The effect of the size,shape, and structure of metal nanoparticles on the dependence of their optical properties on the refractive index of a disperse medium

The effect of the size, shape, and structure of gold and silver nanoparticles on the dependence of their extinction and integral scattering spectra on the dielectric environment has been investigated. Calculations were performed using the Mie theory for spheres and nanoshells and the T-matrix method for chaotically oriented bispheres, spheroids, and s cylinders with hemispherical ends. The sensitivity of plasmon resonances to variations in the refractive index of the environment in the range 1.3–1.7 for particles of different equivolume size, as well as to variations in the thickness of the metal layer of nanoshells, was studied. For nanoparticles with an equivolume diameter of 15 nm, the maximal shifts of plasmon resonances due to variation in the refractive index of the environment are observed for bispheres and the shifts decrease in the series nanoshells, s cylinders or spheroids, and spheres. For particles 60 nm in diameter, the largest shifts of plasmon resonances occur for nanoshells and the shifts decrease in the series bispheres, s cylinders or spheroids, and spheres. All other conditions being the same, silver nanoparticles are more sensitive to the resonance tuning due to a change in the dielectric environment.     

氢离子在固体表面掠角散射与能量损失的数值模拟

利用介电响应理论和镜像反射模型对氢离子在固体表面掠角散射和能量损失进行了数值模拟．离子在表面散射时同时受到表面上原子的库仑排斥作用和表面电子气的动力学相互作用,后者是表面电子受运动的正离子扰动所产生,用线性介电响应理论来确定．在高速和低速情况下,分别采用仅与频率有关的局域介电函数和局域场修正介电函数来确定表面电子气产生的动力学相互作用力．计算结果与实验结果作了比较．发现入射速度很低时能量损失随入射角度变化不太明显,而当速度很高时能量损失随入射角度的变大而有所增加. 关键词：     

任意方位双球粒子体系散射极化特征与单个球的比较

本文用T矩阵与场方程叠加相结合的方法，系统研究任意方位双球粒子体系散射矩阵各元素随两球球心的间距变化规律。 详细推导了双球粒子体系T矩阵的具体形式，并将T矩阵所求得的散射矩阵与单个球的情况作了比较。数值计算表明，球心间间距的增加对该体系的散射矩阵影响不大，得出任意方位即对方位求平均的情况下，双球粒子体系的散射矩阵与体系中有较大尺寸参数的单球相似的结论.     

Radiative heat transfer in a planar medium with anisotropic scattering and directional boundaries

Radiation heat transfer in an absorbing, emitting and scattering medium has been the subject of many previous investigations. Most solutions are numerically complex and the existing analytical solutions are restricted in application by the simplifying assumptions involved. A plane-parallel medium is considered which scatters anisotropically. The boundaries are considered to be specular reflectors, as predicted by Fresnel's relations, while the diffusely incident radiation is refracted according to Snell's law. The emission is restricted to a medium with a uniform temperature distribution. Approximate closed-form solutions for the radiative heat flux and incident intensity are presented for dielectric layers and linear anisotropic scattering. Numerical results are also presented and show that the effects of directional boundaries, anisotropic scattering, scattering albedo and optical depth are accurately predicted by the approximate solution.     

Characterization of Submillimeter Wave Absorbers from 200–600 GHz

This paper presents measurements of both specular and non-specular scattering from several submillimeter wave absorber materials designed for antenna testing and from low-cost carpet materials. The frequency range is 200–600 GHz in specular scattering, and 300–400 GHz in non-specular scattering measurements. The constructed bistatic test bench allows testing of the full continuous angular range of 0°–90°. The measurement results show large differences in performance of different materials. It is shown that reflectivities below –50 dB over limited angular ranges are possible with a correct alignment of the material. Also, low-cost carpet materials have lower than –15 dB reflectivities in most angles, and may be useful in non-critical parts of the antenna test range. The results can be used to optimise the absorber placement inside an antenna range, concerning both best performance and lowest cost.     

Analysis of Frequency Selective Surfaces with Metallic and Dielectric Losses at Millimeter Wave Range

In this paper, a theoretical analysis of scattering from a doubly frequency selective surfaces (FSS) with dielectric and metallic losses in the millimeter wave range is presented. The theoretical analysis involves the solution of the electric field integral equation relating the induced current in the FSS in the presence of anisotropic dielectric layers. The method of moment is employed to obtain numerical results. The frequency selective surface structure considered is composed by conducting patch elements sandwiched between two anisotropic dielectric layers. Three different anisotropic materials are considered: Epsilam-10, Alumina, and Sapphire. The sapphire presents low losses when compared with the other two dielectric materials. The most common metals, as copper and aluminum, are considered in this analysis. None significant metallic losses were observed for any considered metal. Numerical results are presented for the scattering characteristics and for dielectric and metallic losses parameters.     

Microwave Doppler spectra of sea return at small incidence angles: specular point scattering contribution

It is well known that the sea return echo contains contributions from at least two scattering mechanisms. In addition to the resonant Bragg scattering, the specular point scattering plays an important role as the incidence angle becomes smaller (≤20o). Here, in combination with the Kirchhoff integral equation of scattering field and the stationary phase approximation, analytical expressions for Doppler shift and spectral bandwidth of specular point scattering, which are insensitive to the polarization state, are derived theoretically. For comparison, the simulated results related to the two-scale method (TSM) and the method of moment (MOM) are also presented. It is found that the Doppler shift and the spectral bandwidth given by TSM are insufficient at small incidence angles. However, a comparison between the analytical results and the numerical simulations by MOM in the backscatter configuration shows that our proposed formulas are valid for the specular point scattering case. In this work, the dependences of the predicted results on incidence angle, radar frequency, and wind speed are also discussed. The obtained conclusions seem promising for a better understanding of the Doppler spectra of the specular point scattering fields from time-varying sea surfaces.     

An alternative approach for measuring the scattered acoustic pressure field of immersed single and multiple cylinders

The form function of an elastic target can be obtained from the scattered signal through a deconvolution process. The deconvolution process uses the signal measured from an acoustically hard target (reference signal) to compensate for the impulse response of the measurement system. In this paper, it is shown that this approach limits the usable frequency range of the signal and leads to inaccuracies in the final results. An alternative approach is proposed in which the reference signal is replaced by the specular echo. A procedure is described for extracting the specular echo from the measured signal even in cases where it is not completely isolated from the resonant components. Modifications are made to the existing deconvolution formulation and it is further extended to be applicable to multiple scattering measurements. Experimental results show that the new approach provides improved accuracy and wider usable frequency range in both single and multiple scattering experiments.     

Fast iterative approach to the difference scattering from a dielectric target above a rough surface

1 Introduction Electromagnetic scattering from the target above or beneath a rough surface has at- tracted much interest during recent years, because of extensive applications to radar surveillance, target detection, ground radar probing, and so on[1―3]. In order to numeri- cally simulate scattering from composite model of the target and underlying rough sur- face, some fast numerical methods, such as general forward backward method and spec- trum acceleration algorithm (GFBM/SAA)[4,5], fin…     

Fast iterative approach to the difference scattering from a dielectric target above a rough surface

The difference field RCS (d-RCS) has been defined to analyze the scattering from the target above a rough surface. The electric field integral equations (EFIEs) of the difference induced currentJ _sd on the rough surface, the induced electric currentJ _o and magnetic currentK _o on the dielectric target under a TE wave incidence are derived. A small portion of the rough surface towards the target along the specular direction is taken to compute the scattering contributionE _s0 from the rough surface towards the target, which improves the computation speed. A numerical iterative approach is developed to solve the EFIEs and bistatic d-RCS. The surface length for iterations is dependent on the scattering angle and discussed for comparison with Johnson’s method. Using the Monte-Carlo method to generate the Pierson-Morkowitz (P-M) ocean-like rough surface, bistatic d-RCS of the dielectric target, e.g. a cylinder or a square column, above the rough surface is numerically simulated. The induced electric and magnetic currents on the dielectric target and the difference induced current on the rough surface are numerically discussed.     

Atom-surface elastic scattering with additive potential

An additive corrugated potential with linear repulsion and long range attractive well is proposed for atom-surface scattering. The computational procedure yielding the scattering probabilities (essentially linear algebra) proves to be much simpler than with other potentials. For a given shape of the corrugation function and for high values of the steepness parameter one obtains results close to those of the hard corrugated wall model, while an important enhancement of the specular intensity appears, in particular at large angles of incidence, when the steepness parameter is small.     

Acoustic characteristics of urban streets in relation to scattering caused by building facades

The relationship between scattering and the acoustic characteristics of urban streets is examined by computer simulation. The simulation method is a combination of the image method for specular reflection and the radiosity method for scattering reflection. The findings are as follows: (1) the effect of scattering on the SPL appears as an increase at short distances and as a decrease at great distances. The range of the increase in SPL is larger in high-facade streets. In low-facade streets, the primary effect of scattering on SPL is a decrease in SPL. (2) In low-facade streets the reverberation time is determined by the sum of absorption coefficient and scattering coefficient. In contrast, in high-facade streets, the reverberation time is determined by the absorption coefficient. (3) The simulated result for the reverberation time shows good agreement with measured value in actual streets. (4) The estimated values for the sum of absorption coefficient and scattering coefficient of facades of actual urban streets range from 0.1 to 0.25.     

An angular cutoff composite model for investigation on electromagnetic scattering from two-dimensional rough sea surfaces

Based on the local configuration angle division to select the corresponding method for electromagnetic scattering calculation from rough sea surface,this paper presents an angular cutoff composite model:when the local scattered angle is in the specular region that is given by an approximately 20 degrees cone around the specular direction,the Kirchhoff approximation is applied to evaluate the specular reflection,which dominates the total scattering in this region;the small perturbation method is employed to handle the diffuse reflection which is predominant as the local scattered angle is situated out of the specular region.Numerical results are compared with those of experimental and theoretical models in several configurations as a function of incident angle,wind speed,wind direction.The comparison of numerical results of other experimental and theoretical models in several configurations shows that the new composite model is robust to give accurate numerical evaluations for the sea surface scattering.     

Disclination dipoles as the basic structural elements of dielectric glasses

We show that the experimentally observed behavior of thermal conductivity of dielectric glasses over a wide temperature range can be explained by a combination of two scattering processes: phonon scattering due to biaxial dipoles of wedge disclinations and Rayleigh type scattering. The results obtained support the cluster picture suggested earlier for glassy materials.     

Microwave localization due to defects in the arrays of dielectric cylinders: Multiple scattering approach

Microwaves propagation and scattering by dielectric cylinders in an uniform and defected media are simulated by using multiple scattering method. Formation of localized state due to the presence of a defect is observed in our simulations. Our theoretical results are compared with the previous experimental findings, yielding quantitative agreements in the transmission coefficients for a certain range of frequencies. In addition, our results point out some possible inconsistency in the experimental observations.     

Light scattering by cylindrical nanoparticles: Limits of applicability of the Rayleigh-Gans-Debye approximation

Applicability of the Rayleigh-Gans-Debye (RGD) approximation for describing light scattering by nanoparticles with large dielectric losses (such as carbon nanotubes) is analyzed. By a comparison of the approximate results with exact ones, it is shown that the presence of dielectric losses expands the range of applicability of the RGD approximation. This conclusion is illustrated by a differential cross-section diagram of scattering by a multiwall carbon nanotube.     

A New Method for Measuring Scattering of Light from Optical Surfaces with Random Roughness

In this letter we report a new method for measuring light scattered from optically rough surfaces. By collecting scattered light in a given solid angle, the measurement system does not require a detection unit with an extremely large dynamic range. This in turn significantly simplifies the system configuration. Measurements of scattering close to specular reflection (the so-called small angle or near-specular scattering) also can be completed without any difficulty. Unlike in the common angle resolved scattering (ARS) measurement system, in this system a linear movement instead of rotation is adopted to scan scattered light. In this way, the angular resolution of scattering measurements is independent of the resolution of the translation stages and may be adjusted.     

Random distribution of islands explains the oscillatory intensity in He/Si(111)-(7 × 7)

It is shown that the oscillatory specular beam intensity observed in He/Si(111)-(7 × 7) scattering is consistent with a random distribution of islands of height ~3.05 Å. Each of these islands may be reconstructed, totally or partially, in a (7 × 7) structure according to the more favourable models proposed by LEED. This could be a possibility to explain, with the same (7 × 7) unit cell, He scattering and LEED experiments.     

Energy accommodation and reactivity of O2 on tungsten

We have determined by direct molecular beam velocity measurements that translational energy accommodation of O₂ molecules scattered from a hot polycrystalline tungsten target is inefficient at high surface temperatures. Translational energy accommodation is inefficient whether the surface is clean or covered with oxygen to a varying extent, even though in the latter case the scattering is diffuse. On a clean tungsten surface the scattering of the O₂ was approximately specular and the reaction probability of O₂ was constant and greater than 90% over the temperature range 1000K to 2800 K. It was shown by simultaneous helium scattering that atomic surface roughness of an oxygen chemilayer, rather than trapping, is a major cause of the observed diffuse scattering of oxygen. At the lowest surface temperature of 1000 K, with an oxygen chemilayer present, the velocity of the most probable number density of the scattered O₂ was lower than in the incoming beam or than that expected for complete equilibration with the surface.