Modeling of UV pulsed-laser ablation of metallic targets

A model to describe the laser ablation of metallic targets is presented. It accounts for the main physical processes involved in the laser–solid–plasma interaction by considering the photon absorption and the ionization mechanisms that are active in the plasma, as well as the laser-produced plasma kinetics. The model is used to simulate the laser ablation of aluminum targets irradiated with a 6-ns UV laser pulse at 0.35 μm, and the results are compared with experimental findings. Calculations show that all the investigated plasma parameters strongly depend on the laser intensity until a roll-off is reached at irradiance ≥1.5 GW cm^-2. The satisfactorily good agreement between model predictions and experimental findings confirms that laser–plasma interaction processes and plasma kinetics play a relevant role during nanosecond laser ablation of metals in the laser intensity range of concern in this study. Received: 12 February 1999 / Accepted: 12 April 1999 / Published online: 7 July 1999     

Compact X-ray radiograph based on a plasma gun

The results of the experiments on the formation of a plasma emitter with small spatial dimensions for pulsed radiography in the soft X-ray spectral range are presented. Emitting hot plasma was formed as a result of compression of the plasma jet by a current pulse with amplitude I _m = 215 kA and rise time T _fr = 200 ns. For the jet formation, we used a plasma gun based on the arc discharge (I _m = 8.5 kA and T _fr = 6 μs) initiated by breakdown over the surface of a dielectric in vacuum. The experiments were carried out with aluminum, tin, copper, and iron plasma jets. A single emitter, i.e., point Z-pinch (PZ-pinch), was formed when an interelectrode gap of a high current generator of 1.3–1.5 mm was used. The smallest spatial dimensions of the emitting region were obtained with the use of aluminum and tin. For a tin jet, the diameter of the emitting region was 7 ± 2 μm and its height was 17 ± 2 μm. The emission pulse duration at half-height was 2–3 ns. The total emission yield per pulse in the spectral range 1.56–1.90 keV was 30–50 mJ for the aluminum pinch and 10–30 mJ for the tin pinch. The developed method makes it possible to carry out radiographic examination of microobjects (including biological ones) 1–1000 μm in thickness, with spatial (10–20 μm) and time (2–3 ns) resolution.     

Investigation of the turbulent mixing of thin layers of materials of different density during the laser acceleration of flat multilayer targets in the Iskra-4 facility

The results of the first experiments devised to investigate the mixing of thin layers of Al and Au during the laser acceleration of flat three-layer targets of Si (5 μm), Al (2 μm), and Au (0.05–0.26 μm) by radiation converted to the second harmonic from the Iskra-4 iodine laser with an intensity of 4×10¹³−7×10¹³ W/cm² (τ _0.5∼1 ns), which acts on the Si side of the target. A method for detecting the occurrence of mixing is developed. It is established that under the experimental conditions the thickness of the mixing region is at least ∼0.15 μm. The results of a theoretical analysis of the evolution of the disturbances leading to mixing are presented. Zh. éksp. Teor. Fiz. 111, 882–888 (March 1997) Deceased.     

Dynamics of plasma formation during quasicontinuous laser irradiation of metals in high-pressure nitrogen atmospheres

This is a study of target destruction and the dynamics of surface plasma formation during the interaction of quasicontinuous laser radiation (λ = 1.06 μm, q = 1–7 MW/cm², τ ∼ 1.5 msec) with D16T duraluminum and bismuth in nitrogen atmospheres at pressures p = 1–20 atm. High speed photography and spectroscopy of the erosion plasma flare are used to determine the onset time for vaporization of the target, as well as the times of appearance of erosion and nitrogen plasmas for different gas pressures and laser energy fluxes q. The emergence of the plasma front from the vapor zone into the surrounding nitrogen is detected experimentally and the properties of the nitrogen plasma are studied.     

Anomalous burn-through of thin foils by high-intensity laser radiation

The paper presents results of experiments performed on the Pico facility in which foils were heated by laser radiation, and anomalously fast burn-through of foils by a structured laser beam was detected. Comparison with two-dimensional calculations has allowed us to suggest a tentative mechanism for the effect under investigation. The targets in the experiments were thin aluminum foils of thickness 3 to 40 μm. The flux density of laser radiation on the target surface varied between 10¹³ and 10¹⁴ W/cm². We detected a strong dependence of the transmitted energy on the foil thickness and the shortening of the transmitted laser pulse. Penetration of laser radiation through foils with thicknesses considerably larger than 3 μm has been observed, although it was stated in earlier publications [V. V. Ivanov, A. K. Knyazev, A. V. Kutsenko, et al., Kratk. Soobshch. Fiz. FIAN No. 7–8, 37 (1997)]; A. é. Bugrov, I. N. Burdonskii, V. V. Gol’tsov et al., Zh. éksp. Teor. Fiz. 111, 903 (1997) [JETP 84, 903 (1997)] that, at the laser radiation parameters used in our experiment, the evaporated layer of the foil could not be thicker than 2 μm. Two-dimensional calculations have allowed us to interpret this effect in terms of local “piercing” of the target at spots on the target surface where the radiation intensity has its peaks. The possibility of reducing these peaks by using a symmetrizing prepulse is discussed in the paper. Zh. éksp. Teor. Fiz. 116, 1287–1299 (October 1999)     

Femtosecond fiber laser based methane optical clock

An optical clock based on an Er³⁺ fiber femtosecond laser and a two-mode He–Ne/CH₄ optical frequency standard (λ=3.39 μm) is realized. Difference-frequency generation is used to down convert the 1.5-μm frequency comb of the Er³⁺ femtosecond laser to the 3.4-μm range. The generated infrared comb overlaps with the He–Ne/CH₄ laser wavelength and does not depend on the carrier–envelope offset frequency of the 1.5-μm comb. In this way a direct phase-coherent connection between the optical frequency of the He–Ne/CH₄ standard and the radio frequency pulse repetition rate of the fiber laser is established. The stability of the optical clock is measured against a commercial hydrogen maser. The measured relative instability is 1×10⁻¹² at 1 s and for averaging times less than 50 s it is determined by the microwave standard, while for longer times a drift of the He–Ne/CH₄ optical standard is dominant.     

The Muonic Hydrogen Lamb Shift Experiment at PSI

A measurement of the 2S Lamb shift in muonic hydrogen (μ⁻p) is being prepared at the Paul Scherrer Institute (PSI). The goal of the experiment is to measure the energy difference ΔE(2⁵ P _3/2−2³ S _1/2) by laser spectroscopy (λ≈6μm) to a precision of 30 ppm and to deduce the root mean square (rms) proton charge radius with 10⁻³ relative accuracy, 20 times more precise than presently known. An important prerequisite to this experiment is the availability of long-lived μp_2S -atoms. A 2S-lifetime of ∼1 μs – sufficiently long to perform the laser experiment – at H₂ gas pressures of 1–2 hPa was deduced from recent measurements of the collisional 2S-quenching rate. A new low-energy negative muon beam yields an order of magnitude more muon stops in a small low-density gas volume than a conventional cloud muon beam. A stack of ultra-thin carbon foils is the key element of a fast detector for keV-muons. The development of a 2 keV X-ray detector and a 3-stage laser system providing 0.5 mJ laser pulses at 6 μm is on the way. This revised version was published online in August 2006 with corrections to the Cover Date.     

Characterization of compact bright soft X-ray source based on picosecond laser plasma

Radiation emission of silicon and aluminum plasmas produced by 40-ps laser pulses with peak intensity above 10¹⁴ W/cm² was studied. High-resolution soft X-rayspectra of H-like and He-like ions were analyzed to determine plasma parameters. We compared the line shape of resonance transitions and their intensity ratios to corresponding dielectronic satellites and the intensities of the intercombination lines of He-like ions with the results of model calculations. Such comparisons gave average values of the electron number density N_e=(1-1.9)×10²¹ cm^-3 and the electron temperature T_e=460–560 eV for Si plasmas and about 560 eV for Al plasmas produced by the first and the second laser harmonics. The plasma size is about 100 μm. According to our estimations, more than 10¹² photons were produced within the resonance line spectral width and in the solid angle 2π during the total decay period. PACS 41.50.+h; 52.25.Os; 52.50.Jm     

Near IR laser light visualizators using nonlinear GaSe and other layered crystallites

Two methods of preparation of the devices for visualization of pulsed and continuous near-IR (near infrared) are described and the results of conversion of pulsed and continuous IR (800–1360 nm) laser radiation into the visible range of spectra (400–680 nm) by using a transparent substrate covered with the particles (including nanoparticles) of effective nonlinear materials of GaSe _x S_{1 − x} (0.2 ≤ x ≤ 0.8) are presented. Converted light can be detected in transmission or reflection geometry as a visible spot corresponding to the real size of the incident laser beam. Developed device structures can be used for checking if the laser is working or not, for optical adjustment, for visualization of distribution of laser radiation over the cross of the beam and for investigation of the content of the laser radiation. Low energy (power density) limit for visualization of the IR laser pulses with 2–3 ps duration for these device structures are: between 4.6–2.1 μJ (3 × 10⁻⁴−1 × 10⁻⁴ W/cm²) at 1200 nm; between 8.4–2.6 μJ (4.7 × 10⁻⁴−1.5 × 10⁻⁴ W/cm²) at 1300 nm; between 14.4–8.1 μJ (8.2 × 10⁻⁴–4.6 × 10⁻⁴ W/cm²) at 1360 nm. Threshold damage density is more than 10 MW/cm² at λ = 1060 nm, pulse duration τ = 35 ps. The results are compared with commercially existing laser light visualizators.     

Formation of a plane layer of plasma under irradiation by a soft X-ray source

We investigate theoretically the formation of a plasma in a plane layer of polymer foam (density ρ = 0.002 g/cm³ and thickness 800 μm) under the action of an external source of soft X-ray radiation under the conditions of PHELIX experiments. The incident flux is assumed to have a Planck’s distribution over the spectrum with T _rad = 20–40 eV. In numerical calculations, the flux of incident X-ray radiation and the spectral constants of the target substance are varied. The action of an external X-ray radiation source on a low-density foam substance with a density of 2 mg/cm³ causes a plasma to be formed with relatively homogeneous profiles of density and temperature T = 15–35 eV. Absorption of externalradiation energy is distributed in the volume. The plasma temperature increases with increase in the external energy, and the energy passed through the plasma also increases. The results prove to be sensitive to the values of optical constants used in numeral simulation. The spectral flux of external radiation passed through the plasma is chosen as a criterion of correctness of the optical constants used in the calculations. In future experiments using the PHELIX facility, we plan to investigate the slowing-down of an ion beam in a plasma formed as a result of indirect heating of low-density polymer triacetate cellulose (TAC) foam with densities ρ = 0.001–0.01 g/cm³ under the action of a pulse of X-ray radiation, into which the laser radiation is preliminarily transformed.     

Calculation of the parameters of excimer light sources on the basis of a positive column glow discharge

We calculate the concentration of plasma and gas-temperature components in a contracted filament of a glow capillary discharge (R = 0.75 mm) in xenon for pressures of P = 100 and 400 Torr and currents of I = 6–15 mA for cases of with and without cryogenic cooling of the discharge. We find that the gas temperature in the channel of the glow discharge has a value of 1000–2000 K, the concentration of xenon excimers attains a maximum at the boundary of the filament with a value of 10¹⁰–10¹¹ cm⁻³, and the efficiency of electric energy transformation into excimer radiation energy has a value of 0.1–5%.     

Crystallization of a dusty plasma in the positive column of a glow discharge

The formation of macroscopic ordered structures in the standing striations of a stationary glow discharge in Ne is observed. A Coulomb quasicrystal is formed by spherical glass particles with diameters of 50–63 μm and charge Z _p~7·10⁵ e. The interparticle distance is approximately 300 μm. This corresponds to a nonideality parameter Γ~5·10⁴, which leads to crystallization in the Yukawa model. The factors leading to the formation of a quasicrystal in the striations are discussed. Pis’ma Zh. éksp. Teor. Fiz. 64, No. 2, 86–91 (25 July 1996)     

<Emphasis Type="Italic">K</Emphasis><Subscript>α</Subscript> radiation of foil under interaction with laser pulse of relativistic intensity

An analytical model of K _α radiation of thin laser targets has been developed. It has been shown that, for such targets, the motion of fast electrons is significant not only in the target itself but also in vacuum. The considered dependences for the free path length of a fast electron and for the absorption coefficient of laser radiation on the laser intensity with allowance for the electron motion in vacuum make it possible to match the results of the proposed model with the experimental data on generation of K _α radiation in wide ranges of laser intensities (10¹⁸–10²¹ W/cm²) and thicknesses (1–100 μm) of targets.     

Laser radiation tunable within the range of 4.35–5.45 <Emphasis Type="Italic">μ</Emphasis>m in a ZnTe crystal doped with Fe<Superscript>2+</Superscript> ions

We realized laser generation on a Fe²⁺:ZnTe crystal for first time. The crystal was pumped at room temperature by 40 ns pulses of an Er:YAG laser operating at a wavelength of 2.94 μm in the Q-switching mode. The output energy of the Fe²⁺:ZnTe laser was 0.18 mJ at a slope efficiency of 2.4% with respect to absorbed pumping energy. We achieved tuning of the Fe²⁺:ZnTe laser generation wavelength within the range of 4.35–5.45 μm using a prism-dispersion cavity.     

Physical processes in a laser-greenhouse target: Experimental results, theoretical models, and numerical calculations

The paper is devoted to recent results concerning investigation of physical processes occurring in a “laser greenhouse” target. Results of experimental and theoretical studies of laser-pulse interaction with a low-density absorber of the target, namely, with a porous substance having density close to the plasma critical density, are presented. On the basis of a vast cycle of experiments carried out in a number of laboratories, it is shown that the absorption of the laser radiation in porous media, including those with a density exceeding the critical one by at least a factor of 4 to 6, has a bulk nature and is distributed over the target depth. In particular, the laser-radiation absorption region in a porous substance with density 10⁻³–10⁻² g/cm³ is extended into the target 400–100 μm, respectively. The coefficient of absorption of laser radiation with intensity 10¹⁴–10¹⁵ W/cm² in porous substances, including those of the supercritical density, is 70–90%. Experiments have not shown enhanced (compared to a solid-state target) radiation intensity associated with a possible development of parametric instabilities in an extended laser plasma of low-density porous media, as well as noticeable contribution of fast electrons to the energy balance and their effect on the energy transfer. In this paper, theoretical models are developed explaining features of the laser-radiation absorption and energy transfer in porous media. These models are based on the phenomenon of laser-radiation interaction with solid components of a porous substance and plasma production inside pores and cells of the medium. The efficiency of energy conversion in the vicinity of the ignition threshold for the laser-greenhouse target is investigated in the case of an absorber having the above properties. Numerical calculations have shown that a thermonuclear-gain coefficient of 1 to 2 (with respect to the energy absorbed) is attained for a laser-radiation energy of 100 kJ. Translated from Preprint No. 58 of the P. N. Lebedev Physical Institute, Moscow (1999).     

Laser-induced cavities and solitons in overcritical hydrogen plasma

A picosecond CO₂ laser was used successfully in a number of experiments exploring advanced methods of particle acceleration [1]. Proton acceleration from gas-jet plasma exemplifies another advantage of employing the increase in laser wavelength from the optical to the mid-IR region. Recent theoretical- and experimental-studies of ion acceleration from laser-generated plasma point to better ways to control the ion beam’s energy when plasma approaches the critical density. Studying this regime with solid-state lasers is problematic due to the dearth of plasma sources at the critical electron density ∼10²¹ cm⁻³, corresponding to laser wavelength λ = 1 μm. CO₂ laser offers a solution. The CO₂ laser’s 10 μm wavelength shifts the critical plasma density to 10¹⁹ cm⁻³, a value attainable with gas jets. Capitalizing on this approach, we focused a circular polarized 1-TW CO₂ laser beam onto a hydrogen gas jet and observed a monoenergetic proton beam in the 1–2 MeV range. Simultaneously, we optically probed the laser/plasma interaction region with visible light, revealing holes bored by radiation pressure, as well as quasi-stationary soliton-like plasma formations. Our findings from 2D PIC simulations agree with experimental results and aid in their interpretation.     

Optical absorption in early stage low temperature laser produced plasma

We describe a new technique to measure the UV/visible absorption spectrum of the ablated material during the laser pulse. The technique utilizes the continuum emission from one laser produced plasma as a light source to measure the absorption properties of a second laser produced plasma which is formed on a semi-transparent target with an array of 40 μm holes. A 6 ns, 1064 nm laser was used to ablate a Ag target and the plasma absorption was measured in the range 450–625 nm for a laser fluence of 1 J cm⁻². The total absorption cross-section is (0.5–1.5)×10⁻¹⁷ cm² in the range 450–540 nm. By comparing the measured absorption with a calculation using the plasma spectroscopy code FLYCHK it can be concluded that, in the wavelength region examined here, the absorption is mainly due to bound-bound transitions.     

Shaping dynamics and structure of large-scale surface plasma formations under single-pulse laser action on various materials

It is established that, in the case of laser action on materials in large illuminated spots in atmospheric-pressure air for a laser radiation power density q≤2 MW/cm² (λ=1.315 μm), an evaporative regime with plane scattering of the laser-produced erosion plasma is realized while, for q≈5–17 MW/cm², the plasma front is transferred to the air, leading to plasma screening of the target and shaping of a subsonic radiation wave in the air. As the duration of the laser pulses increases (τ∼160 μsec), in spite of the large illuminated spots (S∼150 cm²) the evaporative regime of the laser action with plane plasma scattering goes over into a regime with jet outlow and formation of a quasistationary shock wave. Deceased. Institute of Molecular and Atomic Physics, National Academy of Sciences of Belarus, 70, F. Skorina Ave., Minsk, 220072, Belarus. Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 65, No. 2, pp. 261–268, March–April, 1998.     

Stepwise synthesis of fine crystalline Ce-doped yttrium aluminum garnet in water medium in subcritical and supercritical conditions

In this paper the continuous stepwise method of a production of fine crystalline yttrium aluminum garnet doped with cerium (YAG: Ce³⁺) in supercritical water fluid (SCWF) are represented. The synthesis was carried out in water medium in two stages: first in subcritical conditions and then in an atmosphere of supercritical water fluid. The stoichiometric mixture of yttrium oxide and aluminum hydroxide in a water solution of cerium nitrate was maintained the certain time at 280°C and under vapor water pressure 6.3 MPa. Then temperature and pressure were risen up to a supercritical condition (T = 392–400°C, P_{H2 O}P_{H_2 O} = 22 MPa). The concentration of cerium ions in reaction medium was changed in the interval 0.012–0.706 wt %. The products, obtained on various stages of synthesis, were investigated by physical-chemical methods. During the first stage, the crystals of boehmite and yttrium hydroxide under hydrothermal conditions were arising, and eventually poorly formed YAG: Ce³⁺ were appearing. At this stage, the diffusion of cerium ions into intermediate products takes place. Because of this, at the second step of synthesis, in supercritical conditions, YAG: Ce³⁺, phosphor with high luminescence intensity at 530 nm, was obtained. In supercritical conditions well-faceted crystals of 0.5–3.0 μm with rhombododecahedral habitus were produced.