300 Femtosecond pulses at 497 nanometer generated by an excimer laser pumped cascade of distributed feedback dye lasers

The setup is a cascade of 3 lasers: A competing cavity dye laser pumped by a XeCl excimer laser, followed by two distributed feedback dye lasers. The typical durations of the pulses from the lasers are 100 ps, 5 ps, and 300 fs, respectively. The output pulses at 497 nm are amplified up to 500 MW. The shortest pulse duration obtained was 198 fs.     

Tunable sub-100 femtosecond dye-laser pulses generated with a nanosecond pulsed pumping

Subpicosecond pulses at a fixed wavelength produced with a low-Q cavity dye laser pumped by a single, nanosecond laser (Q-switched Nd:YAG) are converted into tunable high-power sub-100 femtosecond pulses by generation, spectral selection, amplification and compression of a supercontinuum. The tunable, chirped, high-energy pulses obtained are compressed with a prism pair. Energies up to 50 J in sub-100 fs pulses were obtained in the 540 to 650 nm range using 40 mJ of the Nd: YAG-laser pumping pulses at 532 nm. The whole sub-100 fs system including the low-Q dye laser uses only one Nd:YAG laser as a pump source.     

Generation and amplification of sub-picosecond pulses using a frequency-doubled neodymium YAG pumping source

Stable, tunable, sub-picosecond pulses have been obtained by synchronously pumping a Rhodamine 6G dye laser with a frequency-doubled CW modelocked neodymium YAG laser. Careful attention has been paid to minimize amplitude and timing instabilities, resulting in dye laser pulses shorter than 500 fs. The main advantage of this new pumping source over current synchronously pumped dye lasers is that it is particularly well suited to short pulse amplification. Using this technique amplification of 2 × 10⁶ has been achieved.     

Generation of pulses shorter than 70 fs with a synchronously-pumped CW dye laser

Pulses shorter than 70 fs are generated with a synchronously-pumped cw dye laser using a dye medium composed of a mixture of rhodamine 6G and a fast recovery saturable absorber, DQOCI. The laser pulses exhibit no satellites. A stable output of 30 mW is obtained for only 300 mW of pump power.     

Generation of femtosecond pulses by two-photon pumping supercontinuum-seeded collinear traveling wave amplification in a dye solution

Visible femtosecond (fs) laser pulses have been obtained in a dye solution with a very simple traveling wave collinear configuration. A femtosecond Ti:sapphire laser (790 nm) pumps the dye solution by two-photon absorption and simultaneously generates supercontinuum, which seeds a light-amplification mechanism. Cross-correlation frequency-resolved optical gating measurements reveal a chirped structure in the dye pulse. The shortest pulse duration achieved is 170 fs and the overall energy efficiency of the process is typically 25%. Received: 22 March 2001 / Revised version: 4 July 2001 / Published online: 19 September 2001     

Femtosecond transform-limited Kerr-lens mode-locked dye lasers

Using SF6 glass plates as intracavity Kerr lenses and double-prism pairs for dispersion compensation, we achieve tunable femtosecond passive mode locking in rhodamine 590 (R6G) and 4-dicyanomethylene-2-methyl-16-p-dimethylaminostyryl-4H-pyran (DCM) dye lasers. The R6G laser produces transform limited 240–500 fs pulses between 577 and 606 nm, and the DCM laser produces 150 fs transform-limited pulses between 650 and 671 nm. We use dilute intracavity saturable-absorber jets to make the mode locking self-starting. Characteristics of the pulses and the stability regions of the lasers agree with general theories of passive mode locking.     

Synchronously pumped femtosecond dye oscillator-amplifier system at 815 nm

A tunable dye oscillator-amplifier system that produces 0.25 mJ, 105 fs pulses at 815 nm is demonstrated. The system consists of a synchronously pumped femtosecond dye laser followed by a dye amplifier that is quasi-longitudinally pumped using the frequency-doubled output from a Nd:YAG regenerative amplifier.     

用腔倒空Nd：YAG激光器对fs超短脉冲的同步放大

实现了用腔倒空Nd:YGA激光器对fs超短脉冲放大器的同步泵浦。由碰撞锁模环形染料激光器产生的80fs脉冲经二级染料放大后,实现放大倍数6.2×10~4,输出超短脉冲峰值功率～2×10~7W。     

超短飞秒光脉冲产生技术

本文叙述了群速弥散补偿被动锁模环型染料激光器的特性;研究了产生极短飞秒光脉冲的条件和光脉冲强度分布的非对称性。该技术产生的最短光脉冲宽度为21 fs;光脉冲宽度可调范围从最短到500fs以上。实验和理论数据拟合证明光强分布为非对称双曲正割平方,非对称因子r在7到11之间。     

Subpicosecond UV pulse generation for a multiterawatt KrF laser

A 180-fs UV pulse has been generated based on a hybrid synchronously pumped mode-locked dye laser for a multiterawatt KrF laser system. The pulse width was measured by the single shot autocorrelation technique with the three-photon fluorescence of the XeF C-A transition. The pulse width broadening due to dispersive media was investigated. The results show that the observed pulse width broadening from 210 fs to 390 fs through the entire system is explained mostly by the linear dispersion of the optical elements for near-transform-limited input pulses.     

Generation of femtosecond vacuum-ultraviolet pulses

High power femtosecond pulses in the Vacuum Ultra Violet (VUV) have been generated through the nonlinear interaction of femtosecond KrF pulses with xenon and argon gas. Under near resonant two photon excitation of xenon by a femtosecond KrF laser, parametric four wave mixing processes lead to VUV pulses at 147 and 108 nm with pulse energies in the 10 µJ range. Tuning is demonstrated by mixing the KrF pulse with a 500 fs dye laser pulse at 497 nm, resulting in 165 nm emission. In argon, a three photon resonance leads to third harmonic generation at 83 nm and micro joule level pulses near 127 nm generated by a six wave mixing process. Since the spectra of the VUV pulses show an ionization-induced blue shift with increasing KrF laser intensity, the VUV pulses can be shown to have temporal duration less than the pulse width (450 fs) of the KrF laser. Blue shifting of the third harmonic of the KrF laser in argon is dominated by a reduction in the neutral gas density rather than by an increase in the electron density.     

YAG激光同步泵浦染料激光器产生38fs光脉冲

研究表明,不用碰撞脉冲锁模技术,而由一台简单的线型腔染料激光器,就可成功地产生短达38飞秒的光脉冲。这种激光器用六镜折叠腔,其中有Rh6G和DOPCI两个喷流和一个棱镜对色散补偿器,用连续锁模Nd:YAG激光器的倍频输出同步泵浦。染料激光脉冲的平均功率为20mW,脉冲重复频率近100MHz。     

飞秒激光脉冲产生研究

本文报导了一种用于超快速同步扫描诊断技术的高稳定CPM环型染料激光器,激光器通过多层电介质反射镜弥散进行啁啾补偿,激光器输出脉宽45fs。     

Spectral optimisation of a synchronously mode locked femtosecond dye laser

Through optimisation of the spectrum and dispersion parameters of a synchronously mode locked Rhodamine B dye laser, pulses as short as 270 fs have been directly generated without using any saturable absorber or pulse compressor. In addition a system of tunable output coupling with well characterised dispersion has been demonstrated.     

Time evolution of synchronously pumped dye laser pulses: Picosecond pulse formation studies

The pulse-by-pulse evolution and compression of the output of a synchronously pumped dye laser as a function of the number of pump pulses was investigated with a high resolution, variably triggered streak camera. The measured pulse durations and energies for the pulse compression process are demonstrated to be in disagreement with the predictions of recent classical rate equation models. This is shown not to be due to the complete breakdown of the model but, rather, is caused by the failure to include two key loss terms in the rate equation treatment, namely, excited state absorption and thermal lensing. In addition, a highly durable dye laser compatible with the 100 MHz output of commercially available QS and ML YAG lasers is presented which is capable of 50 μJ, 20–30 ps transform limited pulses without the need of amplification. Further refinements of this laser system are discussed, based on the experimental work reported, which will lead to tunable ～ 100 fs pulses with energies in the μJ range from a single laser pump source.     

Generation of 49 fs pulses in a CPM laser pumped by a small-frame Ar+ laser

A colliding pulse mode-locked ring dye laser, pumped by an all-line small frame Ar⁺ laser has been used to generate stable pulses as short as 49 fs with pulse duration and stability similar to those obtained with the usual configuration where a single line of the pump is used. The effects of cavity alignment on the absorber saturation are presented and explained in terms of an analysis of stability of the ring cavity.     

同步泵浦PML飞秒激光研究

采用CW锁模YAG倍频激光器同步泵浦PML飞秒染料激光器,产生了平均脉宽约55fs、功率为15mW的光脉冲。文章在理论和实验上还研究了同步泵浦飞秒激光脉冲产生技术。     

Single crystal formation of amino acid with high temporal controllability by combining femtosecond and continuous wave laser trapping

We investigated laser trapping crystallization of glycine by using femtosecond (fs) laser as a trapping light source. Impulsively exerted fs laser pulses crystallized glycine more effectively than that induced by continuous wave (CW) laser trapping. Highly efficient crystallization and crystal growth behavior indicates fs laser irradiation increased the concentration not only at the focal spot, but also around the laser focus. Furthermore, we found that irradiation of fs pulses to CW laser-induced locally high supersaturation region enables immediate crystallization. Spatiotemporally controlled triggering of a single crystal formation with sub-second time resolution has achieved by integrating fs and CW laser trapping techniques.     

飞秒和纳秒激光脉冲作用下等离子体X射线辐射特性

对飞秒和纳秒激光作用下的Ａｌ和Ｃｕ等离子体的Ｘ射线辐射进行了测量、分析和比较．实验结果表明在飞秒激光脉冲下等离子体Ｘ射线峰值向短波方向移动．同时Ａｌ等离子体的的电离阶数和温度在飞秒下比纳秒高．     

Pulse Compression by Filamentation in Argon with an Acoustic Optical Programmable Dispersive Filter for Predispersion Compensation

We have experimentally demonstrated pulses 0.4 mJ in duration smaller than 12 fs with an excellent spatial beam profile by self-guided propagation in argon. The original 52 fs pulses from the chirped pulsed amplification laser system are first precompressed to 32 fs by inserting an acoustic optical programmable dispersive filter instrument into the laser system for spectrum reshaping and dispersion compensation, and the pulse spectrum is subsequently broadened by filamentation in an argon cell. By using chirped mirrors for post-dispersion compensation, the pulses are successfully compressed to smaller than 12 fs.