共查询到20条相似文献,搜索用时 31 毫秒
1.
Using the time-dependent multilevel approach, we have calculated the
coherent population transfer between the quantum states of potassium
atom by a single frequency-chirped laser pulse. The result shows that
a pair of sequential `broadband' frequency-chirped laser pulses can
efficiently transfer population from the initial state of the ladder
system to the target state. It is also found that the population can
be efficiently transferred to a target state and trapped there by
using an `intuitive' or a `counterintuitive' frequency sweep laser
pulse in the case of `narrowband' frequency-chirped laser pulse. Our
research shows that the complete population transfer is related to
the pulse duration, chirp rate, and amplitude of the laser pulse. 相似文献
2.
Coherent population transfer in Rydberg potassium atom by a single frequency-chirped laser pulse 下载免费PDF全文
By using the time-dependent multilevel approach, we have calculated the coherent
population transfer among the quantum states of potassium atom by a single
frequency-chirped laser pulse. The results show that the population can be
efficiently transferred to a target state and be trapped there by using an
`intuitive' or a `counter-intuitive' frequency sweep laser pulse in the case of
`narrowband' frequency-chirped laser pulse. It is also found that a pair of
sequential `broadband' frequency-chirped laser pulses can efficiently transfer
population from one ground state of the \La atom to the other one. 相似文献
3.
采用含时多态展开方法研究了高斯啁啾激光激发钾原子布局数跃迁的动力学过程,得到了不同激光脉冲强度、频率啁啾场中里德堡钾原子布局数跃迁,实现了布局数向目标态的跃迁. 相似文献
4.
In this paper, the dynamics of coherent laser control of potassium
atoms is studied by using the time-dependent multilevel approach
(TDMA). The calculation results of population transfer are presented
with different laser fields. The results show that the population can
be transferred to target state completely by a specially designed
laser field. 相似文献
5.
R. Unanyan S. Guérin B. W. Shore K. Bergmann 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2000,8(3):443-449
In traditional schemes of multilevel multilaser excitation, each laser pulse interacts with only one pair of states, and the
rotating wave approximation (RWA) is applicable. Here we study the population transfer process in a three-state system when
each of the two lasers interacts with each of the pair of states and when the Rabi frequencies characterizing the interaction
strengths of the system are comparable to or larger than the difference of the transition frequencies. We show that complete
and robust population transfer is possible under conditions more general than those hitherto considered necessary for stimulated
Raman adiabatic passage (STIRAP) or for successive π pulses. Using adiabatic Floquet theory we show that successful population transfer can be interpreted as adiabatic passage
by means of a transfer state which connects the initial and final states. The Floquet picture offers a convenient interpretation
of the population transfer as accompanied by multiple absorption of photons from or emission into the laser fields. 相似文献
6.
频率啁啾激光场中锂原子的激发与态囚禁 总被引:1,自引:1,他引:0
采用含时多态展开方法,对不同频率啁啾激光场中里德堡锂原子布居数的相干迁移特性进行了计算研究。结果表明:布居数跃迁几率对激光脉冲形状、激光场强度、啁啾率等参数非常敏感,在合适的激光参数下,可以实现布居数在四个量子态之间的完全迁移和量子态的囚禁。 相似文献
7.
Adiabatic passage induced by a frequency-chirped laser pulse in four-level ladder systems is investigated. Two different strategies for efficient population transfer (intuitive and counterintuitive laser pulse) are analyzed. For the larger detuning, the four-level ladder system can be reduced to a two-level system with which we are familiar. For the smaller detuning, the main conditions for realization of population transfer are the following: the width of the transform-limited laser pulse envelope frequency spectrum (without chirp) must be smaller and the peak Rabi frequency of the pulse must be larger than the detuning ε21 and ε21∼ε32 in the case of the three-photon resonance. With this laser pulse, it is possible to achieve complete population via the intermediate levels by three successive adiabatic passages. Complete inversion is also obtained by a counterintuitive direction of the frequency sweep. 相似文献
8.
9.
利用"反直觉"频率啁啾激光脉冲分析了偶能级ladder系统的布局数迁移,其中在缀饰激光场作用下N-2个中间态进行耦合.作为偶能级ladder系统的代表,我们着重分析了四能级ladder系统.研究发现如果缀饰激光场足够强且发生共振,则在能级1和能级4之间发生完全布局数迁移必须要求有一个恰当的脉冲叠加面积,调谐pump激光和stokes激光,使其中一个缀饰中间态发生共振,则可以使这个四能级系统简化为三能级系统. 相似文献
10.
《Comptes Rendus de l''Academie des Sciences Series IV Physics》2001,2(7):1001-1012
Electrostriction, population transfer caused by absorption of laser energy and subsequent thermalization are the most important mechanisms responsible for the formation of laser-induced gratings. Applying time resolved light diffraction from electrostrictive gratings allows for the measurements of thermodynamic properties like temperature, gas composition, and flow velocity. Thermal gratings can be employed as a very sensitive spectroscopic tool.The Two-Colour Four-Wave Mixing (TCFWM) signal formed by a non-resonant pump laser and a resonant probe laser in an acetylene/air diffusion flame comprises of contributions due to soot and C2, the latter is generated by vaporising the soot. Profile measurements across the flame have shown that the signal composition changes within the flame.Intermediate level labelling by Two-Colour Resonant Four-Wave Mixing Spectroscopy (TC-RFWM) is applied to reduce the spectral complexity of molecular spectra. In addition, we observe extra resonances forbidden by a conventional three-level scheme in OH- and NH-containing flames. A detailed investigation shows that the newly observed TC-RFWM resonances are induced by collisional energy transfer within the population, alignment and orientation gratings formed in both electronic states that are coupled to the laser fields. 相似文献
11.
Sola IR Chang BY Santamaria J Malinovsky VS Krause JL 《Physical review letters》2000,85(20):4241-4244
In this Letter we describe a method for population transfer using intense, ultrafast laser pulses. The selectivity is accomplished by careful shaping of light-induced potentials (LIPs). Creation and control of the LIPs is accomplished by choosing pairs of pulses with proper frequency detunings and time delays. As an example, selective population transfer is demonstrated for a three-state model of the sodium dimer. 相似文献
12.
13.
A theoretical analysis is presented of the effect of correlation between fluctuations of laser pulse amplitudes on population
transfer between the states of a three-level atom coupled by the laser field. The carrier frequencies of the pulses are tuned
to resonance with the transitions between the ground and excited states, |〈 and | 2〈, and the excited and metastable states,
|2〈 and |3〈, in a lambda-type configuration. The laser pulses are timed so that population transfer between states |1〈 and
| 3〈 is made possible by stimulated Raman adiabatic passage (STIRAP) in the absence of fluctuations. STIRAP does not occur
when the laser fields are not correlated. When the fluctuations of one pulse amplitude duplicate those of the other, STIRAP
can be observed for pulse amplitudes larger than those required in the absence of fluctuations. 相似文献
14.
Controlling Population Transfer and Dissociation Rate of Na2 Molecules with Ultra-Short Intense Laser Pulses 下载免费PDF全文
A scheme used for controlling the population transfer and the dissociation rate of Na2 molecules is described by using the quantum wavepacket dynamical method. It is theoretically shown that the population transfer and the dissociation rate of Na2 molecules can be controlled by pump and probe laser pulses with appropriate widths of pulses, sequence and intensities. 相似文献
15.
Adiabatic population transfer in effective three-level systems driven by laser beams 总被引:1,自引:0,他引:1 下载免费PDF全文
The population transfer in effective three-state systems driven by laser beams has been studied based on the theory of Lewis-Riesenfeld Hermitian invariants in the full- and partial-adiabatic approximations. A strict formulation of adiabatic conditions is given, and a new adiabatic condition for inducing a complete population transfer is found. 相似文献
16.
V.S. Malinovsky J.L. Krause 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2001,14(2):147-155
We present a general theory of adiabatic rapid passage (ARP) with intense, linearly chirped laser pulses. For pulses with
a Gaussian profile and a fixed bandwidth, we derive a rigorous formula for the maximum temporal chirp rate that can be sustained
by the pulse. A modified Landau-Zener formula displays clearly the relationships among the pulse parameters. This formula
is used to derive the optimal conditions for efficient, robust population transfer. As illustrations of the theory, we present
results for two- and four-level systems, and selective vibronic excitation in the I2 molecule. We demonstrate that population transfer with chirped pulses is more robust and more selective than population transfer
with transform-limited pulses.
Received 6 September 2000 and Received in final form 25 September 2000 相似文献
17.
This paper investigates the effect of carried-envelope phase on transient process in a cascade-type atomic system, which is driven by two ultrashort laser pulses (probe and signal laser). It is found that the one- and two-photon processes corresponding to pathway |0〉→|1〉and |0〉→|1〉→|2〉 can be enhanced or ,suppressed by modulating the carried-envelope phases of probe laser pulse. Our numerical results also show that the transient populations of two excited states can be periodically affected by the carried-envelope phase of probe laser pulse. With certain time, the partial population transfer between two exited states can be realized just by adjusting the carried-envelope phase of probe laser pulse. 相似文献
18.
<正>Using the time-dependent multilevel approach(TDML),this paper studies the dynamics of coherent control of Rydberg lithium atoms and demonstrates that Rydberg lithium atoms can be transferred to states of higher principal quantum number by exposing them to specially designed frequency-chirped laser pulses.The population transfer from n= 70 to n= 75 states of lithium atoms with efficiency of more than 90%is achieved by means of the sequential adiabatic rapid passages.The results agree well with the experimental ones and show that the coherent control of the population transfer from the lower n to the higher n states can be accomplished by the optimization of the chirping parameters and the intensity of laser field. 相似文献
19.
X. H. Yang Z. H. Zhang Z. Wang X. N. Yan 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2010,57(2):253-258
We investigate ultrafast coherent population transfer driven by few-cycle pump and Stokes laser pulses in the Λ-type three-level
system with the stimulated Raman adiabatic passage technique beyond the rotating-wave approximation. In contrast to the case
with the rotating wave approximation, the most efficient population transfer may be realized without the satisfaction of the
one-photon resonances or two-photon resonance and the transfer efficiency depends critically on the Rabi frequencies and initial
optical phases of the two laser fields when the peak Rabi frequencies are much larger than the respective transition frequencies.
Moreover, complete and robust population transfer can still be obtained with the variations of the Rabi frequencies, pulse
durations, and one-photon or two-photon detuning in a moderate range, though a considerable transient population may reside
in the excited state. These abnormal behaviors result from the counterrotating terms, which are not taken into account in
the traditional rotating wave approximation. 相似文献
20.
Millimeter/submillimeter rotational absorption spectroscopy has been used as a diagnostic probe of a cw HCN discharge laser. This sensitive technique allowed in situ absolute population measurements of a number of vibrational states of HCN (including the upper lasing state) and other pertinent molecules. This unique set of data, which was obtained under a variety of discharge and laser conditions, is directly related to excitation, inversion, and relaxation processes. Along with elucidating several fundamental aspects of inversion and relaxation these results also strongly indicate that the primary laser excitation mechanism is near-resonant energy transfer from vibrationally excited nitrogen, N2 (v=1), to the fundamental symmetric stretching mode of hydrogen cyanide, HCN(100), and subsequent thermal population exchange between HCN (100) and the upper laser state, HCN (110).Work supported by ARO Contract DAAG-29-83-K-0078 相似文献