Density of states and extent of wave function: two crucial factors for small polaron hopping conductivity in 1D

Abstract

We introduce a theoretical model to scrutinize the conductivity of small polarons in 1D disordered systems, focusing on two crucial – as will be demonstrated – factors: the density of states and the spatial extent of the electronic wave function. The investigation is performed for any temperature up to 300 K and under electric field of arbitrary strength up to the polaron dissociation limit. To accomplish this task, we combine analytical work with numerical calculations.     

Tailoring Anderson localization by disorder correlations in 1D speckle potentials

We study Anderson localization of single particles in continuous, correlated, one-dimensional disordered potentials. We show that tailored correlations can completely change the energy-dependence of the localization length. By considering two suitable models of disorder, we explicitly show that disorder correlations can lead to a nonmonotonic behavior of the localization length versus energy. Numerical calculations performed within the transfer-matrix approach and analytical calculations performed within the phase formalism up to order three show excellent agreement and demonstrate the effect. We finally show how the nonmonotonic behavior of the localization length with energy can be observed using expanding ultracold-atom gases.     

Anderson localization and propagation of electromagnetic waves through disordered media

We have used the dynamic method to calculate the frequency dependence of the localization length in a disordered medium, using the amplitude change and the redshift of the spectral density of the propagating incident pulse. The frequency dependence of the localization length in an effectively one-dimensional disordered medium is computed in terms of the strength of the disorder. The results obtained with the dynamic method are confirmed by computing the same results using the transfer-matrix method.     

Anderson localization in a two-dimensional random gap model

We study the properties of the spinor wavefunction in a strongly disordered environment on a two-dimensional lattice. By employing a transfer-matrix calculation we find that there is a transition from delocalized to localized states at a critical value of the disorder strength. We prove that there exists an Anderson localized phase with exponentially decaying correlations for sufficiently strong scattering. Our results indicate that suppressed backscattering is not sufficient to prevent Anderson localization of surface states in topological insulators.     

Optical third-harmonic generation in coupled microcavities based on porous silicon

The resonance features of the third-harmonic generation have been observed in 1D coupled microcavities consisting of three Bragg reflectors and two identical half-wave layers of mesoporous silicon. The third-harmonic intensity increases by a factor of about 10³ in the resonance of fundamental radiation with each of the modes of coupled microcavities. It has been shown that the resonance positions in the angular spectra of the third-harmonic intensity depend on the coupling between microcavities that is determined by the transmission of the intermediate Bragg reflector. In the framework of the transfer-matrix method with nonlinear sources, it has been shown that the basic mechanism of the enhancement of the third-harmonic generation in coupled microcavities based on porous silicon is the constructive interference of the partial third-harmonic waves that are generated by near-surface layers.     

Incommensurate-commensurate phase transitions in an anisotropic antiferromagnetic model on triangular lattice

An anisotropic antiferromagnetic model on a triangular lattice with competing interactions is investigated by the cluster transfer-matrix method. A phase diagram with ferrimagnetic, incommensurate, and disordered phases is found. Three order parameters are introduced. At commensurate-incommensurate and incommensurate-disorder phase transition lines two of them change in continuous and one in discontinuous way.     

光子晶体对太赫兹波的调制特性研究

利用传输矩阵方法研究了掺杂半导体n-GaAs/聚碳酸脂一维光子晶体的太赫兹波透射谱.研究结果发现,与一般由两种介电材料组成的一维光子晶体不同,由于掺杂半导体中自由载流子对太赫兹波存在较强的吸收,所以这种材料组成的一维光子晶体除可形成光子带隙外,还可以增强n-GaAs对太赫兹波的透射.同时还提出了一种基于这种一维光子晶体的太赫兹波调制器,通过外加电压控制半导体中电子浓度的大小可实现对太赫兹透射波幅度的调制. 关键词： 掺杂半导体光子晶体 太赫兹波 太赫兹波的调制     

Localized mode hybridization by fine tuning of two-dimensional random media

We study numerically the interaction of spatially localized modes in strongly scattering two-dimensional (2D) media. We move eigenvalues in the complex plane by changing gradually the index of a single scatterer. When spatial and spectral overlap is sufficient, localized states couple, and avoided level crossing is observed. We show that local manipulation of the disordered structure can couple several localized states to form an extended chain of hybridized modes crossing the entire sample, thus changing the nature of certain modes from localized to extended in a nominally localized disordered system. We suggest such a chain in 2D random systems is the analog of one-dimensional necklace states, the occasional open channels predicted by Pendry [Physics 1, 20 (2008).] through which the light can sneak through an opaque medium.     

Incommensurate structure in the lattice-gas ANNNI model

The phase diagram of the two-dimensional lattice-gas ANNNI model is investigated using the cluster transfer-matrix method. The numerical calculations have shown commensurate, disordered, and floating incommensurate phases. The properties of the incommensurate phase are studied in detail and the position of the Lifshitz point is discussed.     

无规结构全角高反一维光子晶体的场强分布

因一维光子晶体的许多应用由其场强分布特性所决定，本文研究了无规全角高反一维光子晶体场强分布的性质，结果表明在带隙内,两者的场强分布无明显差别,但在研究各种应用和器件关系最密切的带隙边缘, 周期结构的场强分布只有对称性的一种；无规结构光子晶体的谱带边缘电场分布特性则完全可按应用要求进行设计和控制，为光子晶体器件设计提供了全新的思路. 关键词： 光子晶体 无规结构 光子能隙 全角高反 场强分布     

Magnetic-field effects on two-Leg heisenberg antiferromagnetic ladders: thermodynamic properties

Using the recently developed transfer-matrix renormalization group method, we have studied the thermodynamic properties of two-leg antiferromagnetic ladders in a magnetic field. Based on different magnetization behaviors, we found a disordered spin liquid, the Luttinger liquid, spin-polarized phases, and a classical regime. Our calculations in the Luttinger liquid regime suggest that both the divergence of the NMR relaxation rate and the anomalous specific heat behavior observed on Cu2(C5H12N2)2Cl4 are due to a quasi-one-dimensional effect rather than three-dimensional ordering.     

Delocalization of quasiparticles in quasi-two-dimensional disordered superconductors with s-wave pairing

We investigate localization behavior of quasiparticles in disordered multi-plane superconductors with s-wave pairing. By introducing disorder with random site energies, the spatial fluctuations of Bogoliubov-de Gennes pairing potential are self-consistently determined. The size dependence of rescaled localization length for a long bar is calculated by using the transfer-matrix method. From the finite-size scaling analysis we show that there exists a critical point of the disorder strength W_c which separates the extended and localized quasiparticle states in such quasi-two-dimensional systems. The associated critical behavior is studied and the relationship of the results to the number of planes is discussed.     

Room-Temperature 2.5 eV Pulsed Cathodoluminescence Band of High-Purity Silicon Dioxide

We study the room-temperature (RT) pulsed cathodoluminescence (PCL) spectra of a set of pure synthetic (both crystalline and amorphous) silicon dioxide samples. We show that the PCL spectra of all samples (both amorphous and crystalline) possess bands with intensity maxima in the region of 487 – 500 nm (2.54 – 2.48 eV). These bands are the most intense in the PCL spectra of disordered materials. We investigate the annealing behavior of RT PCL spectra of the crystalline and amorphous samples. Annealing has no significant effect on this emission. We demonstrate that the surface area of the material plays no role in the emission of PCL bands at 415 and 490 nm in the spectra of α-quartz single crystal and crystalline powder with grain sizes of 10 – 100 μm. Our results show that the bands in the region of 2.5 eV are the universal property of all synthetic pure SiO₂ samples. The nature of the SiO₂ emission band in the region of 2.5 eV is not clear; we discuss two possible explanations. The first one is based on considering the intrinsic emission due to self-trapped exciton (STE) decay with the transient O-O (oxygen–oxygen) bond formation. The second one is based on the role of Li ions in the emission process.     

Metastable heterophase system of the Ising type

A modified Ising model is introduced, which gives the possibility to consider metastable states corresponding to a partially ordered and partially disordered system. The thermodynamics of such a system for the case of a square lattice is exactly analysed by means of the transfer-matrix method.     

Electronic transport in double-strand poly(dG)-poly(dC) DNA segments

We study the electronic properties of a double-strand quasiperiodic DNA molecule modeled by a one-dimensional effective Hamiltonian, which includes contributions from the nucleobasis system as well as the sugar-phosphate backbone. Our theoretical approach makes use of Dyson's equation together with a transfer-matrix treatment, considering an electronic tight-binding Hamiltonian model to investigate the electronic density of states (DOS) and the electronic transmissivity of sequences of DNA finite segments. To mimic the DNA segments, we consider the finite quasiperiodic sequences of Fibonacci's type, in a poly(dG)-poly(dC) configuration, whose building blocks are the bases guanine G and cytosine C. We compared the electronic transport found for the quasiperiodic structure to those using a sequence of natural DNA, as part of the human chromosome Ch22.     

Electronic density of states in sequence dependent DNA molecules

We report in this work a numerical study of the electronic density of states (DOS) in π-stacked arrays of DNA single-strand segments made up from the nucleotides guanine G, adenine A, cytosine C and thymine T, forming a Rudin-Shapiro (RS) as well as a Fibonacci (FB) polyGC quasiperiodic sequences. Both structures are constructed starting from a G nucleotide as seed and following their respective inflation rules. Our theoretical method uses Dyson’s equation together with a transfer-matrix treatment, within an electronic tight-binding Hamiltonian model, suitable to describe the DNA segments modelled by the quasiperiodic chains. We compared the DOS spectra found for the quasiperiodic structure to those using a sequence of natural DNA, as part of the human chromosome Ch22, with a remarkable concordance, as far as the RS structure is concerned. The electronic spectrum shows several peaks, corresponding to localized states, as well as a striking self-similar aspect.     

Critical behavior of nanoemitter radiation in a percolation material

We studied the field radiation of disordered optical nanoemitters incorporated into three-dimensional (3D) spanning cluster in a percolation material. In supercritical state, the field intensity is large enough to produce a dynamic high-density coherent field. The resulting state becomes different for lossless and lossy mediums. For material with small losses the long-term coherence arises in the supercritical area close to the percolation threshold. As a result, the dynamic non-monotonic behavior of the field order parameter raises that allows to reach the optimal field intensity. This effect can allow optimization of the disordered optical nanostructures with incorporated radiating nanoemitters in various applications of information technology.     

含单负特异材料一维无序扰动周期结构中的光子局域特性研究

采用传输矩阵法研究了电磁波在由单负特异材料组成的一维无序扰动周期结构中的Anderson局域(Anderson Localization)行为,分别讨论了色散和非色散两种模型.结果发现,在对应周期结构的通带位置,无序的引入对局域长度的影响较大,而在带隙位置,影响较小,几乎可以忽略.该性质与我们曾讨论的随机结构有较明显不同.导致这种局域性质的主要原因应为,光在单负材料组成的系统中的传输主要依赖于两种单负材料间的界面.在无序扰动结构中,该界面数相对于周期结构并没有减少,因此对光的传输性质影响较小,而随机结构中     

Leading Branches of the Transfer-Matrix Spectrum for Lattice Spin Systems (Quasi-Particles of Different Species)

For lattice systems under high temperatures T with compact or finite spin we construct three invariant subspaces of the transfer-matrix, which can be interpreted as the spaces of states for quasi-particles of two different species and the space of states for two particles of the first species. We formulate a condition on a priori distribution guaranteeing that the spectrum of the transfer-matrix on these subspaces are not overlapping.     

Transport length scales in disordered graphene-based materials: strong localization regimes and dimensionality effects

We report on a numerical study of quantum transport in disordered two dimensional graphene and graphene nanoribbons. By using the Kubo and the Landauer approaches, transport length scales in the diffusive (mean free path and charge mobilities) and localized regimes (localization lengths) are computed, assuming a short range disorder (Anderson-type). The electronic systems are found to undergo a conventional Anderson localization in the zero-temperature limit, in agreement with localization scaling theory. Localization lengths in weakly disordered ribbons are found to strongly fluctuate depending on their edge symmetry, but always remain several orders of magnitude smaller than those computed for 2D graphene for the same disorder strength. This pinpoints the role of transport dimensionality and edge effects.