Rotational properties of the odd-Z transfermium nucleus 255Lr by a particle-number-conserving method in the cranked shell model

Experimentally observed ground state band based on the 1/2-[521] Nilsson state and the first exited band based on the 7/2-[514]Nilsson state of the odd-Z nucleus ~(255)Lr are studied by the cranked shell model(CSM) with the paring correlations treated by the particle-number-conserving(PNC) method. This is the first time the detailed theoretical investigations are performed on these rotational bands. Both experimental kinematic and dynamic moments of inertia(J~(1)and J~(2)) versus rotational frequency are reproduced quite well by the PNC-CSM calculations. By comparing the theoretical kinematic moment of inertia J~(1) with the experimental ones extracted from different spin assignments, the spin 17/2~-→13/2~- is assigned to the lowest-lying 196.6(5) ke V transition of the 1/2~-[521] band, and 15/2~-→11/2~- to the 189(1) ke V transition of the 7/2~-[514] band, respectively. The proton N = 7 major shell is included in the calculations. The intruder of the high- j low-? 1 j_((15)/2)(1/2~-[770]) orbital at the high spin leads to band-crossings at ω≈0.20( ω≈0.25) Me V for the 7/2~-[514] α =-1/2(α = +1/2) band, and at ω≈0.175 Me V for the1/2~-[521] α =-1/2 band, respectively. Further investigations show that the band-crossing frequencies are quadrupole deformation dependent.     

Study of low-lying states in151Eu via (n,n′γ) reaction

The levels of¹⁵¹Eu have been investigated in the (n,n′γ) reaction using nuclear reactor fast neutrons. The energies, intensities and angular distributions of theγ-rays have been measured with the Ge(Li) spectrometer. Four rotational bands with the following band heads and Nilsson configurations have been identified: ground state band, 5/2⁺ [402]; 21.5 keV, 7/2⁺[404]; 196.5 keV, 3/2⁺[411]; 260.5 keV, 5/2⁺[413]. The low spin states at 332.2 and 336.2 keV have been tentatively assigned to the l/2⁺[411] Nilsson orbital, but 522.8, 580.0 and 587.0 keV states to the 1/2⁺[420] Nilsson orbital. The negative parity levels at 353.7, 522.1 and probably 546.2 keV have been proposed basing on theh _11/2 proton state.     

Time constants of radiative transitions from the 5<Emphasis Type="Italic">d</Emphasis>[3/2]<Subscript>1</Subscript> level of a xenon atom

Integral yields of spontaneous emission at wavelengths of 1.73, 2.03, and 2.65 μm have been measured upon excitation of pure xenon by a pulsed electron beam. These yields have been analyzed and experimental data have been obtained on time constants of radiative transitions 5d[3/2]₁ → 6p[5/2]₂, 5d[3/2]₁ → 6p[3/2]₁, and 5d[3/2]₁ → 6p[1/2]₀ of XeI, which appeared to be equal to (2300 ± 400) × 10^?9, (300 ± 40) × 10^?9, and (1300 ± 200) × 10^?9 s, respectively. It is shown that the experimental data are in a qualitative agreement with the results of computational and theoretical investigations. The results of averaging the experimental and calculated data are proposed for use as recommended values of the corresponding constants.     

High-j proton alignments in 101Pd

High-spin states in ¹⁰¹Pd have been investigated by means of in-beam γ-ray spectroscopic techniques via the ⁷⁶Ge(²⁸Si, 3n) reaction at beam energies of 85 and 95 MeV. The previously known d _5/2 and 1/2^?[550] bands were extended to higher spins, and the unfavored signature branch of the 1/2^?[550] band was built. The band crossings observed experimentally are explained by the alignment of g _9/2 protons. The band properties in ¹⁰¹Pd are compared with those in the neighboring nuclei and are discussed within the framework of the cranked shell model (CSM).     

Gammaübergänge und Energieniveaus in Dy 165

220 neutron capture Gamma rays of Dy 165 were measured with the Risø curved crystal spectrometer. The intense transitions permitted the construction of a level scheme for this oddN nucleus. The rotational bandsK=7/2⁺[633],K=1/2^?[521] andK=5/2^?[512] were precisely localized, including the spin 11/2 states. Gammavibrational bands built on these Nilsson orbits were observed with their band heads at 538.6, 573.5 and 570.2 keV. TheI=5/2 term at 533 keV can be considered as the 5/2^?[523] Nilsson state. The branching ratios allowed the determination of (g _K?g^R)²-factors for the [633], [521] and [512] bands and yieldedE 1-hindrance factors.     

Collective and intrinsic structures in 183W

The structure of ¹⁸³W has been studied by employing the ¹⁷⁶Yb(¹⁴C,α3n) reaction at 68 MeV. Five previously known rotational structure with one-quasiparticle configurations have been extended to higher spin states, and five new rotational bands with three- and five-quasiparticle configurations and a γ-vibration of a one-quasiparticle structure have been newly identified. In the ν7/2⁻[503] and ν11/2⁺[615] rotational structures, a signal of an admixture of an octupole-vibrational structure has been observed in their in-band B(M1)/B(E2) ratios and g_K factors. In the K^π=19⁻ rotational band, a Coriolis effect on the ν1/2⁻[510] neutron has been identified. In all, 17 K-forbidden transitions have been observed. Energies of intrinsic states below 4 MeV have been calculated based on the Blocked BCS theory, and they are used in support of the configuration assignments.     

High-temperature VUV spectroscopy of KYF4 crystals doped with Nd3+, Er3+ and Tm3+ ions

Thermal quenching of 5d-4f luminescence from Nd³⁺, Er³⁺ and Tm³⁺ ions doped into KYF₄ crystals has been investigated in the temperature range up to ∼750 K where this luminescence is completely quenched. The obtained temperatures of thermal quenching (T_q) are ∼270, 495, 450 K for Nd³⁺, Er³⁺, Tm³⁺, respectively. At high temperatures, thermal quenching of 5d-4f luminescence from Nd³⁺ and Er³⁺ is accompanied by the appearance of 4f-4f luminescence from the lower-energy 4f levels. It has been shown that the dominating mechanism of thermal quenching for Nd³⁺ and Er³⁺ ions is thermally stimulated non-radiative transitions (intersystem crossing) from the 5d states to lower-energy 4f levels, namely ²G(2)_9/2 and ²F(2)_7/2, respectively, whereas for the Tm³⁺ ion, thermally stimulated ionization of 5d electrons to the conduction band states is responsible for thermal quenching of 5d-4f luminescence. The energy gap between the lowest Tm³⁺ 5d level and the bottom of the KYF₄ conduction band has been estimated to be 0.66 eV.     

Time-resolved Fourier transform infrared spectroscopy: Application to pulsed discharges

Time-resolved Fourier transform spectroscopy (TR-FTS) is reviewed, with emphasis on synchronous FTS using continuously scanning interferometers. By using a high-resolution Bruker IFS 120 HR, a TR-FTS method has been developed with the help of a microcontroller SX, where a maximum of 64 time-resolved data are recorded with a preset time interval in a single scan of the interferometer. The time resolution is 1 μs, limited by the response time of the detector system used. This method has been applied to a pulsed discharge in an Ar and H₂ mixture to observe time profiles of ArH⁺ and ArH emission spectra. Electronic transitions of He₂ have been observed in the infrared region with this method, and from the time profiles, He₂ in Rydberg states with higher energy than the b³Π state is found to be produced efficiently in afterglow plasma. Fifteen bands in the 2300-8000 cm⁻¹ region have been assigned by using previously reported data from the optical region. A new band from the 5f state has been assigned for the first time through the 5f-4d band in the 2600 cm⁻¹ region.     

On the correlation between the composition of Pr doped garnet type materials and their photoluminescence properties

Lu₃(Al,Ga)₅O₁₂ and (Y,Lu)₃(Al,Mg,Si)₅O₁₂ samples doped with 1% Pr³⁺ were prepared by two aqueous sol-gel chemistry approaches, such as citrate and glycolate methods. All samples were characterised by powder X-ray diffraction (XRD), thermal quenching (TQ), fluorescence lifetime measurements and photoluminescence (PL) techniques. It turned out that the Pr³⁺ emission is very sensitive to the composition of the garnet host lattice. Lu₃Al₅O₁₂:Pr³⁺ samples showed mainly [Xe]4f¹5d¹→[Xe]4f² broad band emission in UV-blue region, whereas [Xe]4f²-[Xe]4f² line emission of Pr³⁺ dominated in Lu₃Ga₅O₁₂ samples. Modification of garnet crystals with Mg²⁺-Si⁴⁺ pair has led to generation of strong crystal field strength resulting in energy transfer from 5d to 4f orbitals. Y₃AlMg₂Si₂O₁₂ composition generated the strongest crystal field splitting out of all synthesised samples and showed practically only Pr³⁺ [Xe]4f²-[Xe]4f² line emission in the red spectral region.     

Properties of the 3/2−[521] band in the odd-N rare-earth nuclei

High-spin states in ¹⁶¹Er have been studied experimentally via the ¹⁵⁰Nd(¹⁶O, 5n) reaction at a beam energy of 86 MeV. Three rotational bands built on the 5/2⁺[642], 3/2⁻[521], and 11/2⁻[505] configurations have been extended up to high-spin states, and particularly, the α = −1/2 branch of the ground state 3/2⁻[521] band has been revised significantly. It is found that signature inversion occurs in the 3/2⁻[521] band after the band crossing in ¹⁶¹Er. The systematics of the signature inversion associated with the 3/2⁻[521] configuration in the rare-earth region is discussed. The band properties are analyzed within the framework of a triaxial particle-rotor model, and a triaxial deformation is proposed to the 3/2⁻[521] band.

     

In-beam spectroscopy of231Pa

Information on energy levels and onE 2 andM 1 matrix elements in²³¹Pa has been obtained using conversion-electron and gamma-ray spectroscopy following the²³²Th(p, 2n)²³¹Pa reaction and Coulomb excitation of the radioactive target²³¹Pa by⁴He and³²S ions. The results are analyzed in the framework of the rotational model, applied to the rotational band built on the 1/2^?[530] Nilsson state whose 3/2^? member forms the ground state of this nucleus. The deviations of the level energies from the rigid-rotor values can be described by Coriolis couplings. The analysis of the Coulomb-excitation process shows that a constant set of rotational parameters Q₀, g_R, g_K, andb can fairly well account for the measured line intensities.     

Half-life measurements of intrinsic states in deformed odd-mass nuclei

The half-lives of the following intrinsic states in deformed odd-mass nuclei has been measured by delayed coincidences with a time-to-amplitude converter:

1. 5/2 5/2⁺[642] at 86.5 keV in¹⁵⁵Gd:T _1/2=6.7±0.3 ns, which results in the determination of theE1,ΔK=1 transition probability to the ground state 3/2 3/2^?[521] and first rotational state 5/2 3/2^?[521], yielding hindrance factors ofF _N ≈5.5 and ≈1.8 (F _W =3.1×10⁴ and 2.3×10⁴) respectively.
2. (3) 5/2 5/2^?[512] at 191.4 keV in¹⁶⁹Yb:T _1/2=3.35±0.15 ns and at 122.39 keV in¹⁷¹Yb:T _1/2=265±20 ns which results in the determination of the transition probabilities of theE1,ΔK=1 transitions to the ground states 7/2 7/2⁺[633], of theK-forbiddenM1 transitions to the 5/2 and 3/2 1/2^?[521] and of theE2 transitions to the 5/2, 3/2 and 1/2 1/2^?[521] states in both nuclei.

TheE1 transition probabilities are compared to the transitions between the same Nilsson states in¹⁷³Yb and¹⁷⁵Hf discussing the influence of the position of the Fermi surface — obtained from recent stripping and pick-up reactions — on these transition probabilities. Additional information on the decay scheme of¹⁷¹Lu→¹⁷¹Yb is obtained by delayed coincidence measurements. For testing the used time-to-amplitude converter the well known half-lives of the 482 keV level in¹⁸¹Ta (T _1/2=10.4±0.3 ns) and of the 279 keV level in²⁰³Tl (T _1/2=0.285 ±0.015 ns) were measured, in good agreement with other measurements.     

On the level scheme of the159Tm nucleus

Level in¹⁵⁹Tm have been excited in the¹⁵⁰Sm(¹⁴N,5n reaction. The yrast band 7/2^?[523] observed up to spin 45/2^? is built on a isomeric state at 166 keV (T _1/2=37±5ns). Connections between the 7/2^?[523] and 7/2⁺ [404] bands fix the band-head energies.     

New rotational bands in 174Ta

Three new bands in ¹⁷⁴Ta have been identified by using the ¹⁶⁰Gd(¹⁹F,5n) reaction at beam energies of 87 MeV and 96 MeV. Nilsson configurations are assigned to these bands. In the 9/2⁻[514]_p+5/2⁻[512]_n band, the AB neutron crossing occurs at a rotational frequency of 0.30 MeV. This is indicative of the disappearance of the evidence for a reduction in neutron pair correlations. Received: 30 March 1998     

Levels of233Pa excited in helium-induced single-proton transfer reactions

The²³³Th(³He,d)²³³Pa and²³³Th(α, t)²³³Pa reactions were studied with 28.5-MeV³He and 30-MeV α-particles, respectively. The reaction results are interpreted in terms of a distorted-wave Born-approximation analysis. Transferred angular momenta are deduced from (α, t) and (³He,d) cross-section ratios,R=dσ(α, t)/dσ(³He,d). Theoretical cross sections, calculated in the framework of the Nilsson model with pairing and Coriolis interactions included, are in reasonable agreement with experiment. Rotational bands built on the following Nilsson proton configurations are identified in²³³Pa: 1/2_?[530↑], 3/2⁺[651↑], 1/2⁺[660↑], 5/2⁺[642↑], 5/2_?[5231↓], and 3/2_?[521↑].     

Luminescence study of the 4f5d configuration of Nd in LiYF4, LiLuF4 and BaY2F8 crystals

Ultraviolet fluorescence of Nd³⁺ ions induced by triphotonic excitation process was studied in Nd-doped LiYF₄, LiLuF₄ and BaY₂F₈ crystals using a technique of time-resolved spectroscopy. The observed ultraviolet luminescence was due to transitions between the bottom of 4f²5d configuration and 4f³ states of Nd³⁺ ions. Narrow emission lines superposed to the broadband emissions were observed. A detailed analysis of luminescence spectrum revealed that the narrow emissions are due to parity and spin allowed radiative transitions from the Stark levels of ⁴K_11/2(5d) state created by the electrostatic interaction between the 5d electron and the two electrons of the 4f² configuration. The narrow emissions are related to the high spin state (S=3/2) which gives f-f characteristics to the f-d broadband emissions. The narrow emissions superposed to the wide emission correspond to 18%, 34% and 43% of the integrated broadband emission at 262 nm observed in LiYF₄, LiLuF₄ and BaY₂F₈ crystals, respectively. Although the 5d-4f² interaction is observed to be weaker than 5d-crystal field interaction, it is stronger enough to select only the radiative transitions from 4f²5d configuration to 4f³ states that preserves the total spin S=3/2.     

Behavior of the excitation cross sections of the perturbed series of the xenon atom

Behavior of the excitation cross sections of the perturbed 6s[3/2]_n°?np[1/2]₀ spectral series of the xenon atom is experimentally studied. By using the methods of extended electron beam and optical spectroscopy, the cross sections are measured and the optical excitation functions are recorded for the transitions of this series with n=6–13. A deviation of the dependence Q=f(n) from a power-law function is revealed, as well as changes in the form of optical excitation functions and in the nature of the branching caused by perturbation of the 7p[1/2]₀ level by levels of the 5p ⁵(² P _1/2°)6p configuration.     

New investigation of the decay of the high-spin isomer in 151Er

The decay of the T _1/2 = 420 ns isomer in ¹⁵¹Er has been reinvestigated. The multipolarities of the decaying transitions have been established by measuring the electron conversion coefficients. An I ^π = 67/2⁻ assignment is proposed for this isomer with a π[h ₁₁^2/4 d ₃^2/1 d ₅^2/−1]⊗ν[f _7/2 h _9/2 h ₁₁^2/−1] configuration.     

Photoluminescence and tunneling charge transfer in CaF2: RE2+-CdF2 superlattices on Si(111)

The nonstationary behavior of Eu²⁺ and Sm²⁺ photoluminescence in continuously optically pumped CaF₂:RE²⁺-CdF₂superlattices was considered. The transient character of the photoluminescence is due to spontaneous electron tunneling from the excited 4f5d states into the conduction band of the adjacent CdF₂ layer. Coupled balance equations were constructed and numerically analyzed. It is shown that photoionization energies of the 4f5d states can be derived from the experimentally measured variation of the photoluminescence intensity in superlattices with CaF₂ and CdF₂ layers 10 to 20 monolayers thick.