Lasing of middle-infrared free-election lasers using the storage ring NIJI-IV

We report for the first time to our knowledge the experimental realization of a storage ring free-electron laser (FEL) in the middle-infrared (MIR) region. A technique to adjust the optical cavity using higher harmonic FELs was developed for a fundamental FEL in the MIR region. The MIR FELs were oscillated in the wavelength region of 2475 to 2673 nm, and the relative linewidth was 5×10??. A quasi-monochromatic x-ray beam with an energy of 700 keV was generated using FEL Compton backscattering. We were able to realize a quasi-monochromatic x-ray beam, whose energy is difficult to generate even in advanced synchrotron radiation facilities.     

Cavity-enhanced absorption spectroscopy for shocktubes: Design and optimization

Cavity-enhanced absorption spectroscopy (CEAS) has generated much interest in shocktube kinetics studies because of its recent success in achieving improved sensitivity and high time resolution with robust optical alignment. While recent progress demonstrated experimental schemes including off-axis scanned-wavelength approach and on-axis ps-pulsed laser approach, that both successfully suppressed the laser-cavity coupling noise, this paper develops a theoretical model to predict the CEAS sensor performance that can be used as a design tool applicable to more generalized cases. The method models the optical field in the cavity based on the decentered Gaussian beam model, from which the cavity transmission spectrum and the laser-cavity coupling noise can be numerically calculated. The simulation results predict sensor performance for different cavity configurations and laser characteristics, including various degrees of laser-cavity mode-matching, laser linewidths, scanning rates, and cavity filling conditions. Simulation with example wavelengths in the ultraviolet, near-infrared, and mid-infrared showed increasing mode-matched beam waist size for increasing wavelengths. An off-axis alignment scheme was found to be capable of suppressing the coupling noise by two orders-of-magnitude at a moderate laser linewidth of 1?GHz. Coupling noise level on the order of 1e-5 for scanned-wavelength off-axis alignment case with a narrowband mid-infrared laser was obtained by model calculation and agreed with experimental results within acceptable uncertainty range. The developed method can serve to guide future design and optimization of CEAS system in shocktube studies.     

基于频域近红外光谱法的生物组织光学参数的检测与三维重构

生物组织的光学特性参数与组织的各种生理、生化以及病理过程密切相关。光学特性参数的检测与三维重构可以在一定程度上了解组织的内部结构及特性。基于频域近红外光谱法,使用美国ISS公司的频域近红外光谱检测系统,采用多光源多检测器技术,将830 nm的激光经过调制后,照射进放置了具有一定吸收系数和散射系数的异质体小球的牛奶中,检测出射光的光强和相位,然后应用光学扩散层析成像技术,通过计算含有异质体小球的牛奶的光学参数,重构出了牛奶中异质体的具体位置。实验结果表明,利用频域近红外光谱法得到的出射光的光强和相位信息,能够较准确地计算出牛奶及异质体小球的吸收系数和散射系数等组织光学参数,并可进一步定位出牛奶中异质体小球的位置。因此,可以考虑将该方法应用在分析及定位水果病变等农产品品质检测领域。     

吲哚菁绿对大鼠脑皮层血管近红外光学特性及光学相干层析成像的影响

研究观察了吲哚菁绿(ICG)对大鼠脑皮层血管近红外光谱学特性及光学相干层析成像(OCT)的影响。实验中,将SD大鼠颞部开颅,暴露并标记大脑中动脉,给予动物尾静脉注射ICG溶液,应用可见-近红外反射光谱仪和OCT系统检测脑皮层血管反射光谱的动态变化和衰减系数的特征性变化。结果显示,ICG注射后,大脑中动脉的反射光谱在ICG的吸收峰(800nm)左右出现一个特异性的低反射峰并随时间而逐渐变化;在注射ICG 3min时,本特异性低反射峰值达到最强,反射光谱的特征性变化可以为实现最佳OCT图像效果提供时间点。此外,ICG注射后的脑动脉OCT信号衰减系数为24.692±1.471,明显高于未注射ICG时15.088±1.602(p<0.01)。实验结果说明ICG可以增加血管对近红外光的吸收,为增强血管的检测能力提供理论参考,也为无损监测血管病变、肿瘤血管新生及血液动力学变化提供一种可行性检测手段。     

Fiber-optic ring-down spectroscopy using a tunable picosecond gain-switched diode laser

Visible and near-infrared laser light pulses were coupled into two different types of optical fiber cavities. One cavity consisted of a short strand of fiber waveguide that contained two identical fiber Bragg gratings. Another cavity was made using a loop of optical fiber. In either cavity ∼40 ps laser pulses, which were generated using a custom-built gain-switched diode laser, circulated for a large number of round trips. The optical loss of either cavity was determined from the ring-down times. Cavity ring-down spectroscopy was performed on 200 pL volumes of liquid samples that were injected into the cavities using a 100 μm gap in the fiber loop. A detection limit of 20 ppm of methylene blue dye in aqueous solution, corresponding to a minimum absorptivity of εC<6 cm^-1, was realized. PACS 42.62.Fi; 42.81.-i     

Electronic and optical properties of van der Waals vertical heterostructures based on two-dimensional transition metal dichalcogenides: First-principles calculations

Four vertical heterostructures based on two-dimensional transition-metal dichalcogenides (TMDs) – MoS₂/GeC, MoSe₂/GeC, WS₂/GeC, and WSe₂/GeC, were studied by density functional theory calculations to investigate their structure, electronic characteristics, principle of photogenerated electron–hole separation, and optical-absorption capability. The optimized heterostructures were formed by van der Waals (vdW) forces and without covalent bonding. Their most stable geometric configurations and band structures display type-II band alignment, which allows them to spontaneously separate photogenerated electrons and holes. The charge difference and built-in electric field across the interface of these vdW heterostructures also contribute to preventing the photogenerated electron–hole recombination. Finally, the high optical absorption of the four TMD-based vdW heterostructures in the visible and near-infrared regions indicates their suitability for photocatalytic, photovoltaic, and optical devices.     

Thermally tunable optical constants of vanadium dioxide thin films measured by spectroscopic ellipsometry

Smart materials with reversible tunable optical constants from visible to near-infrared wavelengths could enable excellent control over the resonant response in metamaterials, tunable plasmonic nanostructures, optical memory based on phase transition and thermally tunable optical devices. Vanadium dioxide (VO₂) is a promising candidate that exhibits a dramatic change in its complex refraction index or complex dielectric function arising from a structural phase transition from semiconductor to metal at a critical temperature of 70 °C. We demonstrated the thermal controllable reversible tunability of optical constants of VO₂ thin films. The optical/dielectric constants showed an abrupt thermal hysteresis which confirms clearly the electronic structural changes. Temperature dependence of dielectric constants as well as optical conductivity of sputtered VO₂ thin films was also reported and compared to previous theoretical and experimental reports.     

Controllable optical bistability and multistability in a rare-earth-ion-doped optical fiber

We investigated the optical bistability and multistability in an Er³⁺-doped ZrF₄–BaF₂–LaF₃–AlF₃–NaF optical fiber inside an optical ring cavity. It is found that the optical bistability and multistability can be easily controlled via adjusting properly the parameters of the corresponding system. Our scheme may provide some new possibilities for technological applications in optoelectronics and optical-fiber communication.     

Design of integrated optical circulator based on photonic crystals

Photonic crystals containing defects produce enhanced Faraday rotation. They have opened up the possibility of fabricating very compact magneto-optics structures. In this work, we have designed a two-dimensional photonic crystal waveguide for use in optical packaging and integrated optical circuits. For design purposes, a temporal coupled mode theory was utilized at the first step. It examined the coupling between cavity and optical ports. After acquiring a general solution, it would be applied to specific problem in hand. Then, optical characteristics of photonic crystal were investigated to design the practical parts such as cavity and waveguides which eventually a triangular crystal lattice of air holes in Bi:YIG (BIG) was considered to be the best candidate. Finally, the results of analytical investigations were evaluated using OptiFDTD software and then were confirmed.     

相干谐波储存环自由电子激光

相干谐波自由电子激光不用光学谐振腔及反射镜,可望工作在紫外和真空紫外光波段,是第四代同步辐射光源的可能途径之一。由于对束流品质要求很高,相干谐波自由电子激光首先是以储存环作为驱动器而发展起来的。由于光阴极微波电子枪的发展和直线加速器技术的进步,目前,已开始有直线加速器驱动的高增益相干谐波自由电子激光的建议。文章介绍了相干谐波储存环自由电子激光的原理、现状及展望。     

微型化光纤法布里-珀罗传感器腔长一致性的控制研究

研究了光纤法布里-珀罗腔传感器的腔长一致性的控制技术.通过三维调整架组成微调装置来控制全光纤法布里-珀罗腔的腔长;结合法布里-珀罗腔的工作原理,利用光谱分析仪实时检测加工过程中法布里-珀罗腔的腔长并用装置予以修正;以热熔接的方法将毛细玻璃管与光纤加工成法布里-珀罗腔;利用超景深光学显微系统检查加工的法布里-珀罗腔的关键部位的结构,并对熔接点的牢固性进行了检测.实验结果和数据分析显示:法布里-珀罗腔的腔长得到了较好的控制及一致性,熔接部位的变形和对法布里-珀罗腔的性能的影响也很小.该工艺可用于制备全光纤法布里-珀罗腔传感器.     

Demonstration for a two-axis interferometric tilt sensor in KAGRA

Recently, a folded Mach–Zehnder interferometer with homodyne in- and quadrature-phase detection was proposed as a high-precision, wide-dynamic range tilt sensor. By way of a practical application and to validate actual performance, two-axis tilt sensors were developed and installed for one mirror of the input mode cleaner cavity in KAGRA, the large-scale cryogenic gravitational-wave telescope in Kamioka, Gifu, Japan. Building on previous work, we have demonstrated that the two-axis tilt sensor has properly sensed the tilt angle changes of the mirror motion with high precision and without calibration. Compared with our initial angular sensor, an optical lever, which is calibrated by using the interferometer tilt sensor, we found that both sensors showed actual tilt motions of the mirror at low frequencies, and the two-axis interferometer sensor has a better sensitivity at higher frequencies.     

AlxGa1-xAs/AlyGa1-yAs微腔中的激子吸收增强效应

文章采用Al_xGa_1-xAs/Al_yGa_1-yAs微腔结构,研究了微腔中激子的吸收行为,在室温下观察到了激子吸收的增强效应,激子的峰值吸收强度是自由空间中激子吸收强度的2,6倍;我们从激子与光波场相互作用和腔中模函数的分布建立了计算.激子先吸收的模型,文中给出的微腔结构的数值计算表明激子的吸收增强与实验结果相一致;数值计算表明,微腔中激子吸收的强弱不仅与上、下两腔镜的反射率和腔长有关,而且还取决于量子阱在腔中的位置.     

Quasi-linear theory of multimode free-electron lasers with an inhomogeneous frequency broadening

assuming that the number of excited modes is large and their phases are random a quasi-linear theory of interaction of ultrarelativistic electron beam with the field of a high-quality cavity is developed. The saturation effects in FELs with an inhomogeneous frequency broadening are described. It is shown that in the case of very large excesses over threshold the efficiency of FELs tends to 50% but the emitted energy is distributed in a very wide spectral interval.     

环圈光纤的失效预测

以光纤的机械可靠性为主线综述了光纤材料中固有裂纹的生长和传播所导致的光纤断裂机制.在该断裂力学的基础上推导了传统通信光纤在平直应用中的寿命预测模型.继而分析了处于弯曲构型中的传感环圈光纤表面的应力分布,然后在与传统理论相同的基本断裂机理下,类比于通信光纤可靠性模型的推导,据此应力分析给出了评估这种环圈光纤的机械可靠性的一般模型.进而从工程应用的角度简化了所推导出的一般模型,使之能够快速简单地给出环圈光纤失效概率的保守评估.在此简化模型的基础上,数值计算了目前常见的几种传感环圈中的光纤在服役期间的累积失效概率;其结果同时也显示了该环圈光纤的失效概率对光纤参量、环圈参量以及工艺参量的依赖关系.根据这一依赖关系,不仅可以快速评估在各种服役应力条件下具有不同寿命要求的光纤环圈的失效概率,同时也能对这些环圈的设计提供参考.     

All-optical switch based on photonic crystal microcavity with multi-resonant modes

We present a design of all-optical switches based on one-dimensional photonic crystals (1D PhC) doped with nonlinear optical materials. The 1D PhC switch structure is composed of a PhC cavity sandwiched by two accessional PhC microcavities. The center PhC cavity has two resonant frequencies with nearly the same quality factors (Q), while the accessional PhC cavities have the same resonant frequency, which is equal to one of the resonant frequencies of the center cavity. The two accessional PhC cavities cause reduction of Q value in this resonant frequency and result in different Q values of two modes. We realize all-optical switch effect by selecting pump light wavelength at the low Q mode and probe light wavelength at the other mode. The theoretical simulations by using the finite difference time domain method show that the pump light intensity required to realize optical switch effect in the designed switch is 50 times smaller than that in one-dimensional photonic crystals cavity with only one resonant mode.     

多腔耦合微波表面波PECVD法沉积 DLC薄膜研究

报道了利用多腔耦合微波表面波等离子体增强化学气相沉积(PECVD)的方法制备类金刚石(DLC)薄膜。通过发射光谱(OES)测量,对Ar等离子体中的各种放电参数以及全部四个腔室内放电的均匀性作出评估。采用表面轮廓仪测量了薄膜的厚度;薄膜的表面形貌、组成结构通过原子力显微镜(AFM)、激光拉曼光谱和X射线衍射光谱(XPS)进行了表征。在12.5μm厚度的有机薄膜聚酯(PET)表面沉积一定厚度DLC后,通过测量水蒸气透过率(WVTR)对DLC薄膜的阻隔性能进行了研究。结果表明,这种多腔耦合微波表面波等离子体装置,不仅能够实现四个腔室同时相对均匀的放电,也能够实现单个腔室的轴向均匀放电。制备的DLC薄膜结构致密、成分均匀,可以使PET薄膜阻隔性能提高约20倍。     

New plastic optical fiber using polycarbonate core and fluorescence-doped fiber for high temperature use

This article describes the development of a plastic optical fiber composed of a polycarbonate core with a glass transition temperature of 150°C, and a cladding of newly developed poly-4-methyl penten-1, which softens at 173°C. This cladding is suitable for use at temperatures up to 130°C. The minimum optical attenuation is 0.8 dB/m at 765 nm in the near-infrared region. The cause of the attenuation of the PC-core fiber was analyzed and the intrinsic loss limit was estimated to be 0.4 dB/m at 765 nm. The fiber has excellent characteristics, including thermal stability up to 125°C, high flexibility, high strength, and self-extinguishing properties.

The polycarbonate core fiber, doped organic fluorescing materials, has also been developed for automotive uses such as light guide and illuminator. Light can be transmitted through this fiber with incident optical beam perpendicular to the fiber as well as the beam parallel to the fiber.     

Single-shot tomography by means of VIPA and spatial phase modulator installed optical interferometer

A VIPA (virtually imaged phased array) installed optical interferometer has been proposed for scanless tomography. Also, a spatial phase modulator and a line-image sensor were installed into the interferometer to realize single-shot measurement by displaying the delay time on a line-image sensor. The correlation peak function was observed on the line-sensor at same time. The envelope of the peak was given by the inverse Fourier transformation of the light source spectrum. The peak position on the image-sensor reflects the sample structure. Furthermore, the correlation peaks are appeared repeatedly along the delay time of the interferometer. The repeated correlation function raise an alignment flexibility of the sample set position, which has been limited in the traditional time-domain interferometry involving the delay time to be zero. The flexibility was experimentally confirmed at 25 mm related to the VIPA coherency. The resolution was experimentally 52.5 μm when the ASE (amplified spontaneous emission) light source of the optical fiber amplifier was used. The single-shot measurement was realized by a line-image sensor of the 30 frames per second. The repeatability of the interfered peak position was 5 μm by the tunable mirror position. The one-dimensional scanless measurement was demonstrated by use of 3-layer glass plates.     

Trace-gas analysis using diode lasers in the near-IR and long-path techniques

Room-temperature, near-infrared, semiconductor diode lasers continue to gain importance for gas monitoring applications owing to their compactness, ease of use, reasonable cost and compatibility with telecommunications-grade optical fiber components. They may probe overtone or combination vibrational bands for a large variety of atmospheric relevant molecular species. These spectral bands exhibit line strengths orders of magnitude lower than those of fundamental vibrations, occurring in the mid-infrared. As a consequence, they are often used in conjunction with long-path techniques, enabling one to perform high sensitivity local measurements through long absorption path-lengths. At this purpose, resonant optical cavities can be fruitfully employed. This paper is devoted to a discussion of the main features of cavity-enhanced absorption spectrometers, operating with near-infrared diode lasers. We report on the operating principle as well as the achievable performance of these devices, also compared to more traditional apparatus, based on the multiple reflection cells. Experimental results on water vapour and oxygen detection are reported.