Field applied (FMD) computer simulation of the frequency doubled optical Stark effect |
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| Authors: | M. W. Evans |
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| Affiliation: | (1) Institute of Physical Chemistry, University of Zürich, Winterthurerstrasse 190, CH-8057 Zürich, Switzerland;(2) Present address: 433 Theory Center, Cornell University, 14853 Ithaca, NY, USA |
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| Abstract: | It is shown by field applied molecular dynamics computer simulation (FMD) of liquid water that the frequency doubled optical Stark effect is accompanied by novel second order rise transients which have no known counterpart in orientational theory, based on Langevin/Kielich functions. In the statistically stationary, post transient, steady state, correlation function have been computed which are intricately dependent on the frequency of the pump laser. These transients can be obtained experimentally by modifications of optical Stark effect apparatus for measurement on a femtosecond time scale. |
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