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Optical and microscopy investigations of soot structure alterations by laser-induced incandescence
Authors:R.L. Vander Wal  T.M. Ticich  A.B. Stephens
Affiliation:(1) NCMR@NASA-Lewis Research Center, M.S. 110-3, 21 000 Brookpark Rd., Cleveland, OH 44135, USA (E-mail: randy@rvander.lerc.nasa.gov), US;(2) Department of Chemistry, Centenary College of Louisiana, 2911 Centenary Blvd., Shreveport, LA 71134, USA (E-mail: tticich@centenary.edu), US
Abstract:2 at 1064 nm, vaporization/fragmentation of soot primary particles and aggregates occurs. Optical measurements are performed using a second laser pulse to probe the effects of these changes upon the LII signal. With the exception of very low fluences, the structural changes induced in the soot lead to a decreased LII intensity produced by the second laser pulse. These two-pulse experiments also show that these changes do not alter the LII signal on timescales less than 1 μs for fluences below the vaporization threshold. Received: 20 October 1997/Revised version: 16 February 1998
Keywords:PACS: 42.62 Hk   78.20.Dj   82.40.Py
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