Correlation effects obtained from optical spectra of Fe-pnictides using an extended Drude-Lorentz model analysis

We introduce an analysis model, an extended Drude–Lorentz model, and apply it to Fe-pnictide systems to extract their electron–boson spectral density functions (or correlation spectra). The extended Drude–Lorentz model consists of an extended Drude mode for describing correlated charge carriers and Lorentz modes for interband transitions. The extended Drude mode can be obtained by a reverse process starting from the electron–boson spectral density function and extending to the optical self-energy and, eventually, to the optical conductivity. Using the extended Drude–Lorentz model, we obtained the electron–boson spectral density functions of K-doped BaFe₂As₂ (Ba-122) at four different doping levels. We discuss the doping-dependent properties of the electron–boson spectral density function of K-doped Ba-122. We also can include pseudogap effects in the model using this approach. Therefore, this approach is very helpful for understanding and analyzing measured optical spectra of strongly correlated electron systems, including high-temperature superconductors (cuprates and Fe-pnictides).     

Doping dependent evolution of infrared spectra in underdoped YBa2Cu3Oy in terms of two-component optical conductivity

In access to optical spectroscopy of heavily underdoped detwinned YBa₂Cu₃O_y (YBCO) crystals, we re-examine the doping dependent evolution of infrared spectra in the CuO₂ plane of underdoped YBCO in terms of two-component optical conductivity. The extended Drude model analysis is applied to the two-component conductivity, and the results are compared with experimental data in the pseudogap state. We demonstrate that a model consisting of a Drude and Lorentz oscillator components reproduces characteristics of infrared spectra in underdoped YBCO.     

Electron-phonon interaction and charge carrier mass enhancement in SrTiO3

We report a comprehensive THz, infrared and optical study of Nb-doped SrTiO3 as well as dc conductivity and Hall effect measurements. Our THz spectra at 7 K show the presence of an unusually narrow (<2 meV) Drude peak. For all carrier concentrations the Drude spectral weight shows a factor of three mass enhancement relative to the effective mass in the local density approximation, whereas the spectral weight contained in the incoherent midinfrared response indicates that the mass enhancement is at least a factor two. We find no evidence of a particularly large electron-phonon coupling that would result in small polaron formation.     

High-resolution electron energy-loss spectroscopy at epitaxially grown GaAs(100)

High-Resolution Electron Energy-Loss Spectroscopy (HREELS) is shown to be a very sensitive tool to investigate the space-charge regime of n-respectively p-type semiconductors. The most simple model we applied to fit experimental spectra is based on a step-like distribution of free carriers with the Drude dielectric response function. In this case, the dispersion of surface plasmon excitations is neglected, but it is considered in the Thomas-Fermi and the Debye-Hückel models. We use these models to fit HREELS-spectra, obtained from heavily Si-doped GaAs(100), which was grown by Molecular Beam Epitaxy (MBE). A comparison shown that the Drude model overestimates both the free-carrier concentration and the plasmon damping factor. The use of a more realistic smooth free-carrier profile, obtained by the self-consistent solution of the Schrödinger and Poisson equations, leads to plasmon excitations with lower frequencies. Besides Ohmic damping, the calculations show that Landau damping should be incorporated in order to obtain a better fit, particularly at intermediate frequencies.     

Investigation of the linear and nonlinear properties of a Drude model photonic crystal

The optical transmission properties of a one-dimensional Drude model photonic crystal are investigated. The linear wave propagation is studied by the transfer matrix method. Using a delta-function approximation a nonlinear 2-d map is obtained and used to explore the global transmission properties of nonlinear wave propagation in this system. Inclusion of a frequency-dependent refractive index represented by the Drude model results in a considerable modification of the characteristics of the linear and nonlinear wave propagation of the one-dimensional photonic crystal.     

贵金属Ag中光学和磁光性质的研究实验

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Measurements of terahertz electrical conductivity of intense laser-heated dense aluminum plasmas

We report the electrical conductivity of laser-produced warm dense aluminum plasmas measured using single-shot ultrafast terahertz (THz) frequency spectroscopy. In contrast with experiments performed at optical frequencies, measurements based upon THz probe reflectivity directly determine a quasi-dc electrical conductivity, and therefore the analysis does not require a free-electron Drude model based extrapolation to recover the near zero frequency conductivity. In fact, our experimental results indicate that the Drude model breaks down for warm (>0.6 eV), moderate-dense (<1.6 g/cm(3)) aluminum at THz frequencies. A calculation of THz reflectivity over a non-Fresnel boundary in dense plasmas is also presented.     

Reflectivity spectra of new organic metal (BEDO-TTF)5[CsHg(SCN)4]2

The polarized reflectivity and optical conductivity spectra of microcrystals of the new organic conductor (BEDO-TTF)₅[CsHg(SCN)₄]₂ based on the donor molecule bis(ethylenedioxy)tetrathiafulvalene (BEDO-TTF) have been studied in the spectral ranges 600–6500 and 9000–40000 cm^?1 at 300 K for three principal lattice directions. The optical evidence for the quasi-two-dimensional character of the conducting electronic system is obtained. The conclusion is made that the studied crystal is the quasi-two-dimensional semimetal with overlapping electron energy bands. The basic parameters of the electronic system of the crystal are determined in the framework of the Drude model. It is found that the allowed electron energy bands of the crystal are somewhat narrower than those of the previously studied structurally allied superconductor based on the same molecule. The features of vibrational structure are identified in the σ(ω) spectra for the specified three polarizations.     

Infrared investigations of the one-dimensional organic conductors (perylene)<Subscript>2</Subscript> M (mnt)<Subscript>2</Subscript>, M = Au,Pt

The optical properties of the one-dimensional organic conductor (perylene)₂Pt(mnt)₂ and its Au analogue have been investigated at ambient and low temperatures. The spectra along the stacks of the molecules show a simple Drude behavior with no detectable influence of electron-electron interactions. Basing on the spectra for different polarizations an assignment of the vibrational modes is made. Perpendicular to the stacks, a wide band observed in the mid-infrared range evidences a charge transfer between perylene and anion stacks. The electronic properties are discussed in comparison with other quasi-one-dimensional synthetic metals.     

Charge carrier interaction with a purely electronic collective mode: plasmarons and the infrared response of elemental bismuth

We present a detailed optical study of single-crystal bismuth using infrared reflectivity and ellipsometry. Large changes in the plasmon frequency are observed as a function of temperature due to charge transfer between hole and electron Fermi pockets. In the optical conductivity, an anomalous temperature dependent midinfrared absorption feature is observed. An extended Drude model analysis reveals that it can be connected to a sharp upturn in the scattering rate, the frequency of which exactly tracks the temperature dependent plasmon frequency. We interpret this absorption and increased scattering as direct optical evidence for a charge carrier interaction with a collective mode of purely electronic origin, here electron-plasmon scattering. The observation of a plasmaron as such is made possible only by the unique coincidence of various energy scales and exceptional properties of semimetal bismuth.     

Optical properties of new organic conductors based on the BEDT-TSeF molecule (the κ-(BETS)4Hg2.84Br8 superconductor and κ-(BETS)4Hg3Cl8 Metal) in the range 300–15 K

Polarized reflectance and optical conductivity spectra of single crystals of two new isostructural organic conductors based on the BEDT-TSeF molecule, namely, the κ-(BETS)₄Hg_2.84Br₈ superconductor (T _c =2 K) and the κ-(BETS)₄Hg₃Cl₈ metal, which undergoes a smooth transition to the dielectric state near 35 K, have been obtained in the spectral region 700–6500 cm⁻¹ at temperatures of 300–15 K. At 300 K, the spectra of both compounds are nearly identical and differ from the Drude spectrum characteristic of metals. The nature of the observed difference is discussed, and the spectra are described in terms of a cluster approach with inclusion of electron-electron correlations in the Hubbard approximation combined with the Drude model. The parameters of the theory were determined, including the electron transfer integrals between molecules in a cluster. The spectra in the conducting plane of the crystals were found to be essentially anisotropic, which should be assigned to specific features of in-plane interaction between molecules. The spectra of the superconductor and the metal become increasingly different as the temperature is lowered. The spectra of the metal obtained for T<150 K exhibit splitting of the broad electronic maximum in the mid-IR region into two bands, which is accompanied by a splitting of a vibronic feature deriving from electron interaction with intramolecular BETS vibrations of ν₃(A _g ) symmetry. No such splitting is observed in the superconductor spectra with decreasing temperature. __________ Translated from Fizika Tverdogo Tela, Vol. 46, No. 11, 2004, pp. 1921–1929. Original Russian Text Copyright ? 2004 by Vlasova, Drichko, Petrov, Semkin, Zhilyaeva, Lyubovskaya, Olejniczak, A. Kobayashi, H. Kobayashi.     

Ultrafast deflection of spatial solitons in AlxGa(1-x)As slab waveguides

We demonstrate ultrafast all-optical deflection of spatial solitons in an AlxGa(1-x)As slab waveguide, using 190 fs, 1550 nm pulses to generate and deflect the spatial soliton. The steering beam is focused onto the top of the waveguide near the soliton pathway, and the soliton is steered by refractive-index changes induced by optical Kerr, or free-carrier (Drude), effects. Angular deflections up to 8 mrad are observed.     

Nonequilibrium phase change in gold films induced by ultrafast laser heating

Ultrafast laser-induced melting in a gold thin film is simulated by an integrated continuum-atomistic method with the extended Drude model for dynamic optical properties. The local order parameter of atoms is used to identify solid and liquid regions. It is shown that the film is superheated in the early nonequilibrium stage and the melted region grows very quickly with a very high rate of melting up to ～13,300 m/s. It is also found that the continuum approach could significantly underestimate the ultrafast phase-change response, and temperature-dependent optical properties should be considered in atomic-level modeling for ultrafast laser heating.     

Incoherent c-axis interplane response of the iron chalcogenide FeTe(0.55)Se(0.45) superconductor from infrared spectroscopy

We report on the interplane c-axis electronic response of FeTe(0.55)Se(0.45) investigated by infrared spectroscopy. We find that the normal-state c-axis electronic response of FeTe(0.55)Se(0.45) is incoherent and bears significant similarities to those of mildly underdoped cuprates. The c-axis optical conductivity σ(c)(ω) of FeTe(0.55)Se(0.45) does not display well-defined Drude response at all temperatures. As temperature decreases, σ(c)(ω) is continuously suppressed. The incoherent c-axis response is found to be related to the strong dissipation in the ab-plane transport: a pattern that holds true for various correlated materials as well as FeTe(0.55)Se(0.45).     

Coherent heavy quasiparticles in a CePt5 surface alloy

We report on the results of a high-resolution angle-resolved photoemission study on the ordered surface alloy CePt(5). The temperature dependence of the spectra show the formation of the coherent low-energy heavy-fermion band near the Fermi level. These experimental data are supported by a multiband model calculation in the framework of the dynamical mean-field theory.     

Optical reflectivity of (SN)x-single crystals

The optical reflectivity of (SN)_x single crystals was measured in the visible region and the near infrared with light polarized parallel and perpendicular to the polymer chain axis. Whereas the reflectivity for light polarized perpendicular to the chain axis is approximately constant in this region, the reflectance for light polarized parallel to the chain axis exhibits a pronounced plasma edge at 2.72 eV. A simple Drude model was used to analyse the data. Differences between these results and those of previous film measurements are discussed.     

金属薄膜亚波长近场成像特性研究

采用基于等离子体物理模型的时域有限差分方法模拟了金属薄膜近场成像特性;采用薄膜传输矩阵方法计算了金属薄膜对倏逝波分量的放大作用.实现了周期为1μm的Cr光栅的成像实验,验证了平板金属薄膜的模拟成像特性. 关键词： 时域有限差分 金属薄膜 近场亚波长成像 传输矩阵方法     

大孔径空间外差干涉光谱成像技术多谱段成像仿真

在大孔径空间外差干涉光谱成像技术（LASHIS）的基础上提出了一种多谱段成像方案.其采用LASHIS的外差探测原理,一方面,可通过较少的采样点数实现很高的光谱分辨率,保留了LASHIS的高光谱分辨率、高稳定性和高探测灵敏度的特点;另一方面,利用光栅的多级衍射性质,实现同一系统的多谱段同时探测,拓宽了光谱探测范围.首先,阐述了LASHIS多谱段成像方案的基本原理;然后,分析了多谱段探测与谱段解混方式;最后,对该方案进行了计算机仿真模拟,通过ZEMAX光线追迹的干涉图结果与理论计算结果相符合,验证了方案的正确性.基于LASHIS的多谱段成像方案所具有的高光谱分辨率、高探测灵敏度以及可实现同一系统的多谱段同时探测特点,尤其适合温室气体等高稳定性、高探测灵敏度的多谱段高光谱探测应用.     

Optical investigations of polycrystalline Mg1−xB2 near metal-insulator transition

We measured reflectivity spectra of polycrystalline Mg_1−xB₂ samples, which show a metal-insulator transition with x. After performing the Kramers-Kronig analysis, the obtained optical conductivity spectra σ(ω) of MgB₂ show a narrow Drude peak in the far-infrared region and a broad peak in the mid-infrared region. As x increases, the spectral weight of the Drude peak is strongly suppressed and that of the broad peak becomes enhanced a little. The existence of the broad mid-infrared peak in the insulating sample suggests that this peak might not be related to the free carriers in MgB₂. In the far-infrared region, we also observe that the low energy dielectric constant of Mg_1−xB₂ diverges near the metal-insulator phase boundary (i.e. x=0.08). This result implies the possibility of a phase separation and a percolative metal-insulator transition in Mg_1−xB₂.