The turbulent flow of non-Newtonian fluids in the absence of anomalous wall effects

For Newtonian fluids, the engineering predictions for pressure drop in turbulent pipe flow are well established. However, in the case of non-Newtonian liquids, only a few design techniques have been proposed and these do not share a common basis with the approach for Newtonian systems. This present work attempts to provide a common basis for both Newtonian and non-Newtonian systems in situations where anomalous wall effects are absent. Previously published experimental data suggest that if the Reynolds number is calculated on the basis of the apparent viscosity at the wall then the standard Newtonian correlations can be used for the prediction of pressure drop. The use of the wall viscosity in defining the Reynolds number also serves as a test for anomalous behaviour. Any departure of the experimental data from the Newtonian turbulent friction factor correlation indicates anomalous behaviour.     

Interaction between Taylor bubbles rising in stagnant non-Newtonian fluids

The interaction between Taylor bubbles rising in stagnant non-Newtonian solutions was studied. Aqueous solutions of carboxymethylcellulose (CMC) and polyacrylamide (PAA) polymers were used to study the effect of different rheological properties: shear viscosity and viscoelasticity. The solutions studied covered a range of Reynolds numbers between 10 and 714, and Deborah numbers up to 14. The study was performed with pairs of Taylor bubbles rising in a vertical column (0.032 m internal diameter) filled with stagnant liquid. The velocities of the leading and trailing bubbles were measured by sets of laser diodes/photocells placed along the column. The velocity of the trailing bubble was analysed together with the liquid velocity profile in the wake of a single rising bubble (Particle Image Velocimetry data obtained from the literature). For the less concentrated CMC solutions, with moderate shear viscosity and low viscoelasticity, the interaction between Taylor bubbles was similar to that found in Newtonian fluids. For the most concentrated CMC solution, which has high shear viscosity and moderate viscoelasticity, a negative wake forms behind the Taylor bubbles, inhibiting coalescence since the bubbles maintain a minimum distance of about 1D between them. For the PAA solutions, with moderate shear viscosity but higher viscoelasticity than the CMC solutions, longer wake lengths are seen, which are responsible for trailing bubble acceleration at greater distances from the leading bubble. Also in the PAA solutions, the long time needed for the fluid to recover its initial shear viscosity after the passage of the first bubble makes the fluid less resistant to the trailing bubble flow. Hence, the trailing bubble can travel at a higher velocity than the leading bubble, even at distances above 90D.     

CFD study on rise and deformation characteristics of buoyancy-driven spheroid bubbles in stagnant Carreau model non-Newtonian fluids

The bubbles are almost ubiquitous in many chemical and processing industries; and many of the polymeric solutions obey non-Newtonian rheological characteristics. Therefore, in this work the rise and deformation characteristics of spheroid bubbles in Carreau model non-Newtonian fluids are numerically investigated using a level set method. To demonstrate the validity of the moving bubble interface, the present simulations are compared with existing numerical and experimental results available in the literature; and for these comparisons, the computational geometries are considered same as reported in corresponding literatures. The present bubble deformation characteristics are satisfactorily agreeing with their literature counterparts. After establishing the validity of the numerical solution procedure, the same method is applied to obtain the deformation characteristics of an air bubble in Carreau model non-Newtonian fluids. Further, the results in terms of the volume fraction images, streamlines, and viscosity profiles around the deforming bubbles are presented as function of the bubble rise time.     

The minimum in-line coalescence height of bubbles in non-Newtonian fluid

The minimum in-line coalescence height of bubbles generated from a submerged nozzle was investigated experimentally in shear thinning non-Newtonian fluid at lower Reynolds number (2∼60). Carboxymethyl cellulose sodium (CMC) aqueous solution and carbon dioxide were used as the liquid phase and the gas phase, respectively. The process of the formation, movement and in-line coalescence of bubbles was visualized and recorded by a high-speed digital camera. The influences of bubble size, bubble generation frequency and liquid property on the minimum in-line coalescence height of bubbles were investigated by changing nozzle diameter, gas flow rate and the mass concentration of CMC aqueous solutions. For a given liquid, the generating frequency and size of bubbles increased but the minimum coalescence height of in-line bubbles decreased when the nozzle diameter and gas flow rate were increased. When the nozzle diameter and gas flow rate were fixed, the shear-thinning effect of CMC aqueous solution became stronger with increasing CMC mass concentration, which led to the increase in both the terminal rise velocity and average acceleration of the trailing bubble, consequently, the minimum in-line coalescence height of bubbles decreased. An empirical correlation for estimating the minimum in-line bubble coalescence height was proposed, the calculating values accords well with experimental data with a mean relative deviation only 7.6%.     

Shapes of ellipsoidal bubbles in infinite stagnant liquids

Aspect ratios E of ellipsoidal bubbles in infinite stagnant clean liquids are measured for log M = −6.6, −5.5, −4.9 and −3.9, where M is the Morton number. An empirical correlation of E applicable to a wide range of the Morton number is proposed by making use of the present data and Sugihara's data at log M = −11 (2007). The aspect ratio in this correlation is expressed in terms of the combination of the Eötvös number and the bubble Reynolds number to account for the effects of the inertial, viscous, buoyant and surface tension forces on E. Terminal velocities of ellipsoidal bubbles are accurately predicted by using the proposed correlation and a drag correlation proposed by Rastello et al. (2011).     

Cavitation structures formed during the rebound of a sphere from a wetted surface

We use high-speed imaging to observe the dynamics of cavitation, caused by the impact and subsequent rebound of a sphere from a solid surface covered with a thin layer of highly viscous liquid. We note marked qualitative differences between the cavitation structures with increase in viscosity, as well as between Newtonian and non-Newtonian liquids. The patterns observed are quite unexpected and intricate, appearing in concentric ring formations around the site of impact. In all cases, we identify a distinct radius from which the primary bubbles emanate. This radius is modelled with a modified form of Hertz contact theory. Within this radius, we show that some fine cavitation structure may exist or that it may be one large cavitation bubble. For the non-Newtonian fluids, we observe foam-like structures extending radially with diminishing bubble sizes with increase in radial position. Whereas for the Newtonian fluids, the opposite trend is observed with increasing bubble size for increasing radial position. Finally, we compare our experimental observations of cavitation to the maximum tension criterion proposed by Joseph (J Fluid Mech 366:367–378, 1998) showing that this provides the lower limit for the onset of cavitation in our experiments.     

Bubble stability in a class of non-Newtonian fluids with shear dependent viscosities

Using elementary dynamical systems theory we delineate the locally asymptotically stable, stable, and unstable equilibrium states of a spherical vapor bubble immersed in an unbounded non-Newtonian fluid with shear dependent viscosity; stability results for the equilibrium states of bubbles immersed in a Newtonian fluid are obtained as special cases.     

Dynamics of a Taylor bubble in steady and pulsatile co-current flow of Newtonian and shear-thinning liquids in a vertical tube

A computational analysis is carried out to ascertain the effects of steady and pulsatile co-current flow, on the dynamics of an air bubble rising in a vertical tube containing water or a solution of Carboxymethylcellulose (CMC) in water. The mass fraction (m_f) of CMC in the solution is varied in the range 0.1% ⩽ m_f ⩽ 1% to accommodate zero-shear dynamic viscosities in the range 0.009–2.99 Pa-s. It was found that the transient and time-averaged velocities of Taylor bubbles are independent of the bubble size under both steady as well as pulsatile co-current flows. The lengths of the Taylor bubbles under the Newtonian conditions are found to be consistently greater than the corresponding shear-thinning non-Newtonian conditions for any given zero-shear dynamic viscosity of the liquid. In contrast to observations in stagnant liquid columns, an increase in the dynamic viscosity of the liquid (under Newtonian conditions) results in a concomitant increase in the bubble velocity, for any given co-current liquid velocity. In shear-thinning liquids, the change in the bubble velocity with an increase in m_f is found to be relatively greater at higher co-current liquid velocities. During pulsatile shear-thinning flows, distinct ripples are observed to occur on the bubble surface at higher values of m_f, the locations of which remain stationary with reference to the tube for any given pulsatile flow frequency, while the bubble propagated upwards. In such a pulsatile shear-thinning flow, a localised increase in dynamic viscosity is accompanied near each ripple, which results in a localised re-circulation region inside the bubble, unlike a single re-circulation region that occurs in Newtonian liquids, or shear-thinning liquids with low values of m_f. It is also seen that as compared to frequency, the amplitude of pulsatile flow has a greater influence on the oscillating characteristics of the rising Taylor bubble. The amplitude of oscillation in the bubble velocity increases with an increase in the CMC mass fraction, for any given value of pulsatile flow amplitude.     

Oscillations of a gas bubble in a non-Newtonian liquid under the action of an acoustic field

The evolution of the radius of a spherical cavitation bubble in an incompressible non-Newtonian liquid under the action of an external acoustic field is investigated. Non-Newtonian liquids having relaxation properties and also pseudoplastic and dilatant liquids with powerlaw equation of state are studied. The equations for the oscillation of the gas bubble are derived, the stability of its radial oscillation and its spherical form are investigated, and formulas are given for the characteristic frequency of oscillations of the cavitation hollow in a relaxing liquid. The equations are integrated numerically. It is shown that in a relaxing non-Newtonian liquid the viscosity may lead to the instability of the radial oscillations and the spherical form of the bubble. The results obtained here are compared with the behavior of a gas bubble in a Newtonian liquid.     

Rising behavior of single bubble in infinite stagnant non-Newtonian liquids

This work is an experimental study of the rising behavior of single air bubbles in infinite stagnant non-Newtonian liquids. Aqueous solutions of carboxymethyl cellulose (CMC) are selected to study the effect of rheological properties. The high speed photography is employed to record the bubble motion in CMC solutions. The bubble size, rising trajectory, bubble shape and velocities are determined by digital image processing technique. As expected, the rheological properties have great influence on the rising behavior of single bubble. In the less concentrated CMC solutions, the bubble rising process can be divided into three stages according to spatial evolution of bubble shape. The deformation changes the trajectories of rising bubbles and bubble hydrodynamics. As the solution concentration increases, the transitional stage gradually disappears. In the most concentrated CMC solution, the first continuous shape flattening stage is directly followed by a rising process with bubble shape basically constant, the rectilinear path and constant rising velocity. Dimensional analysis is performed to formulate a general dimensionless correlation for the deformation and motion of bubbles in infinite liquids by considering the rheological properties.     

Interfacial area concentration in gas–liquid bubbly to churn flow regimes in large diameter pipes

This study performed a survey on existing correlations for interfacial area concentration (IAC) prediction and collected an IAC experimental database of two-phase flows taken under various flow conditions in large diameter pipes. Although some of these existing correlations were developed by partly using the IAC databases taken in the low-void-fraction two-phase flows in large diameter pipes, no correlation can satisfactorily predict the IAC in the two-phase flows changing from bubbly, cap bubbly to churn flow in the collected database of large diameter pipes. So this study presented a systematic way to predict the IAC for the bubbly-to-churn flows in large diameter pipes by categorizing bubbles into two groups (group 1: spherical or distorted bubble, group 2: cap bubble). A correlation was developed to predict the group 1 void fraction by using the void fraction for all bubble. The group 1 bubble IAC and bubble diameter were modeled by using the key parameters such as group 1 void fraction and bubble Reynolds number based on the analysis of Hibiki and Ishii (2001, 2002) using one-dimensional bubble number density and interfacial area transport equations. The correlations of IAC and bubble diameter for group 2 cap bubbles were developed by taking into account the characteristics of the representative bubbles among the group 2 bubbles and the comparison between a newly-derived drift velocity correlation for large diameter pipes and the existing drift velocity correlation of Kataoka and Ishii (1987) for large diameter pipes. The predictions from the newly-developed two-group IAC correlation were compared with the collected experimental data in gas–liquid bubbly to churn flow regimes in large diameter pipes and their mean absolute relative deviations were obtained to be 28.1%, 54.4% and 29.6% for group 1, group 2 and all bubbles respectively.     

A numerical study of the motion of a spherical drop rising in shear-thinning fluid systems

The dynamical processes of a Newtonian spherical drop rising freely through shear-thinning fluids expressed by the generalized Cross-Carreau (Carreau–Yasuda) model were considered experimentally and computationally. The local effects of shear-thinning on the drop motion, which are hard to evaluate from an experimental approach, are clearly revealed by the numerical results. The relation between the drop motion and the change in viscosity is clearly indicated and considered in detail for the cases in which the non-Newtonian fluids are highly and weakly pseudoplastic. In addition, the modified Reynolds and Morton numbers are discussed in order to describe the drop or bubble free motion in shear-thinning fluids using a more convenient and practical form.     

Bubble cluster formation in shear-thinning inelastic bubbly columns

The mean rise velocity of bubble swarms ascending in shear-thinning fluids was experimentally measured in a rectangular bubble column. Great care was taken to produce nearly mono-dispersed bubble swarms and to use shear-thinning fluids with negligible elastic effects. In this manner, it was possible to isolate the effect of the hydrodynamic interaction between bubbles in the column caused by the thinning behavior of the liquid. It was found that the mean rise velocity of the bubbles was larger than that of an individual bubble, in accordance with previous studies. The magnitude of the swarm velocity was found to be greatly influenced by the appearance of bubble clusters. The bubble clusters, which appeared for certain values of the flow index and bubble diameter, were found to have a very different structure from those observed in Newtonian liquids. Furthermore, it was found that the appearance of clusters produced a dramatic increase of the agitation within the column. A set of conditions was identified for the appearance of bubble clusters in shear-thinning inelastic bubbly columns.     

GPU accelerated simulations of three-dimensional flow of power-law fluids in a driven cube

Newtonian fluid flow in two- and three-dimensional cavities with a moving wall has been studied extensively in a number of previous works. However, relatively a fewer number of studies have considered the motion of non-Newtonian fluids such as shear thinning and shear thickening power law fluids. In this paper, we have simulated the three-dimensional, non-Newtonian flow of a power law fluid in a cubic cavity driven by shear from the top wall. We have used an in-house developed fractional step code, implemented on a Graphics Processor Unit. Three Reynolds numbers have been studied with power law index set to 0.5, 1.0 and 1.5. The flow patterns, viscosity distributions and velocity profiles are presented for Reynolds numbers of 100, 400 and 1000. All three Reynolds numbers are found to yield steady state flows. Tabulated values of velocity are given for the nine cases studied, including the Newtonian cases.     

The influence of flow-induced non-Newtonian fluid properties on turbulent drag reduction

Friction factors and velocity profiles in turbulent drag reduction can be compared to Newtonian fluid turbulence when the shear viscosity at the wall shear rate is used for the Reynolds number and the local shear viscosity is used for the non-dimensional wall distance. On this basis, an apparent maximum drag reduction asymptote is found which is independent of Reynolds number and type of drag reducing additive. However, no shear viscosity is able to account for the difference between the measured Reynolds stress and the Reynolds stress calculated from the mean velocity profile (the Reynolds stress deficit). If the appropriate local viscosity to use with the velocity fluctuation correlations includes an elongational component, the problem can be resolved. Taking the maximum drag reduction asymptote as a non-Newtonian flow, with this effective viscosity, leads to agreement with the concept of an asymptote only when the solvent viscosity is used in the non-dimensional wall distance.     

Theoretical prediction of the mass transfer coefficients in bubble columns operating in churn-turbulent flow regime. Study in Newtonian and non-Newtonian fluids under different operation conditions

 A comprehensive experimental study of the volumetric transfer coefficient k _L a with Newtonian and non-Newtonian fluids in bubble columns using CO₂ as gas phase is the objective of this work. The evaluation of the hydrodynamic characteristics of the bubble columns and delineated the different hydrodynamic regimes considering column geometry, gas flow, liquid height and type of fluid (Newtonian and non-Newtonian) suggest a general applicability of the proposed model. An explanation about of the k _L a values in non-Newtonian fluid is offered take into account shear rate, column geometry, viscosity and results reported in the literature previously. Received on 31 July 1999     

PIV measurements of slow flow of a viscoelastic fluid within a porous medium

Particle image velocimetry (PIV) and pressure loss measurements were used to investigate slow flow through a square array of cylinders having a solid fraction of 10%. The test fluids were a Newtonian fluid and a Boger fluid, both of high viscosity such that the Reynolds number did not exceed 0.1. The pressure loss data reveal that the onset of elastic effects occurred at a Deborah number around 0.5 and that flow resistance was up to several times Newtonian values at Deborah numbers up to 3. PIV showed that the transverse velocity profiles for the Newtonian and non-Newtonian fluid were the same at Deborah numbers below onset. Above onset, the profiles became skewed, increasingly so as the Deborah number increased. In the wake regions between cylinders in a column, periodic flow structures formed in the spanwise direction. The structures were staggered from column to column, consistent with the skewing and were offset. These flow patterns are the result of an apparent elastic instability.     

粗糙表面滑动轴承非牛顿介质润滑的计算

分析了轴承润滑中非牛顿介质的流变特性以及轴承表面形貌对润滑效果的影响,推导出了修正的雷诺方程,在方程中用差分粘度和第一正应力差函数表征非牛顿介质的流变特性,采用流量因子表征表面形貌的作用.结果表明:差分粘度的变化是影响润滑结果的主要因素,它取决于不同介质的动态参数和剪切频率范围,非牛顿介质润滑的承载力并非总高于或低于牛顿介质;在动载荷条件下,第一正应力差效应使油膜压力明显增大;影响流量因子的2个因素为表面形貌的粗糙度和纹理,但其作用远小于非牛顿介质流变特性的影响.     

Electrorheology of dielectric liquids

Dielectric liquids that show striking electrorheological (ER) effects are formulated by controlling the conductivity. Although the viscosity is increased on the application of a d.c. field, the flow of electrified fluids is Newtonian in the plain electrodes with smooth surfaces. When the liquids are sandwiched between the electrodes with flocked fabrics, the viscosity behavior is converted from Newtonian to shear-thinning flow. In electric fields, the convective flow is induced over the system due to the electrohydrodynamic(EHD) effect. The interactions between EHD convection and external shear give rise to the additional energy dissipation and in turn the increase in viscosity. The ER effects of simple liquids are very attractive in application to new fluid devices.