Investigation of excess enthalpies of selected binary and ternary solutions and mixtures |
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Authors: | L. Vogel |
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Affiliation: | (1) Department of Chemistry, Applied Thermodynamics Teaching and Research Team, Martin-Luther-University Halle-Wittenberg, 4020 Halle, Germany |
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Abstract: | The excess enthalpies were investigated for 12 binary and 4 ternary systems, including mixtures and solutions of electrolytes and non-electrolytes. The excess enthalpies of mixtures and integral heats of solutions were measured with an isoperibol calorimeter at 35 °C. Heats of fusion and heat capacities as functions of temperature were measured with a Perkin Elmer Corp., DSC-2. Integral heats, heats of fusion and heat capacities allow investigations of excess enthalpies of solutions. For modelling of the experimental results, the modified Redlich-Kister equation was used with good success.
Zusammenfassung Für 12 binäre und temäre Systeme, darunter Mischungen und Lösungen von Elektrolyten und Nichtelektrolyten, wurden die Exzessenthalpien untersucht. Die Exzessenthalpien der Mischungen und die integralen Lösungsenthalpien wurden mit einem isoperibolen Kalorimeter bei 35 °C gemessen. Die Schmelzwärmen und spezifischen Wärmekapazitäten in Abhängigkeit von der Temperatur wurden mit einem DSC 2 der Fa. Perkin-Elmer bestimmt. Die integralen Wärmen, Schmelzwärmen und Wärmekapazitäten erlauben, die Exzessenthalpien der Lösungen zu untersuchen. Die Versuchsergebnisse lassen sich erfolgreich mit modifizierten Redlich-Kister-Gleichungen modellieren.
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-![Kcy](/content/xl32573420287344/xxlarge1050.gif) ![icy](/content/xl32573420287344/xxlarge1080.gif) ![scy](/content/xl32573420287344/xxlarge1089.gif) ![tcy](/content/xl32573420287344/xxlarge1090.gif) ![iecy](/content/xl32573420287344/xxlarge1077.gif) ![rcy](/content/xl32573420287344/xxlarge1088.gif) .
The author expresses his gratitude to the leader of the Teaching and Research TEAM, Prof. Dr. H. Schuberth, and to Dr. G. Figurski, for help and discussions. |
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