共查询到20条相似文献,搜索用时 15 毫秒
1.
A. Paolone P. Roy A. Pimenov A. Loidl A.A. Mukhin A.M. Balbashov 《The European Physical Journal B - Condensed Matter and Complex Systems》2000,16(2):245-250
The optical conductivity of La0.85Sr0.15MnO3 single crystals was studied by means of submillimeter and infrared spectroscopy for frequencies cm-1 and temperatures 10 K <
T
<300 K. The submillimeter conductivity follows the temperature dependence of the dc-data. The phonon spectrum of La0.85Sr0.15MnO3 changes considerably below K revealing a structural phase transition induced by charge or orbital order. At T
=10 K a number of phonon modes can be identified in addition to the room-temperature spectrum. The optical conductivity () in the mid-infrared reveals the characteristics of small polaron absorption. Below the magnetic ordering temperature the
polaron binding energy is highly reduced, but the onset of charge order interrupts the formation of free charge carriers with
a Drude-like behavior. The frequency and temperature dependence of in this regime qualitatively resembles the small polaron predictions by Millis et al. (Phys. Rev. B 54, 5405 (1996)).
Received 5 November 1999 相似文献
2.
Li Zhang Hong-Jing Xie Chuan-Yu Chen 《The European Physical Journal B - Condensed Matter and Complex Systems》2002,27(4):577-582
Within the framework of the dielectric continuum model, interface optical(IO) and surface optical(SO) phonon modes and the
Fr?hlich electron-IO (SO) phonon interaction Hamiltonian in a multi-shell spherical system were derived and studied. Numerical
calculation on CdS/HgS/H2O and CdS/HgS/CdS/H2O spherical systems have been performed. Results reveal that there are two IO modes and one SO mode for the CdS/HgS/H2O system, one SO mode and four IO modes whose frequencies approach the IO phonon frequencies of the single CdS/HgS heterostructure
with the increasing of the quantum number l for CdS/HgS/CdS/H2O. It also showed that smaller l and SO phonon compared with IO phonon, have more significant contribution to the electron-IO (SO) phonon interaction.
Received 16 October 2001 and Received in final form 23 January 2002 Published online 25 June 2002 相似文献
3.
H.-D. Zhou R.-K. Zheng G. Li S.-J. Feng F. Liu X.-J. Fan X.-G. Li 《The European Physical Journal B - Condensed Matter and Complex Systems》2002,26(4):467-471
The transport properties of the La1-xCaxMnO3 ( 0.5 ?
x
< 1) system in magnetic fields up to 14 T were studied. We found that the relationship between the charge ordering temperature
T
CO
and Mn4+ content n
Mn4 +
obeys the formula T
CO
/
T
max
= 1 -
a
(
n
Mn4 +
-
n
0
)
2
, here n0 and a are constants and T
max
is the maximum of T
CO
. For x
= 0.65, T
CO
arrives at the maximum value of 249.5 K in zero magnetic field, while the charge ordered (CO) state is most stable around
x
= 0.75. For x
= 0.5 when H
< 6 T the resistivity displays Mott's variable-range hopping (VRH) behavior, when 6 <
H
< 12 T it is suggested that two kinds of conduction mechanism, i.e., VRH and magnetic polarons, coexist in the material, and when H
> 12 T the resistivity shows metallic-like behavior and the transport mechanism is attributed to coexistence of magnetic polarons
and free carriers. For x
= 0.95, the conduction mechanism accords with the coexistence of VRH and magnetic polarons.
Received 4 January 2002 and Received in final form 28 January 2002 相似文献
4.
G. Li S.-J. Feng F. Liu Y. Yang R.-K. Zheng T. Qian X.-Y. Guo X.-G. Li 《The European Physical Journal B - Condensed Matter and Complex Systems》2003,32(1):5-11
The magnetic transport properties have been measured for La0.67-xYxCa0.33MnO3 ( 0 ⩽
x
⩽ 0.14) system. It was found that the transition temperature T
p
almost linearly moves to higher temperature as H increases. Electron spin resonance confirms that above T
p
, there exist ferromagnetic clusters. From the magnetic polaron point of view, the shift of T
p
vs. H was understood, and it was estimated that the size of the magnetic polaron is of 9.7 ∼ 15.4 ? which is consistent with the magnetic correlation length revealed by the small-angle neutron-scattering technique. The
transport properties at temperatures higher than T
p
conform to the variable-range hopping mechanism.
Received 27 August 2002 / Received in final form 2 December 2002 Published online 14 March 2003 相似文献
5.
Zhi Ping Wang Xi Xia Liang 《The European Physical Journal B - Condensed Matter and Complex Systems》2003,33(3):265-271
Rayleigh-Schr?dinger perturbation theory and an improved Wigner-Brillouin perturbation theory has been used to study the cyclotron
resonance of the polarons in ternary mixed crystals in the zero-temperature limit. The interaction between an electron and
two branches of longitudinal optical phonon modes is taken into account in the framework of the random-element-isodisplacement
model. The numerical results for several ternary mixed crystals show that the polaronic cyclotron energy and mass split successively
twice related to the higher and lower branches of longitudinal optical phonon modes of ternary mixed crystals. A non-linear
dependence of the polaronic cyclotron energy and mass on the composition x is found.
Received 19 March 2002 / Received in final form 21 March 2003 Published online 20 June 2003
RID="a"
ID="a"e-mail: xxliang@imu.edu.cn 相似文献
6.
7.
F. Fauth E. Suard V. Caignaert B. Domengès I. Mirebeau L. Keller 《The European Physical Journal B - Condensed Matter and Complex Systems》2001,21(2):163-174
The oxygen deficient cobaltites LnBaCo2O5 (Ln = Tb, Dy, Ho) exhibit two successive crystallographic transitions at T
N
∼340 K and at T
CO
∼210 K. Whereas the first transition (P4/mmm to Pmmm) is related to the long-range antiferromagnetic ordering of the Co ions
(spin ordering), the second transition (Pmmm to Pmmb) corresponds to the long-range ordering of the Co2+ and Co3+ species (charge ordering) occurring in 1:1 ratio in the structure. The charge ordered (CO) state was directly evidenced by
the observation of additional superstructure peaks using neutron and electron diffraction techniques. The CO state was also
confirmed indirectly from refinement of high resolution neutron diffraction data as well as from resistivity and DSC measurements.
From the refined saturated magnetic moment values only, ∼3.7
and ∼2.7
, the electronic configuration of the Co ions in LnBaCo2O5 remains conjectural. Two pictures, with Co3+ ions either in intermediate spin state ( t
5
2g
e
1
g
) or in high spin state ( t
4
2g
e
2
g
), describe equally well our experimental data. In both cases, the observed magnetic structure can be explained using the
qualitative Goodenough-Kanamori rules for superexchange. Finally, in contrast to the parent Ln = Y compound [Vogt et al. , Phys. Rev. Lett. 84, 2969 (2000)], we do not report any spin transition in LnBaCo2O5 (Ln = Tb, Dy, Ho).
Received 13 December 2000 相似文献
8.
J.E. Lorenzo H. Requardt 《The European Physical Journal B - Condensed Matter and Complex Systems》2002,28(2):185-186
Eur. Phys. J. B 24, 315 (2001) Here we comment on a recently published paper on the presence of a phason contribution in the low temperature heat capacity data of the charge-density-wave compounds K0.3MoO3 and (TaSe4)2I. We have shown that the anomaly in the C
P
/
T
3
data reported by Odin et al. is straightforwardly interpreted in terms of low energy phonon modes resulting from the peculiar topology of these compounds.
Received 21 February 2002 Published online 19 July 2002 相似文献
9.
R. Ramakumar K. Yamaji 《The European Physical Journal B - Condensed Matter and Complex Systems》2001,24(1):71-75
A simple model is developed to understand superconductivity in α
′
-TTF[Pd(dmit)2]2. We include electron-intra molecular and intermolecular phonon interactions as the mechanism of superconductivity. Intramolecular vibrations included are the eight symmetric Ag modes of the Pd(dmit)2 molecule. Intermolecular vibrations included are the longitudinal acoustic and transverse acoustic (LA and TA) modes of the Pd(dmit)2 column. All the electron-phonon coupling constants are calculated from first principles. We find that largest el-intramolecular vibration coupling is to the Ag mode with the highest frequency (1449 cm-1). The el-intermolecular coupling to the LA mode is found to be larger than the total el-intramolecular couplings. We also find el-(TA)phonon coupling to be at least an order of magnitude smaller than el-(LA)phonon coupling.
Estimate of superconducting transition temperature is comparable to experimental result. We also provide a detailed discussion,
employing the results of recent numerical calculations on two-chain Hubbard model and the specific material parameters, on
the relative importance of el-ph and Coulomb-origin mechanisms of superconductivity in α
′
-TTF[Pd(dmit)2]2 and TTF[Ni(dmit)
2
]
2
.
Received 29 March 2001 and Received in final form 7 August 2001 相似文献
10.
M. Tsuchiizu P. Donohue Y. Suzumura T. Giamarchi 《The European Physical Journal B - Condensed Matter and Complex Systems》2001,19(2):185-193
We investigate the physical properties of two coupled chains of electrons, with a nearly half-filled band, as a function of
the interchain hopping t
⊥ and the doping. We show that upon doping, the system undergoes a metal-insulator transition well described by a commensurate-incommensurate
transition. By using bosonization and renormalization we determine the full phase diagram of the system, and the physical
quantities such as the charge gap. In the commensurate phase two different regions, for which the interchain hopping is relevant
and irrelevant exist, leading to a confinement-deconfinement crossover in this phase. A minimum of the charge gap is observed
for values of t
⊥ close to this crossover. At large t
⊥ the region of the commensurate phase is enhanced, compared to a single chain. At the metal-insulator transition the Luttinger
parameter takes the universal value K
ρ
* = 1, in agreement with previous results on special limits of this model.
Received 31 July 2000 相似文献
11.
T. Kautzsch W.B. Walters M. Hannawald K.-L. Kratz V.I. Mishin V.N. Fedoseyev W. Böhmer Y. Jading P. Van Duppen B. Pfeiffer A. Wöhr P. Möller I. Klöckl V. Sebastian U. Köster M. Koizumi J. Lettry H.L. Ravn the ISOLDE Collaboration 《The European Physical Journal A - Hadrons and Nuclei》2000,9(2):201-206
A chemically selective laser ion source has been used in a β-decay study of heavy Ag isotopes into even-even Cd nuclides.
Gamma-spectroscopic techniques in time-resolving event-by-event and multiscaling modes have permitted the identification of
the first 2+ and 4+ levels in 126Cd78, 128Cd80, and tentatively the 2+ state in 130Cd82. From a comparison of these new states in 48Cd with the E(2+) and E(4+)/E(2+) level systematics of 46Pd and 52Te isotopes and several recent model predictions, possible evidence for a weakening of the spherical N = 82 neutron-shell below double-magic 132Sn is obtained.
Received: 13 July 2000 / Accepted: 12 October 2000 相似文献
12.
V. Mohaček-Grošev D. Kirin 《The European Physical Journal B - Condensed Matter and Complex Systems》2001,20(1):85-90
Methyl-mercury(II) halides CH3HgX (X = Cl, Br and I) were studied by means of temperature dependent Raman spectroscopy from 10 K to 410 K. In addition to
the previously reported soft phonons, new changes in the low frequency spectra were observed at T
≈ 70 K in CH3HgBr and at T
≈ 100 K in CH3HgI. The bandwidths of the two internal modes in CH3HgBr, the CH3 symmetric stretching band and the C-Hg-Br bending band, rise towards a local maximum at T
≈ 50 K as the temperature is raised from 10 K to 300 K. On the other hand the bandwidths of the two corresponding modes in CH3HgI crystals monotonously increase with temperature, obeying an Arrhenius law. Besides the three phonon modes present in the
Raman spectra of CH3HgCl at room temperature, the fourth phonon band that has been observed at temperatures below 245 K might correspond to the
freezing of methyl librations. The huge bandwidth of the C-Hg-Br bending mode could suggest the presence of additional weak
bonding of a mercury atom with bromine atoms from other molecules, thus inducing positional disorder.
Received 19 November 1999 and Received in final form 10 November 2000 相似文献
13.
B. Pilawa I. Keilhauer G. Fischer S. Knorr J. Rahmer A. Grupp 《The European Physical Journal B - Condensed Matter and Complex Systems》2003,33(3):321-330
The magnetic properties of the cyclic compound [Fe6(bicine)6] LiClO4
. 2MeOH are reported. The cluster Fe6(bicine)6 forms an antiferromagnetically coupled ring structure of Fe III ions. The magnetic susceptibility is measured between 2 and 300 K and yields the exchange coupling of J/k
B = - 27.5±0.5 K. The field dependence of the magnetic moment is studied at 3 and 6 K in magnetic fields up to 5 T. The zero-field
splitting of the first excited spin states with S = 2 and 3 are determined by ESR at 94 GHz. The intra-molecular interactions of the Fe III ions are analyzed and the on-site anisotropy of the Fe III due to the ligand-configuration is determined to d /k
B = - 0.633±0.008K.
Received 28 October 2002 / Received in final form 22 February 2003 Published online 20 June 2003
RID="a"
ID="a"e-mail: bernd@piobelix.physik.uni-karlsruhe.de 相似文献
14.
E. Hasmonay E. Dubois S. Neveu J.-C. Bacri R. Perzynski 《The European Physical Journal B - Condensed Matter and Complex Systems》2001,21(1):19-29
A dynamic probing of magnetic liquids is performed experimentally, using a static magnetic field modulated by another smaller
field, normal and alternating. The optical magneto-birefringence under these crossed magnetic fields is recorded as a function
of the frequency for different field intensities and different sizes of the magnetic nanoparticles. A general reduced behavior
is found for the in-phase and the out-of-phase optical response which is well-described by a simple mechanical model. Depending
on the value H
ani of the anisotropy field of the nanoparticles, we can distinguish two different high magnetic field regimes: - a rigid dipole
regime (large anisotropy energy with respect to k
B
T) for cobalt ferrite nanoparticles with a relaxation time inversely proportional to the field intensity H
C(H
C < H
ani), - a soft dipole regime (anisotropy energy of the order of k
B
T) for maghemite nanoparticles with a relaxation time independent of the field intensity H
C(H
C > H
ani).
Received 5 June 2000 and Received in final form 8 January 2001 相似文献
15.
Y. Ōno R. Bulla A.C. Hewson 《The European Physical Journal B - Condensed Matter and Complex Systems》2001,19(3):375-384
The Mott metal-insulator transition in the two-band Hubbard model in infinite dimensions is studied by using the linearized
dynamical mean-field theory recently developed by Bulla and Potthoff. The phase boundary of the metal-insulator transition
is obtained analytically as a function of the on-site Coulomb interaction at the d-orbital, the charge-transfer energy between the d- and p-orbitals and the hopping integrals between p-d, d-d and p-p orbitals. The result is in good agreement with the numerical results obtained from the exact diagonalization method.
Received 5 October 2000 and Received in final form 8 December 2000 相似文献
16.
Catherine A. Kennedy 《Solid State Communications》2005,134(4):271-276
In order to investigate the relationship between negative thermal expansion and other thermal properties, the thermal conductivity of the α-phase of ZrW2O8 has been determined from 1.9 to 390 K. In addition, the heat capacity was measured from 1.9 to 300 K. The thermal conductivity of ZrW2O8 is low, glass-like and close to its theoretical minimum value. The phonon-phonon coupling of the highly anharmonic low-frequency modes which are responsible for negative thermal expansion in ZrW2O8 appears to be highly efficient, leading to short phonon mean free paths and exceptionally low thermal conductivity. 相似文献
17.
W. Boujelben A. Cheikh-Rouhou J.C. Joubert 《The European Physical Journal B - Condensed Matter and Complex Systems》2001,24(4):419-423
Deficiency effects in the A site upon the structural, magnetic and electrical properties in the lacunar perovskite manganite
oxides Pr0.7Sr0.3-x
xMnO3 ( 0 ?
x
? 0.3) and Pr0.7-x
xSr0.3MnO3 ( 0 ?
x
? 0.23) have been investigated. This study focuses on the different parameters which govern the magnetic and electrical properties
in such samples. The powder X-ray diffraction patterns for all samples could be indexed either with a rhombohedral perovskite
structure and R
c space group for x
? 0.2 in strontium deficient samples and for x
? 0.1 for praseodymium deficient ones. For other values of x the samples could be indexed in the orthorhombic structure with Pbnm space group. Magnetic and electrical investigations
show that praseodymium and strontium vacancies do not have similar effects on the lacunar compounds. Magnetization measurements
versus temperature show that all our samples exhibit a magnetic transition when the temperature decreases. All the praseodymium
deficient samples exhibit a paramagnetic-ferromagnetic transition when the temperature decreases while the strontium deficient
ones exhibit this transition only for low x values. The magnetic transition temperature shifts to lower values as the strontium deficiency increases (from 265 K for
x
= 0 to 90 K for x
= 0.3) and to higher values with the praseodymium deficiency increase (from 265 K for x
= 0 to 315 for x
= 0.23). Resistivity measurements as a function of temperature show a semiconducting-metallic transition for all x values in the praseodymium lacunar samples and only for low x values ( 0 ?
x
? 0.1) in the strontium lacunar ones when the temperature decreases.
Received 12 April 2000 and Received in final form 8 January 2001 相似文献
18.
A new and rather trivial model is suggested with mechanism that implies simultaneous violation of the zeroth and the second
laws of thermodynamics. Mathematically rigorous quantum theory reduces to a trivial application of the Golden rule formula.
It yields exciton on-energy-shell diffusion caused by bath-nonassisted excitation hopping between tails of different exciton
site levels ε1 < ε2 broadened by bath-assisted finite life-time effects. The elastic character of the hopping implies 1 ↔ 2-symmetric transfer
rate W. Thus the net diffusion exciton flow W(P
1 - P
2) and also, as argued, the net energy flow are possible due to different near-to-equilibrium exciton populations P
1 > P
2. As the sites are provided with two different baths, the population imbalance and the flows survive even for slightly different
local bath temperatures T
1 < T
2 < T
1ε2/ε1. Thus spontaneous exciton and also energy flows against temperature step become possible, in contradiction with the Clausius
form of the second law. Violations of both the laws disappear in the high-temperature, i.e. classical limit
Received 16 May 2001 and Received in final form 20 September 2001 相似文献
19.
Interplay of charge, spin, orbital and lattice correlations in colossal magnetoresistance manganites
A. Weiße H. Fehske 《The European Physical Journal B - Condensed Matter and Complex Systems》2002,30(4):487-494
We derive a realistic microscopic model for doped colossal magnetoresistance manganites, which includes the dynamics of charge,
spin, orbital and lattice degrees of freedom on a quantum mechanical level. The model respects the SU(2) spin symmetry and the full multiplet structure of the manganese ions within the cubic lattice. Concentrating on the hole
doped domain ( 0≤x≤0.5) we study the influence of the electron-lattice interaction on spin and orbital correlations by means of exact diagonalisation
techniques. We find that the lattice can cause a considerable suppression of the coupling between spin and orbital degrees
of freedom and show how changes in the magnetic correlations are reflected in dynamic phonon correlations. In addition, our
calculation gives detailed insights into orbital correlations and demonstrates the possibility of complex orbital states.
Received 4 September 2002 / Received in final form 8 November 2002 Published online 31 December 2002 相似文献
20.
It has been shown over the last few years that the dynamics close to the glass transition is strongly heterogeneous, both
by measuring the diffusion coefficient of tagged particles or by NMR studies. Recent experiments have also demonstrated that
the glass transition temperature of thin polymer films can be shifted as compared to the same polymer in the bulk. We propose
here first a thermodynamical model for van der Waals liquids, which accounts for experimental results regarding the bulk modulus
of polymer melts and the evolution of the density with temperature. This model allows us to describe the density fluctuations
in such van der Waals liquids. Then, by considering the thermally induced density fluctuations in the bulk, we propose that
the 3D glass transition is controlled by the percolation of small domains of slow dynamics, which allows to explain the heterogeneous
dynamics close to T
g. We show then that these domains percolate at a lower temperature in the quasi-2D case of thin suspended polymer films and
we calculate the corresponding glass transition temperature reduction, in quantitative agreement with experimental results
of Jones and co-workers. In the case of strongly adsorbed films, we show that the strong adsorption amounts to enhance the
slow domains percolation. This effect leads to 1) a broadening of the glass transition and 2) an increase of T
g in quantitative agreement with experimental results. For both strongly and weakly adsorbed films, the shift in T
g is given by a power law, the exponent being the inverse of that of the correlation length of 3D percolation.
Received 21 March 2000 and Received in final form 4 December 2000 相似文献