Quasi-static bubble in a yield stress fluid: elasto-plastic model

The influence of the yield stress of Carbopol® gel dispersions on the behaviour of quasi-static bubbles was investigated. Many fluids, from many different industrial fields, have yield stress behaviour. Most of them contain gas bubbles. To study bubble behaviour in such suspensions, a transparent model fluid (dispersion of Carbopol® in water) was used. The experimental device allowed to quasi-statically increase bubble internal pressure with small pressure step to reach a maximum target internal pressure and the pressure setpoint was inverted to return to the initial pressure. Hysterical behaviour of the bubbles was highlighted as they did not regain their initial shape because of yield stress. We show that the rheological behaviour is related to the internal pressure, bubble geometry and yield stress in quasi-static conditions. A modification of the Laplace law depending on the yield stress of the fluid and bubble sphericity was proposed and validated.     

Dynamics of a small bubble in a compressible fluid

An efficient (simplified) method for solving problems of spherically symmetric dynamics of a small gas bubble in a compressible fluid is proposed. The method is based on the joint use of the full problem statement (the gas dynamics equations for the gas and the fluid) and its relevant simplifications. Some approximate statements are discussed. In the proposed method, the rarefaction and compression of the gas during the slow motion of the bubble surface is assumed to be uniform over the bubble volume. At the same time the fluid in the thin zone adjacent to the bubble is considered to be slightly compressible. Otherwise the gas dynamics equations are used for the gas and the fluid. The dynamics of the fluid in the thick external zone are described by the linear acoustics only. The proposed simplified method and two others used in literature are estimated by comparison of their numerical results with those obtained in full statement. Copyright © 2000 John Wiley & Sons, Ltd.     

Robust numerical analysis of the dynamic bubble formation process in a viscous liquid

The dynamics of bubble formation from a submerged nozzle in a highly viscous liquid with relatively fast inflow gas velocity is studied numerically. The numerical simulations are carried out using a sharp interface coupled level set/volume-of-fluid (CLSVOF) method and the governing equations are solved through a hydrodynamic scheme with formal second-order accuracy. Numerical results agree well with experimental results and it is shown that the sharp interface CLSVOF method enables one to reproduce the bubble formation process for a wide range of inflow gas velocities. From numerical results, one can improve their understanding of the mechanisms regarding the dynamics of bubble formation. For example, it is found that for some sets of parameters that the bubble formation process reaches steady state after several bubbles are released from the nozzle. At steady state, bubbles uniformly rise freely in the viscous liquid. It is observed that the fluid flow around a formed bubble has a significant role in determining the overall dynamic process of bubble formation; e.g. the effect of the fluid flow from the preceding bubble can be seen on newly formed bubbles.     

Oscillatory Marangoni convection around the air bubble in a vertical surfactant stratificationConvection de Marangoni oscillante autour d'une bulle d'air dans une stratification verticale surfactante

The solutocapillary Marangoni convection around a gas bubble in the inhomogeneous binary mixture of miscible fluids with a vertical surfactant concentration gradient was studied experimentally. A new phenomenon, the oscillatory instability of the surfactant mass transfer, near the bubble boundary, was detected and investigated. The interpretation of this effect as an interaction between the surfactant adsorption at the bubble free surface and solutocapillary and buoyancy convective mechanisms is proposed. The experimental data on oscillation period in relation to bubble dimensions, time, liquid layer thickness, physico-chemical fluid parameters and concentration gradients are presented and discussed. To cite this article: K. Kostarev et al., C. R. Mecanique 332 (2004).     

A numerical strategy for the direct 3D simulation of the expansion of bubbles into a molten polymer during a foaming process

In the framework of the foam process modelling, this paper presents a numerical strategy for the direct 3D simulation of the expansion of gas bubbles into a molten polymer. This expansion is due to a gas overpressure. The polymer is assumed to be incompressible and to behave as a pseudo‐plastic fluid. Each bubble is governed by a simple ideal gas law. The velocity and the pressure fields, defined in the liquid by a Stokes system, are subsequently extended to each bubble in a way of not perturbing the interface velocity. Hence, a global velocity–pressure‐mixed system is solved over the whole computational domain, thanks to a discretization based on an unstructured first‐order finite element. Since dealing with an Eulerian approach, an interface capturing method is used to follow the bubble evolution. For each bubble, a pure advection equation is solved by using a space–time discontinuous‐Galerkin method, coupled with an r‐adaptation technique. Finally, the numerical strategy is achieved by considering a global mesh expansion motion, which conserves the amount of liquid into the computational domain during the expansion. The expansion of one bubble is firstly considered, and the simulations are compared with an analytical model. The formation of a cellular structure is then investigated by considering the expansion of 64 bubbles in 2D and the expansion of 400 bubbles in 3D. Copyright © 2007 John Wiley & Sons, Ltd.     

Dissolved gas effects on thermocapillary convection during boiling in reduced gravity environments

The mechanisms by which thermocapillary convection arises during boiling of nominally pure fluids in low-g environments are currently not known. It has recently been suggested that small amounts of dissolved gas within the bulk liquid can accumulate within the vapor bubble, forming localized concentration gradients that results in a temperature gradient to form along the liquid–vapor interface that drives thermocapillary convection. This hypothesis was tested by boiling > 99.3% pure n-perfluorohexane with and without noncondensible gas in a low-g environment using a 7.0 × 7.0 mm² microheater array to measure time and space resolved heat transfer at various wall superheats. The thermocapillary convection around the primary bubble that formed in the gassy fluid was found to be much weaker than in the degassed fluid, and the primary bubble diameter was much larger in the gassy fluid due to the accumulation of noncondensible gas within the bubble. The results suggest that the accumulation of noncondensible gas in the bubble can result in temperature variations along the interface but due to the increased vapor/gas bubble size, the driving thermocapillary temperature gradient along the interface is significantly reduced and result in much weaker thermocapillary flow. The highest CHF values in a reduced gravity environment (19 W/cm²) occurred when the fluid was highly subcooled and degassed.     

A conservative local interface sharpening scheme for the constrained interpolation profile method

A conservative local interface sharpening scheme has been developed for the constrained interpolation profile method with the conservative semi‐Lagrangian scheme, because the conservative semi‐Lagrangian scheme does not feature a mechanism to control the interface thickness, thus causing an increase of numerical error with the advance of the time step. The proposed sharpening scheme is based on the conservative level set method proposed by Olsson and Kreiss. However, because their method can cause excessive deformation of the free‐surface in certain circumstances, we propose an improvement of the method by developing a local sharpening technique. Several advection tests are presented to assess the correctness of the advection and the improved interface sharpening scheme. This is followed by the validations of dam‐breaking flow and the rising bubble flows. The mass of the fluid is exactly conserved and the computed terminal velocity of the rising bubble agrees well with the experiments compared with other numerical methods such as the volume of fluid method (VOF), the front tracking method, and the level set method. Copyright © 2011 John Wiley & Sons, Ltd.     

Countercurrent gas/liquid flow and mixing: Implications for water disinfection

Experimental and numerical results are presented from investigations into the hydrodynamics of a bench scale bubble column reactor. Countercurrent bubble column reactors are most commonly used in water disinfection for effecting mass transfer of ozone to the aqueous phase. In the reactor column used in this study, gas is introduced at the bottom of the column via a spherical diffuser and water is introduced to the top of the column through a manifold packed with glass spheres. Residence time distribution (RTD) studies were conducted for a range of gas flow rates chosen to span the dispersed flow bubble regime. A multiphase computational fluid dynamics (CFD) model was used to simulate the flow in the bubble column and to gain insights into the fluid dynamics of countercurrent flow bubble columns. The CFD model accurately predicted trends in mixing. Use of CFD in bubble column design and scale-up thus may yield better designs than those based on empirical relations.     

Numerical simulation of a single bubble by compressible two‐phase fluids

The present work deals with the numerical investigation of a collapsing bubble in a liquid–gas fluid, which is modeled as a single compressible medium. The medium is characterized by the stiffened gas law using different material parameters for the two phases. For the discretization of the stiffened gas model, the approach of Saurel and Abgrall is employed where the flow equations, here the Euler equations, for the conserved quantities are approximated by a finite volume scheme, and an upwind discretization is used for the non‐conservative transport equations of the pressure law coefficients. The original first‐order discretization is extended to higher order applying second‐order ENO reconstruction to the primitive variables. The derivation of the non‐conservative upwind discretization for the phase indicator, here the gas fraction, is presented for arbitrary unstructured grids. The efficiency of the numerical scheme is significantly improved by employing local grid adaptation. For this purpose, multiscale‐based grid adaptation is used in combination with a multilevel time stepping strategy to avoid small time steps for coarse cells. The resulting numerical scheme is then applied to the numerical investigation of the 2‐D axisymmetric collapse of a gas bubble in a free flow field and near to a rigid wall. The numerical investigation predicts physical features such as bubble collapse, bubble splitting and the formation of a liquid jet that can be observed in experiments with laser‐induced cavitation bubbles. Opposite to the experiments, the computations reveal insight to the state inside the bubble clearly indicating that these features are caused by the acceleration of the gas due to shock wave focusing and reflection as well as wave interaction processes. While incompressible models have been used to provide useful predictions on the change of the bubble shape of a collapsing bubble near a solid boundary, we wish to study the effects of shock wave emissions into the ambient liquid on the bubble collapse, a phenomenon that may not be captured using an incompressible fluid model. Copyright © 2009 John Wiley & Sons, Ltd.     

DISCRETE MODELLING OF TWO-DIMENSIONAL LIQUID FOAMS

Liquid foam is a dense random packing of gas or liquid bubbles in a small amount of immiscible liquid containing surfactants. The liquid within the Plateau borders, although small in volume, causes considerable difficulties to the investigation of the spatial structure and physical properties of foams, and the situation becomes even more complicated as the fluid flows. To solve these problems, a discrete model of two-dimensional liquid foams on the bubble scale is proposed in this work. The bubble surface is represented with finite number of nodes, and the liquid within Plateau borders is discretized into lattice particles. The gas in bubbles is treated as ideal gas at constant temperatures. This model is tested by choosing an arbitrary shape bubble as the initial condition. This then automatically evolves into a circular shape, which indicates that the surface energy minimum routine is obeyed without calling external controlling conditions. Without inserting liquid particle among the bubble channels, periodic ordered and disordered dry foams are both simulated, and the fine foam structures are developed. Wet foams are also simulated by inserting fluid among bubble channels. The calculated coordination number, as a function of liquid fractions, agrees well with the standard values.     

Convective and diffusive surfactant transfer in multiphase liquid systems

Laser interferometry was used to investigate diffusive and convective mass transfer in a multicomponent fluid mixture with a liquid–liquid or liquid–gas interface. For this purpose, an immobile gas bubble or insoluble fluid droplet, having the shape of a short cylinder with a free lateral surface, was inserted into a thin liquid layer. In the case of non-uniform distribution of the dissolved surfactant component, the Marangoni convection near the drop/bubble was initiated by the surface tension inhomogeneities, depending on the surfactant concentration. The applied experimental techniques allowed us to study the structure and evolution of the convective flows and concentration fields in a liquid layer, which due to its small thickness were nearly two-dimensional. Making use of both the vertical and horizontal orientation of the liquid layer, we investigated the mass transfer process at different levels of the interaction between gravity and capillary forces. During the experiments, we detected new solutocapillary phenomena, which were found to be caused by oscillatory regimes of solutal convection occurring around air bubbles and chlorobenzene drops in heterogeneous aqueous solutions of alcohol with a vertical surfactant concentration gradient. The role of the oscillatory instability in the processes of drop saturation by the surfactant from its water solution and an inverse process of surfactant extraction from the drop into the surrounding homogeneous fluid (water) was determined. A reasonable explanation for the driving mechanisms of the discovered effects has been proposed.     

NUMERICAL ANALYSIS ON THE VELOCITY AND PRESSURE FIELDS INDUCED BYMULTI-OSCILLATIONS OF AN UNDERWATER EXPLOSION BUBBLE

假设水下爆炸气泡的内部气体在膨胀收缩过程中满足绝热条件,周围流体无黏无旋不可压缩. 基于势流理论,采用边界元法研究气泡动力学行为,重点关注气泡引起的流场脉动载荷以及滞后流特性,给出了相关的理论推导和数值计算方法. 通过将数值结果与解析解、实验值进行对比,数值模型的收敛性和有效性能够得到保证. 利用编写的程序进行计算和分析,发现在气泡加速膨胀阶段,流场压力在气泡径向不一定是逐渐衰减,还有可能以先增后减的规律变化;气泡射流后,为了能够继续描述环状气泡的运动以及流场特性,将此时的流场分为无旋场和一个布置在气泡内部涡环的叠加,计算过程中采用了一些数值技巧处理气泡的拓扑结构,得以连续模拟多个周期的气泡运动. 环状气泡具有相对较高的上浮迁移速度,而且在其顶部和底部附近分别形成两个高压区,顶部的高压区峰值相对较大,底部的高压区范围相对较大. 环状气泡中心轴上的流场速度会在气泡中心有一个加速过程,在气泡顶部附近又迅速减小.     

Certain hydrodynamic characteristics of the evolution of a solitary spherical bubble in the finite compression regime

The characteristics of unsteady incompressible fluid flow around a gas or vapor bubble compressed to a finite size are theoretically investigated. The velocity on the bubble boundary, the integral flow-rate and kinetic energy, and the form of the pressure distribution in the fluid are analyzed. Certain general qualitative regularities independent of viscosity, surface tension, and the intensity of the heat and mass transfer processes are revealed. The general results obtained are illustrated and specified with reference to a simplified polytropic model.     

Numerical simulation of bubble and droplet deformation by a level set approach with surface tension in three dimensions

In this paper we present a three‐dimensional Navier–Stokes solver for incompressible two‐phase flow problems with surface tension and apply the proposed scheme to the simulation of bubble and droplet deformation. One of the main concerns of this study is the impact of surface tension and its discretization on the overall convergence behavior and conservation properties. Our approach employs a standard finite difference/finite volume discretization on uniform Cartesian staggered grids and uses Chorin's projection approach. The free surface between the two fluid phases is tracked with a level set (LS) technique. Here, the interface conditions are implicitly incorporated into the momentum equations by the continuum surface force method. Surface tension is evaluated using a smoothed delta function and a third‐order interpolation. The problem of mass conservation for the two phases is treated by a reinitialization of the LS function employing a regularized signum function and a global fixed point iteration. All convective terms are discretized by a WENO scheme of fifth order. Altogether, our approach exhibits a second‐order convergence away from the free surface. The discretization of surface tension requires a smoothing scheme near the free surface, which leads to a first‐order convergence in the smoothing region. We discuss the details of the proposed numerical scheme and present the results of several numerical experiments concerning mass conservation, convergence of curvature, and the application of our solver to the simulation of two rising bubble problems, one with small and one with large jumps in material parameters, and the simulation of a droplet deformation due to a shear flow in three space dimensions. Furthermore, we compare our three‐dimensional results with those of quasi‐two‐dimensional and two‐dimensional simulations. This comparison clearly shows the need for full three‐dimensional simulations of droplet and bubble deformation to capture the correct physical behavior. Copyright © 2009 John Wiley & Sons, Ltd.     

Shock structure in bubbly liquids: comparison of direct numerical simulations and model equations

Shock wave structure in a bubbly mixture composed of a cluster of gas bubbles in a quiescent liquid with initial void fractions around 10% inside a 3D rectangular domain excited by a sudden increase in the pressure at one boundary is investigated using the front tracking/finite volume method. The effects of bubble/bubble interactions and bubble deformations are, therefore, investigated for further modeling. The liquid is taken to be incompressible while the bubbles are assumed to be compressible. The gas pressure inside the bubbles is taken uniform and is assumed to vary isothermally. Results obtained for the pressure distribution at different locations along the direction of propagation show the characteristics of one-dimensional unsteady shock propagation evolving towards steady-state. The steady-state shock structures obtained by the present direct numerical simulations, which show a transition from A-type to C-type steady-state shock structures, are compared with those obtained by the classical Rayleigh–Plesset equation and by a modified Rayleigh–Plesset equation accounting for bubble/bubble interactions in the mean-field theory.      

Assessment of regularized delta functions and feedback forcing schemes for an immersed boundary method

We present an improved immersed boundary method for simulating incompressible viscous flow around an arbitrarily moving body on a fixed computational grid. To achieve a large Courant–Friedrichs–Lewy number and to transfer quantities between Eulerian and Lagrangian domains effectively, we combined the feedback forcing scheme of the virtual boundary method with Peskin's regularized delta function approach. Stability analysis of the proposed method was carried out for various types of regularized delta functions. The stability regime of the 4‐point regularized delta function was much wider than that of the 2‐point delta function. An optimum regime of the feedback forcing is suggested on the basis of the analysis of stability limits and feedback forcing gains. The proposed method was implemented in a finite‐difference and fractional‐step context. The proposed method was tested on several flow problems, including the flow past a stationary cylinder, inline oscillation of a cylinder in a quiescent fluid, and transverse oscillation of a circular cylinder in a free‐stream. The findings were in excellent agreement with previous numerical and experimental results. Copyright © 2008 John Wiley & Sons, Ltd.     

Direct 2D simulation of small gas bubble clusters: from the expansion step to the equilibrium state

A numerical strategy, based on an adaptive finite element method, is proposed for the direct two‐dimensional simulation of the expansion of small clusters of gas bubbles within a Newtonian liquid matrix. The velocity and pressure fields in the liquid are first defined through the Stokes equations and are subsequently extended to the gas bubbles. The liquid–gas coupling is imposed through the stress exerted on the liquid by gas pressure (ruled by an ideal gas law) and by surface tension. A level set method, combined with a mesh adaptation technique, is used to track liquid–gas interfaces. Many numerical simulations are presented. The single bubble case allows to compare the simulations to an analytical model. Simulations of the expansion of small clusters are then presented showing the interaction and evolution of the gas bubbles to an equilibrium state, involving topological rearrangements induced by Plateau's rule. Copyright © 2006 John Wiley & Sons, Ltd.     

不同发射深度下导弹水下点火气水流体动力计算

从流体动力角度研究了不同发射深度下，导弹水下点火这一非定常非线性过程。整个系统分为外部水流场、喷管流场和燃气泡流场三个区域加以考虑。水流场采用不可压势流模型，用边界元方法求解；喷管内流场采用非定常一元流动模型，用特征线差分法求解，并设置了激波检测功能；燃气泡采用基于质量和能量守恒的零维计算模型。在时间域中用步进方法实现了三个流场的耦合求解。给出了四种发射深度下的数值计算结果，展示了导弹水下点火的一     

Formation of the finely dispersed gas phase in upward and downward fluid flows

The influence of the fluid and gas flow rate parameters on the diameter of bubbles separating from a single capillary immersed in a fluid flow in a channel of 1×1 cm cross-section is investigated. The dependences of the mean bubble diameter on the fluid velocity and the gas flow rate through the capillary are obtained. The frequency of the bubble detachment from the capillary is estimated. It is shown that the histogram of the bubble size distribution changes qualitatively with the excess of a certain critical bubble detachment frequency, which is associated with the transition from the discrete to jet mode of detachment.     

Development of level set method with good area preservation to predict interface in two‐phase flows

A two‐step conservative level set method is proposed in this study to simulate the gas/water two‐phase flow. For the sake of accuracy, the spatial derivative terms in the equations of motion for an incompressible fluid flow are approximated by the coupled compact scheme. For accurately predicting the modified level set function, the dispersion‐relation‐preserving advection scheme is developed to preserve the theoretical dispersion relation for the first‐order derivative terms shown in the pure advection equation cast in conservative form. For the purpose of retaining its long‐time accurate Casimir functionals and Hamiltonian in the transport equation for the level set function, the time derivative term is discretized by the sixth‐order accurate symplectic Runge–Kutta scheme. To resolve contact discontinuity oscillations near interface, nonlinear compression flux term and artificial damping term are properly added to the second‐step equation of the modified level set method. For the verification of the proposed dispersion‐relation‐preserving scheme applied in non‐staggered grids for solving the incompressible flow equations, three benchmark problems have been chosen in this study. The conservative level set method with area‐preserving property proposed for capturing the interface in incompressible fluid flows is also verified by solving the dam‐break, Rayleigh–Taylor instability, bubble rising in water, and droplet falling in water problems. Good agreements with the referenced solutions are demonstrated in all the investigated problems. Copyright © 2010 John Wiley & Sons, Ltd.