Measurements of lifetime andg-factor of the 32S(4 1 + ) state at 4.459 MeV

Precessions of the very short-lived 2 ₁ ⁺ - and 4 ₁ ⁺ -states in³²S have been measured using the transient field technique. The deducedg-factor of the 4 ₁ ⁺ -state g=+0.40(15) agrees with the known value of the 2 ₁ ⁺ -state and with theoretical predictions. In addition, the lifetimes of both states were redetermined and are consistent with previous results.     

g-factors of the lowest 2+ and 4+ states in198, 200, 202Hg

Theg-factors of the 2 ₁ ⁺ and 4 ₁ ⁺ states in^198,200,202Hg were simultaneously measured by means of the transient-field perturbed angular correlation method in Coulomb excitation using multi-isotopic targets and thin polarized Gd foils as ferromagnetic host. Theg(2 ₁ ⁺ ) andg(4 ₁ ⁺ ) were found identical within errors in^{198, 200}Hg, while in²⁰⁰Hg lowerg-factor values have been determined. The experimentalg-factors were compared with the predictions of the pairing-plus-quadrupole, dynamical deformation and interacting boson models.     

g-factor of the 4 1 + rotational state of160Dy

By use of Ge-detectors of the OSIRIS-collaboration [1] in connection with the 12 detector IPAC apparatus of our laboratory [2] a precise measurement of theg-factor of the 4 ₁ ⁺ rotational state of¹⁶⁰Dy was performed. The directional correlations of the threeγ-γ cascades, 1003-197 keV, 1103-197 keV and 1115-197 keV, which are weakly populated in the decay of 72.3 d¹⁶⁰Tb were observed simultaneously. The integral rotations in the static hyperfine field of DyTb at 4.2 K were measured. Theg-factorg(4 ₁ ⁺ )=+0.350(20) was derived. By comparison with the magnetic splitting of the 2 ₁ ⁺ rotational state observed in the same environment by a Mössbauer experiment [3] the ratio of the twog-factors was derived as g(4 ₁ ⁺ )/g(2 ₁ ⁺ )=+ 0.91(5). For the high energy lines we derived from the measured directional correlations the E1/M2 mixing parameters: δ(1003 keV)=+0.005(4); δ(1103 keV)=?0.020(22), and δ(1115 keV)=+0.010(4)     

Remeasurement of the lifetime of the 4 1 + -state of156Gd and recalculation of itsg-factor

The half-life of the 4 ₁ ⁺ -state of¹⁵⁶Gd has been remeasured by the delayed coincidence technique. The excellent time resolution which can now be achieved by use of small BaF₂ detectors allows a more reliable determination than with previously applied methods. The resultT _1/2(¹⁵⁶Gd,4 ₁ ⁺ )=108(2) ps is smaller than previously published data, but it fits well into the systematics of theB(E2) values of the rotational transitions of this nucleus. A recalculation of the previously measuredg-factor of the same state givesg(¹⁵⁶Gd,4 ₁ ⁺ ) =0.327(19). This value is still smaller than theg-factor of the 2 ₁ ⁺ state, but the magnitude of the reduction can now easier be interpreted by nuclear structure calculations.     

Gyromagnetic ratios of excited states in186W

The gyromagnetic ratios of the 4 ₁ ⁺ , 6 ₁ ⁺ , and 2 ₂ ⁺ states in¹⁸⁶W were measured relative to that of the 2 ₁ ⁺ level by means of the transient field implantation perturbedγ-ray angular distribution technique. The nuclei in the states of interest were Coulomb excited using a beam of 220-MeV⁶³Cu projectiles and recoiled swiftly through a thin, polarized Fe foil. The present measurements yielded ratiosg(4 ₁ ⁺ )/g(2 ₁ ⁺ )=1.04±0.07,g(6 ₁ ⁺ )/g(2 ₁ ⁺ )=1.03 ±0.20 andg(2 ₂ ⁺ )/g(2 ₁ ⁺ )=0.63±0.13. The sizable disparity between the measuredg-factors of the ground- and excited-band is examined within the context of the interacting boson approximation model.     

g-factor of the second 4+ state in24Mg

The transient field technique has been used to determine theg-factor of the 4 ₂ ⁺ state at 6.010MeV excitation in²⁴Mg. The deduced value ofg=+0.5(4) is consistent with collective model expectations. Further, the equality within experimental accuracies, of the g-factors of the 2 ₁ ⁺ , 2 ₂ ⁺ , 4 ₁ ⁺ and 4 ₂ ⁺ states agrees with theoretical predictions for thisT=0 self-conjugate nucleus, in contrast to the results for²⁰Ne.     

g-factors of the ground state rotational band of158Dy

Theg-factors of the four lowest states of the ground state rotational band of¹⁵⁸Dy have been determined asg(2 ₁ ⁺ )=+0.362(23),g(4 ₁ ^su+ )=+0.340(20),g(6 ₁ ^su+ )=+0.207(36) andg(8 ₁ ^su+ )=+0.21(11). Theg-factors of the 2⁺ and 4⁺ states were measured by the IPAC method with radioactive samples of 2.4 h¹⁵⁸Er in external magnetic fields. To investigate the higher states, for the first time an on-line γ—γ IPAC experiment was performed with the reaction¹⁵⁶Gd(α, 2n)¹⁵⁸Dy by use of the static hyperfine field of DyGd.     

Magnetic moments of the 2 1 + states in102, 104Mo

Theg factors of the first excited 2⁺ levels in the neutron-rich nuclei¹⁰²Mo and¹⁰⁴Mo have been studied through the measurement of the perturbed angular correlations for theγ-γ cascades between the 0 ₂ ⁺ -2 ₁ ⁺ -0 ₁ ⁺ level sequences. The results of g=0.42±0.07 for¹⁰²Mo and ofg= _?0.11 ^+0.12 for¹⁰⁴Mo agree with the prediction of the vibrational-rotational model. In terms of IBA, with the assumption ofN _π=3 for the Mo isotopes which takes into consideration a two particle, two-hole excitation across the Z=40 subshell, the proton-bosong factor is deduced to beg _π=1.00±0.23. It is shown that this value provides evidence for subshell effects in¹⁰⁰Zr.     

g-Factor of the first 2+ state in theN=82 nucleus138Ba

The 2 ₁ ⁺ level of¹³⁸Ba has been Coulomb excited with a 105 MeV³²S beam. The precession of the gamma ray angular distribution induced by the transient magnetic field when traversing a 2.14 mg/cm² iron foil, has been measured to be 15.6(1.7) mr. A value of g(¹³⁸Ba 2 ₁ ⁺ )=0.72(11) was obtained assuming for the transient field strength the Chalk River calibration. The field parametrization has been checked using the first 2⁺ state in¹⁵⁰Sm as probe. Theg value obtained is sensibly lower than predicted by large scale shell model calculations in a proton subspace. Theg-factor of the first 2⁺ state in¹⁴⁸Sm has been remeasured yieldingg(¹⁴⁸Sm 2 ₁ ⁺ )=0.246(22).     

EPR of a fullerene-molecule-derived paramagnetic center as a mesoscopic conducting object

Discussion of theg-factor value of fullerene is based on the model of itinerant electrons restricted to the surface of the fullerene molecule C₆₀. The Ag shift, i.e., the difference between the experimentalg-factor and theg-factor of free electron Δg = g ? 2.0023 for C ₆₀ ^?1 is negative as for a very small metallic conducting particle.g-factor value is proportional to the interaction between itinerant electrons in the conduction band, thus the Δg is negative for C ₆₀ ^?1 and C ₆₀ ^?3 having less than half filled conduction band, while Δg is positive for C ₆₀ ⁺ where the conduction band is almost filled.     

B(E2)-values of even-a nuclei with 82 neutrons

Coulomb excitation of the first excited 2⁺-state was measured usingα-particles to determine reduced transition probabilities,B(E2; 0 _gs ⁺ →2 ₁ ⁺ ), in nuclei with a closed shell of 82 neutrons. TheB(E2; 0 _gs ⁺ →2 ₁ ⁺ -values are 10.2 single-particle units (spu) for¹³⁸Ba, 13.5 spu for¹⁴⁰Ce, 11.9 spu for¹⁴²Nd and 11.6 spu for¹⁴⁴Sm. The uncertainty ranges from 1.3 % to 2.3 %.     

g-factors of rotational states in176Hf,177Hf,and180Hf

g-factors of rotational states in¹⁷⁶Hf and¹⁸⁰Hf were measured with the twelve detector IPAC-apparatus of our laboratory [1]. The natural radioactivity 3.78·10¹⁰y¹⁷⁶Lu and the 5.5 h isomer^180mHf were used which populate the ground-state rotational bands of¹⁷⁶Hf and¹⁸⁰Hf. The integral rotations ofγ-γ directional correlations in strong external magnetic fields and in static hyperfine fields of (Lu→Hf)Fe₂ and HfFe₂ were observed. The following results were obtained: $$\begin{array}{l} ^{176} Hf: g\left( {4_1^ + } \right) = + 0.334\left( {38} \right) \\ ^{180} Hf: g\left( {2_1^ + } \right) = + 0.305\left( {14} \right) \\ g\left( {4_1^ + } \right) = + 0.358\left( {43} \right) \\ {{ g\left( {6_1^ + } \right)} \mathord{\left/ {\vphantom {{ g\left( {6_1^ + } \right)} {g\left( {4_1^ + } \right)}}} \right. \kern-\nulldelimiterspace} {g\left( {4_1^ + } \right)}} = + 0.95\left( {12} \right) \\ \end{array}$$ . The hyperfine field in (Lu→Hf)Fe₂ was calibrated by observing the integral rotation of the 9/2^? first excited state of¹⁷⁷Hf populated in the decay of 6.7d¹⁷⁷Lu. Theg-factor of this state was redetermined in an external magnetic field as $$^{177} Hf: g\left( {{9 \mathord{\left/ {\vphantom {9 {2^ - }}} \right. \kern-\nulldelimiterspace} {2^ - }}} \right) = + 0.228\left( 7 \right)$$ . Finally theg-factor of the 2 ₁ ⁺ state of¹⁷⁶Hf was derived from the measuredg(2 ₁ ⁺ ) of¹⁸⁰Hf by use of the precisely known ratiog(2 ₁ ⁺ ,¹⁷⁶Hf)/g(2 ₁ ⁺ ,¹⁸⁰Hf) [2] as $$^{176} Hf: g\left( {2_1^ + } \right) = + 0.315\left( {30} \right)$$ .     

Untersuchung des Zerfalls von134Cs durch γ-γ-Winkelkorrelationsmessungen

γ-γ-angular correlation measurements with Ge(Li) detectors and NaJ(Tl) detectors provided theE2/M1 mixing ratios of the following gamma transitions: 3 ₁ ⁺ →2 ₂ ⁺ (475.3 keV), 2 ₂ ⁺ →2 ₁ ⁺ (563.3 keV), 4 ₂ ⁺ →4 ₁ ⁺ (569.4 keV), 3 ₁ ⁺ →2 ₁ ⁺ (1,039 keV). The angular correlation measurements were only consistent with spin 3 of the 1,643 keV level. The half life of the 1,401 keV level was determined by delayed coincidence techniques to beT _1/2 (1,401 keV)≦30 ps.     

Gyromagnetic ratios of 4+ and 6+ states in156Gd and158Gd

The followingg-factors have been derived from time integral measurements of γ-γ angular correlations in the static magnetic hyperfine field of magnetized gadolinium metal probes:¹⁵⁶Gd:g(4 ₁ ⁺ )=+0.310(19)g(6 ₁ ⁺ )=+0.25(21)g(4 ₃ ⁺ , 1511 keV)=+0.809(27)¹⁵⁸Gd:g(4 ₁ ⁺ )=+0.409(15). The 5.35d ¹⁵⁶Tb sources were produced by the reaction¹⁵⁶Gd(d, 2n)¹⁵⁶Tb in our cyclotron. A carrier-free 150y ¹⁵⁸Tb source was obtained from ISOLDE/CERN. In comparison with the precisely knowng-factors of the 2 ₁ ⁺ states,g(2 ₁ ^su+ ,¹⁵⁶Gd) =+0.386(4) andg(2 ₁ ⁺ ,¹⁵⁸Gd)=0.381(4), we observe a large reduction for the¹⁵⁶Gd 4 ₁ ⁺ state whereasg increases slightly for¹⁵⁸Gd. The half-life of the 4 ₁ ⁺ state of¹⁵⁸Gd was remeasured as¹⁵⁸Gd:T _1/2(4 ₁ ⁺ )=148(2) ps. A measurement of the rotation in the 4 ₃ ⁺ state of¹⁵⁶Gd in external magnetic fields of various strengths up toB _ext=9.5 T did not confirm the anomalous dependence of the magnetic hyperfine field in gadolinium metal on the external field, which has been reported by Persson et al. [29].     

E2 andE3 transition strengths in some rare-earth nuclei

Coulomb excitation byα-particles of vibrational-like states in even-mass rare-earth nuclei is used to determine the reduced transition probabilitiesB(E2; 0 _gs ⁺ →2 _γ ⁺ ),B(E2; 0 _gs ⁺ →2 _β ⁺ ),B(E2; 2 _gs ⁺ →0 _β ⁺ ) andB(E2; 0 _gs ⁺ →3 _oct ^? ) in¹⁵⁰Nd,^{152, 154}Sm,^{154, 158}Gd,¹⁶⁴Dy and¹⁶⁶Er. TheB(Eλ; 0 _gs ⁺ →I=λ)-values range from 2.4 to 6.5 single-particle units for transitions to the 2 _γ ⁺ -states, 0.8 single-particle units for the 2 _β ⁺ -states and from 14.1 to 21.7 single-particle units for the 3^?-states.     

Gyromagnetic ratio of the 2+ rotational state of184W and observation of a large hyperfine anomaly with respect to183Wg in iron

Theg-factor of the 2⁺ rotational state of¹⁸⁴W was redetermined by an IPAC measurement in an external magnetic field of 9.45 (5)T as: $$g_{2^ + } (^{184} W) = + 0.289(7).$$ In the evaluation the remeasured half-life of the 2⁺ state: $$T_{{1 \mathord{\left/ {\vphantom {1 2}} \right. \kern-\nulldelimiterspace} 2}} (2^ + ) = 1.251(12)ns$$ was used. TDPAC-measurements with a sample of carrierfree¹⁸⁴Re in high purity iron gave the hyperfine fields: $$B_{300 K}^{hf} (^{184} W_2 + \underline {Fe} ) = 70.1(21)T$$ and $$B_{40 K}^{hf} (^{184} W_{2^ + } \underline {Fe} ) = 71.8(22)T.$$ A comparison with the hyperfine field known from a spin echo experiment with¹⁸³W _g Fe leads to the hyperfine anomaly: $$^{184} W_{2^ + } \Delta ^{183} W_g = + 0.145(36).$$ The hyperfine splitting observed in a Mössbauer source experiment with another sample of carrierfree^184m Re in high purity iron indicates that the smaller splitting, measured previously by a Mössbauer absorber experiment is due to the high tungsten concentration in the absorber. The new value for theg-factor of the 2⁺ state together with the result of the Mössbauer experiment allow an improved calibration for our recent investigation of theg _R -factors of the 4⁺ and 6⁺ rotational states. The recalculated values are: $$g_{4^ + } (^{184} W) = + 0.293(23)$$ and $$g_{6^ + } (^{184} W) = + 0.299(43).$$ The remeasured 792-111 keVγ-γ angular correlation $$W(\Theta ) = 1 - 0.034(4) \cdot P_2 + 0.325(6) \cdot P_4 $$ gives for the mixing ratio of theK-forbidden 792keV transition: $$\delta ({{E2} \mathord{\left/ {\vphantom {{E2} {M1}}} \right. \kern-\nulldelimiterspace} {M1}}) = - \left( {17.6\begin{array}{*{20}c} { + 1.8} \\ { - 1.5} \\ \end{array} } \right).$$ A detailed investigation of the attenuation ofγ-γ angular correlations in liquid sources of¹⁸⁴Re and^184m Re revealed the reason for erroneous results of early measurements of the 2⁺ g _R -factor: The time dependence of the perturbation is not of a simple exponential type. It contains an unresolved strong fast component.     

Measurement of theg-factor of the 21 + state of192Pt in an external magnetic field

Theg-factor of the 2₁ ⁺ state of¹⁹²Pt has been measured by the IPAC technique in an external magnetic field as:g(2₁ ⁺,¹⁹²Pt)=+0.287(17). An additional IPAC experiment with an¹⁹²IrFe sample was performed with the same level in order to investigate the hyperfine field. The result:ω _L τ(2₁ ⁺,¹⁹²PtFe)=0.1115(9) gives the hyperfine field:B _hf ^4.2k (PtFe)=126.8(71) T. The result of an LTNO experiment with the same level is compatible with the assumption that 100% of the¹⁹²Ir atoms were on unique sites.     

Confrontation between the quasiparticle-phonon nuclear model and the interacting boson model for deformed nuclei

TheK ^π=0⁺, 2⁺ and 4⁺ states are considered in doubly even deformed nuclei. It is shown that in the quasiparticle-phonon nuclear model (QPNM) and in the interacting boson model (IBM) a vibrational state has one dominating component. The states withK _n ^π =0 ₃ ⁺ , 0 ₄ ⁺ 0 ₅ ⁺ 2 ₂ ⁺ , 2 ₃ ⁺ , 4 ₁ ⁺ and 4 ₂ ⁺ have a dominating one-phonon component within the QPNM and a two- or three-boson component within the IBM. According to the QPNM the contribution of two-phonon components to the wave functions of these states is less than 10%, i.e. there is a qualitative discrepancy in describing the structure of these states within the QPNM and the IBM. The experimental data indicate the existence in these states of one-phonon or two-quasiparticle components. They are rather well described within the QPNM. These states cannot be described within the IBM. This is due to the fact that the IBM takes into account only a small part of the space of two-quasiparticle states, just the one entering intoΒ- andγ-vibrational states.     

g-factors of rotational states in 176Hf, 177Hf,and 180Hf

g-factors of rotational states in ¹⁷⁶Hf and ¹⁸⁰Hf were measured with the twelve detector IPAC-apparatus of our laboratory [1]. The natural radioactivity 3.78 · 10¹⁰y ¹⁷⁶Lu and the 5.5 h isomer ^180mHf were used which populate the ground-state rotational bands of ¹⁷⁶Hf and ¹⁸⁰Hf. The integral rotations of γ-γ directional correlations in strong external magnetic fields and in static hyperfine fields of (Lu → Hf)Fe₂ and HfFe₂ were observed. The following results were obtained: The hyperfine field in (Lu → Hf)Fe₂ was calibrated by observing the integral rotation of the 9/2^? first excited state of ¹⁷⁷Hf populated in the decay of 6.7d ¹⁷⁷Lu. The g-factor of this state was redetermined in an external magnetic field as Finally the g-factor of the 2 ₁ ⁺ state of ¹⁷⁶Hf was derived from the measured g(2 ₁ ⁺ ) of ¹⁸⁰Hf by use of the precisely known ratio g(2 ₁ ⁺ , ¹⁷⁶Hf)/g(2₁ ⁺, ¹⁸⁰Hf) [2] as      

Multiplicities of charged particles prior to fission

Electric monopole transitions between the 0 ₂ ⁺ , 0 ₁ ⁺ and 2 ₂ ⁺ , 2 ₁ ⁺ levels in⁷⁶Se, populated in the decay of⁷⁶Br, were investigated by means of conversion electrons and gammaray spectroscopy. TheK-electron intensity ratios ofE0 andE2 transitions connecting the 0 ₂ ⁺ level to the 0 ₁ ⁺ and 2 ₁ ⁺ levels and of theE0 andE2 components in the 2 ₂ ⁺ →2 ₁ ⁺ transition were determined. The ratioX(E0/E2) of theE0 toE2 reduced transition probabilities and, from the available lifetimes, theE0 strength parameters ρ(E0) were deduced for the two transitions. The results are compared with the predictions of current models.