here we apply quantum optimal control theory to coherently manipulate the single-electron charge distribution in quantum-dot lattices of various sizes. In particular, we show that to control the charge distribution it is sufficient to optimize the gate voltage acting on a single quantum dot in the lattice. We generally find yields around 99% in the picosecond time scale when using realistic models for the quantum-dot lattices on a real-space grid. We analyze and discuss both the limitations of the model regarding the gate parameters as well as the potential of the scheme for applications as quantum-dot cellular automata.