Manifestation of new interference effects in a superconductor-ferromagnet spin valve

Superconductor-ferromagnet (S/F) spin valve effect theories based on the S/F proximity phenomenon assume that the superconducting transition temperature Tc of F1/F2/S or F1/S/F2 trilayers for parallel magnetizations of the F1 and F2 layers (T(c)(P)) are smaller than for the antiparallel orientations (T(c)(AP)). Here, we report for CoOx/Fe1/Cu/Fe2/In multilayers with varying Fe2-layer thickness the sign-changing oscillating behavior of the spin valve effect ΔT(c) = T(c)(AP) - T(c)(P). We observe the full direct effect with T(c)(AP) > T(c)(P) for Fe2-layer thickness d(Fe2) < 1 nm and the full inverse (T(c)(AP) < T(c((P)) effect for d(Fe2) ≥ 1 nm. Interference of Cooper pair wave functions reflected from both surfaces of the Fe2 layer appear as the most probable reason for the observed behavior of ΔT(c).     

Andreev reflections and magnetoresistance in ferromagnet-superconductor mesoscopic structures

An analysis is made of the change in the resistance of a nanostructure consisting of a diffusive ferromagnetic (F) wire and normal metal electrodes, due to the onset of superconductivity (S) in the normal electrode and Andreev scattering processes. The superconducting transition results in an additional contact resistance arising from the necessity to match the spin-polarized current in the F-wire to the spinless current in the S reservoir, which is comparable to the resistance of a piece of F wire with length equal to the spin relaxation length. It is also shown that in the absence of spin relaxation the resistance of a two-domain structure is the same for a ferro-or antiferromagnetic configuration if one electrode is in the superconducting state. Pis’ma Zh. éksp. Teor. Fiz. 69, No. 7, 497–502 (10 April 1999) Published in English in the original Russian journal. Edited by Steve Torstveit.     

Angular dependence of the superconducting transition temperature in ferromagnet-superconductor-ferromagnet trilayers

The superconducting transition temperature T(c) of a ferromagnet (F)-superconductor (S)-ferromagnet trilayer depends on the mutual orientation of the magnetic moments of the F layers. This effect has been previously observed in F/S/F systems as a T(c) difference between parallel and antiparallel configurations of the F layers. Here we report measurements of T(c) in CuNi/Nb/CuNi trilayers as a function of the angle between the magnetic moments of the CuNi ferromagnets. The observed angular dependence of T(c) is in qualitative agreement with a F/S proximity theory that accounts for the odd triplet component of the condensate predicted to arise for noncollinear orientation of the magnetic moments of the F layers.     

Microscopic theory of non local pair correlations in metallic F/S/F trilayers

We consider a microscopic theory of F/S/F trilayers with metallic or insulating ferromagnets. The trilayer with metallic ferromagnets is controlled by the formation of non local pair correlations among the two ferromagnets which do not exist with insulating ferromagnets. The difference between the insulating and ferromagnetic models can be understood from lowest order diagrams. Metallic ferromagnets are controlled by non local pair correlations and the superconducting gap is larger if the ferromagnetic electrodes have a parallel spin orientation. Insulating ferromagnets are controlled by pair breaking and the superconducting gap is smaller if the ferromagnetic electrodes have a parallel spin orientation. The same behavior is found in the presence of disorder in the microscopic phase variables and also in the presence of a partial spin polarization of the ferromagnets. The different behaviors of the metallic and insulating trilayers may be probed in experiments. Received 4 July 2001 and Received in final form 8 November 2001     

Recent experimental results on the superconductor/ferromagnet proximity effect

The recent experimental results on the proximity effect in heterostructures composed of superconducting and ferromagnetic thin films are reviewed. First, the experimental observation and investigation of the spin screening effect, i.e., a spin polarization in the V layer developing in the superconducting state under the influence of a spin polarization of conduction electrons in the ferromagnetic layer are discussed. This effect was predicted theoretically by Bergeret et al. [F. S. Bergeret, A. F. Volkov, and K. B. Efetov, EPL 66, 111 (2004); Phys. Rev. B 69, 174504 (2004)]. Then, the progress concerning the experimental realization of the superconducting spin switch device based on the superconductor/ferromagnet proximity effect is presented.     

Tunneling conductance on surface of topological insulator ferromagnet/insulator/(s- or d-wave) superconductor junction: Effect of magnetically-induced relativistic mass

We investigate the tunneling conductance on the surface of topological insulator ferromagnet (F)/insulator (I)/superconductor (S) junction where superconducting type is either s- or d-wave paring. Topological insulators (TI) are insulating in bulk but conducting on the surface with the Dirac-fermion-like carriers. In contrast to the Dirac fermions in graphene, relativistic mass of the Dirac fermions in TI can be easily caused by applying magnetic field perpendicular to its surface. In this work, we emphatically focus on the effect of the magnetically-induced relativistic mass on the tunneling conductance of a TI-based F/I/S junction. We find that, due to the effect of spinless fermions as carriers in TI, the behavior of the tunneling conductance in a TI-based NIS junction resembles that in a nonmagnetic graphene-based NIS junction. In case of the d-wave paring F/I/S junction, increasing magnetically-induced relativistic mass changes the zero bias conductance dip (peak) to a zero bias conductance peak (dip). This behavior cannot be observed in a graphene-based F/I/S junction.     

Critical temperature oscillations and reentrant superconductivity due to the FFLO like state in F/S/F trilayers

Ferromagnet/Superconductor/Ferromagnet (F/S/F) trilayers, in which the establishing of a Fulde‐Ferrell Larkin‐Ovchinnikov (FFLO) like state leads to interference effects of the superconducting pairing wave function, form the core of the superconducting spin valve. The realization of strong critical temperature oscillations in such trilayers, as a function of the ferromagnetic layer thicknesses or, even more efficient, reentrant superconductivity, are the key condition to obtain a large spin valve effect, i.e. a large shift in the critical temperature. Both phenomena have been realized experimentally in the Cu₄₁Ni₅₉/Nb/Cu₄₁Ni₅₉ trilayers investigated in the present work.     

Antiferromagnetic spin fluctuations above the dome-shaped and full-gap superconducting states of LaFeAsO1-xFx revealed by (75)As-nuclear quadrupole resonance

We report a systematic study by (75)As nuclear-quadrupole resonance in LaFeAsO(1-x)F(x). The antiferromagnetic spin fluctuation found above the magnetic ordering temperature T(N) = 58 K for x = 0.03 persists in the regime 0.04 ≤ x ≤ 0.08, where superconductivity sets in. A dome-shaped x dependence of the superconducting transition temperature T(c) is found, with the highest T(c) = 27 K at x = 0.06, which is realized under significant antiferromagnetic spin fluctuation. With increasing x further, the antiferromagnetic spin fluctuation decreases, and so does T(c). These features resemble closely the cuprates La(2-x)Sr(x)CuO(4). In x = 0.06, the spin-lattice relaxation rate (1/T(1)) below T(c) decreases exponentially down to 0.13T(c), which unambiguously indicates that the energy gaps are fully opened. The temperature variation of 1/T(1) below T(c) is rendered nonexponential for other x by impurity scattering.     

Multigap superconductivity in sesquicarbides La2C3 and Y2C3

A complex structure of the superconducting order parameter in Ln2C3 (Ln=La,Y) is demonstrated by muon spin relaxation measurements in their mixed state. The muon depolarization rate sigma v(T)] exhibits a characteristic temperature dependence that can be perfectly described by a phenomenological double-gap model for nodeless superconductivity. While the magnitude of two gaps is similar between La2C3 and Y2C3, a significant difference in the interband coupling between those two cases is clearly observed in the behavior of sigma v(T).     

Pressure Studies of the Unconventional Superconductors CeTIn 5 (T: Co,Ir)

In the quest for new superconductor compounds which adopt the superconducting state at increasingly higher transition temperatures T c , a non-phonon mediated coupling between the charge carriers seems to play a key role. In order to enhance our understanding of such unconventional coupling mechanisms, we studied a new family of heavy fermion (HF) superconductors CeTIn 5 (T: transition metal) whose properties point toward the realization of unconventional superconductivity (SC): the specific heat, thermal conductivity and nuclear spin-lattice relaxation rate of CeIrIn 5 and CeCoIn 5 decrease as a power law of temperature instead of exponentially for T < T c . We report on measurements of the heat capacity of CeIrIn 5 and CeCoIn 5 at hydrostatic pressures p h 1.6 GPa. In both compounds, T c increases with increasing pressure, while the mass of the quasi-particles m eff decreases, as indicated by the ratio C / T | T c . As a working hypothesis based on theories of a nearly antiferromagnetic Fermi-liquid (NAFFL), this may be interpreted as the stabilization of the superconducting state by an increase of the characteristic spin fluctuation temperature T_{\rm SF}\ (T_{\rm SF}\propto k_{\rm F}^{2}/m_{\rm eff}).     

Superconducting spin-valve and triplet superconductivity

Recent experimental results on the superconducting spin-valve effect and generation of the long-range triplet superconductivity in a F1/F2/S structure are reviewed (here, F1 and F2 are uncoupled ferromagnetic layers, and S is the superconducting layer). The main results are the following: (i) the maximum of the magnitude of the superconducting spin-valve effect increases with decreasing the exchange field h in the ferromagnetic layer; (ii) a full switching between the normal and superconducting states may be realized with the aid of the triplet contribution to the spin-valve effect.     

EuS/Ta异质结的极大磁电阻效应

在铁磁/超导异质结中,铁磁体的交换场通过近邻效应将导致超导体准粒子态密度的塞曼劈裂.基于该效应,在外磁场不强的情况下,通过外加磁场可以有效地调节铁磁/超导界面处的交换作用,从而实现超导体在正常态和超导态之间转换,产生极大磁电阻.本文利用脉冲激光沉积方法制备了EuS/Ta异质结并研究了其电磁特性.Ta在3.6 K以下为超导态,EuS在20 K以下为铁磁态.在2 K时,EuS/Ta异质结中可观测蝴蝶型磁滞回线,证明在低磁场下(<±0.18 T)异质结中EuS铁磁态和Ta超导态共存.磁输运测试表明,通过施加外磁场可以有效调节EuS的交换场,随着交换场的增大,同时也加强了界面处的交换作用,从而抑制Ta的超导态,实现了Ta在超导态和正常态之间的转变,在EuS/Ta异质结中观测到了高达144000%的磁电阻.本文制备的EuS/Ta异质结具有极大磁电阻效应,在自旋电子学器件中有潜在的应用前景.     

Field-suppressed interfacial spin scattering in YBa2Cu3O7−δ/La0.67Sr0.33MnO3 heterostructures

The superconductivity and magnetoresistance (MR) of epitaxial bilayers consisting of YBa₂Cu₃O_7?δ (YBCO) and La_0.67Sr_0.33MnO₃ (LSMO) are investigated with respect to the proximity and spin polarization effects. In the region of the mixed vortex state near the onset temperature of the superconducting transition, the diffusion of the spin-polarized quasiparticles from the LSMO to the YBCO is evidenced by their distinct magnetotransport behaviors, which are characterized by two superconducting transitions. It is revealed that the second transition is strongly dependent on the applied magnetic field, demonstrating an abnormal pair-breaking effect. This effect, together with the reduced MR, is believed to arise from an increase in the spin injection efficiency induced by the suppressed interfacial spin scattering, disclosing a new perspective for understanding the magnetotransport phenomena in proximity-coupled superconductor/ferromagnet (S/F) hybrids.     

Multiple-quantum J-resolved NMR spectroscopy (MQ-JRES): measurement of multiple-quantum relaxation rates and relative signs of spin coupling constants

The technique of multiple-quantum J-resolved NMR spectroscopy (MQ-JRES) is introduced and applied to the spin system SI(3)-M (such as in the example given here, the (13)CH(3)-(12)CH in alanine). The SI(3) spin system was excited to its highest quantum state (8S(y)I(x)I(y)I(y)), which consists of four coherences: quadruple quantum of (3I + S), double quantum of (3I - S), double quantum of (I + S), and zero quantum of (I - S). In the MQ spectrum generated from the projection onto the F(1) dimension, the resonances of the different multiple-quantum coherences are resolved by their coupling constants to the remote spin (M). The absorptive lineshapes in both F(1) and F(2) dimensions enable accurate measurements of transverse relaxation rates, and both amplitude and relative signs of the long-range coupling constants are to be derived from either frequency or time domain data. The selective detection of MQ-JRES spectra of the individual MQ coherences using either phase cycling or pulsed field gradients is presented.     

Nondemolition measurements of a single quantum spin using Josephson oscillations

We consider a single localized spin-1/2 between the singlet superconducting leads of a Josephson junction (e.g., a superconducting STM). For the spin subject to a dc magnetic field B parallel z, we study the spin dynamics and the possibility to measure the spin state via transport through the junction embedded in a dissipative circuit. Turning on the tunneling or a voltage bias induces oscillations of the Josephson current, with an amplitude sensitive to the initial value of the z component of the spin, S(z)=+/-1/2. At low temperatures, when effects of quasiparticles are negligible, this procedure realizes a quantum nondemolition measurement of S(z).     

Microscopic theory of equilibrium properties of F/S/F trilayers with weak ferromagnets

The aim of this paper is to explain the non monotonic temperature dependence of the self-consistent superconducting gap of ferromagnet/superconductor/ferromagnet (F/S/F) trilayers with weak ferromagnets in the parallel alignment (equivalent to F/S bilayers). We show that this is due to Andreev bound states that compete with the formation of a minigap. Using a recursive algorithm we discuss in detail the roles of various parameters (thicknesses of the superconductor and ferromagnets, relative spin orientation of the ferromagnets, exchange field, temperature, disorder, interface transparencies).Received: 23 January 2004, Published online: 29 June 2004PACS: 74.78.Na Mesoscopic and nanoscale systems - 74.45. + c Proximity effects; Andreev effect; SN and SNS junctions - 74.50. + r Tunneling phenomena; point contacts, weak links, Josephson effects     

Superconducting spin valve effect of a v layer coupled to an antiferromagnetic [Fe/V] superlattice

We studied superconducting V layers deposited on an antiferromagnetically coupled [Fe(2)V(11)](20) superlattice. The parallel upper critical magnetic field exhibits an anomalous T dependence up to the ferromagnetic saturation field of the superlattice, indicating that the superconducting transition temperature T(S) decreases when rotating the relative sublattice magnetization directions of the superlattice from antiparallel to parallel. This proves that the pair breaking effect of a Fe2 layer is reduced if at a distance of 1.5 nm a second Fe2 layer with antiparallel spin orientation exists.     

Change in the sign of the magnetoresistance effect in bilayer superconductor/ferromagnet structures under change in the type of the domain structure in the ferromagnet

The magnetoresistance effects in the bi- and trilayer hybrid planar superconductor/ferromagnet (S/F) structures based on Py (permalloy) and Nb near the superconducting transition temperature T _C are considered. It has been experimentally shown that the sign of the observed magnetoresistance peaks in the bilayer S/F systems changes from negative to positive at the permalloy layer thickness corresponding to the change in the type of domain walls from Néel to Bloch. For the Néel walls at the ferromagnet coercive fields, the negative magnetoresistance effect, which is due to a decrease in the depairing action of the exchange field E _ex, is observed in the S/F bilayers. For the Bloch domain walls, the magnetoresistance of the bilayer S/F structures is determined by the dissipative motion of Abrikosov vortices in the superconducting layer. In the trilayer F/S/F structures, the magnetoresistance is mainly due to the suppression of the superconducting order parameter in the superconducting layer under the action of the accumulation of the spin-polarized carriers near the S/F interfaces.     

Optimum spin-state selection for all multiplicities in the acquisition dimension of the HSQC experiment

Most conventional heteronuclear spin-state-selective (S(3)) NMR experiments only work for a specific multiplicity, typically IS spin systems. Here, we introduce a general and efficient IPAP strategy to achieve S(3) editing simultaneously for all multiplicities in the acquisition dimension of the HSQC experiment. Complementary in-phase (HSQC-IP) and anti-phase (HSQC-AP) data are separately recorded with a simple phase exchange of two 90 degrees proton pulses involved in the mixing process of the F2-coupled sensitivity-improved HSQC pulse sequence. Additive and subtractive linear combination of these IP/AP data generates simplified F2-alpha/beta-spin-edited HSQC subspectra for all IS, I(2)S, and I(3)S spin systems and combines enhanced and optimized sensitivity with excellent tolerance to unwanted cross-talk contributions over a considerable range of coupling constants. Practical aspects such as pulse phase settings, transfer efficiency dependence, inter-pulse delay optimization, and percentage of cross-talk are theoretically analyzed and discussed as a function of each I(n)S multiplicity. Particular emphasis on the features associated to spin-editing in diastereotopic I(2)S spin systems and application to the measurement of long-range proton-carbon coupling constants are also provided.     

Enhancement of the Josephson current by an exchange field in superconductor-ferromagnet structures

We calculate the dc Josephson current for two superconductor/ferromagnet (S/F) bilayers separated by a thin insulating film. It is demonstrated that the critical Josephson current I(c) in the junction strongly depends on the relative orientation of the effective exchange field h of the bilayers. We found that in the case of an antiparallel orientation I(c) increases at low temperatures with increasing h and at zero temperature has a singularity when h equals the superconducting gap Delta. This striking behavior contrasts with the suppression of the critical current by the magnetic moments aligned in parallel and is an interesting new effect of the interplay between superconductors and ferromagnets.