Electro-optic spectral tuning in a continuous-wave, asymmetric-duty-cycle, periodically poled LiNbO(3) optical parametric oscillator

We demonstrate electro-optic spectral tuning in a continuous-wave periodically poled LiNbO(3) (PPLN) optical parametric oscillator (OPO). We achieve 8.91 cm(-1) of rapid spectral tuning, with a linear tuning rate of 2.89 cm(-1) /(kV/mm), by applying electric fields up to +/-1.5 kV/mm across the crystal while it is operating within the OPO. Intentionally poling the PPLN crystal with an asymmetric domain structure enables tuning, and numerical predictions closely match the experimental observations. The tuning is considerably larger than the typical operational bandwidth of the OPO, indicating that we are in fact shifting the gain curve of the PPLN crystal.     

Optical parametric oscillation in periodically poled lithium niobate driven by a diode-pumped Q-switched erbium fiber laser

We describe what is to our knowledge the first nanosecond periodically poled lithium niobate (PPLN) optical parametric oscillator (OPO) driven by a fiber laser. The source was frequency doubled by a PPLN sample before pumping a second, 20-mm-long, PPLN crystal. The OPO threshold was <10muJ, with pump depletions of as much as 45% and a tunable signal range of 945-1450 nm (1690-4450-nm idler range). We demonstrated 130-nm signal tuning by varying the pump wavelength and doubling crystal's temperature. Also, we achieved 15-nm tuning with all crystals at a constant temperature. The results demonstrate the potential of the fiber laser:PPLN combination for practical, versatile, and tunable sources.     

Low-threshold singly-resonant continuous-wave optical parametric oscillator based on MgO-doped PPLN

We present a 532 nm-pumped singly-resonant cw optical parametric oscillator based on MgO-doped PPLN with a minimum threshold pump power of 0.3 W. The OPO with a two-mirror standing-wave cavity is optimized by using a tunable diode laser on the path of the resonant signal beam. The maximum output power is 200 mW at an idler wavelength near 1330 nm at a pump power of 2 W. We report the degradation of the output power and beam characteristics at high pump power indicating a strong thermal lensing in the crystal. The continuous tuning range of the OPO is measured to be 800 MHz which is close to 90% of the free spectral range of the OPO cavity.     

Few‐cycle,broadband, mid‐infrared optical parametric oscillator pumped by a 20‐fs Ti:sapphire laser

A few‐cycle, broadband, singly‐resonant optical parametric oscillator (OPO) for the mid‐infrared based on MgO‐doped periodically‐poled LiNbO₃ (MgO:PPLN), synchronously pumped by a 20‐fs Ti:sapphire laser is reported. By using crystal interaction lengths as short as 250 µm, and careful dispersion management of input pump pulses and the OPO resonator, near‐transform‐limited, few‐cycle idler pulses tunable across the mid‐infrared have been generated, with as few as 3.7 optical cycles at 2682 nm. The OPO can be continuously tuned over 2179‐3732 nm (4589‐2680 cm^‐1) by cavity delay tuning, providing up to 33 mW of output power at 3723 nm. The idler spectra exhibit stable broadband profiles with bandwidths spanning over 422 nm (FWHM) recorded at 3732 nm. The effect of crystal length on spectral bandwidth and pulse duration is investigated at a fixed wavelength, confirming near‐transform‐limited idler pulses for all grating interaction lengths. By locking the repetition frequency of the pump laser to a radio‐frequency reference, and without active stabilization of the OPO cavity length, an idler power stability better than 1.6% rms over >2.75 hours is obtained when operating at maximum output power, in excellent spatial beam quality with TEM₀₀ mode profile. Photograph shows a multigrating MgO:PPLN crystal used as a nonlinear gain medium in the few‐cycle femtosecond mid‐IR OPO. The visible light is the result of non‐phase‐matched sum‐frequency mixing between the interacting beams.     

板条放大器同步泵浦的宽调谐MgO:PPLN中红外光参量振荡器（英）

搭建了Nd:YVO4/SESAM锁模激光器,采用LDA泵浦的Innoslab对其进行功率放大,最后同步泵浦MgO:PPLN实现了宽调谐皮秒中红外光参量运转。通过改变MgO:PPLN的温度和通道,实现了信号光1415~1557 nm、闲频光3362~4290 nm范围的宽调谐输出,其中最高的光光转换效率为17.5%。同步泵浦功率为16 W,脉冲重复频率为116.9 MHz时,同时获得1.33 W的1518 nm信号光和1.26 W的3558 nm闲频光输出。     

双共振准相位匹配光学参量振荡器的调谐特性

利用全固化单频Nd：YVO4激光器泵浦双共振难相位匹配铌酸锂连续光学参量振荡器，实验研究了该光学参量振荡器下转换光的调谐特性。通过改变PPLN晶体的温度及OPO的腔长，下转换光的调谐范围分别为189nm和175nm，通过改变泵浦光频率，信号光频率连续调谐375MHz。实验结果与理论计算值基本吻合。     

低阈值温度调谐PPMgLN红外光参量振荡

研究了温度调谐下周期极化镁掺杂铌酸锂晶体的红外光参量振荡特性。采用外电场短脉冲极化技术,在大小为7.0mm×50.0mm×1.0mm的Z切高镁掺杂(摩尔分数0.05)铌酸锂上制备出了准相位匹配光学微结构器件,极化周期为30.0μm。以输出波长为1064nm的声光调QNd:YAG固体激光器作为基频泵浦光开展了光参量振荡研究。实验表明:泵浦该PPMgLN晶体,实现了室温下低阈值红外光参量振荡产生,阈值功率仅为45mW(重复频率1kHz)。在泵浦输入功率为225mW时,有36mW信号光输出,转换效率达到16.0%,通过调谐晶体温度(20~180℃),获得了调谐范围为1503~1550nm波段的OPO信号光,实现了低阈值可调谐红外光的稳定输出。     

Study of quasi-phase matching wavelength acceptance bandwidth for periodically poled LiNbO3 crystal-based difference-frequency generation

The temperature tuning characteristics of quasi-phase matching (QPM) wavelength acceptance bandwidth in a uniform periodically poled lithium niobate (PPLN) based on difference-frequency generation (DFG) are studied theoretically and experimentally. This paper proposes a PPLN device consisting of several segments of different temperatures to obtain a more desirable performance for the QPM-DFG. The result shows that through the tuning of temperature, the bandwidth can be changed considerably and the method was proved suitable and accurate to calculate QPM wavelength acceptance bandwidth of DFG in a uniform PPLN crystal for temperatures between room temperature and 180 °C and mid-infrared (mid-IR) wavelengths ranging from 2.8 to 4.8 μm.     

Rapid infrared wavelength access with a picosecond PPLN OPO synchronously pumped by a mode-locked diode laser

We theoretically and experimentally investigate wavelength tuning of synchronously pumped optical parametric oscillators (OPOs) on changing the cavity length or the pump-repetition rate. Conditions for rapid and wide-range wavelength access are derived. Using an OPO pumped directly by a mode-locked diode-laser master-oscillator power-amplifier (MOPA) system, an all-electronically controlled access to near- and mid-infrared wavelengths is demonstrated. The singly (signal) resonant OPO is based on periodically poled lithium niobate (PPLN) and emits 8 ps idler pulses at a repetition rate of 2.5 GHz in the wavelength range 1986 to 2348 nm (signal: 1530 to 1737 nm). Wavelength tuning over 114 nm (signal) and 189 nm (idler) is achieved solely by electronically varying the repetition rate of the diode-laser oscillator over 720 kHz. By controlling the repetition rate with a programmable driver, an arbitrary emission sequence of the OPO on two wavelength channels is generated, with access times as short as 10 μs. 11 OPO wavelengths equally spaced in the range 1627–1689 nm (signal) or 2054–2154 nm (idler) could be addressed. Received: 6 September 2000 / Revised version: 16 March 2001 / Published online: 23 May 2001     

All-optical wavelength tuning in Ti:PPLN Šolc filter via the photorefractive effect

We demonstrate fine-wavelength tuning of a periodically poled Ti:LiNbO₃ (Ti:PPLN) Šolc filter by use of the photorefractive (PR) effect. The center wavelength of a Ti:PPLN Šolc filter is controlled by the PR effect, which is induced by second-harmonic generation (SHG). The refractive index change caused by the PR effect is calculated from the measured shift in center wavelength from the Ti:PPLN Šolc filter. The experimental results show that all-optical fine-wavelength tuning in a Ti:PPLN Šolc filter is possible by the use of a second-order nonlinear effect and that a Ti:PPLN waveguide has much higher resistance to PR damage than a Ti:LiNbO₃ waveguide. The measured wavelength tuning rate as a function of the pump beam power is about − 0.033 nm/mW.     

窄线宽1064 nm光纤激光泵浦高效率中红外3.8μm MgO:PPLN光参量振荡器

采用放大1064?nm掺镱光纤激光器作为泵浦源,实现了中红外3.8?μm?MgO:PPLN光参量振荡(OPO)激光输出.在泵浦源中,采用分布式反馈激光器(DFB)作为种子源来实现光纤激光窄线宽的调制,实现线宽2.5?nm到0.1?nm的压缩,最大平均输出功率可达40?W.进一步对不同泵浦线宽条件下中红外3.8?μm?M...     

Spectroscopic diagnostics of chemical processes: applications of tunable optical parametric oscillators

Optical parametric oscillator (OPO) and amplifier (OPA) devices are useful for spectroscopic sensing of chemical processes in laboratory, industrial, and environmental settings. This is particularly true of nanosecond-pulsed, continuously tunable OPO/OPA systems, for which we survey a variety of instrumental strategies, together with actual spectroscopic measurements. The relative merits of OPO wavelength control by intracavity gratings and by injection seeding are considered. A major innovation comprises an OPO with a ring cavity based on periodically poled lithium niobate (PPLN) and injection-seeded by a single-mode tunable diode laser (TDL). Active cavity control by an ‘intensity dip’ method yields an optical bandwidth ≤0.005 cm^-1 (150 MHz), which compares favourably with the performance of advanced grating-tuned OPO/OPA systems. A novel adaptation of this TDL-seeded PPLN OPO employs a compact, inexpensive multimode pump laser, with which it is still possible to obtain continuously tunable single-mode signal output. Cavity ringdown (CRD) spectroscopy also figures prominently, with infrared (IR) CRD spectra from both grating-scanned and TDL-seeded OPOs reported. Finally, a tunable ultraviolet (UV) source, combining a TDL-seeded passive-cavity OPO and a sum-frequency generation stage, is developed for measurements of time-resolved IR-UV double resonance spectra of acetylene and UV laser-induced fluorescence spectra of nitric oxide. Received: 28 March 2000 / Published online: 13 September 2000     

Widely tunable difference frequency generation around 3.4 μm using index dispersion property of PPLN

In this paper, the wide difference frequency generation (DFG) tuning characteristics around 3.4 μm are investigated by using the index dispersion property of PPLN. With a ytterbium doped fiber laser (YDFL) and an erbium doped fiber laser (EDFL) as the fundamental light sources, our simulation results show that the quasi-phase matching (QPM) wavelength acceptance bandwidth (BW) for the pump is much larger than that for the signal. Although the positions of the broadened QPM pump bands vary with the poling period and the signal wavelength, the corresponding idler tuning ranges center around 3.4 μm. With a signal wavelength of 1.57 μm, an idler tuning range of greater than 170 nm is experimentally obtained in the 30 uniform grating PPLN. When the signal wavelength and the poling period are respectively changed to 1.55 and 29.50 μm, wide DFG tuning operations around 3.4 μm are also achieved with the crystal temperature adjusted to adapt the change.     

Widely tunable PPLN/IOPO driven by a diode-end-pumped Q-switched Nd:YVO<Subscript>4</Subscript> laser

This paper reported a broadband tuning intracavity optical parametric oscillator (IOPO), based on the multiple grating periodical poled lithium niobate (PPLN) pumped by a acoustic-optical (AO) Q-switched Nd:YVO₄ laser. The widely tunable OPO output signal wavelength range from 1390 to 1605 nm, which was obtained by changing PPLN poling period from 27.8 to 31.6 μm at a certain temperature of 46°C, while the continuous tuning range was measured from 1475 to 1592 nm with the PPLN poling period of 30 μm by varying the temperature of nonlinear crystal PPLN from 50 to 120°C. The maximum output power of 0.92 W at 1534 nm with the minimum pulse width of 5.17 ns was generated under the incident pump power of 9.6 W at 808 nm. The corresponding peak power and single pulse energy were calculated to be 5.94 kW and 30.7 μJ, respectively. The M ₂-factor was measured to be 2.01 at the signal power of 0.4 W.     

Quasi-phase-matched generation of tunable blue light in a quasi-periodic structure

We present what is to our knowledge a new approach to generating tunable blue light by cascaded nonlinear frequency conversion in a single LiTaO3 crystal. Simultaneous quasi-phase matching of an optical parametric generation process and a sum-frequency mixing process is achieved by means of structuring the crystal with a quasi-periodic optical superlattice. The spectral (wavelength tuning and bandwidth) and power characteristics of the blue-light generation are studied with a fixed-wavelength 532-nm picosecond laser and a wavelength-tunable nanosecond optical parametric oscillator (OPO) as the pump sources. By tuning the OPO wavelength, we could tune the blue output over approximately 20 nm. Temperature tuning of the blue output at a fixed pump wavelength of 532 nm was limited to approximately 1.5 nm. A maximum blue power of 15 microW was generated at a pump power of 0.5 mW, corresponding to an efficiency of 3%.     

Tuning and stability of a continuous-wave mid-infrared high-power single resonant optical parametric oscillator

A 2.2-W continuous-wave, continuously tunable, single-frequency OPO has been developed in the 3.0–3.8 μm wavelength range for the detection of molecular trace gasses. The oscillation threshold, output power and stability of the single resonant OPO were improved by optimizing pump beam waist and OPO cavity length. Both air-spaced and solid etalons were tested to frequency stabilize and tune the OPO, from which the solid etalon gave a better performance. Temperature oscillations in the PPLN crystal caused oscillations in the idler wavelength of less than 200 MHz over 300 s; the short-term stability was less than 3 MHz over 1 s. The high laser power, in combination with photoacoustic spectroscopy, achieved a detection limit of 10 parts-per-trillion for ethane in nitrogen. Received: 9 April 2002 / Revised version: 14 June 2002 / Published online: 2 September 2002 RID="*" ID="*"Corresponding author. Fax:+31-24/3653311, E-Mail: maartenh@sci.kun.nl     

Synchronously pumped femtosecond optical parametric oscillator of congruent and stoichiometric MgO-doped periodically poled lithium niobate

A synchronously pumped femtosecond optical parametric oscillator based on congruent MgO-doped periodically poled lithium niobate (c-MgO:PPLN) is reported. The system, operating at room temperature, was pumped by a mode-locked Ti:sapphire laser. The wavelengths of the signal and idler waves were tuned from 870 nm to 1.54 μm and 1.58 to 5.67 μm, respectively, by changing the pump wavelength, the grating period or the cavity length. Pumped by 1.1 W of 755 nm laser radiation, the OPO generated 310 mW of 1080 nm radiation. This signal output corresponds to a total conversion efficiency of 50%. Without dispersion compensation the OPO generated phase-modulated signal pulses of 200 fs duration. Besides the OPO of c-MgO:PPLN, an OPO of stoichiometric (s) MgO:PPLN was investigated. Because of the reduced sensitivity to photorefractive damage, both crystals allowed efficient OPO operation at room temperature. Received: 19 August 2002 / Revised version: 11 December 2002 / Published online: 19 March 2003 RID="*" ID="*"Corresponding author. Fax: +49-631/205-3906, E-mail: andres@physik.uni-kl.de     

Tunable mid-infrared optical parametric oscillator with intracavity parametric amplification based on a dual-grating PPLN crystal

Intracavity amplification of the idler radiation of a nanosecond optical parametric oscillator (OPO) is achieved within a single dual-grating PPLN crystal composed of a uniform-grating section followed by a fan-out grating section. While all the OPO wavelength-tuning capabilities are preserved, this configuration leads to a 60?% increase of the 4-??m idler power and a significant beam quality improvement when compared to a conventional singly resonant OPO.     

Combined wide pump tuning and high power of a continuous-wave, singly resonant optical parametric oscillator

A new singly resonant, single-frequency optical parametric oscillator (OPO) has been developed for the 2.6–4.7 m infrared wavelength region, using a high power (>20 W), widely tunable (1024–1034 nm) Yb:YAG pump source. With the OPO frequency stabilized with an intracavity etalon, the OPO achieved an idler output power of 3 W at 2.954 m. Tuning of the idler frequency was achieved by longitudinal mode-hop tuning of the pump source (FSR 100 MHz). In this way an idler frequency scan of 100–150 GHz could be obtained, after which the signal frequency hops ahead over the FSR of the intracavity etalon of the OPO (207 GHz). Due to un-optimized mirror coatings for the OPO cavity and PPLN crystal, the frequency stability was limited to 90 MHz over 1 s, with an unaffected long-term frequency stability of 250 MHz over 200 seconds. PACS 42.65.Yj; 82.80.Kq; 42.62.Fi     

基于准相位匹配产生近中红外波段的特性分析

基于周期极化晶体的Sellmeier方程和准相位匹配理论,对准相位匹配光参变振荡器的调谐特性进行了理论分析.通过数值模拟计算,得到了PPRTA晶体光参变振荡的调谐特性与极化反转光栅周期、晶体温度和抽运光波长等参量的关系曲线.并且与PPKTP晶体和PPLN晶体光参变振荡器的调谐特性进行了比较,研究了三者的不同之处,得出了PPRTA晶体的参量调谐特性优于PPKTP晶体和PPLN晶体的结论,与国外已报道的实验数据相吻合.证实了PPRTA晶体是一种可以产生可调谐近中红外光的理想准相位匹配非线性光学晶体.